2026
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Meier, T. N. G.; Back, C. Thermal stability of skyrmions Journal Article J. Phys.: Condens. Matter 38, 423004 (2026), datadoi: 10.14459/2026mp1859939. @article{meierThermalStabilitySkyrmions2026,
title = {Thermal stability of skyrmions},
author = {T. N. G. Meier and C. Back},
url = {http://dx.doi.org/10.1088/1361-648X/aeb085},
doi = {10.1088/1361-648x/aeb085},
issn = {1361-648X},
year = {2026},
date = {2026-10-23},
urldate = {2026-10-01},
journal = {J. Phys.: Condens. Matter},
volume = {38},
number = {42},
pages = {423004},
publisher = {IOP Publishing},
abstract = {Magnetic skyrmions are vortex-like magnetic textures with a topologically nontrivial spin structure making a continuous transformation from the skyrmion to the uniform state impossible. Hence skyrmions are regarded as topologically protected attracting large interest concerning applications in data storage, neuromorphic computing, and digital logic. For such kind of applications an extraordinary stability of the skyrmion state against thermal fluctuations is required. In real matter, due to its discrete nature, topological protection translates into the existence of an energy barrier between the skyrmion and the uniform state leading to a finite skyrmion lifetime. Therefore the experimental determination of the skyrmion lifetime becomes important. Within this work we focus on experimental studies of the skyrmion lifetime in a variety of magnetic systems ranging from monolayers to bulk samples. We discuss previous experimental studies on the thermal stability of magnetic skyrmions in systems based on Fe/Ir(111) and in B20-materials. New experimental results on skyrmion nucleation and decay are obtained for thin Ni/Fe-films on Cu(001) using threshold photoemission magnetic circular dichroism in combination with photoemission electron microscopy (TP-MCD-PEEM). The results are interpreted using an Arrhenius-like activation behavior and evaluated regarding energy barriers and pre-exponential factors of the skyrmion dynamics.},
note = {datadoi: 10.14459/2026mp1859939},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
Magnetic skyrmions are vortex-like magnetic textures with a topologically nontrivial spin structure making a continuous transformation from the skyrmion to the uniform state impossible. Hence skyrmions are regarded as topologically protected attracting large interest concerning applications in data storage, neuromorphic computing, and digital logic. For such kind of applications an extraordinary stability of the skyrmion state against thermal fluctuations is required. In real matter, due to its discrete nature, topological protection translates into the existence of an energy barrier between the skyrmion and the uniform state leading to a finite skyrmion lifetime. Therefore the experimental determination of the skyrmion lifetime becomes important. Within this work we focus on experimental studies of the skyrmion lifetime in a variety of magnetic systems ranging from monolayers to bulk samples. We discuss previous experimental studies on the thermal stability of magnetic skyrmions in systems based on Fe/Ir(111) and in B20-materials. New experimental results on skyrmion nucleation and decay are obtained for thin Ni/Fe-films on Cu(001) using threshold photoemission magnetic circular dichroism in combination with photoemission electron microscopy (TP-MCD-PEEM). The results are interpreted using an Arrhenius-like activation behavior and evaluated regarding energy barriers and pre-exponential factors of the skyrmion dynamics. |  |
Ranaut, D.; Unnikrishnan, G.; M, Samraj; Channarayappa, S. K.; Mukharjee, P. K.; Saravanan, P.; Gegenwart, P.; Jaiswal-Nagar, D. Frustrated Garnet Gd3Te2Li3O12 for High-Performance Sub-Kelvin Adiabatic Demagnetization Refrigeration Journal Article ACS Appl. Electron. Mater. (2026). @article{ranautFrustratedGarnetGd3Te2Li3O122026,
title = {Frustrated Garnet Gd_{3}Te_{2}Li_{3}O_{12} for High-Performance Sub-Kelvin Adiabatic Demagnetization Refrigeration},
author = {D. Ranaut and G. Unnikrishnan and Samraj M and S. K. Channarayappa and P. K. Mukharjee and P. Saravanan and P. Gegenwart and D. Jaiswal-Nagar},
url = {https://doi.org/10.1021/acsaelm.6c01619},
doi = {10.1021/acsaelm.6c01619},
issn = {2637-6113},
year = {2026},
date = {2026-10-22},
urldate = {2026-10-01},
journal = {ACS Appl. Electron. Mater.},
abstract = {Owing to the limited availability and high cost of 3He, adiabatic demagnetization refrigeration (ADR) has gained considerable attention as an efficient technology for ultralow-temperature applications. Here, we demonstrate the frustrated garnet Gd3Te2Li3O12 (GTLG) as a high-performance ADR material with substantially improved cooling capability over the commercial benchmark Gd3Ga5O12 (GGG). Direct ADR measurements reveal a minimum temperature of 165 mK for GTLG, nearly two-fold lower than that of GGG (320 mK). Under a cryostat bath temperature of 1.8 K, GTLG maintains temperatures below 1 K for more than 12 h and below the 3He-temperature (0.4 K) for over 3 h, demonstrating excellent temperature stability for prolonged cryogenic operation. Magnetic and thermodynamic measurements show that GTLG undergoes antiferromagnetic ordering at TN ∼ 0.25 K while retaining strong magnetic frustration and a large magnetic entropy reservoir favorable for efficient demagnetization cooling. Field-dependent heat capacity and magnetic Grüneisen parameter measurements further reveal the presence of field-induced critical behavior that enables cooling below TN through enhanced entropy accumulation near the critical region. These findings establish GTLG as a promising next-generation magnetic refrigerant and highlight field-induced criticality as an effective design principle for developing advanced materials for ultralow-temperature refrigeration.},
keywords = {B1, B3},
pubstate = {published},
tppubtype = {article}
}
Owing to the limited availability and high cost of 3He, adiabatic demagnetization refrigeration (ADR) has gained considerable attention as an efficient technology for ultralow-temperature applications. Here, we demonstrate the frustrated garnet Gd3Te2Li3O12 (GTLG) as a high-performance ADR material with substantially improved cooling capability over the commercial benchmark Gd3Ga5O12 (GGG). Direct ADR measurements reveal a minimum temperature of 165 mK for GTLG, nearly two-fold lower than that of GGG (320 mK). Under a cryostat bath temperature of 1.8 K, GTLG maintains temperatures below 1 K for more than 12 h and below the 3He-temperature (0.4 K) for over 3 h, demonstrating excellent temperature stability for prolonged cryogenic operation. Magnetic and thermodynamic measurements show that GTLG undergoes antiferromagnetic ordering at TN ∼ 0.25 K while retaining strong magnetic frustration and a large magnetic entropy reservoir favorable for efficient demagnetization cooling. Field-dependent heat capacity and magnetic Grüneisen parameter measurements further reveal the presence of field-induced critical behavior that enables cooling below TN through enhanced entropy accumulation near the critical region. These findings establish GTLG as a promising next-generation magnetic refrigerant and highlight field-induced criticality as an effective design principle for developing advanced materials for ultralow-temperature refrigeration. |  |
Prodan, L.; Evans, D. M.; Puntigam, L.; Kézsmárki, I.; Tsurkan, V. Universality of magnetic susceptibility in the conical state of kagome ferromagnet Fe3Sn2 Journal Article Appl. Phys. Lett. 129, 151905 (2026), datadoi: 10.5281/zenodo.15367272. @article{prodan2026universalitymagneticsusceptibilityconical,
title = {Universality of magnetic susceptibility in the conical state of kagome ferromagnet Fe_{3}Sn_{2}},
author = {L. Prodan and D. M. Evans and L. Puntigam and I. Kézsmárki and V. Tsurkan},
url = {https://doi.org/10.1063/5.0342307},
doi = {10.1063/5.0342307},
year = {2026},
date = {2026-10-13},
urldate = {2026-10-01},
journal = {Appl. Phys. Lett.},
volume = {129},
pages = {151905},
abstract = {We report universal behavior of the differential magnetic susceptibility (DMS) in the conical phase that mediates the spin-reorientation (SR) transition of the kagome ferromagnet Fe3Sn2. Within the SR temperature range, the DMS isotherms exhibit extremely narrow crossing regions, forming isosbestic points. Using an isosbestic-invariance analysis, we show that the isotherms collapse onto a single temperature-independent curve, revealing quadratic-in-temperature corrections to the susceptibility. Complementary field-dependent magnetic-force-microscopy measurements uncover the evolution of spin textures from stripe-like domains at low fields to isolated bubble-like domains near the isosbestic field ( textasciitilde0.6T), a behavior not previously reported in bulk Fe3Sn2 within the conical state. These findings point to a universal mechanism for the emergence of complex magnetic textures near isosbestic points, driven by the competition between magnetocrystalline anisotropy, dipolar interactions, and external magnetic field.},
note = {datadoi: 10.5281/zenodo.15367272},
keywords = {A1, A4},
pubstate = {published},
tppubtype = {article}
}
We report universal behavior of the differential magnetic susceptibility (DMS) in the conical phase that mediates the spin-reorientation (SR) transition of the kagome ferromagnet Fe3Sn2. Within the SR temperature range, the DMS isotherms exhibit extremely narrow crossing regions, forming isosbestic points. Using an isosbestic-invariance analysis, we show that the isotherms collapse onto a single temperature-independent curve, revealing quadratic-in-temperature corrections to the susceptibility. Complementary field-dependent magnetic-force-microscopy measurements uncover the evolution of spin textures from stripe-like domains at low fields to isolated bubble-like domains near the isosbestic field ( textasciitilde0.6T), a behavior not previously reported in bulk Fe3Sn2 within the conical state. These findings point to a universal mechanism for the emergence of complex magnetic textures near isosbestic points, driven by the competition between magnetocrystalline anisotropy, dipolar interactions, and external magnetic field. |  |
Liu, Y. -J.; Xu, W. -T.; Pollmann, F.; Knap, M. Information-Theoretic Principle of Emergent 1-Form Symmetries Journal Article PRX Quantum 7, (2026), datadoi: 10.5281/zenodo.17652054. @article{liuInformationTheoreticPrincipleEmergent2026,
title = {Information-Theoretic Principle of Emergent 1-Form Symmetries},
author = {Y. -J. Liu and W. -T. Xu and F. Pollmann and M. Knap},
url = {https://doi.org/10.1103/d6qf-5chk},
doi = {10.1103/d6qf-5chk},
issn = {2691-3399},
year = {2026},
date = {2026-10-09},
urldate = {2026-10-01},
journal = {PRX Quantum},
volume = {7},
number = {4},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.17652054},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Schneider, M.; Butcher, T. A.; Wagner, S.; Metternich, D.; Klose, C.; Malm, E.; Battistelli, R.; Deinhart, V.; Fuchs, J.; Wittrock, S.; Karaman, T.; Joy, K. Puzhekadavil; Patra, M.; Büttner, F.; Wintz, S.; Weigand, M.; Günther, C. M.; Engel, D.; Gaal, P.; Schwarzkopf, J.; Pfau, B.; Eisebitt, S. Linear dichroic soft x-ray microscopy of ferroelectric stripe domains in epitaxial K0.6Na0.4NbO3 Journal Article Phys. Rev. B 114, L231401 (2026), datadoi: 10.5281/zenodo.22250213.. @article{schneiderLinearDichroicSoft2026,
title = {Linear dichroic soft x-ray microscopy of ferroelectric stripe domains in epitaxial K_{0.6}Na_{0.4}NbO_{3}},
author = {M. Schneider and T. A. Butcher and S. Wagner and D. Metternich and C. Klose and E. Malm and R. Battistelli and V. Deinhart and J. Fuchs and S. Wittrock and T. Karaman and K. Puzhekadavil Joy and M. Patra and F. Büttner and S. Wintz and M. Weigand and C. M. Günther and D. Engel and P. Gaal and J. Schwarzkopf and B. Pfau and S. Eisebitt},
url = {https://link.aps.org/doi/10.1103/kcjc-dtj6},
doi = {10.1103/kcjc-dtj6},
year = {2026},
date = {2026-10-02},
urldate = {2026-10-01},
journal = {Phys. Rev. B},
volume = {114},
number = {23},
pages = {L231401},
publisher = {American Physical Society},
abstract = {Functional properties of ferroelectric thin films are governed by domains that can be engineered by epitaxial strain. Soft x-ray microscopy can image domain structures with elemental and electronic sensitivity, but hitherto its application to strain-stabilized domains has been hindered by the absorption of soft x-rays in epitaxial substrates. Here, it is demonstrated how this limitation can be overcome by locally back-thinning the (110) TbScO3 substrate of epitaxial K0.6Na0.4NbO3 ferroelectric thin films to achieve soft x-ray transparency at the O K-edge around 530 eV. Strain-induced ferroelectric stripe domains with periods down to 44 nm were resolved by scanning transmission x-ray microscopy and coherent diffractive imaging by exploiting the x-ray linear dichroism of hybridized O 2𝑝–Nb 4𝑑 states, providing sensitivity to in-plane polarization components under normal incidence. The results establish soft x-ray microscopy for nanoscale imaging of epitaxial ferroelectric domain structures and open perspectives for time-resolved studies thereof.},
note = {datadoi: 10.5281/zenodo.22250213.},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
Functional properties of ferroelectric thin films are governed by domains that can be engineered by epitaxial strain. Soft x-ray microscopy can image domain structures with elemental and electronic sensitivity, but hitherto its application to strain-stabilized domains has been hindered by the absorption of soft x-rays in epitaxial substrates. Here, it is demonstrated how this limitation can be overcome by locally back-thinning the (110) TbScO3 substrate of epitaxial K0.6Na0.4NbO3 ferroelectric thin films to achieve soft x-ray transparency at the O K-edge around 530 eV. Strain-induced ferroelectric stripe domains with periods down to 44 nm were resolved by scanning transmission x-ray microscopy and coherent diffractive imaging by exploiting the x-ray linear dichroism of hybridized O 2𝑝–Nb 4𝑑 states, providing sensitivity to in-plane polarization components under normal incidence. The results establish soft x-ray microscopy for nanoscale imaging of epitaxial ferroelectric domain structures and open perspectives for time-resolved studies thereof. |  |
Mangeolle, L.; Knolle, J. Probing topology in thin films with quantum Sondheimer oscillations Journal Article Phys. Rev. B 114, 225108 (2026). @article{mangeolleProbingTopologyThin2026,
title = {Probing topology in thin films with quantum Sondheimer oscillations},
author = {L. Mangeolle and J. Knolle},
url = {https://link.aps.org/doi/10.1103/l1gl-xdvv},
doi = {10.1103/l1gl-xdvv},
year = {2026},
date = {2026-10-01},
journal = {Phys. Rev. B},
volume = {114},
number = {22},
pages = {225108},
publisher = {American Physical Society},
abstract = {Sondheimer oscillations (SO) are magnetoresistance oscillations occurring in thin films due to the commensurability between cyclotron motion and sample thickness, and are traditionally regarded as a purely semiclassical size effect. Here we develop a general quantum theory of SO for thin-film conductors in the quantum limit of a large magnetic field. We show that corrections arising from band topology modify the SO frequency, in contrast to Shubnikov–de Haas oscillations where topological information appears only in the phase. As a consequence, quantum SO provide a direct and robust probe of the full Landau level spectrum. Applying our framework to a minimal model with tunable Berry phase, we demonstrate how topology manifests itself in experimentally accessible magneto-oscillation spectra and discuss damping mechanisms including surface roughness.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Sondheimer oscillations (SO) are magnetoresistance oscillations occurring in thin films due to the commensurability between cyclotron motion and sample thickness, and are traditionally regarded as a purely semiclassical size effect. Here we develop a general quantum theory of SO for thin-film conductors in the quantum limit of a large magnetic field. We show that corrections arising from band topology modify the SO frequency, in contrast to Shubnikov–de Haas oscillations where topological information appears only in the phase. As a consequence, quantum SO provide a direct and robust probe of the full Landau level spectrum. Applying our framework to a minimal model with tunable Berry phase, we demonstrate how topology manifests itself in experimentally accessible magneto-oscillation spectra and discuss damping mechanisms including surface roughness. | |
Zhang, Y. -S.; Yang, Z.; Xiao, C.; Isobe, M.; Minola, M.; Takagi, H.; Huang, D. Substrate tuning of the structural and electronic transition in thin flakes of the excitonic insulator candidate Ta2NiSe5 Journal Article Commun. Phys. 9, 309 (2026), datadoi: 10.5281/zenodo.22107443. @article{zhangSubstrateTuningStructural2026,
title = {Substrate tuning of the structural and electronic transition in thin flakes of the excitonic insulator candidate Ta_{2}NiSe_{5}},
author = {Y. -S. Zhang and Z. Yang and C. Xiao and M. Isobe and M. Minola and H. Takagi and D. Huang},
url = {https://doi.org/10.1038/s42005-026-02888-x},
doi = {10.1038/s42005-026-02888-x},
year = {2026},
date = {2026-09-29},
urldate = {2026-09-01},
journal = {Commun. Phys.},
volume = {9},
pages = {309},
abstract = {Ta2NiSe5 continues to draw interest for its Tc = 326 K phase transition, whose dual electronic and structural nature reflects a complex interplay of electron-hole (excitonic) and electron-lattice interactions. The majority of studies that have attempted to decipher the relative importance of these interactions, particularly through charge tuning, have been focused on bulk samples. Here, we utilize an all-dry exfoliation and transfer protocol to isolate ultrathin flakes of Ta2NiSe5 on insulating Al2O3 and conducting Au. Using polarized Raman spectroscopy, we uncover the following substrate dependence: Four layers of Ta2NiSe5 on Al2O3 show a sharp structural and electronic transition that is lowered by roughly 40 K from the bulk Tc. Meanwhile, four layers of Ta2NiSe5 on Au undergo a structural and electronic transition that is much more gradual with respect to temperature and finishes roughly 150 K below the bulk Tc. The pronounced broadening points to an atomic-scale interface effect, wherein electrostatic screening and charge transfer from Au produces a Tc gradient perpendicular to the layers of the flake. We discuss the role of excitonic physics and suggest the possibility for interface engineering to pattern nanoscale junctions in Ta2NiSe5.},
note = {datadoi: 10.5281/zenodo.22107443},
keywords = {A3},
pubstate = {published},
tppubtype = {article}
}
Ta2NiSe5 continues to draw interest for its Tc = 326 K phase transition, whose dual electronic and structural nature reflects a complex interplay of electron-hole (excitonic) and electron-lattice interactions. The majority of studies that have attempted to decipher the relative importance of these interactions, particularly through charge tuning, have been focused on bulk samples. Here, we utilize an all-dry exfoliation and transfer protocol to isolate ultrathin flakes of Ta2NiSe5 on insulating Al2O3 and conducting Au. Using polarized Raman spectroscopy, we uncover the following substrate dependence: Four layers of Ta2NiSe5 on Al2O3 show a sharp structural and electronic transition that is lowered by roughly 40 K from the bulk Tc. Meanwhile, four layers of Ta2NiSe5 on Au undergo a structural and electronic transition that is much more gradual with respect to temperature and finishes roughly 150 K below the bulk Tc. The pronounced broadening points to an atomic-scale interface effect, wherein electrostatic screening and charge transfer from Au produces a Tc gradient perpendicular to the layers of the flake. We discuss the role of excitonic physics and suggest the possibility for interface engineering to pattern nanoscale junctions in Ta2NiSe5. |  |
Jawale, M.; Nandi, S.; Mukharjee, P. K.; Gegenwart, P.; Mahajan, A. V. Low-temperature magnetism and spin dynamics in the disordered triangular-lattice Yb3+ compound LiCaYb5(BO3)6 Journal Article Phys. Rev. B 114, 165140 (2026). @article{jawaleLowtemperatureMagnetismSpin2026,
title = {Low-temperature magnetism and spin dynamics in the disordered triangular-lattice Yb^{3+} compound LiCaYb_{5}(BO_{3})_{6}},
author = {M. Jawale and S. Nandi and P. K. Mukharjee and P. Gegenwart and A. V. Mahajan},
url = {https://link.aps.org/doi/10.1103/px8x-fcqp},
doi = {10.1103/px8x-fcqp},
year = {2026},
date = {2026-09-25},
urldate = {2026-09-01},
journal = {Phys. Rev. B},
volume = {114},
number = {16},
pages = {165140},
publisher = {American Physical Society},
abstract = {The interplay between geometric frustration, spin-orbit coupling, and structural disorder can give rise to unconventional magnetic ground states in rare-earth triangular-lattice magnets. We report low-temperature magnetic and 7Li NMR investigations of the disordered triangular-lattice compound LiCaYb5(BO3)6 (LCYBO). Rietveld refinement confirms a hexagonal 𝑃6522 structure with partial Ca/Yb antisite disorder and fractional Li occupancy. Magnetic susceptibility and magnetization measurements indicate a well-isolated effective 𝐽eff=1/2 Kramers doublet with weak antiferromagnetic interactions (𝜃CW≈−0.54K). The specific heat reveals a weak anomaly near 0.43 K, suggesting the development of short-range correlated magnetism rather than conventional long-range order. 7Li NMR spectra broaden strongly upon cooling, consistent with increasingly inhomogeneous internal magnetic fields. The spin-lattice relaxation exhibits two relaxation components consistent with disorder-induced distributions of local magnetic environments arising from antisite disorder and competing exchange pathways. Our results establish LCYBO as a structurally disordered frustrated triangular-lattice magnet with correlated low-energy spin dynamics.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
The interplay between geometric frustration, spin-orbit coupling, and structural disorder can give rise to unconventional magnetic ground states in rare-earth triangular-lattice magnets. We report low-temperature magnetic and 7Li NMR investigations of the disordered triangular-lattice compound LiCaYb5(BO3)6 (LCYBO). Rietveld refinement confirms a hexagonal 𝑃6522 structure with partial Ca/Yb antisite disorder and fractional Li occupancy. Magnetic susceptibility and magnetization measurements indicate a well-isolated effective 𝐽eff=1/2 Kramers doublet with weak antiferromagnetic interactions (𝜃CW≈−0.54K). The specific heat reveals a weak anomaly near 0.43 K, suggesting the development of short-range correlated magnetism rather than conventional long-range order. 7Li NMR spectra broaden strongly upon cooling, consistent with increasingly inhomogeneous internal magnetic fields. The spin-lattice relaxation exhibits two relaxation components consistent with disorder-induced distributions of local magnetic environments arising from antisite disorder and competing exchange pathways. Our results establish LCYBO as a structurally disordered frustrated triangular-lattice magnet with correlated low-energy spin dynamics. |  |
Gimpel, T.; Büttgen, N.; Prodan, L.; Tsurkan, V.; Tsirlin, A. A.; Nakamura, H.; Kézsmárki, I. Magnetic symmetry and hyperfine fields of V_4 tetrahedral clusters in the multiferroic lacunar spinel GeV4S8 Journal Article Phys. Rev. B 114, 154418 (2026), datadoi: (10.5281/zenodo.20604906). @article{xn3r-b7g6,
title = {Magnetic symmetry and hyperfine fields of V_4 tetrahedral clusters in the multiferroic lacunar spinel GeV_{4}S_{8}},
author = {T. Gimpel and N. Büttgen and L. Prodan and V. Tsurkan and A. A. Tsirlin and H. Nakamura and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/xn3r-b7g6},
doi = {10.1103/xn3r-b7g6},
year = {2026},
date = {2026-09-18},
urldate = {2026-09-01},
journal = {Phys. Rev. B},
volume = {114},
number = {15},
pages = {154418},
abstract = {We use 51V nuclear magnetic resonance (NMR) spectroscopy to investigate the magnetic ground state of the lacunar spinel GeV4S8, which undergoes a structural distortion at 𝑇JT≈30K followed by an antiferromagnetic (AFM) ordering at 𝑇𝑁≈15K. According to our zero- and finite-field NMR data, the four V-sites of V4 clusters become magnetically inequivalent in the AFM state: Two of them share the same internal field, while the other two sites are characterized by different internal fields. The angular dependence of the 51V NMR lines, upon rotation of an external magnetic field about the pseudocubic [110] and [100] axes, reveals that the internal fields are either parallel to the orthorhombic 𝑎 axis at all four V-sites of the V4 tetrahedra, or they form an orthogonal pattern, where two V-sites have internal field along the 𝑎 axis and the other two along the 𝑏 axis. Based on these results, further supported by the observation of distinct spin-echo modulations of the inequivalent V-sites, we conclude that the magnetic space group of the AFM state is 𝑃𝑏𝑚𝑛21 or 𝑃𝑚𝑛′2′1.},
note = {datadoi: (10.5281/zenodo.20604906)},
keywords = {B3, B4},
pubstate = {published},
tppubtype = {article}
}
We use 51V nuclear magnetic resonance (NMR) spectroscopy to investigate the magnetic ground state of the lacunar spinel GeV4S8, which undergoes a structural distortion at 𝑇JT≈30K followed by an antiferromagnetic (AFM) ordering at 𝑇𝑁≈15K. According to our zero- and finite-field NMR data, the four V-sites of V4 clusters become magnetically inequivalent in the AFM state: Two of them share the same internal field, while the other two sites are characterized by different internal fields. The angular dependence of the 51V NMR lines, upon rotation of an external magnetic field about the pseudocubic [110] and [100] axes, reveals that the internal fields are either parallel to the orthorhombic 𝑎 axis at all four V-sites of the V4 tetrahedra, or they form an orthogonal pattern, where two V-sites have internal field along the 𝑎 axis and the other two along the 𝑏 axis. Based on these results, further supported by the observation of distinct spin-echo modulations of the inequivalent V-sites, we conclude that the magnetic space group of the AFM state is 𝑃𝑏𝑚𝑛21 or 𝑃𝑚𝑛′2′1. |  |
Chatterjee, S.; Agarwal, A.; Borkenhagen, R.; Kuntscher, C. A.; Winiarski, M. J.; Pavlosiuk, O.; Wiśniewski, P.; Kaczorowski, D. Anisotropic magnetotransport and optical response of the multiband low-carrier antiferromagnet DyPtSb Journal Article Phys. Rev. B 114, 154412 (2026). @article{chatterjeeAnisotropicMagnetotransportOptical2026,
title = {Anisotropic magnetotransport and optical response of the multiband low-carrier antiferromagnet DyPtSb},
author = {S. Chatterjee and A. Agarwal and R. Borkenhagen and C. A. Kuntscher and M. J. Winiarski and O. Pavlosiuk and P. Wiśniewski and D. Kaczorowski},
url = {https://link.aps.org/doi/10.1103/lqnh-7d73},
doi = {10.1103/lqnh-7d73},
year = {2026},
date = {2026-09-14},
urldate = {2026-09-01},
journal = {Phys. Rev. B},
volume = {114},
number = {15},
pages = {154412},
abstract = {We report a combined study of the magnetic, electrical transport, optical reflectivity, and electronic properties of single-crystalline DyPtSb, a half-Heusler antiferromagnet that orders at 2.2 K. The electrical resistivity exhibits semiconductor-like behavior and the Hall response becomes strongly nonlinear at low temperatures, indicating multiband transport with hole- and electron-type pockets. Angular magnetoresistance measurements revealed occurrence of twofold and fourfold symmetry components, both of which change sign near magnetic field of 4 T at 2 K, suggesting a field-induced modification of the electronic structure near the crossover from the antiferromagnetic to the spin-polarized regime. The optical spectroscopy revealed a temperature-dependent plasma edge and a Drude response, consistent with the bulk electrical transport data. In contrast to the characteristic feature of three-dimensional Dirac and Weyl semimetals, the optical conductivity of DyPtSb does not exhibit clear linear-in-frequency behavior at low energy. The results of ab initio electronic band-structure calculations revealed that the compound is a narrow-gap semiconductor, showing pronounced anisotropy of valence bands and strong sensitivity to magnetic polarization. DyPtSb was characterized as a multiband low-carrier antiferromagnet whose electrical transport properties are closely tied to the evolution of its electronic structure.},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
We report a combined study of the magnetic, electrical transport, optical reflectivity, and electronic properties of single-crystalline DyPtSb, a half-Heusler antiferromagnet that orders at 2.2 K. The electrical resistivity exhibits semiconductor-like behavior and the Hall response becomes strongly nonlinear at low temperatures, indicating multiband transport with hole- and electron-type pockets. Angular magnetoresistance measurements revealed occurrence of twofold and fourfold symmetry components, both of which change sign near magnetic field of 4 T at 2 K, suggesting a field-induced modification of the electronic structure near the crossover from the antiferromagnetic to the spin-polarized regime. The optical spectroscopy revealed a temperature-dependent plasma edge and a Drude response, consistent with the bulk electrical transport data. In contrast to the characteristic feature of three-dimensional Dirac and Weyl semimetals, the optical conductivity of DyPtSb does not exhibit clear linear-in-frequency behavior at low energy. The results of ab initio electronic band-structure calculations revealed that the compound is a narrow-gap semiconductor, showing pronounced anisotropy of valence bands and strong sensitivity to magnetic polarization. DyPtSb was characterized as a multiband low-carrier antiferromagnet whose electrical transport properties are closely tied to the evolution of its electronic structure. |  |
Scopa, S.; Zechmann, P.; Knap, M.; Nardis, J. De; Bastianello, A. Generalized Hydrodynamics of Bloch Oscillations in the Absence of a Lattice Journal Article Phys. Rev. Lett. 137, (2026), datadoi: 10.5281/zenodo.20272044. @article{scopaGeneralizedHydrodynamicsBloch2026,
title = {Generalized Hydrodynamics of Bloch Oscillations in the Absence of a Lattice},
author = {S. Scopa and P. Zechmann and M. Knap and J. De Nardis and A. Bastianello},
url = {https://doi.org/10.1103/yfjc-r69d},
doi = {10.1103/yfjc-r69d},
issn = {1079-7114},
year = {2026},
date = {2026-09-11},
urldate = {2026-09-01},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {11},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.20272044},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Cônsoli, P. M.; Day-Roberts, E.; Knolle, J.; Botana, A. S.; Erten, O. Tuning the Magnetic Properties of Kitaev Materials via the Antiferromagnetic Proximity Effect: Novel Phases and Application to an α-RuCl3/MnPS3 Bilayer Journal Article Nano Lett. 26, 12491–12499 (2026). @article{consoliTuningMagneticProperties2026,
title = {Tuning the Magnetic Properties of Kitaev Materials via the Antiferromagnetic Proximity Effect: Novel Phases and Application to an α-RuCl_{3}/MnPS_{3} Bilayer},
author = {P. M. Cônsoli and E. Day-Roberts and J. Knolle and A. S. Botana and O. Erten},
url = {https://doi.org/10.1021/acs.nanolett.6c03321},
doi = {10.1021/acs.nanolett.6c03321},
issn = {1530-6984},
year = {2026},
date = {2026-09-08},
urldate = {2026-09-01},
journal = {Nano Lett.},
volume = {26},
number = {37},
pages = {12491–12499},
abstract = {In recent years, the increasing level of control over van der Waals (vdW) heterostructures has opened new routes to tune the properties of quantum materials. Motivated by these developments, we examine the potential consequences of interfacing a Kitaev honeycomb magnet, such as α-RuCl3, with a nearly lattice-matched vdW antiferromagnet. By combining perturbation theory, exact diagonalization, and a classical energy-minimization method, we show that an effective staggered magnetic field originating from the vdW antiferromagnet can drive a monolayer of a Kitaev material into various novel phases, including an antichiral Kitaev spin liquid, a nonmagnetic nematic phase, and different types of skyrmion crystals. We then apply first-principles simulations to assess the prospect of concretely realizing this setup in a heterobilayer of α-RuCl3 and the easy-axis antiferromagnet MnPS3.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
In recent years, the increasing level of control over van der Waals (vdW) heterostructures has opened new routes to tune the properties of quantum materials. Motivated by these developments, we examine the potential consequences of interfacing a Kitaev honeycomb magnet, such as α-RuCl3, with a nearly lattice-matched vdW antiferromagnet. By combining perturbation theory, exact diagonalization, and a classical energy-minimization method, we show that an effective staggered magnetic field originating from the vdW antiferromagnet can drive a monolayer of a Kitaev material into various novel phases, including an antichiral Kitaev spin liquid, a nonmagnetic nematic phase, and different types of skyrmion crystals. We then apply first-principles simulations to assess the prospect of concretely realizing this setup in a heterobilayer of α-RuCl3 and the easy-axis antiferromagnet MnPS3. |  |
Wang, Y.; Wu, Z.; Bhupendra, K. C.; Zhang, D.; Wang, L.; Khare, S. V.; Prodan, L.; Tsurkan, V. Pressure-induced electronic delocalization and superconductivity in GaNb4Se8 Journal Article Phys. Rev. B 114, 175107 (2026). @article{8b8c-2wm3,
title = {Pressure-induced electronic delocalization and superconductivity in GaNb_{4}Se_{8}},
author = {Y. Wang and Z. Wu and K. C. Bhupendra and D. Zhang and L. Wang and S. V. Khare and L. Prodan and V. Tsurkan},
url = {https://link.aps.org/doi/10.1103/8b8c-2wm3},
doi = {10.1103/8b8c-2wm3},
year = {2026},
date = {2026-09-04},
urldate = {2026-09-01},
journal = {Phys. Rev. B},
volume = {114},
number = {17},
pages = {175107},
publisher = {American Physical Society},
abstract = {Understanding how electronic transport evolves from localized to itinerant regimes in correlated cluster solids remains an important challenge in condensed-matter physics. Here, we investigate the pressure-dependent transport properties of the lacunar spinel GaNb4Se8, a cluster Mott insulator at ambient conditions. At ambient pressure, the resistivity follows Efros-Shklovskii variable-range hopping, indicating Coulomb gap–controlled carrier localization. A pressure-induced electronic delocalization process begins at low pressures (∼5 GPa), as evidenced by the continuous suppression of room-temperature resistance. Upon further compression, the system undergoes a broad insulator-to-metal-like crossover in low-temperature transport, culminating in a fully metallic-like ground state at ∼17–18 GPa. In contrast, the crystallographic transition from the cubic phase to the monoclinic 𝐶2 phase starts at ∼20 GPa and ends near ∼32 GPa, demonstrating that the pressure-induced electronic evolution is completed before the onset of long-range structural symmetry breaking. At higher pressures, superconductivity (with a superconducting coherence length ξ(0) ≈ 80–90 Å) emerges from a pressure-induced metallic-like regime. These results establish GaNb4Se8 as a platform for studying correlation-driven evolution of electronic transport in cluster-based solids.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
Understanding how electronic transport evolves from localized to itinerant regimes in correlated cluster solids remains an important challenge in condensed-matter physics. Here, we investigate the pressure-dependent transport properties of the lacunar spinel GaNb4Se8, a cluster Mott insulator at ambient conditions. At ambient pressure, the resistivity follows Efros-Shklovskii variable-range hopping, indicating Coulomb gap–controlled carrier localization. A pressure-induced electronic delocalization process begins at low pressures (∼5 GPa), as evidenced by the continuous suppression of room-temperature resistance. Upon further compression, the system undergoes a broad insulator-to-metal-like crossover in low-temperature transport, culminating in a fully metallic-like ground state at ∼17–18 GPa. In contrast, the crystallographic transition from the cubic phase to the monoclinic 𝐶2 phase starts at ∼20 GPa and ends near ∼32 GPa, demonstrating that the pressure-induced electronic evolution is completed before the onset of long-range structural symmetry breaking. At higher pressures, superconductivity (with a superconducting coherence length ξ(0) ≈ 80–90 Å) emerges from a pressure-induced metallic-like regime. These results establish GaNb4Se8 as a platform for studying correlation-driven evolution of electronic transport in cluster-based solids. |  |
Magnaterra, M.; Hopfer, K.; Sahle, C. J.; Sala, M. Moretti; Monaco, G.; Attig, J.; Hickey, C.; Pietsch, I. -M.; Breitner, F.; Gegenwart, P.; Upton, M. H.; Kim, J.; Trebst, S.; Loosdrecht, P. H. M.; Brink, J.; Grüninger, M. RIXS observation of bond-directional excitations in the Kitaev material Na2IrO3 Journal Article npj Quantum Mater. 11, 85 (2026). @article{magnaterraRIXSObservationBonddirectional2026,
title = {RIXS observation of bond-directional excitations in the Kitaev material Na_{2}IrO_{3}},
author = {M. Magnaterra and K. Hopfer and C. J. Sahle and M. Moretti Sala and G. Monaco and J. Attig and C. Hickey and I. -M. Pietsch and F. Breitner and P. Gegenwart and M. H. Upton and J. Kim and S. Trebst and P. H. M. Loosdrecht and J. Brink and M. Grüninger},
url = {https://doi.org/10.1038/s41535-026-00938-9},
doi = {10.1038/s41535-026-00938-9},
year = {2026},
date = {2026-09-03},
urldate = {2026-09-01},
journal = {npj Quantum Mater.},
volume = {11},
pages = {85},
abstract = {Spin-orbit coupling locks spin direction and spatial orientation and generates, in semi-classical magnets, a local spin easy-axis and associated ordering. Quantum spin-1/2’s defy this fate: rather than spins becoming locally anisotropic, the spin-spin interactions do. Consequently interactions become dependent on the spatial orientation of bonds between spins, prime theoretical examples of which are Kitaev magnets. Bond-directional interactions imply the existence of bond-directional magnetic modes, spin excitations that render crystallographically equivalent bonds magnetically inequivalent, which yet have remained elusive experimentally. Here we show that resonant inelastic X-ray scattering allows us to explicitly probe the bond-directional character of magnetic excitations. To do so, we use a scattering plane spanned by one bond and the corresponding spin component and scan a range of momentum transfer that encompasses multiple Brillouin zones. Applying this approach to Na2IrO3 we establish the different bond-directional characters of magnetic excitations at textasciitilde10 meV and textasciitilde45 meV. The bond-directional nearest-neighbor excitations are a fingerprint of the dominant Kitaev interactions and even prevail in the magnetically ordered state.},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Spin-orbit coupling locks spin direction and spatial orientation and generates, in semi-classical magnets, a local spin easy-axis and associated ordering. Quantum spin-1/2’s defy this fate: rather than spins becoming locally anisotropic, the spin-spin interactions do. Consequently interactions become dependent on the spatial orientation of bonds between spins, prime theoretical examples of which are Kitaev magnets. Bond-directional interactions imply the existence of bond-directional magnetic modes, spin excitations that render crystallographically equivalent bonds magnetically inequivalent, which yet have remained elusive experimentally. Here we show that resonant inelastic X-ray scattering allows us to explicitly probe the bond-directional character of magnetic excitations. To do so, we use a scattering plane spanned by one bond and the corresponding spin component and scan a range of momentum transfer that encompasses multiple Brillouin zones. Applying this approach to Na2IrO3 we establish the different bond-directional characters of magnetic excitations at textasciitilde10 meV and textasciitilde45 meV. The bond-directional nearest-neighbor excitations are a fingerprint of the dominant Kitaev interactions and even prevail in the magnetically ordered state. |  |
Zhang, Y. -S.; Isobe, M.; Takagi, H.; Huang, D. Electronic tuning of the soft-phonon transport anomaly in Ta2Ni(SxSe1-x)5 Journal Article Phys. Rev. Lett. 137, 106503 (2026), datadoi: 10.5281/zenodo.21493304. @article{l5xq-2yrt,
title = {Electronic tuning of the soft-phonon transport anomaly in Ta_{2}Ni(S_{x}Se_{1-x})_{5}},
author = {Y. -S. Zhang and M. Isobe and H. Takagi and D. Huang},
url = {https://link.aps.org/doi/10.1103/l5xq-2yrt
https://doi.org/10.5281/zenodo.21493304},
doi = {10.1103/l5xq-2yrt},
year = {2026},
date = {2026-09-02},
urldate = {2026-09-02},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {10},
pages = {106503},
abstract = {Ta2NiSe5 continues to be investigated for its phase transition at 𝑇c=326 K, where it develops both an electronic gap and a distortion of its Ta/Ni chains. One intriguing feature at 𝑇c seen in thermal transport is the giant anisotropic scattering of phonons moving perpendicular to the chains, which is apparently associated with the softening of a transverse acoustic phonon, but whose microscopic origin and significance demand clarification. By tuning the normal-state band overlap or gap with S substitution, we uncover a close connection between this soft-phonon transport anomaly and underlying electronic instabilities: when Ta2Ni(S𝑥Se1−𝑥)5 approaches a band insulator at high 𝑥, and signatures of the electronic transition are suppressed, the soft-phonon transport anomaly concomitantly vanishes. Our results establish the following picture for the Ta2Ni(S𝑥Se1−𝑥)5 family: near the S end, a sole lattice instability gives rise to a weak structural transition with 𝑇c approaching 130 K. Near the Se end, additional electronic instabilities boost 𝑇c up to 326 K and amplify experimental signatures of the transition. The strong interaction between electrons, holes, and the lattice is manifested as a soft-phonon transport anomaly accompanied by electronic fluctuations, which include excitonic and hybridization-gap fluctuations.},
note = {datadoi: 10.5281/zenodo.21493304},
keywords = {A3},
pubstate = {published},
tppubtype = {article}
}
Ta2NiSe5 continues to be investigated for its phase transition at 𝑇c=326 K, where it develops both an electronic gap and a distortion of its Ta/Ni chains. One intriguing feature at 𝑇c seen in thermal transport is the giant anisotropic scattering of phonons moving perpendicular to the chains, which is apparently associated with the softening of a transverse acoustic phonon, but whose microscopic origin and significance demand clarification. By tuning the normal-state band overlap or gap with S substitution, we uncover a close connection between this soft-phonon transport anomaly and underlying electronic instabilities: when Ta2Ni(S𝑥Se1−𝑥)5 approaches a band insulator at high 𝑥, and signatures of the electronic transition are suppressed, the soft-phonon transport anomaly concomitantly vanishes. Our results establish the following picture for the Ta2Ni(S𝑥Se1−𝑥)5 family: near the S end, a sole lattice instability gives rise to a weak structural transition with 𝑇c approaching 130 K. Near the Se end, additional electronic instabilities boost 𝑇c up to 326 K and amplify experimental signatures of the transition. The strong interaction between electrons, holes, and the lattice is manifested as a soft-phonon transport anomaly accompanied by electronic fluctuations, which include excitonic and hybridization-gap fluctuations. |  |
Lao, H.; Kronseder, M.; Yuan, Z.; Narr, T.; Meier, T. N. G.; Mundigl, N.; Qu, X.; Wang, Z.; Back, C. H.; Chen, L. Alloying‐controlled tuning of interfacial spin‐orbit interaction and magnetic damping in crystalline FeCo thin films grown on GaAs(001) Journal Article Adv. Mater. (2026). @article{laoAlloyingcontrolledTuningInterfacial2026,
title = {Alloying‐controlled tuning of interfacial spin‐orbit interaction and magnetic damping in crystalline FeCo thin films grown on GaAs(001)},
author = {H. Lao and M. Kronseder and Z. Yuan and T. Narr and T. N. G. Meier and N. Mundigl and X. Qu and Z. Wang and C. H. Back and L. Chen},
url = {http://dx.doi.org/10.1002/adma.74841},
doi = {10.1002/adma.74841},
issn = {1521-4095},
year = {2026},
date = {2026-08-28},
urldate = {2026-08-01},
journal = {Adv. Mater.},
publisher = {Wiley},
abstract = {The discovery of intrinsic spin–orbit fields in non-centrosymmetric ferromagnets have attracted considerable interest for both fundamental studies and technological applications. However, once such materials are synthesized, the strength of the spin-orbit fields is difficult to tune because it is primarily a bulk property. Here, we demonstrate that the interfacial spin-orbit interaction (SOI) in single-crystalline Fe1−xCox thin films grown on GaAs(001) can be continuously tuned via alloying. Using spin-orbit ferromagnetic resonance, we find that the Landé g-factor, the Gilbert damping α, and the interfacial spin-orbit fields exhibit a common nonmonotonic dependence on Co concentration. A pronounced minimum occurs near x ≈ 0.2 where an ultra-low damping α ≈ 0.0015 is achieved. Furthermore, we observe linear scaling between α and (g − 2)2, suggesting that interfacial SOI may also contribute to magnetic relaxation. These results identify alloying as an effective knob to engineer interfacial SOI and damping in single crystalline ferromagnet/semiconductor heterostructures.},
keywords = {A2},
pubstate = {published},
tppubtype = {article}
}
The discovery of intrinsic spin–orbit fields in non-centrosymmetric ferromagnets have attracted considerable interest for both fundamental studies and technological applications. However, once such materials are synthesized, the strength of the spin-orbit fields is difficult to tune because it is primarily a bulk property. Here, we demonstrate that the interfacial spin-orbit interaction (SOI) in single-crystalline Fe1−xCox thin films grown on GaAs(001) can be continuously tuned via alloying. Using spin-orbit ferromagnetic resonance, we find that the Landé g-factor, the Gilbert damping α, and the interfacial spin-orbit fields exhibit a common nonmonotonic dependence on Co concentration. A pronounced minimum occurs near x ≈ 0.2 where an ultra-low damping α ≈ 0.0015 is achieved. Furthermore, we observe linear scaling between α and (g − 2)2, suggesting that interfacial SOI may also contribute to magnetic relaxation. These results identify alloying as an effective knob to engineer interfacial SOI and damping in single crystalline ferromagnet/semiconductor heterostructures. |  |
Salgado-Linares, I.; Mook, A.; Mangeolle, L.; Knolle, J. Thermal Hall conductivity from semiclassical spin dynamics simulations: Implementation and applications to chiral ferromagnets and Kitaev magnets Journal Article Phys. Rev. B 114, 125123 (2026). @article{salgado-linaresThermalHallConductivity2026,
title = {Thermal Hall conductivity from semiclassical spin dynamics simulations: Implementation and applications to chiral ferromagnets and Kitaev magnets},
author = {I. Salgado-Linares and A. Mook and L. Mangeolle and J. Knolle},
url = {https://link.aps.org/doi/10.1103/b1r9-1l3f},
doi = {10.1103/b1r9-1l3f},
year = {2026},
date = {2026-08-21},
urldate = {2026-08-21},
journal = {Phys. Rev. B},
volume = {114},
number = {12},
pages = {125123},
publisher = {American Physical Society},
abstract = {We investigate thermal Hall transport in magnetic systems, using semiclassical spin dynamics simulations. Building on a linear response framework, we discuss the intricacies of computing the thermal Hall conductivity from real-time energy current correlations and the energy magnetization. We then apply this methodology to two models: a square-lattice chiral magnet with in-plane Dzyaloshinskii-Moriya interaction, and the antiferromagnetic Kitaev model in a field. Our results demonstrate the efficiency of semiclassical spin dynamics to study thermal Hall transport capturing quantitative effects beyond the simple intrinsic noninteracting approximation. They can serve as a benchmark for comparison with experiments in regimes where nonlinearities from magnon-magnon interactions and strong thermal fluctuations play a crucial role.},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
We investigate thermal Hall transport in magnetic systems, using semiclassical spin dynamics simulations. Building on a linear response framework, we discuss the intricacies of computing the thermal Hall conductivity from real-time energy current correlations and the energy magnetization. We then apply this methodology to two models: a square-lattice chiral magnet with in-plane Dzyaloshinskii-Moriya interaction, and the antiferromagnetic Kitaev model in a field. Our results demonstrate the efficiency of semiclassical spin dynamics to study thermal Hall transport capturing quantitative effects beyond the simple intrinsic noninteracting approximation. They can serve as a benchmark for comparison with experiments in regimes where nonlinearities from magnon-magnon interactions and strong thermal fluctuations play a crucial role. |  |
Sun, X.; Le, Y.; Naus, S.; Tsai, R. B. -S.; Picard, L. R. B.; Murciano, S.; Knap, M.; Alicea, J.; Endres, M. Observation of conformal field theory spectra in a quantum simulator Journal Article Nature 657, 98–106 (2026). @article{sunObservationConformalField2026,
title = {Observation of conformal field theory spectra in a quantum simulator},
author = {X. Sun and Y. Le and S. Naus and R. B. -S. Tsai and L. R. B. Picard and S. Murciano and M. Knap and J. Alicea and M. Endres},
url = {https://doi.org/10.1038/s41586-026-10904-x},
doi = {10.1038/s41586-026-10904-x},
issn = {1476-4687},
year = {2026},
date = {2026-08-19},
urldate = {2026-08-01},
journal = {Nature},
volume = {657},
number = {8130},
pages = {98–106},
publisher = {Springer Science and Business Media LLC},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Fazlizhanov, I.; Seidov, Z. Y.; von Nidda, H. -A. Krug; Krellner, C.; Klingner, C.; Pedrero, L.; Lausberg, S.; Brando, M.; Geibel, C.; Steglich, F.; Sichelschmidt, J. Evolution of low-temperature electron spin resonance in Y(Rh0.73Co0.27)2Si2 upon entering ferromagnetic order Journal Article Phys. Rev. B 114, 115117 (2026). @article{fazlizhanovEvolutionLowtemperatureElectron2026,
title = {Evolution of low-temperature electron spin resonance in Y(Rh_{0.73}Co_{0.27})_{2}Si_{2} upon entering ferromagnetic order},
author = {I. Fazlizhanov and Z. Y. Seidov and H. -A. Krug von Nidda and C. Krellner and C. Klingner and L. Pedrero and S. Lausberg and M. Brando and C. Geibel and F. Steglich and J. Sichelschmidt},
url = {https://link.aps.org/doi/10.1103/csyd-6npb},
doi = {10.1103/csyd-6npb},
year = {2026},
date = {2026-08-17},
urldate = {2026-08-01},
journal = {Phys. Rev. B},
volume = {114},
number = {11},
pages = {115117},
publisher = {American Physical Society},
abstract = {We report electron spin resonance (ESR) experiments conducted on oriented powder of the heavy-fermion ferromagnet Yb(Rh0.73Co0.27)2Si2 in the temperature range 0.75≤𝑇≤4K, which includes the transition between the paramagnetic and ferromagnetic ordered phases below the Curie temperature 𝑇C=1.3K. The ESR measurements were performed using a home-built 3He cryostat at 𝑋-band frequencies. In the ferromagnetic ordered phase the ESR spectra of Yb(Rh0.73Co0.27)2Si2 are split into two lines. While the resonance in the paramagnetic phase features an easy-plane crystalline electric field induced anisotropy of the 𝑔 tensor perpendicular to the 𝑐 axis of the tetragonal crystal structure, the split lines in the ordered phase can be related to ferromagnetic resonance modes with a uniaxial exchange-type anisotropy along the 𝑐 axis. The corresponding effective anisotropy field can be determined.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
We report electron spin resonance (ESR) experiments conducted on oriented powder of the heavy-fermion ferromagnet Yb(Rh0.73Co0.27)2Si2 in the temperature range 0.75≤𝑇≤4K, which includes the transition between the paramagnetic and ferromagnetic ordered phases below the Curie temperature 𝑇C=1.3K. The ESR measurements were performed using a home-built 3He cryostat at 𝑋-band frequencies. In the ferromagnetic ordered phase the ESR spectra of Yb(Rh0.73Co0.27)2Si2 are split into two lines. While the resonance in the paramagnetic phase features an easy-plane crystalline electric field induced anisotropy of the 𝑔 tensor perpendicular to the 𝑐 axis of the tetragonal crystal structure, the split lines in the ordered phase can be related to ferromagnetic resonance modes with a uniaxial exchange-type anisotropy along the 𝑐 axis. The corresponding effective anisotropy field can be determined. |  |
Yue, X.; Pichler, F.; Knap, M.; Stern, A. Electromagnetic Response of a Half-Filled Chern Band near Topological Criticality Journal Article Phys. Rev. Lett. 137, (2026). @article{yueElectromagneticResponseHalfFilled2026,
title = {Electromagnetic Response of a Half-Filled Chern Band near Topological Criticality},
author = {X. Yue and F. Pichler and M. Knap and A. Stern},
url = {https://doi.org/10.1103/v44d-7jr4},
doi = {10.1103/v44d-7jr4},
issn = {1079-7114},
year = {2026},
date = {2026-08-14},
urldate = {2026-08-01},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {7},
publisher = {American Physical Society (APS)},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Sebastian, S. J.; Islam, S. S.; Kolay, R.; Mohanty, S.; Ding, Q. -P.; Skourski, Y.; Sichelschmidt, J.; Baenitz, M.; Krieger, J. A.; Hicken, T. J.; Luetkens, H.; Tsirlin, A. A.; Furukawa, Y.; Nath, R. Dynamic spin fluctuations in the S = ⁵⁄₂ tetratrillium lattice antiferromagnet KBaFe2(PO4)3 Journal Article Phys. Rev. B 114, L080403 (2026). @article{xcr2-rxv6,
title = {Dynamic spin fluctuations in the S = ⁵⁄₂ tetratrillium lattice antiferromagnet KBaFe_{2}(PO_{4})_{3}},
author = {S. J. Sebastian and S. S. Islam and R. Kolay and S. Mohanty and Q. -P. Ding and Y. Skourski and J. Sichelschmidt and M. Baenitz and J. A. Krieger and T. J. Hicken and H. Luetkens and A. A. Tsirlin and Y. Furukawa and R. Nath},
url = {https://link.aps.org/doi/10.1103/xcr2-rxv6},
doi = {10.1103/xcr2-rxv6},
year = {2026},
date = {2026-08-11},
urldate = {2026-08-01},
journal = {Phys. Rev. B},
volume = {114},
number = {8},
pages = {L080403},
abstract = {The three-dimensional (3D) magnet KBaFe2(PO4)3 hosts an effective tetratrillium spin lattice of Fe3+ (𝑆=5/2) ions, offering a prototypical platform to study frustration-driven phenomena in 3D. Through magnetization, specific heat, 31P nuclear magnetic resonance (NMR), and muon spin relaxation (µSR) experiments, supported by first-principles calculations, we uncover an unconventional ground state. Despite strong antiferromagnetic interactions with a large Curie-Weiss temperature 𝜃CW=−70(2)K, no magnetic long-range order is observed down to 30 mK. Below 𝑇*≃3.5K, the NMR linewidth becomes nearly field independent and the spin-spin relaxation rate 1/𝑇2 saturates, accompanied by a two-component relaxation in the transverse nuclear magnetization 𝑀𝑥𝑦. The latter indicates the emergence of short-range dynamical correlations, which was further corroborated by a robust and field-insensitive broad maximum in specific heat. In µSR, we detect neither a static internal field nor spin freezing; instead, the spins remain dynamic down to 30 mK and the asymmetry curves are best described by two coexisting dynamic relaxation channels: a dominant fast (sporadic) channel and a slower Markovian component. Their differing weights and fluctuation rates suggest microscopic inhomogeneity in spin dynamics. These persistent low-temperature spin fluctuations are found to be intrinsic to the 3D frustrated tetratrillium geometry, exemplifying KBaFe2(PO4)3, a rare 3D antiferromagnet with a classical spin that fosters unconventional dynamics.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
The three-dimensional (3D) magnet KBaFe2(PO4)3 hosts an effective tetratrillium spin lattice of Fe3+ (𝑆=5/2) ions, offering a prototypical platform to study frustration-driven phenomena in 3D. Through magnetization, specific heat, 31P nuclear magnetic resonance (NMR), and muon spin relaxation (µSR) experiments, supported by first-principles calculations, we uncover an unconventional ground state. Despite strong antiferromagnetic interactions with a large Curie-Weiss temperature 𝜃CW=−70(2)K, no magnetic long-range order is observed down to 30 mK. Below 𝑇*≃3.5K, the NMR linewidth becomes nearly field independent and the spin-spin relaxation rate 1/𝑇2 saturates, accompanied by a two-component relaxation in the transverse nuclear magnetization 𝑀𝑥𝑦. The latter indicates the emergence of short-range dynamical correlations, which was further corroborated by a robust and field-insensitive broad maximum in specific heat. In µSR, we detect neither a static internal field nor spin freezing; instead, the spins remain dynamic down to 30 mK and the asymmetry curves are best described by two coexisting dynamic relaxation channels: a dominant fast (sporadic) channel and a slower Markovian component. Their differing weights and fluctuation rates suggest microscopic inhomogeneity in spin dynamics. These persistent low-temperature spin fluctuations are found to be intrinsic to the 3D frustrated tetratrillium geometry, exemplifying KBaFe2(PO4)3, a rare 3D antiferromagnet with a classical spin that fosters unconventional dynamics. |  |
Belbase, B. P.; Unnikrishnan, A.; Feng, S.; Choi, E. S.; Knolle, J.; Banerjee, A. Finite spinon density of states in triangular lattice delafossite TlYbSe2 Journal Article Phys. Rev. Res. 8, L032021 (2026), datadoi: 10.5281/zenodo.21481296. @article{belbaseFiniteSpinonDensity2026,
title = {Finite spinon density of states in triangular lattice delafossite TlYbSe_{2}},
author = {B. P. Belbase and A. Unnikrishnan and S. Feng and E. S. Choi and J. Knolle and A. Banerjee},
url = {https://link.aps.org/doi/10.1103/tc4h-cq9c},
doi = {10.1103/tc4h-cq9c},
year = {2026},
date = {2026-08-11},
urldate = {2026-08-01},
journal = {Phys. Rev. Res.},
volume = {8},
number = {3},
pages = {L032021},
publisher = {American Physical Society},
abstract = {We introduce the rare-earth delafossite compound TlYbSe2 — extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the dc magnetization suggests magnetic exchange interactions on the order of several kelvin, the zero-field ac magnetization and heat capacity measurements reveal no signs of long-range magnetic order down to 20 mK, indicating a quantum-disordered ground state. We observe a spin-freezing transition near ∼30mK at zero field that is suppressed by an applied magnetic field of ∼0.02T. A broad anomaly in the heat capacity measurements between 2 and 5 K is indicative of short-range spin correlations. Below 350 mK, we observe a robust linear temperature dependence of the heat capacity, accompanied by the complete absence of long-range order at low fields. We propose that a phenomenological theory, based on the interplay between spinons and thermally excited gauge flux excitations, can account for the linear temperature dependence of the heat capacity, and could be widely applicable to similar critical quantum spin liquid candidate materials. The results establish the low-temperature, low-field regime of TlYbSe2 as a prime candidate for field-tunable triangular quantum spin liquid behavior and highlight the importance of thermally excited gauge field excitations.},
note = {datadoi: 10.5281/zenodo.21481296},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
We introduce the rare-earth delafossite compound TlYbSe2 — extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the dc magnetization suggests magnetic exchange interactions on the order of several kelvin, the zero-field ac magnetization and heat capacity measurements reveal no signs of long-range magnetic order down to 20 mK, indicating a quantum-disordered ground state. We observe a spin-freezing transition near ∼30mK at zero field that is suppressed by an applied magnetic field of ∼0.02T. A broad anomaly in the heat capacity measurements between 2 and 5 K is indicative of short-range spin correlations. Below 350 mK, we observe a robust linear temperature dependence of the heat capacity, accompanied by the complete absence of long-range order at low fields. We propose that a phenomenological theory, based on the interplay between spinons and thermally excited gauge flux excitations, can account for the linear temperature dependence of the heat capacity, and could be widely applicable to similar critical quantum spin liquid candidate materials. The results establish the low-temperature, low-field regime of TlYbSe2 as a prime candidate for field-tunable triangular quantum spin liquid behavior and highlight the importance of thermally excited gauge field excitations. |  |
Leeb, V.; Knolle, J. Collinear p-Wave Magnetism and Hidden Orbital Ferrimagnetism Journal Article Phys. Rev. Lett. 137, 106701 (2026), datadoi: 10.5281/zenodo.18456373. @article{leebCollinearpWaveMagnetism2026,
title = {Collinear p-Wave Magnetism and Hidden Orbital Ferrimagnetism},
author = {V. Leeb and J. Knolle},
url = {https://link.aps.org/doi/10.1103/ydjj-6r9l},
doi = {10.1103/ydjj-6r9l},
year = {2026},
date = {2026-08-01},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {10},
pages = {106701},
publisher = {American Physical Society},
abstract = {In the absence of spin-orbit coupling, collinear magnets are classified as even-wave magnets, i.e., either ferromagnets, antiferromagnets, or altermagnets. It is based on the belief that collinear magnets always feature an inversion-symmetric band structure, which forbids odd-parity magnetism. Here, we show that collinear magnets, which break time-reversal symmetry in the nonmagnetic sector, e.g., through loop currents, can have an inversion-symmetry-broken band structure and lead to unconventional types of collinear magnets. Hence, collinear odd-parity magnets do exist, and we explain that a magnetic field-induced Edelstein effect is their unique signature. We propose minimal models based on the coexistence of antiferromagnet order with compensated loop current orders for all types of collinear magnets. Our Letter provides a new perspective on collinear magnets and the spin-space group classification.},
note = {datadoi: 10.5281/zenodo.18456373},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
In the absence of spin-orbit coupling, collinear magnets are classified as even-wave magnets, i.e., either ferromagnets, antiferromagnets, or altermagnets. It is based on the belief that collinear magnets always feature an inversion-symmetric band structure, which forbids odd-parity magnetism. Here, we show that collinear magnets, which break time-reversal symmetry in the nonmagnetic sector, e.g., through loop currents, can have an inversion-symmetry-broken band structure and lead to unconventional types of collinear magnets. Hence, collinear odd-parity magnets do exist, and we explain that a magnetic field-induced Edelstein effect is their unique signature. We propose minimal models based on the coexistence of antiferromagnet order with compensated loop current orders for all types of collinear magnets. Our Letter provides a new perspective on collinear magnets and the spin-space group classification. | |
Gippius, A. A.; Zhurenko, S. V.; Tkachev, A. V.; Gunbin, A. V.; Büttgen, N.; Schaedler, M.; Silkin, I. G.; Morozov, I. V.; Bogach, A. V.; Sobolev, A. V.; Presniakov, I. A.; Moskvin, A. S. Short-range helical magnetic order in FeP1-xAsx (x = 0.33 and 0.5) Journal Article J. Magn. Magn. Mater. 651, 174177 (2026). @article{GIPPIUS2026174177,
title = {Short-range helical magnetic order in FeP_{1-x}As_{x} (x = 0.33 and 0.5)},
author = {A. A. Gippius and S. V. Zhurenko and A. V. Tkachev and A. V. Gunbin and N. Büttgen and M. Schaedler and I. G. Silkin and I. V. Morozov and A. V. Bogach and A. V. Sobolev and I. A. Presniakov and A. S. Moskvin},
url = {https://www.sciencedirect.com/science/article/pii/S0304885326003689},
doi = {10.1016/j.jmmm.2026.174177},
year = {2026},
date = {2026-08-01},
urldate = {2026-08-01},
journal = {J. Magn. Magn. Mater.},
volume = {651},
pages = {174177},
abstract = {Although the FeP1-xAsx solid solution compounds are isostructural with the binary helimagnets FeP and FeAs with MnP-type structure (sp. gr. Pnma) of the B31 family, their magnetic structure remained unclear. We studied two members of this family (x = 0.33 and 0.5) via microscopic site-selective techniques such as Mössbauer and NMR spectroscopy. Our results indicate that the helimagnetic nature of the ground state is preserved, but undergoes significant modifications. In particular, its ordering range seems to become drastically shorter, so that the local fields on the non-magnetic phosphorus atoms decrease several times compared to those in FeP, and even local fields on iron slightly decrease compared to FeP and FeAs. The ordering temperature for these fragmented structures is suppressed down to 20–30 K, which is significantly lower than the TN values for FeP and FeAs. Additionally, both compounds demonstrate higher sustainability to the external field than the parent compound FeP.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
Although the FeP1-xAsx solid solution compounds are isostructural with the binary helimagnets FeP and FeAs with MnP-type structure (sp. gr. Pnma) of the B31 family, their magnetic structure remained unclear. We studied two members of this family (x = 0.33 and 0.5) via microscopic site-selective techniques such as Mössbauer and NMR spectroscopy. Our results indicate that the helimagnetic nature of the ground state is preserved, but undergoes significant modifications. In particular, its ordering range seems to become drastically shorter, so that the local fields on the non-magnetic phosphorus atoms decrease several times compared to those in FeP, and even local fields on iron slightly decrease compared to FeP and FeAs. The ordering temperature for these fragmented structures is suppressed down to 20–30 K, which is significantly lower than the TN values for FeP and FeAs. Additionally, both compounds demonstrate higher sustainability to the external field than the parent compound FeP. |  |
Chmeruk, A.; Jones, D.; Dwadasi, R.; Ebad-Allah, J.; Beiuşeanu, F.; Schilberth, F.; Kassem, M. A.; Schade, U.; Veber, A.; Puskar, L.; Tabata, Y.; Waki, T.; Nakamura, H.; Kuntscher, C. A.; Östlin, A.; Chioncel, L. Suppression of magnetism in Co3Sn2S2 under external pressure Journal Article Phys. Rev. B 114, 024423 (2026). @article{chmerukSuppressionMagnetismCo3Sn2S22025,
title = {Suppression of magnetism in Co_{3}Sn_{2}S_{2} under external pressure},
author = {A. Chmeruk and D. Jones and R. Dwadasi and J. Ebad-Allah and F. Beiuşeanu and F. Schilberth and M. A. Kassem and U. Schade and A. Veber and L. Puskar and Y. Tabata and T. Waki and H. Nakamura and C. A. Kuntscher and A. Östlin and L. Chioncel},
url = {https://link.aps.org/doi/10.1103/v623-m3y4},
doi = {10.1103/v623-m3y4},
year = {2026},
date = {2026-07-28},
urldate = {2026-07-28},
journal = {Phys. Rev. B},
volume = {114},
number = {2},
pages = {024423},
abstract = {The ability to control the magnetic state provides a powerful means to tune the underlying band topology, enabling transitions between distinct electronic phases and the emergence of novel quantum phenomena. In this work, we address the evolution of the ferromagnetic state in Co3Sn2S2 upon applying external pressures up to 10.8 GPa using a combined experimental and theoretical study. The standard ab initio density functional theory computation, including ionic relaxations grossly overestimates the unit cell magnetization as a function of pressure. In our theoretical analysis we identify two possible mechanisms to remedy this shortcoming. Matching the experimental observations is achieved by a symmetry-preserving adjustment of the sulfur atom positions within the unit cell. Alternatively, we explore various combinations of the exchange and correlation parts of the effective potential that reproduce the experimental magnetization, the structural parameters and the measured optical conductivity spectra. Thus, the pressure-dependent behavior of the magnetization demands a careful theoretical treatment and analysis of both theoretical and experimental data.},
keywords = {A1, A5},
pubstate = {published},
tppubtype = {article}
}
The ability to control the magnetic state provides a powerful means to tune the underlying band topology, enabling transitions between distinct electronic phases and the emergence of novel quantum phenomena. In this work, we address the evolution of the ferromagnetic state in Co3Sn2S2 upon applying external pressures up to 10.8 GPa using a combined experimental and theoretical study. The standard ab initio density functional theory computation, including ionic relaxations grossly overestimates the unit cell magnetization as a function of pressure. In our theoretical analysis we identify two possible mechanisms to remedy this shortcoming. Matching the experimental observations is achieved by a symmetry-preserving adjustment of the sulfur atom positions within the unit cell. Alternatively, we explore various combinations of the exchange and correlation parts of the effective potential that reproduce the experimental magnetization, the structural parameters and the measured optical conductivity spectra. Thus, the pressure-dependent behavior of the magnetization demands a careful theoretical treatment and analysis of both theoretical and experimental data. |  |
Lanzini, L.; Das, P.; Knap, M. Theory of Angle Resolved Photoemission Spectroscopy of Altermagnetic Mott Insulators Journal Article Phys. Rev. Lett. 137, (2026), datadoi: 10.5281/zenodo.15553362. @article{lanziniTheoryAngleResolved2026,
title = {Theory of Angle Resolved Photoemission Spectroscopy of Altermagnetic Mott Insulators},
author = {L. Lanzini and P. Das and M. Knap},
url = {https://doi.org/10.1103/1d1n-cssv},
doi = {10.1103/1d1n-cssv},
issn = {1079-7114},
year = {2026},
date = {2026-07-28},
urldate = {2026-07-01},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {5},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.15553362},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Hollricher, M.; Bauer, A.; Maximov, L.; Feenstra, L.; Pfleiderer, C.; Wilde, M. A. Cyclotron mass-selective de Haas–van Alphen measurements using temperature modulation Journal Article Appl. Phys. Lett. 129, 041902 (2026). @article{hollricherCyclotronMassselectiveHaas2026,
title = {Cyclotron mass-selective de Haas–van Alphen measurements using temperature modulation},
author = {M. Hollricher and A. Bauer and L. Maximov and L. Feenstra and C. Pfleiderer and M. A. Wilde},
url = {https://doi.org/10.1063/5.0334928},
doi = {10.1063/5.0334928},
issn = {0003-6951},
year = {2026},
date = {2026-07-27},
urldate = {2026-07-27},
journal = {Appl. Phys. Lett.},
volume = {129},
number = {4},
pages = {041902},
abstract = {We present a temperature-modulated de Haas–van Alphen measurement technique that allows selective addressing of quantum oscillations with different effective masses m∗ using a non-monotonic amplitude evolution with temperature and magnetic field, governed by the temperature derivative of the Lifshitz–Kosevich factor. The technique relies on harmonic modulation of the sample temperature and phase-sensitive detection of quantum oscillations in the voltage induced in a pickup coil. We use a set of frequencies with strong Zeeman-driven harmonic content in the compensated topological semimetal MoSi2 as a natural linear mass comb ranging from 1 m∗ to 13 m∗ to demonstrate the tunability of the mass-dependent quantum oscillation amplitudes experimentally. The technique allows us to reliably isolate weak contributions of heavy orbits that are inaccessible in conventional de Haas–van Alphen frequency spectra because their frequency peaks overlap with much stronger frequency peaks of lighter orbits.},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
We present a temperature-modulated de Haas–van Alphen measurement technique that allows selective addressing of quantum oscillations with different effective masses m∗ using a non-monotonic amplitude evolution with temperature and magnetic field, governed by the temperature derivative of the Lifshitz–Kosevich factor. The technique relies on harmonic modulation of the sample temperature and phase-sensitive detection of quantum oscillations in the voltage induced in a pickup coil. We use a set of frequencies with strong Zeeman-driven harmonic content in the compensated topological semimetal MoSi2 as a natural linear mass comb ranging from 1 m∗ to 13 m∗ to demonstrate the tunability of the mass-dependent quantum oscillation amplitudes experimentally. The technique allows us to reliably isolate weak contributions of heavy orbits that are inaccessible in conventional de Haas–van Alphen frequency spectra because their frequency peaks overlap with much stronger frequency peaks of lighter orbits. |  |
Feng, S.; Zhu, P.; Knolle, J.; Knap, M. Transient localization from fractionalization: Vanishingly small energy transport in gapless quantum magnets Journal Article Phys. Rev. B 114, 034423 (2026), datadoi: 10.5281/zenodo.17151126. @article{fengTransientLocalizationFractionalization2026,
title = {Transient localization from fractionalization: Vanishingly small energy transport in gapless quantum magnets},
author = {S. Feng and P. Zhu and J. Knolle and M. Knap},
url = {https://doi.org/10.1103/crq3-l1r3},
doi = {10.1103/crq3-l1r3},
year = {2026},
date = {2026-07-21},
urldate = {2026-07-21},
journal = {Phys. Rev. B},
volume = {114},
number = {3},
pages = {034423},
abstract = {In this work, we investigate zero-temperature energy transport in a gapless quantum magnet. We find that suppressed energy transport can arise at low frequencies due to transient localization from fractionalization, even in the absence of extrinsic defects or disorder. Concretely, we consider a Kitaev ladder model, whose spin degrees of freedom fractionalize into visons and spinons, in a uniform magnetic field. For moderate magnetic fields, visons are heavy and act as quasistatic disorder that induces transient localization of light spinons even in the translation-invariant model and at zero temperature, which strongly suppresses the residual transport.},
note = {datadoi: 10.5281/zenodo.17151126},
keywords = {B6, C5, C6},
pubstate = {published},
tppubtype = {article}
}
In this work, we investigate zero-temperature energy transport in a gapless quantum magnet. We find that suppressed energy transport can arise at low frequencies due to transient localization from fractionalization, even in the absence of extrinsic defects or disorder. Concretely, we consider a Kitaev ladder model, whose spin degrees of freedom fractionalize into visons and spinons, in a uniform magnetic field. For moderate magnetic fields, visons are heavy and act as quasistatic disorder that induces transient localization of light spinons even in the translation-invariant model and at zero temperature, which strongly suppresses the residual transport. |  |
Ghara, S.; Kinoshita, Y.; Miyake, A.; Ishii, Y.; Prodan, L.; Tsurkan, V.; Skourski, Y.; Wosnitza, J.; Matsuda, Y. H.; Miyahara, S.; Tokunaga, M.; Kézsmárki, I. High-field crossover from linear to nonlinear magnetoelectric effect in Co3O4 Journal Article Phys. Rev. B 114, 024417 (2026), datadoi: 10.5281/zenodo.21078310. @article{gharaHighfieldCrossoverLinear2026,
title = {High-field crossover from linear to nonlinear magnetoelectric effect in Co_{3}O_{4}},
author = {S. Ghara and Y. Kinoshita and A. Miyake and Y. Ishii and L. Prodan and V. Tsurkan and Y. Skourski and J. Wosnitza and Y. H. Matsuda and S. Miyahara and M. Tokunaga and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/j66k-pc7d},
doi = {10.1103/j66k-pc7d},
issn = {2469-9950, 2469-9969},
year = {2026},
date = {2026-07-20},
urldate = {2026-07-20},
journal = {Phys. Rev. B},
volume = {114},
number = {2},
pages = {024417},
abstract = {The 𝐴-site magnetic spinel Co3O4 exhibits a simple Néel-type collinear antiferromagnetic ordering below 𝑇𝑁=30 K, accompanied by a strong linear magnetoelectric effect. Here, we report magnetization and electric polarization measurements on single crystals of Co3O4 up to high magnetic fields. We show that the magnetoelectric polarization undergoes a crossover from linear to nonlinear behavior with increasing magnetic field, followed by complete suppression upon reaching the field-polarized ferromagnetic state, where inversion symmetry is recovered. Our microscopic spin model, reproducing the observed field evolution of the magnetoelectric response, evidences weak anisotropy that is crucial for the effective magnetoelectric control of the antiferromagnetic state [Phys. Rev. Lett. 135, 126704 (2025)].},
note = {datadoi: 10.5281/zenodo.21078310},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
The 𝐴-site magnetic spinel Co3O4 exhibits a simple Néel-type collinear antiferromagnetic ordering below 𝑇𝑁=30 K, accompanied by a strong linear magnetoelectric effect. Here, we report magnetization and electric polarization measurements on single crystals of Co3O4 up to high magnetic fields. We show that the magnetoelectric polarization undergoes a crossover from linear to nonlinear behavior with increasing magnetic field, followed by complete suppression upon reaching the field-polarized ferromagnetic state, where inversion symmetry is recovered. Our microscopic spin model, reproducing the observed field evolution of the magnetoelectric response, evidences weak anisotropy that is crucial for the effective magnetoelectric control of the antiferromagnetic state [Phys. Rev. Lett. 135, 126704 (2025)]. |  |
Opletal, P.; Fikáček, J.; Duverger–Nédellec, E.; Thamizhavel, A.; Hossain, Z.; Tarasenko, R.; Tkáč, V.; Legut, D.; Shen, Bin; Gegenwart, P.; Custers, J. Complex magnetic behavior of the Ce sawtooth chains in CeRhSn2 Journal Article Phys. Rev. B 114, 045118 (2026), datadoi: 10.5281/zenodo.20434110. @article{opletalComplexMagneticBehavior2026,
title = {Complex magnetic behavior of the Ce sawtooth chains in CeRhSn_{2}},
author = {P. Opletal and J. Fikáček and E. Duverger–Nédellec and A. Thamizhavel and Z. Hossain and R. Tarasenko and V. Tkáč and D. Legut and Bin Shen and P. Gegenwart and J. Custers},
url = {https://link.aps.org/doi/10.1103/pkdg-n4yk},
doi = {10.1103/pkdg-n4yk},
year = {2026},
date = {2026-07-17},
urldate = {2026-07-01},
journal = {Phys. Rev. B},
volume = {114},
number = {4},
pages = {045118},
publisher = {American Physical Society},
abstract = {Conflicting reports exist on the ground state of the intermetallic compound CeRhSn2. This can be rooted in the sawtoothlike arrangement of two inequivalent Ce sites in the unit cell, which suggests potential geometric magnetic frustration. To resolve these conflicting reports, we conducted a comprehensive study on high-quality single crystals of CeRhSn2 by means of magnetization (𝑀), specific heat (𝐶p/𝑇), and resistivity (𝜌). The system exhibits strong magnetic anisotropy, confirming the 𝑏 axis as the easy magnetic axis. We establish three successive transitions: an antiferromagnetic order at 𝑇N=3.65K, a first-order ferromagnetic (FM) order at 𝑇C=1.7K and final transition, at 𝑇=1.5K. The transition temperatures are highly field-directional dependent: in a magnetic field, the lowest transition is immediately suppressed while 𝐇∥𝑏 rapidly merges 𝑇C and 𝑇N into a single second-order transition. Conversely, 𝐇∥𝑐 suppresses the FM order and reduces 𝑇N. Additional ab initio calculations affirm the FM ground state of CeRhSn2. The observation of an enhancement of the Sommerfeld coefficient (𝛾=76.5mJ/molK2) may arise from geometric frustration, but it is most consistently attributed to weak Kondo hybridization as frustration cannot be conclusively established through our data.},
note = {datadoi: 10.5281/zenodo.20434110},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
Conflicting reports exist on the ground state of the intermetallic compound CeRhSn2. This can be rooted in the sawtoothlike arrangement of two inequivalent Ce sites in the unit cell, which suggests potential geometric magnetic frustration. To resolve these conflicting reports, we conducted a comprehensive study on high-quality single crystals of CeRhSn2 by means of magnetization (𝑀), specific heat (𝐶p/𝑇), and resistivity (𝜌). The system exhibits strong magnetic anisotropy, confirming the 𝑏 axis as the easy magnetic axis. We establish three successive transitions: an antiferromagnetic order at 𝑇N=3.65K, a first-order ferromagnetic (FM) order at 𝑇C=1.7K and final transition, at 𝑇=1.5K. The transition temperatures are highly field-directional dependent: in a magnetic field, the lowest transition is immediately suppressed while 𝐇∥𝑏 rapidly merges 𝑇C and 𝑇N into a single second-order transition. Conversely, 𝐇∥𝑐 suppresses the FM order and reduces 𝑇N. Additional ab initio calculations affirm the FM ground state of CeRhSn2. The observation of an enhancement of the Sommerfeld coefficient (𝛾=76.5mJ/molK2) may arise from geometric frustration, but it is most consistently attributed to weak Kondo hybridization as frustration cannot be conclusively established through our data. |  |
Boesl, J.; Liu, Y. -J.; Pollmann, F.; Knap, M. Skeleton of Isometric Tensor Network States for Abelian String-Net Models Journal Article Phys. Rev. Lett. 137, (2026), datadoi: 10.5281/zenodo.17427675. @article{boeslSkeletonIsometricTensor2026,
title = {Skeleton of Isometric Tensor Network States for Abelian String-Net Models},
author = {J. Boesl and Y. -J. Liu and F. Pollmann and M. Knap},
url = {https://doi.org/10.1103/d3fz-5755},
doi = {10.1103/d3fz-5755},
issn = {1079-7114},
year = {2026},
date = {2026-07-07},
urldate = {2026-07-01},
journal = {Phys. Rev. Lett.},
volume = {137},
number = {2},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.17427675},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Lamp, M.; Ebad-Allah, J.; Chmeruk, A.; Bura, N.; Schönemann, R.; Balicas, L.; Lee, S. H.; Mao, Z. Q.; Chioncel, L.; Kuntscher, C. A. Charge dynamics in the Weyl semimetals NbIrTe4 and TaIrTe4 under pressure: Signatures of an electronic phase transition Journal Article Phys. Rev. B 114, 065101 (2026), datadoi: 10.5281/zenodo.20604906. @article{lamp:ChargeDynamics2026,
title = {Charge dynamics in the Weyl semimetals NbIrTe_{4} and TaIrTe_{4} under pressure: Signatures of an electronic phase transition},
author = {M. Lamp and J. Ebad-Allah and A. Chmeruk and N. Bura and R. Schönemann and L. Balicas and S. H. Lee and Z. Q. Mao and L. Chioncel and C. A. Kuntscher},
url = {https://link.aps.org/doi/10.1103/pvhn-prsw},
doi = {10.1103/pvhn-prsw},
year = {2026},
date = {2026-07-06},
urldate = {2026-07-01},
journal = {Phys. Rev. B},
volume = {114},
number = {6},
pages = {065101},
abstract = {A high-pressure investigation of the Weyl semimetals NbIrTe4 and TaIrTe4 is presented, using infrared spectroscopy supplemented by density functional theory calculations. The experimental optical conductivity spectra as a function of pressure suggest the occurrence of a pressure-induced phase transition at a critical pressure P_c = 7-8 GPa. This transition is most likely electronic in nature, as Raman scattering measurements provide no evidence of a significant structural phase transition. Above P_c a significant redistribution of spectral weight occurs in the optical conductivity spectrum for both materials. A Drude-Lorentz analysis of the optical data indicates a sharp reduction in the free carrier concentration at P_c, concomitant with the appearance of a low-energy phonon, which was initially screened by free charge carriers. A predominantly electronic origin of the phase transition is supported by the calculated electronic band structure, Fermi surface, and interband optical conductivity as a function of pressure. Our findings provide collective evidence for a pressure-induced, most likely electronic phase transition in both van der Waals materials at P_c=7-8 GPa, highlighting the tunability of their electronic band structure by hydrostatic pressure.},
note = {datadoi: 10.5281/zenodo.20604906},
keywords = {A1, A5},
pubstate = {published},
tppubtype = {article}
}
A high-pressure investigation of the Weyl semimetals NbIrTe4 and TaIrTe4 is presented, using infrared spectroscopy supplemented by density functional theory calculations. The experimental optical conductivity spectra as a function of pressure suggest the occurrence of a pressure-induced phase transition at a critical pressure P_c = 7-8 GPa. This transition is most likely electronic in nature, as Raman scattering measurements provide no evidence of a significant structural phase transition. Above P_c a significant redistribution of spectral weight occurs in the optical conductivity spectrum for both materials. A Drude-Lorentz analysis of the optical data indicates a sharp reduction in the free carrier concentration at P_c, concomitant with the appearance of a low-energy phonon, which was initially screened by free charge carriers. A predominantly electronic origin of the phase transition is supported by the calculated electronic band structure, Fermi surface, and interband optical conductivity as a function of pressure. Our findings provide collective evidence for a pressure-induced, most likely electronic phase transition in both van der Waals materials at P_c=7-8 GPa, highlighting the tunability of their electronic band structure by hydrostatic pressure. |  |
Ojeda-Aristizabal, C.; Zheng, X.; Xu, C.; Nussinov, Z.; Motome, Y.; Banerjee, A.; Tsen, A. W.; Knap, M.; Du, R. -R.; Joshi, G.; Mounce, A.; Kim, Y.; Hunt, B. M; Shcherbakov, D.; Zhou, B.; Jing, R.; Liu, M.; Zhao, H.; Claassen, M.; Erten, O.; Chen, Y. P.; Henriksen, E. A. Lessons from α-RuCl3 for pursuing quantum spin liquid physics in atomically thin materials Journal Article J. Phys. Condens. Matter 38, 263001 (2026). @article{ojeda-aristizabalLessonsARuCl_3Pursuing2026,
title = {Lessons from α-RuCl_{3} for pursuing quantum spin liquid physics in atomically thin materials},
author = {C. Ojeda-Aristizabal and X. Zheng and C. Xu and Z. Nussinov and Y. Motome and A. Banerjee and A. W. Tsen and M. Knap and R. -R. Du and G. Joshi and A. Mounce and Y. Kim and B. M Hunt and D. Shcherbakov and B. Zhou and R. Jing and M. Liu and H. Zhao and M. Claassen and O. Erten and Y. P. Chen and E. A. Henriksen},
url = {https://iopscience.iop.org/article/10.1088/1361-648X/ae7cc8},
doi = {10.1088/1361-648x/ae7cc8},
issn = {1361-648X},
year = {2026},
date = {2026-07-03},
urldate = {2026-07-01},
journal = {J. Phys. Condens. Matter},
volume = {38},
number = {26},
pages = {263001},
publisher = {IOP Publishing},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Breitner, F.; Shen, B.; Jesche, A.; Tsirlin, A. A.; Gegenwart, P. Magnetic and electric properties of the metallic kagome antiferromagnet CrRhAs Journal Article Phys. Rev. Mater. 10, 064204 (2026), datadoi: 10.5281/zenodo.19046826. @article{breitner2026magneticelectricpropertiesmetallic,
title = {Magnetic and electric properties of the metallic kagome antiferromagnet CrRhAs},
author = {F. Breitner and B. Shen and A. Jesche and A. A. Tsirlin and P. Gegenwart},
url = {https://link.aps.org/doi/10.1103/d449-1tfw},
doi = {10.1103/d449-1tfw},
year = {2026},
date = {2026-06-30},
urldate = {2026-06-01},
journal = {Phys. Rev. Mater.},
volume = {10},
number = {6},
pages = {064204},
abstract = {CrRhAs is an antiferromagnetic kagome metal predicted to host a nontrivial spin texture with vector spin chirality [Huang et al., npj Quantum Mater. 8, 32 (2023)]. We report the synthesis and basic characterization of CrRhAs single crystals, which exhibit an antiferromagnetic transition with 𝑇N = 150 K, evidenced by electrical transport, heat capacity, and magnetization measurements. Hall resistivity varies linearly with magnetic field, i.e., there is no nonlinear Hall contribution. Intriguingly, the Hall coefficient changes sign between the configurations of 𝑗∥𝑎𝑏, 𝐻⊥𝑎𝑏 and 𝑗∥𝑐, 𝐻⊥𝑐, which is likely connected to a peculiar topology of the Fermi surface. Furthermore, for 𝑗∥𝑎𝑏, the Hall coefficient shows a pronounced and continuous enhancement below 𝑇N, signaling a significant reconstruction of the Fermi surface or an extra scattering from the magnons. Our results offer guidance for exploring anomalous electrical transport phenomena in exotic magnetic systems.},
note = {datadoi: 10.5281/zenodo.19046826},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
CrRhAs is an antiferromagnetic kagome metal predicted to host a nontrivial spin texture with vector spin chirality [Huang et al., npj Quantum Mater. 8, 32 (2023)]. We report the synthesis and basic characterization of CrRhAs single crystals, which exhibit an antiferromagnetic transition with 𝑇N = 150 K, evidenced by electrical transport, heat capacity, and magnetization measurements. Hall resistivity varies linearly with magnetic field, i.e., there is no nonlinear Hall contribution. Intriguingly, the Hall coefficient changes sign between the configurations of 𝑗∥𝑎𝑏, 𝐻⊥𝑎𝑏 and 𝑗∥𝑐, 𝐻⊥𝑐, which is likely connected to a peculiar topology of the Fermi surface. Furthermore, for 𝑗∥𝑎𝑏, the Hall coefficient shows a pronounced and continuous enhancement below 𝑇N, signaling a significant reconstruction of the Fermi surface or an extra scattering from the magnons. Our results offer guidance for exploring anomalous electrical transport phenomena in exotic magnetic systems. |  |
Bader, T.; Feng, S.; Budaraju, S.; Becca, F.; Knolle, J.; Pollmann, F. Triangular J1-J2 Heisenberg antiferromagnet in a magnetic field Journal Article Phys. Rev. B 113, L241114 (2026), datadoi: 10.5281/zenodo.20510149. @article{baderTriangular$J_1textensuremathJ_2$Heisenberg2026,
title = {Triangular J_{1}-J_{2} Heisenberg antiferromagnet in a magnetic field},
author = {T. Bader and S. Feng and S. Budaraju and F. Becca and J. Knolle and F. Pollmann},
url = {https://link.aps.org/doi/10.1103/rwhz-jf5b},
doi = {10.1103/rwhz-jf5b},
year = {2026},
date = {2026-06-18},
urldate = {2026-06-01},
journal = {Phys. Rev. B},
volume = {113},
number = {24},
pages = {L241114},
publisher = {American Physical Society},
abstract = {The behavior of the paradigmatic 𝐽1−𝐽2 triangular lattice Heisenberg antiferromagnet in a magnetic field remains unsettled despite decades of study. We map out the phase diagram using three complementary approaches, including self-consistent nonlinear spin-wave theory, density-matrix renormalization group, and variational Monte Carlo. This combined analysis resolves the competition among different field-induced magnetic orders and magnetization plateaus across the classically frustrated parameter range. In particular, there is a finite range in the parameter regime around 𝐽2/𝐽1 = 1/8 in which (i) upon the application of the external field, the gapless quantum spin liquid acquires a finite density of monopoles, and (ii) by further increasing the field, two plateaus are clearly obtained at 𝑚=1/3 and 𝑚=1/2. We discuss the experimental importance of the consecutive magnetization plateau transitions as a signature of an underlying quantum spin-liquid phase.},
note = {datadoi: 10.5281/zenodo.20510149},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
The behavior of the paradigmatic 𝐽1−𝐽2 triangular lattice Heisenberg antiferromagnet in a magnetic field remains unsettled despite decades of study. We map out the phase diagram using three complementary approaches, including self-consistent nonlinear spin-wave theory, density-matrix renormalization group, and variational Monte Carlo. This combined analysis resolves the competition among different field-induced magnetic orders and magnetization plateaus across the classically frustrated parameter range. In particular, there is a finite range in the parameter regime around 𝐽2/𝐽1 = 1/8 in which (i) upon the application of the external field, the gapless quantum spin liquid acquires a finite density of monopoles, and (ii) by further increasing the field, two plateaus are clearly obtained at 𝑚=1/3 and 𝑚=1/2. We discuss the experimental importance of the consecutive magnetization plateau transitions as a signature of an underlying quantum spin-liquid phase. |  |
Hemmida, M.; Pakhira, S.; Johnston, D. C.; von Nidda, H. -A. Krug Observation of surface ferromagnons in the axion-insulating phase of the antiferromagnetic topological insulator EuSn2As2 Journal Article Phys. Rev. Research 8, 023309 (2026). @article{dp4g-dyll,
title = {Observation of surface ferromagnons in the axion-insulating phase of the antiferromagnetic topological insulator EuSn_{2}As_{2}},
author = {M. Hemmida and S. Pakhira and D. C. Johnston and H. -A. Krug von Nidda},
url = {https://link.aps.org/doi/10.1103/dp4g-dyll},
doi = {10.1103/dp4g-dyll},
year = {2026},
date = {2026-06-17},
urldate = {2026-06-01},
journal = {Phys. Rev. Research},
volume = {8},
number = {2},
pages = {023309},
abstract = {We report the study of spin dynamics of Eu2+ in the antiferromagnetic axion topological insulator EuSn2As2 by means of antiferromagnetic resonance at 9.34 GHz. Below the Néel temperature (T_N), two types of resonance modes, the conventional bulk antiferromagnetic resonance and additional surface ferromagnetic resonance, are observed. The latter turns out to be characteristic of the axion-insulating phase. Above T_N, we prove the existence of a Kosterlitz-Thouless scenario that is relevant for the spin relaxation in the Eu2+ layers. The absence of Korringa relaxation indicates the strong confinement of the conduction electrons at the Fermi level to the SnAs layers.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
We report the study of spin dynamics of Eu2+ in the antiferromagnetic axion topological insulator EuSn2As2 by means of antiferromagnetic resonance at 9.34 GHz. Below the Néel temperature (T_N), two types of resonance modes, the conventional bulk antiferromagnetic resonance and additional surface ferromagnetic resonance, are observed. The latter turns out to be characteristic of the axion-insulating phase. Above T_N, we prove the existence of a Kosterlitz-Thouless scenario that is relevant for the spin relaxation in the Eu2+ layers. The absence of Korringa relaxation indicates the strong confinement of the conduction electrons at the Fermi level to the SnAs layers. |  |
Koller, E.; Swarup, S.; Knolle, J.; Perkins, N. B. Spin-lattice coupling induced chiral phonons and their signature in Raman Circular Dichroism Journal Article npj Quantum Mater. 11, 57 (2026), datadoi: 10.5281/zenodo.17437560. @article{kollerSpinlatticeCouplingInduced2026,
title = {Spin-lattice coupling induced chiral phonons and their signature in Raman Circular Dichroism},
author = {E. Koller and S. Swarup and J. Knolle and N. B. Perkins},
url = {https://doi.org/10.1038/s41535-026-00893-5},
doi = {10.1038/s41535-026-00893-5},
year = {2026},
date = {2026-06-17},
urldate = {2026-06-01},
journal = {npj Quantum Mater.},
volume = {11},
number = {1},
pages = {57},
note = {datadoi: 10.5281/zenodo.17437560},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
| |
Otsuki, J.; Yoshimi, K.; Nakanishi-Ohno, Y.; Sekania, M.; Chioncel, L.; Mizumaki, M. Compressed Sensing of Compton Profiles for Fermi Surface Reconstruction: Concept and Implementation Journal Article J. Phys. Soc. Jpn. 95, 074707 (2026). @article{otsukiCompressedSensingCompton2026,
title = {Compressed Sensing of Compton Profiles for Fermi Surface Reconstruction: Concept and Implementation},
author = {J. Otsuki and K. Yoshimi and Y. Nakanishi-Ohno and M. Sekania and L. Chioncel and M. Mizumaki},
url = {https://doi.org/10.7566/JPSJ.95.074707},
doi = {10.7566/JPSJ.95.074707},
issn = {0031-9015},
year = {2026},
date = {2026-06-15},
urldate = {2026-07-01},
journal = {J. Phys. Soc. Jpn.},
volume = {95},
number = {7},
pages = {074707},
abstract = {Compton scattering is a well-established technique that can provide detailed information about electronic states in solids. Making use of the principle of tomography, it is possible to determine the Fermi surface from sets of Compton-scattering data with different scattering axes. Practical applications, however, are limited due to the long acquisition time required for measuring along a sufficient number of scattering directions. Here, we propose to overcome this difficulty using compressed sensing. Taking advantage of a hidden sparsity in the momentum distribution, we are able to reconstruct the three-dimensional momentum distribution of bcc-Li, and identify the Fermi surface with as little as 14 directions of scattering data with unprecedented accuracy. This compressed-sensing approach will permit wider applications of the Compton scattering experiments.},
keywords = {A5},
pubstate = {published},
tppubtype = {article}
}
Compton scattering is a well-established technique that can provide detailed information about electronic states in solids. Making use of the principle of tomography, it is possible to determine the Fermi surface from sets of Compton-scattering data with different scattering axes. Practical applications, however, are limited due to the long acquisition time required for measuring along a sufficient number of scattering directions. Here, we propose to overcome this difficulty using compressed sensing. Taking advantage of a hidden sparsity in the momentum distribution, we are able to reconstruct the three-dimensional momentum distribution of bcc-Li, and identify the Fermi surface with as little as 14 directions of scattering data with unprecedented accuracy. This compressed-sensing approach will permit wider applications of the Compton scattering experiments. |  |
Ohanyan, V.; Richter, J.; Sekania, M.; Giambattista, L.; Andreanov, A.; Kollar, M. Flat bands in the J1-J2-J3 XXZ sawtooth chain Journal Article Phys. Rev. B 113, 214418 (2026). @article{ohanyanFlatBandsJ_1J_2J_32026,
title = {Flat bands in the J_{1}-J_{2}-J_{3} XXZ sawtooth chain},
author = {V. Ohanyan and J. Richter and M. Sekania and L. Giambattista and A. Andreanov and M. Kollar},
url = {https://link.aps.org/doi/10.1103/byv6-h2m2},
doi = {10.1103/byv6-h2m2},
year = {2026},
date = {2026-06-04},
urldate = {2026-06-01},
journal = {Phys. Rev. B},
volume = {113},
number = {21},
pages = {214418},
abstract = {We consider a generalization of the XXZ model on the sawtooth spin chain with Dzyaloshinskii-Moriya interactions in which all exchange constants (symmetric, antisymmetric, and axial anisotropy) are different for the three different bonds of each triangle. We derive and resolve algebraic constraints on the exchange constants ensuring the appearance of a flat band in the one-magnon spectrum. The properties of the corresponding flat magnon bands and localized magnon states are analyzed. We further construct the mapping of the flat-band conditions for the Dzyaloshinskii-Moriya constants onto the Katsura-Nagaosa-Balatsky parameters. Based on the mapping, the possibility of the electric-field-driven flat bands with the aid of the magnetoelectric coupling is examined.},
keywords = {C4},
pubstate = {published},
tppubtype = {article}
}
We consider a generalization of the XXZ model on the sawtooth spin chain with Dzyaloshinskii-Moriya interactions in which all exchange constants (symmetric, antisymmetric, and axial anisotropy) are different for the three different bonds of each triangle. We derive and resolve algebraic constraints on the exchange constants ensuring the appearance of a flat band in the one-magnon spectrum. The properties of the corresponding flat magnon bands and localized magnon states are analyzed. We further construct the mapping of the flat-band conditions for the Dzyaloshinskii-Moriya constants onto the Katsura-Nagaosa-Balatsky parameters. Based on the mapping, the possibility of the electric-field-driven flat bands with the aid of the magnetoelectric coupling is examined. |  |
Ishihara, Y.; Nakano, Ryota; Yamada, R.; Nomoto, T.; Baral, P. R.; Hirschmann, M. M.; Gautam, K.; Kolincio, K. K.; Kikkawa, A.; Aji, S.; Saitoh, H.; Matsuda, M.; Taguchi, Y.; Arima, T.; Tokura, Y.; Nakajima, T.; Hirschberger, M. Collinear ferromagnetism with reduced moment length in kagome magnet Nd3Ru4Al12 Journal Article Phys. Rev. B 113, (2026). @article{ishiharaCollinearFerromagnetismReduced2026-06-222026,
title = {Collinear ferromagnetism with reduced moment length in kagome magnet Nd_{3}Ru_{4}Al_{12}},
author = {Y. Ishihara and Ryota Nakano and R. Yamada and T. Nomoto and P. R. Baral and M. M. Hirschmann and K. Gautam and K. K. Kolincio and A. Kikkawa and S. Aji and H. Saitoh and M. Matsuda and Y. Taguchi and T. Arima and Y. Tokura and T. Nakajima and M. Hirschberger},
url = {http://dx.doi.org/10.1103/9pvl-33xc},
doi = {10.1103/9pvl-33xc},
issn = {2469-9969},
year = {2026},
date = {2026-06-02},
urldate = {2026-06-01},
journal = {Phys. Rev. B},
volume = {113},
number = {21},
publisher = {American Physical Society (APS)},
abstract = {We determine the magnetic ground state of the kagome lattice magnet Nd3Ru4Al12 by single-crystal neutron diffraction, supported by experiments with polarized neutrons. We identify this material as a collinear ferromagnet (“hex-FM”) with uniform moment length and ordering vector Q=0, in contrast to a previous, seminal report that proposed unequal moment lengths on two Nd sites, here called the “ortho-FM” state. Our analysis of the flipping ratio in polarized neutron scattering is consistent with the hex-FM state. The results provide a microscopic basis for understanding the large fluctuation-induced Hall and Nernst responses near TC≈41K, as previously reported for Nd3Ru4Al12.},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
We determine the magnetic ground state of the kagome lattice magnet Nd3Ru4Al12 by single-crystal neutron diffraction, supported by experiments with polarized neutrons. We identify this material as a collinear ferromagnet (“hex-FM”) with uniform moment length and ordering vector Q=0, in contrast to a previous, seminal report that proposed unequal moment lengths on two Nd sites, here called the “ortho-FM” state. Our analysis of the flipping ratio in polarized neutron scattering is consistent with the hex-FM state. The results provide a microscopic basis for understanding the large fluctuation-induced Hall and Nernst responses near TC≈41K, as previously reported for Nd3Ru4Al12. |  |
Mangeolle, L.; Knolle, J. Dynamical magnetic breakdown and quantum oscillations from hot-spot scattering Journal Article Phys. Rev. B 113, 245132 (2026). @article{mangeolleDynamicalMagneticBreakdown2026,
title = {Dynamical magnetic breakdown and quantum oscillations from hot-spot scattering},
author = {L. Mangeolle and J. Knolle},
url = {https://link.aps.org/doi/10.1103/ytcj-6zkg},
doi = {10.1103/ytcj-6zkg},
year = {2026},
date = {2026-06-01},
journal = {Phys. Rev. B},
volume = {113},
number = {24},
pages = {245132},
publisher = {American Physical Society},
abstract = {Quantum oscillations (QOs) are a well-established probe of Fermi-surface (FS) geometry and in the presence of long-range density wave order can display new QO frequencies from reconstructed FS pockets. We show that such reconstructed frequencies can arise even in the absence of long-range density order. Considering electrons coupled to a fluctuating bosonic mode that scatters quasiparticles between sharp hot spots on the FS, we develop a semiclassical theory in which the interaction generates time-dependent tunneling processes analogous to magnetic breakdown. This dynamical magnetic breakdown produces new semiclassical orbits corresponding to reconstructed FS areas despite the absence of static order. Because tunneling probabilities depend on the thermal population of bosonic excitations, the resulting oscillation amplitudes exhibit characteristic deviations from standard Lifshitz-Kosevich behavior. Our results provide a mechanism to probe bosonic fluctuations in quantum critical metals and provide a framework for dynamical magnetic breakdown.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Quantum oscillations (QOs) are a well-established probe of Fermi-surface (FS) geometry and in the presence of long-range density wave order can display new QO frequencies from reconstructed FS pockets. We show that such reconstructed frequencies can arise even in the absence of long-range density order. Considering electrons coupled to a fluctuating bosonic mode that scatters quasiparticles between sharp hot spots on the FS, we develop a semiclassical theory in which the interaction generates time-dependent tunneling processes analogous to magnetic breakdown. This dynamical magnetic breakdown produces new semiclassical orbits corresponding to reconstructed FS areas despite the absence of static order. Because tunneling probabilities depend on the thermal population of bosonic excitations, the resulting oscillation amplitudes exhibit characteristic deviations from standard Lifshitz-Kosevich behavior. Our results provide a mechanism to probe bosonic fluctuations in quantum critical metals and provide a framework for dynamical magnetic breakdown. | |
Eto, R.; Salgado-Linares, I.; Mochizuki, M.; Knolle, J.; Mook, A. Fate of Topological Dirac Magnons in van der Waals Ferromagnets at Finite Temperature Journal Article Phys. Rev. X 16, 021053 (2026). @article{etoFateTopologicalDirac2026,
title = {Fate of Topological Dirac Magnons in van der Waals Ferromagnets at Finite Temperature},
author = {R. Eto and I. Salgado-Linares and M. Mochizuki and J. Knolle and A. Mook},
url = {https://link.aps.org/doi/10.1103/tbh2-jq9r},
doi = {10.1103/tbh2-jq9r},
year = {2026},
date = {2026-06-01},
journal = {Phys. Rev. X},
volume = {16},
number = {2},
pages = {021053},
publisher = {American Physical Society},
abstract = {Dirac magnons, the bosonic counterparts of Dirac fermions in graphene, provide a versatile platform to explore symmetry-protected band crossings and quantum geometry in magnetic insulators while promising high-velocity, low-dissipation spin transport for next-generation magnonic technologies. However, their stability under realistic, finite-temperature conditions remains an open question. Here, we develop a microscopic theory of thermal magnon-magnon interactions in van der Waals honeycomb ferromagnets, focusing on both gapless and gapped Dirac magnons. Using nonlinear spin-wave theory with magnon self-energy corrections and a 𝑇-matrix resummation that captures two-magnon bound states, we quantitatively reproduce temperature- and momentum-dependent energy shifts and linewidths observed experimentally in the gapless Dirac magnon material CrBr3, even near the Curie temperature. Our approach provides a consistent interpretation of theoretical predictions and experiment shedding light on the role of bound states in enhancing magnon damping at low temperatures. For gapped Dirac magnon materials such as CrI3, CrSiTe3, and CrGeTe3, we find a thermally induced reduction of the topological magnon gap, while no indication of thermally driven topological phase transitions is observed within the considered parameter range. Classical atomistic spin-dynamics simulations corroborate the gap’s robustness up to the Curie temperature. Furthermore, we establish a practical criterion for observing topological gaps by determining the minimum ratio of Dzyaloshinskii-Moriya interaction to Heisenberg exchange required to overcome thermal broadening throughout the ordered phase, typically around 5%. Taken together, our results elucidate the interplay between thermal many-body effects and topology in low-dimensional magnetic systems and provide a controlled framework for the interpretation of spectroscopic measurements.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Dirac magnons, the bosonic counterparts of Dirac fermions in graphene, provide a versatile platform to explore symmetry-protected band crossings and quantum geometry in magnetic insulators while promising high-velocity, low-dissipation spin transport for next-generation magnonic technologies. However, their stability under realistic, finite-temperature conditions remains an open question. Here, we develop a microscopic theory of thermal magnon-magnon interactions in van der Waals honeycomb ferromagnets, focusing on both gapless and gapped Dirac magnons. Using nonlinear spin-wave theory with magnon self-energy corrections and a 𝑇-matrix resummation that captures two-magnon bound states, we quantitatively reproduce temperature- and momentum-dependent energy shifts and linewidths observed experimentally in the gapless Dirac magnon material CrBr3, even near the Curie temperature. Our approach provides a consistent interpretation of theoretical predictions and experiment shedding light on the role of bound states in enhancing magnon damping at low temperatures. For gapped Dirac magnon materials such as CrI3, CrSiTe3, and CrGeTe3, we find a thermally induced reduction of the topological magnon gap, while no indication of thermally driven topological phase transitions is observed within the considered parameter range. Classical atomistic spin-dynamics simulations corroborate the gap’s robustness up to the Curie temperature. Furthermore, we establish a practical criterion for observing topological gaps by determining the minimum ratio of Dzyaloshinskii-Moriya interaction to Heisenberg exchange required to overcome thermal broadening throughout the ordered phase, typically around 5%. Taken together, our results elucidate the interplay between thermal many-body effects and topology in low-dimensional magnetic systems and provide a controlled framework for the interpretation of spectroscopic measurements. | |
Walther, L.; Willsher, J.; Knolle, J. Persistence of the Berezinskii-Kosterlitz-Thouless Transition with Long-Range Couplings Journal Article Phys. Rev. Lett. 136, 227102 (2026). @article{waltherPersistenceBerezinskiiKosterlitzThoulessTransition2026,
title = {Persistence of the Berezinskii-Kosterlitz-Thouless Transition with Long-Range Couplings},
author = {L. Walther and J. Willsher and J. Knolle},
url = {https://link.aps.org/doi/10.1103/9y2v-ybdb},
doi = {10.1103/9y2v-ybdb},
year = {2026},
date = {2026-06-01},
journal = {Phys. Rev. Lett.},
volume = {136},
number = {22},
pages = {227102},
publisher = {American Physical Society},
abstract = {The Berezinskii-Kosterlitz-Thouless (BKT) transition is an archetypal example of a topological phase transition, which is driven by the proliferation of vortices. In this Letter, we analyze the persistence of the BKT transition in the XY model under the influence of long-range algebraically decaying interactions of the form ∼1/𝑟2+𝜎. The model hosts a magnetized low temperature phase for sufficiently small 𝜎. Crucially, in the presence of long-range interactions, spin waves renormalize the interaction between vortices, which stabilizes the BKT transition. As a result, we find that there is no direct transition from the magnetized to the disordered phase and that the BKT transition persists for arbitrary long-range exponents, which is distinct from previous results. The key methodological advance is the inclusion of coupling between spin wave and topological excitations. We do this by developing Landau-Peierls–type arguments and using higher-order renormalization group calculations, obtaining compatible results. We emphasize that Landau-Peierls–type arguments are a powerful tool for analyzing continuous spin models. We discuss the relevance of our findings for current Rydberg atom experiments, and highlight the importance of long-range couplings for other types of topological defects.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
The Berezinskii-Kosterlitz-Thouless (BKT) transition is an archetypal example of a topological phase transition, which is driven by the proliferation of vortices. In this Letter, we analyze the persistence of the BKT transition in the XY model under the influence of long-range algebraically decaying interactions of the form ∼1/𝑟2+𝜎. The model hosts a magnetized low temperature phase for sufficiently small 𝜎. Crucially, in the presence of long-range interactions, spin waves renormalize the interaction between vortices, which stabilizes the BKT transition. As a result, we find that there is no direct transition from the magnetized to the disordered phase and that the BKT transition persists for arbitrary long-range exponents, which is distinct from previous results. The key methodological advance is the inclusion of coupling between spin wave and topological excitations. We do this by developing Landau-Peierls–type arguments and using higher-order renormalization group calculations, obtaining compatible results. We emphasize that Landau-Peierls–type arguments are a powerful tool for analyzing continuous spin models. We discuss the relevance of our findings for current Rydberg atom experiments, and highlight the importance of long-range couplings for other types of topological defects. | |
Mukharjee, P. K.; Erdmann, S.; Wang, L.; Kaiser, J.; Jesche, A.; Puphal, P.; Isobe, M.; Hepting, M.; Keimer, B.; Gegenwart, P.; Tsirlin, A. A. Anisotropic magnetoelastic coupling in the honeycomb magnet Na3Co2SbO6 Journal Article Phys. Rev. B 113, (2026), datadoi: 10.5281/zenodo.18795732. @article{mukharjee2026anisotropicmagnetoelasticcouplinghoneycomb,
title = {Anisotropic magnetoelastic coupling in the honeycomb magnet Na_{3}Co_{2}SbO_{6}},
author = {P. K. Mukharjee and S. Erdmann and L. Wang and J. Kaiser and A. Jesche and P. Puphal and M. Isobe and M. Hepting and B. Keimer and P. Gegenwart and A. A. Tsirlin},
url = {https://doi.org/10.1103/tn1m-sjdh},
doi = {10.1103/tn1m-sjdh},
year = {2026},
date = {2026-05-26},
urldate = {2026-05-26},
journal = {Phys. Rev. B},
volume = {113},
number = {20},
abstract = {We present magnetization and dilatometry measurements on the honeycomb cobaltate Na3Co2SbO6 and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a strongly anisotropic 𝑐*-axis lattice response, which is dominated by the variation of Co–O–Co bond angles according to ab initio calculations. At 𝑇=0.4K, the magnetization 𝑀(𝐵) exhibits steplike features that are also highly anisotropic. In the case of 𝐵∥𝑏, a small hysteresis observed around the second field-induced magnetic transition (𝐵𝑐2) indicates its first-order character, whereas the apparent divergence of the magnetic Grüneisen parameter at 𝐵𝑐2 is suppressed upon cooling and signals the absence of quantum critical behavior upon entering the field-polarized state. None of our thermodynamic measurements provide evidence for a field-induced quantum spin-liquid state near or above 𝐵𝑐2.},
note = {datadoi: 10.5281/zenodo.18795732},
keywords = {B1, B2},
pubstate = {published},
tppubtype = {article}
}
We present magnetization and dilatometry measurements on the honeycomb cobaltate Na3Co2SbO6 and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a strongly anisotropic 𝑐*-axis lattice response, which is dominated by the variation of Co–O–Co bond angles according to ab initio calculations. At 𝑇=0.4K, the magnetization 𝑀(𝐵) exhibits steplike features that are also highly anisotropic. In the case of 𝐵∥𝑏, a small hysteresis observed around the second field-induced magnetic transition (𝐵𝑐2) indicates its first-order character, whereas the apparent divergence of the magnetic Grüneisen parameter at 𝐵𝑐2 is suppressed upon cooling and signals the absence of quantum critical behavior upon entering the field-polarized state. None of our thermodynamic measurements provide evidence for a field-induced quantum spin-liquid state near or above 𝐵𝑐2. |  |
Zhao, K.; Deng, H.; Chen, H.; Ma, N.; Oefele, N.; Guo, J.; Cui, X.; Tang, C.; Gutmann, M. J.; Mueller, T.; Su, Y.; Hutanu, V.; Jin, C.; Gegenwart, P. Three-dimensional XY universality and nonlinear magnetic susceptibility in a kagome ice compound Journal Article Phys. Rev. X 16, 021043 (2026). @article{xl5f-zj9p,
title = {Three-dimensional XY universality and nonlinear magnetic susceptibility in a kagome ice compound},
author = {K. Zhao and H. Deng and H. Chen and N. Ma and N. Oefele and J. Guo and X. Cui and C. Tang and M. J. Gutmann and T. Mueller and Y. Su and V. Hutanu and C. Jin and P. Gegenwart},
url = {https://link.aps.org/doi/10.1103/xl5f-zj9p},
doi = {10.1103/xl5f-zj9p},
year = {2026},
date = {2026-05-26},
urldate = {2026-05-01},
journal = {Phys. Rev. X},
volume = {16},
number = {2},
pages = {021043},
abstract = {Kagome spin ice is an intriguing class of spin systems constituted by in-plane Ising spins with ferromagnetic interaction residing on the kagome lattice, theoretically predicted to host a plethora of magnetic transitions and excitations. In particular, different variants of kagome spin ice models can exhibit different sequences of symmetry breaking upon cooling from the paramagnetic to the fully ordered ground state. Recently, it has been demonstrated that the frustrated intermetallic HoAgGe stands as a faithful solid-state realization of kagome spin ice. However, whether any of the established symmetry-breaking pathways apply to this material remains unaddressed. Here, we use single-crystal neutron diffuse scattering to map the spin ordering of HoAgGe at various temperatures more accurately; surprisingly, we find that the ordering sequence appears to be different from previously known scenarios: From the paramagnetic state, the system first enters a partially ordered state with fluctuating magnetic charges, in contrast to a charge-ordered paramagnetic phase, before reaching the fully ordered state. Through Monte Carlo simulations and scaling analyses using an extended three-dimensional (3D) spin model for the distorted kagome spin ice in HoAgGe, we elucidate a single 3D XY phase transition into the ground state with broken time-reversal symmetry (TRS). However, the 3D XY transition has a long crossover tail before the fluctuating magnetic charges fully order. More interestingly, we find, both experimentally and theoretically, that the TRS-breaking phase of HoAgGe features an unusual, hysteretic response: Despite their vanishing magnetization, the two time-reversal partners are distinguished and selected by a nonlinear magnetic susceptibility tied to the kagome ice rule. Our discovery not only unveils a new symmetry-breaking hierarchy of kagome spin ice but also demonstrates the potential of TRS-breaking frustrated spin systems for information technology applications.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
Kagome spin ice is an intriguing class of spin systems constituted by in-plane Ising spins with ferromagnetic interaction residing on the kagome lattice, theoretically predicted to host a plethora of magnetic transitions and excitations. In particular, different variants of kagome spin ice models can exhibit different sequences of symmetry breaking upon cooling from the paramagnetic to the fully ordered ground state. Recently, it has been demonstrated that the frustrated intermetallic HoAgGe stands as a faithful solid-state realization of kagome spin ice. However, whether any of the established symmetry-breaking pathways apply to this material remains unaddressed. Here, we use single-crystal neutron diffuse scattering to map the spin ordering of HoAgGe at various temperatures more accurately; surprisingly, we find that the ordering sequence appears to be different from previously known scenarios: From the paramagnetic state, the system first enters a partially ordered state with fluctuating magnetic charges, in contrast to a charge-ordered paramagnetic phase, before reaching the fully ordered state. Through Monte Carlo simulations and scaling analyses using an extended three-dimensional (3D) spin model for the distorted kagome spin ice in HoAgGe, we elucidate a single 3D XY phase transition into the ground state with broken time-reversal symmetry (TRS). However, the 3D XY transition has a long crossover tail before the fluctuating magnetic charges fully order. More interestingly, we find, both experimentally and theoretically, that the TRS-breaking phase of HoAgGe features an unusual, hysteretic response: Despite their vanishing magnetization, the two time-reversal partners are distinguished and selected by a nonlinear magnetic susceptibility tied to the kagome ice rule. Our discovery not only unveils a new symmetry-breaking hierarchy of kagome spin ice but also demonstrates the potential of TRS-breaking frustrated spin systems for information technology applications. |  |
Toyoda, S.; Kocsis, V.; Tokunaga, Y.; Kézsmárki, I.; Taguchi, Y.; Arima, T.; Tokura, Y.; Ogawa, N. All-optical control of antiferromagnetic domains via an inverse optical magnetoelectric effect Journal Article Nat. Mater. 25, 1572 (2026), datadoi: 10.1038/s41563-026-02608-4. @article{toyodaAllopticalControlAntiferromagnetic2026,
title = {All-optical control of antiferromagnetic domains via an inverse optical magnetoelectric effect},
author = {S. Toyoda and V. Kocsis and Y. Tokunaga and I. Kézsmárki and Y. Taguchi and T. Arima and Y. Tokura and N. Ogawa},
url = {https://doi.org/10.1038/s41563-026-02608-4},
doi = {10.1038/s41563-026-02608-4},
year = {2026},
date = {2026-05-15},
urldate = {2026-05-01},
journal = {Nat. Mater.},
volume = {25},
pages = {1572},
abstract = {All-optical control of antiferromagnetic order is essential for realizing next-generation energy-efficient spintronic and high-speed memory applications. However, the optical writing of antiferromagnetic domains remains a fundamental challenge, because conventional opto-magnetic recording techniques rely on net magnetization, which is absent in antiferromagnets. In certain multiferroic antiferromagnets, the magnetic toroidal moment provides an additional degree of freedom through its inherent magnetoelectric coupling, which manifests as directional asymmetry in light propagation. Here we demonstrate the all-optical writing of antiferromagnetic domains using the inverse optical magnetoelectric effect in ferrotoroidic LiNiPO4, driven solely by reversing the light propagation direction. This directional control arises from a strong coupling between the photon linear momentum and the magnetic toroidal moment, enabling non-volatile, deterministic and repeatable switching between time-reversed domains with arbitrary light polarization. Our findings establish an inverse optical magnetoelectric effect as a distinct mechanism for manipulating antiferromagnetic order, opening a new paradigm in opto-magnetism driven by photon momentum.},
note = {datadoi: 10.1038/s41563-026-02608-4},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
All-optical control of antiferromagnetic order is essential for realizing next-generation energy-efficient spintronic and high-speed memory applications. However, the optical writing of antiferromagnetic domains remains a fundamental challenge, because conventional opto-magnetic recording techniques rely on net magnetization, which is absent in antiferromagnets. In certain multiferroic antiferromagnets, the magnetic toroidal moment provides an additional degree of freedom through its inherent magnetoelectric coupling, which manifests as directional asymmetry in light propagation. Here we demonstrate the all-optical writing of antiferromagnetic domains using the inverse optical magnetoelectric effect in ferrotoroidic LiNiPO4, driven solely by reversing the light propagation direction. This directional control arises from a strong coupling between the photon linear momentum and the magnetic toroidal moment, enabling non-volatile, deterministic and repeatable switching between time-reversed domains with arbitrary light polarization. Our findings establish an inverse optical magnetoelectric effect as a distinct mechanism for manipulating antiferromagnetic order, opening a new paradigm in opto-magnetism driven by photon momentum. |  |
Pichler, F.; Hafezi, M.; Knap, M. Purely electronic model for exciton-polaron formation in moiré heterostructures Journal Article Phys. Rev. Res. 8, (2026), datadoi: 10.5281/zenodo.14879210. @article{pichlerPurelyElectronicModel2026,
title = {Purely electronic model for exciton-polaron formation in moiré heterostructures},
author = {F. Pichler and M. Hafezi and M. Knap},
url = {https://doi.org/10.1103/98wg-qcfn},
doi = {10.1103/98wg-qcfn},
issn = {2643-1564},
year = {2026},
date = {2026-05-11},
urldate = {2026-05-01},
journal = {Phys. Rev. Res.},
volume = {8},
number = {2},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.14879210},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Srivastava, A.; Birnkammer, S.; Sim, G.; Knap, M.; Knolle, J. Theory of nonlinear spectroscopy of quantum magnets Journal Article Phys. Rev. B 113, 184421 (2026), datadoi: 10.5281/zenodo.14938103. @article{srivastavaTheoryNonlinearSpectroscopy2026,
title = {Theory of nonlinear spectroscopy of quantum magnets},
author = {A. Srivastava and S. Birnkammer and G. Sim and M. Knap and J. Knolle},
url = {https://link.aps.org/doi/10.1103/2rfx-8ql6},
doi = {10.1103/2rfx-8ql6},
year = {2026},
date = {2026-05-07},
urldate = {2026-05-01},
journal = {Phys. Rev. B},
volume = {113},
number = {18},
pages = {184421},
publisher = {American Physical Society},
abstract = {Two-dimensional coherent spectroscopy (2DCS) is an established method for characterizing molecules and has been proposed in the terahertz regime as a tool for probing exotic excitations of quantum magnets; however, the precise nature of the coupling between pump field and spin degrees of freedom has remained unclear. Here, we develop a general response theory of 2DCS and show how magnetoelectric as well as polarization couplings contribute to 2DCS in addition to the typically assumed magnetization. We propose experimental protocols to probe the presence of polarization couplings, for instance, from exchange-striction or spin-current mechanism, when the electric field couples to quadratic terms in spin operators. We provide example calculations for the paradigmatic twisted Kitaev chain material CoNb2O6 and highlight the crucial role of contributions from cross-coupling between polarization and magnetic nonlinear susceptibilities. Our work paves the way for systematic studies of light-matter couplings in quantum magnets and for establishing 2DCS as a versatile tool for probing fractional excitations of exotic magnetic quantum phases.},
note = {datadoi: 10.5281/zenodo.14938103},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
Two-dimensional coherent spectroscopy (2DCS) is an established method for characterizing molecules and has been proposed in the terahertz regime as a tool for probing exotic excitations of quantum magnets; however, the precise nature of the coupling between pump field and spin degrees of freedom has remained unclear. Here, we develop a general response theory of 2DCS and show how magnetoelectric as well as polarization couplings contribute to 2DCS in addition to the typically assumed magnetization. We propose experimental protocols to probe the presence of polarization couplings, for instance, from exchange-striction or spin-current mechanism, when the electric field couples to quadratic terms in spin operators. We provide example calculations for the paradigmatic twisted Kitaev chain material CoNb2O6 and highlight the crucial role of contributions from cross-coupling between polarization and magnetic nonlinear susceptibilities. Our work paves the way for systematic studies of light-matter couplings in quantum magnets and for establishing 2DCS as a versatile tool for probing fractional excitations of exotic magnetic quantum phases. |  |
Ulrich, Y.; Mitscherling, J.; Classen, L.; Schnyder, A. P. Quantum geometric origin of the intrinsic nonlinear Hall effect Journal Article Phys. Rev. B 113, L201107 (2026). @article{4z8z-4kch,
title = {Quantum geometric origin of the intrinsic nonlinear Hall effect},
author = {Y. Ulrich and J. Mitscherling and L. Classen and A. P. Schnyder},
url = {https://link.aps.org/doi/10.1103/4z8z-4kch},
doi = {10.1103/4z8z-4kch},
year = {2026},
date = {2026-05-04},
urldate = {2026-05-01},
journal = {Phys. Rev. B},
volume = {113},
number = {20},
pages = {L201107},
abstract = {We decompose the intrinsic second-order nonlinear Hall effect (NLHE) of a generic multiband system into its quantum geometric contributions within a fully quantum-mechanical, projector-based formalism. By expanding the nonlinear conductivity in powers of the quasiparticle lifetime 𝜏, we recover the established Berry curvature dipole at order 𝜏 and clarify discrepancies in previous literature concerning the (interband) quantum metric dipole (or Berry curvature polarizability) contribution at order 𝜏0. Crucially, our method reveals an additional contribution at order 𝜏0, determined by the intraband quantum metric dipole (intraQMD), arising from additional virtual interband transitions captured within the fully quantum-mechanical treatment. The intraQMD contribution is generically nonzero in systems with broken time-reversal symmetry and can be distinguished from other geometric contributions by symmetry. Analytical results for low-energy models of topological band crossings, which are hot spots of quantum geometry, demonstrate how band topology influences each contribution. In particular, the intraQMD contribution is especially large in gapped Dirac cones in antiferromagnets. Through a comprehensive symmetry classification of all magnetic space groups, we identify several candidate materials that are expected to exhibit large intrinsic NLHE, including the topological antiferromagnets Yb3Pt4, CuMnAs, and CoNb3S6, as well as the nodal-plane material MnNb3S6.},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
We decompose the intrinsic second-order nonlinear Hall effect (NLHE) of a generic multiband system into its quantum geometric contributions within a fully quantum-mechanical, projector-based formalism. By expanding the nonlinear conductivity in powers of the quasiparticle lifetime 𝜏, we recover the established Berry curvature dipole at order 𝜏 and clarify discrepancies in previous literature concerning the (interband) quantum metric dipole (or Berry curvature polarizability) contribution at order 𝜏0. Crucially, our method reveals an additional contribution at order 𝜏0, determined by the intraband quantum metric dipole (intraQMD), arising from additional virtual interband transitions captured within the fully quantum-mechanical treatment. The intraQMD contribution is generically nonzero in systems with broken time-reversal symmetry and can be distinguished from other geometric contributions by symmetry. Analytical results for low-energy models of topological band crossings, which are hot spots of quantum geometry, demonstrate how band topology influences each contribution. In particular, the intraQMD contribution is especially large in gapped Dirac cones in antiferromagnets. Through a comprehensive symmetry classification of all magnetic space groups, we identify several candidate materials that are expected to exhibit large intrinsic NLHE, including the topological antiferromagnets Yb3Pt4, CuMnAs, and CoNb3S6, as well as the nodal-plane material MnNb3S6. |  |
Hirrle, M.; Röß-Ohlenroth, R.; Reschke, S.; Bredenkötter, B.; von Nidda, H. -A. Krug; Volkmer, D. Tuning of Jahn-Teller distortions via sterically enforced lattice enlargement of Cu(ta)2-type coordination polymers Journal Article J. Phys. Chem. Solids. 212, 113566 (2026). @article{hirrleTuningJahnTellerDistortions2026,
title = {Tuning of Jahn-Teller distortions via sterically enforced lattice enlargement of Cu(ta)_{2}-type coordination polymers},
author = {M. Hirrle and R. Röß-Ohlenroth and S. Reschke and B. Bredenkötter and H. -A. Krug von Nidda and D. Volkmer},
url = {https://www.sciencedirect.com/science/article/pii/S0022369726000521},
doi = {10.1016/j.jpcs.2026.113566},
year = {2026},
date = {2026-05-01},
urldate = {2026-05-01},
journal = {J. Phys. Chem. Solids.},
volume = {212},
pages = {113566},
abstract = {The control of Jahn-Teller distortions in copper-based coordination polymers is crucial for tuning their magnetic and structural properties. Here, we report the synthesis and characterization of two novel Cu(II)-based metal-organic frameworks (MOFs), Cu(mta)2 and Cu(cta)2, derived from modified triazole ligands. By introducing steric bulk through methyl and cyclopentyl substituents, we systematically investigate the effect of lattice enlargement on local coordination environments and magnetic behaviour. Single-crystal and powder X-ray diffraction analyses reveal that Cu(mta)2 exhibits static Jahn-Teller distortions similar to those observed in Cu(ta)2, whereas Cu(cta)2 crystallizes in an undistorted, near-ideal cubic structure. Magnetic susceptibility and electron spin resonance measurements show strong antiferromagnetic interactions and temperature-dependent g-factor anisotropy for Cu(ta)2 and Cu(mta)2, while Cu(cta)2 displays nearly isotropic magnetic behavior and only dynamically JT distortions without a cooperative phase transition. These results demonstrate that steric ligand design offers a powerful strategy to modulate the interplay between lattice structure and magnetic anisotropy. Our findings provide fundamental insights into the suppression of cooperative static Jahn-Teller distortions and open pathways for the targeted design of multifunctional MOFs with tailored structural and magnetic properties.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
The control of Jahn-Teller distortions in copper-based coordination polymers is crucial for tuning their magnetic and structural properties. Here, we report the synthesis and characterization of two novel Cu(II)-based metal-organic frameworks (MOFs), Cu(mta)2 and Cu(cta)2, derived from modified triazole ligands. By introducing steric bulk through methyl and cyclopentyl substituents, we systematically investigate the effect of lattice enlargement on local coordination environments and magnetic behaviour. Single-crystal and powder X-ray diffraction analyses reveal that Cu(mta)2 exhibits static Jahn-Teller distortions similar to those observed in Cu(ta)2, whereas Cu(cta)2 crystallizes in an undistorted, near-ideal cubic structure. Magnetic susceptibility and electron spin resonance measurements show strong antiferromagnetic interactions and temperature-dependent g-factor anisotropy for Cu(ta)2 and Cu(mta)2, while Cu(cta)2 displays nearly isotropic magnetic behavior and only dynamically JT distortions without a cooperative phase transition. These results demonstrate that steric ligand design offers a powerful strategy to modulate the interplay between lattice structure and magnetic anisotropy. Our findings provide fundamental insights into the suppression of cooperative static Jahn-Teller distortions and open pathways for the targeted design of multifunctional MOFs with tailored structural and magnetic properties. |  |
Haghshenas, R.; Chertkov, E.; Mills, M.; Kadow, W.; Lin, S. -H.; Chen, Y. H.; Cade, C.; Niesen, I.; Begušić, T.; Rudolph, M. S.; Cirstoiu, C.; Hémery, K.; Keever, C. Mc; Lubasch, M.; Granet, E.; Baldwin, C. H.; Bartolotta, J. P.; Bohn, M.; Burau, J. J.; Cline, J.; DeCross, M.; Dreiling, J. M.; Foltz, C.; Francois, D.; Gaebler, J. P.; Gilbreth, C. N.; Gray, J.; Gresh, D.; Hall, A.; Hankin, A.; Hansen, A.; Hewitt, N.; Holliman, C. A.; Hutson, R. B.; Iqbal, M.; Kotibhaskar, N.; Lehman, E.; Lucchetti, D.; Madjarov, I. S.; Mayer, K.; Milne, A. R.; Moses, S. A.; Neyenhuis, B.; Park, G.; Perry, A. R.; Ponsioen, B.; Schecter, M.; Siegfried, P. E.; Stephen, D. T.; Tiemann, B. G.; Urmey, M. D.; Walker, J.; Potter, A. C.; Hayes, D.; Chan, G. K. -L.; Pollmann, F.; Knap, M.; Dreyer, H.; Foss-Feig, M. Digital quantum magnetism on a trapped-ion quantum computer Journal Article Nature 653, 56–62 (2026), datadoi: 10.5281/zenodo.18487089. @article{haghshenasDigitalQuantumMagnetism2026,
title = {Digital quantum magnetism on a trapped-ion quantum computer},
author = {R. Haghshenas and E. Chertkov and M. Mills and W. Kadow and S. -H. Lin and Y. H. Chen and C. Cade and I. Niesen and T. Begušić and M. S. Rudolph and C. Cirstoiu and K. Hémery and C. Mc Keever and M. Lubasch and E. Granet and C. H. Baldwin and J. P. Bartolotta and M. Bohn and J. J. Burau and J. Cline and M. DeCross and J. M. Dreiling and C. Foltz and D. Francois and J. P. Gaebler and C. N. Gilbreth and J. Gray and D. Gresh and A. Hall and A. Hankin and A. Hansen and N. Hewitt and C. A. Holliman and R. B. Hutson and M. Iqbal and N. Kotibhaskar and E. Lehman and D. Lucchetti and I. S. Madjarov and K. Mayer and A. R. Milne and S. A. Moses and B. Neyenhuis and G. Park and A. R. Perry and B. Ponsioen and M. Schecter and P. E. Siegfried and D. T. Stephen and B. G. Tiemann and M. D. Urmey and J. Walker and A. C. Potter and D. Hayes and G. K. -L. Chan and F. Pollmann and M. Knap and H. Dreyer and M. Foss-Feig},
url = {https://doi.org/10.1038/s41586-026-10445-3},
doi = {10.1038/s41586-026-10445-3},
issn = {1476-4687},
year = {2026},
date = {2026-04-29},
urldate = {2026-04-01},
journal = {Nature},
volume = {653},
number = {8113},
pages = {56–62},
publisher = {Springer Science and Business Media LLC},
note = {datadoi: 10.5281/zenodo.18487089},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Patra, S. P.; Mohanty, S.; Samanta, S.; Oommen, J. K.; Tsirlin, A. A.; Nath, R. Magnetic transitions in the spin-5/2 triangular lattice antiferromagnet Ba3MnTa2O9 Journal Article Phys. Rev. B 113, 144436 (2026). @article{ynnr-dm9r,
title = {Magnetic transitions in the spin-5/2 triangular lattice antiferromagnet Ba_{3}MnTa_{2}O_{9}},
author = {S. P. Patra and S. Mohanty and S. Samanta and J. K. Oommen and A. A. Tsirlin and R. Nath},
url = {https://link.aps.org/doi/10.1103/ynnr-dm9r},
doi = {10.1103/ynnr-dm9r},
year = {2026},
date = {2026-04-28},
urldate = {2026-04-28},
journal = {Phys. Rev. B},
volume = {113},
number = {14},
pages = {144436},
publisher = {American Physical Society},
abstract = {We report a comprehensive study of the structural and magnetic properties of the two-dimensional 𝑆=5/2 frustrated triangular-lattice antiferromagnet Ba3MnTa2O9 using x-ray diffraction, magnetization, electron spin resonance, and heat-capacity measurements on a polycrystalline sample, combined with density-functional band-structure calculations. The magnetic susceptibility and heat-capacity data reveal the onset of antiferromagnetic long-range order at 𝑇N≃2.6K, which is in sharp contrast with the recent report by Mondal et al. [Phys. Rev. B 112, 155153 (2025)] who did not observe magnetic order in this material. The nearest-neighbor exchange coupling 𝐽/𝑘B≃0.85K is obtained from Monte Carlo fits to the experimental susceptibility data. Combined with the ab initio estimate of the interlayer coupling, this 𝐽/𝑘B value leads to 𝑇N≃2.7K in a perfect agreement with the experiment. Magnetic isotherms reveal a field-induced transition below 𝑇N. The complex 𝐻−𝑇 phase diagram features multiple phases as a consequence of magnetic frustration and anisotropy present in the system.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
We report a comprehensive study of the structural and magnetic properties of the two-dimensional 𝑆=5/2 frustrated triangular-lattice antiferromagnet Ba3MnTa2O9 using x-ray diffraction, magnetization, electron spin resonance, and heat-capacity measurements on a polycrystalline sample, combined with density-functional band-structure calculations. The magnetic susceptibility and heat-capacity data reveal the onset of antiferromagnetic long-range order at 𝑇N≃2.6K, which is in sharp contrast with the recent report by Mondal et al. [Phys. Rev. B 112, 155153 (2025)] who did not observe magnetic order in this material. The nearest-neighbor exchange coupling 𝐽/𝑘B≃0.85K is obtained from Monte Carlo fits to the experimental susceptibility data. Combined with the ab initio estimate of the interlayer coupling, this 𝐽/𝑘B value leads to 𝑇N≃2.7K in a perfect agreement with the experiment. Magnetic isotherms reveal a field-induced transition below 𝑇N. The complex 𝐻−𝑇 phase diagram features multiple phases as a consequence of magnetic frustration and anisotropy present in the system. |  |
Nandi, S.; Das, R.; Hemmida, M.; Akbar, M. U.; von Nidda, H. -A. Krug; Sichelschmidt, J.; Mahapatra, S.; Schuller, M.; Büttgen, N.; Wilkinson, J.; Saravanan, M. P.; Dasgupta, I.; Mahajan, A. V. Novel Quantum Spin Liquid States in the S = 1/2 Three-Dimensional Compound Y3Cu2Sb3O14 Journal Article Phys. Rev. Lett. 136, 166502 (2026). @article{nandiNovelQuantumSpin2025,
title = {Novel Quantum Spin Liquid States in the S = 1/2 Three-Dimensional Compound Y_{3}Cu_{2}Sb_{3}O_{14}},
author = {S. Nandi and R. Das and M. Hemmida and M. U. Akbar and H. -A. Krug von Nidda and J. Sichelschmidt and S. Mahapatra and M. Schuller and N. Büttgen and J. Wilkinson and M. P. Saravanan and I. Dasgupta and A. V. Mahajan},
url = {https://doi.org/10.1103/2bps-xvl8},
doi = {10.1103/2bps-xvl8},
year = {2026},
date = {2026-04-22},
urldate = {2026-04-01},
journal = {Phys. Rev. Lett.},
volume = {136},
pages = {166502},
abstract = {The three-dimensional S=1/2 system Y3Cu2Sb3O14 consists of two inequivalent Cu2+ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility 𝜒(𝑇), specific heat 𝐶𝑝(𝑇), 89Y nuclear magnetic resonance (NMR), muon spin relaxation (μSR), and electron spin resonance (ESR) measurements on this system confirm the absence of any long-range magnetic ordering and the persistence of spin dynamics down to 0.077 K. In 89Y NMR, we find an anomaly at about 120 K, which we suggest arises from a fraction of the spins condensing into a singlet (a valence bond solid, or VBS) state. A plateau in the muon relaxation rate is observed between 60 K and 10 K (signifying the VBS state from a fraction of the spins) followed by an increase and another plateau below about 1 K (presumably signifying the quantum spin liquid state from all the spins). Our density functional theory calculations find a dominant antiferromagnetic interaction along the body diagonal with inequivalent Cu(1) and Cu(2) ions alternately occupying the corners of the cube. All other near-neighbor interactions between the Cu ions are also found to be antiferromagnetic and are thought to drive the frustration.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
The three-dimensional S=1/2 system Y3Cu2Sb3O14 consists of two inequivalent Cu2+ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility 𝜒(𝑇), specific heat 𝐶𝑝(𝑇), 89Y nuclear magnetic resonance (NMR), muon spin relaxation (μSR), and electron spin resonance (ESR) measurements on this system confirm the absence of any long-range magnetic ordering and the persistence of spin dynamics down to 0.077 K. In 89Y NMR, we find an anomaly at about 120 K, which we suggest arises from a fraction of the spins condensing into a singlet (a valence bond solid, or VBS) state. A plateau in the muon relaxation rate is observed between 60 K and 10 K (signifying the VBS state from a fraction of the spins) followed by an increase and another plateau below about 1 K (presumably signifying the quantum spin liquid state from all the spins). Our density functional theory calculations find a dominant antiferromagnetic interaction along the body diagonal with inequivalent Cu(1) and Cu(2) ions alternately occupying the corners of the cube. All other near-neighbor interactions between the Cu ions are also found to be antiferromagnetic and are thought to drive the frustration. |  |
Yun, W.; Nakano, R.; Misawa, R.; Yamada, R.; Akatsuka, S.; Ōnuki, Y.; Baral, P. R.; Esser, S.; Saitoh, H.; Kiyanagi, R.; Ohhara, T.; Nakajima, T.; Arima, T.; Hirschberger, M. Stripe antiferromagnetism in the van der Waals metal HoTe3 decoupled from charge density wave order Journal Article Phys. Rev. B (2026). @article{yunStripeAntiferromagnetismVan2026,
title = {Stripe antiferromagnetism in the van der Waals metal HoTe_{3} decoupled from charge density wave order},
author = {W. Yun and R. Nakano and R. Misawa and R. Yamada and S. Akatsuka and Y. Ōnuki and P. R. Baral and S. Esser and H. Saitoh and R. Kiyanagi and T. Ohhara and T. Nakajima and T. Arima and M. Hirschberger},
url = {https://link.aps.org/doi/10.1103/q39f-b32w},
doi = {10.1103/q39f-b32w},
year = {2026},
date = {2026-04-21},
urldate = {2026-04-01},
journal = {Phys. Rev. B},
publisher = {American Physical Society},
abstract = {The RTe3 (R = rare earth) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains largely unexplored. Combining polarized and unpolarized neutron diffraction on single crystals of HoTe3, we identify two distinct antiferromagnetic (AFM) phases, both exhibiting a collinear ↑↑↓↓ motif within individual vdW layers. The two phases are distinguished by the vdW stacking of magnetic layers: ferromagnetic (FM) stacking in the higher-temperature AFM-II phase, here termed “vertical-stripe”, and AFM stacking in the AFM-I ground state, here termed “tilted-stripe”; the two phases have propagation vectors qm2 = (0.48, 0, 0) and qm1 = (0.5, 0.5, 0), respectively. In contrast to the CDW-driven exotic magnetism in DyTe3, TbTe3, and GdTe3, we find no evidence for coupling between magnetism and CDW in HoTe3. The presence of a checkerboard-type charge order in HoTe3 may be detrimental for realizing coupled spin/charge order parameters in layered vdW systems.},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
The RTe3 (R = rare earth) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains largely unexplored. Combining polarized and unpolarized neutron diffraction on single crystals of HoTe3, we identify two distinct antiferromagnetic (AFM) phases, both exhibiting a collinear ↑↑↓↓ motif within individual vdW layers. The two phases are distinguished by the vdW stacking of magnetic layers: ferromagnetic (FM) stacking in the higher-temperature AFM-II phase, here termed “vertical-stripe”, and AFM stacking in the AFM-I ground state, here termed “tilted-stripe”; the two phases have propagation vectors qm2 = (0.48, 0, 0) and qm1 = (0.5, 0.5, 0), respectively. In contrast to the CDW-driven exotic magnetism in DyTe3, TbTe3, and GdTe3, we find no evidence for coupling between magnetism and CDW in HoTe3. The presence of a checkerboard-type charge order in HoTe3 may be detrimental for realizing coupled spin/charge order parameters in layered vdW systems. |  |
Rojewski, S.; Borkenhagen, R.; Li, R.; Ovalle, D. G.; Tsirkin, S. S.; Kumar, H.; Raju, K.; Sankar, R.; Lei, S.; Schoop, L. M.; Vergniory, M. G.; Kuntscher, C. A. Optical response of the Dirac semimetals GdSb0.56Te1.35 and GdSb0.45Te1.50: Influence of charge density wave distortion and magnetic order Journal Article Phys. Rev. B 113, 155141 (2026), datadoi: (10.5281/zenodo.19235004). @article{rojewskiOpticalResponseDirac2026,
title = {Optical response of the Dirac semimetals GdSb_{0.56}Te_{1.35} and GdSb_{0.45}Te_{1.50}: Influence of charge density wave distortion and magnetic order},
author = {S. Rojewski and R. Borkenhagen and R. Li and D. G. Ovalle and S. S. Tsirkin and H. Kumar and K. Raju and R. Sankar and S. Lei and L. M. Schoop and M. G. Vergniory and C. A. Kuntscher},
url = {https://link.aps.org/doi/10.1103/nygm-n4fv},
doi = {10.1103/nygm-n4fv},
year = {2026},
date = {2026-04-20},
urldate = {2026-04-01},
journal = {Phys. Rev. B},
volume = {113},
number = {15},
pages = {155141},
abstract = {The square-net materials GdSb𝑥Te2−𝑥−𝛿
provide a platform for exploring the effects of charge density wave (CDW) distortion and band filling on the topological electronic band structure. In this work we use infrared spectroscopy to probe the temperature-dependent electronic excitations in GdSb0.56Te1.35 and GdSb0.45Te1.50
single crystals for different polarization directions parallel to the square-net layers. First-principles calculations were also performed to study the electronic band structure and interband optical conductivity of stoichiometric GdSbTe. For GdSb0.56Te1.35 the in-plane optical conductivity is independent of the polarization direction and contains a small Drude term, indicating a weak metallic character, and a pronounced near-infrared absorption band, which may be due to excitations across the CDW gap. Upon cooling, the optical response shows no significant temperature dependence within the experimental uncertainty, and no signatures associated with magnetic ordering are detected. In comparison, for GdSb0.45Te1.50 we observe an in-plane anisotropy and strongly reduced low-frequency optical conductivity, with small temperature dependence. Possible signatures of Dirac fermion excitations in the optical conductivity spectra are also analyzed and discussed. Our results demonstrate that small differences in the stoichiometry have a significant impact on the optical response of GdSb𝑥Te2−𝑥−𝛿 materials.},
note = {datadoi: (10.5281/zenodo.19235004)},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
The square-net materials GdSb𝑥Te2−𝑥−𝛿
provide a platform for exploring the effects of charge density wave (CDW) distortion and band filling on the topological electronic band structure. In this work we use infrared spectroscopy to probe the temperature-dependent electronic excitations in GdSb0.56Te1.35 and GdSb0.45Te1.50
single crystals for different polarization directions parallel to the square-net layers. First-principles calculations were also performed to study the electronic band structure and interband optical conductivity of stoichiometric GdSbTe. For GdSb0.56Te1.35 the in-plane optical conductivity is independent of the polarization direction and contains a small Drude term, indicating a weak metallic character, and a pronounced near-infrared absorption band, which may be due to excitations across the CDW gap. Upon cooling, the optical response shows no significant temperature dependence within the experimental uncertainty, and no signatures associated with magnetic ordering are detected. In comparison, for GdSb0.45Te1.50 we observe an in-plane anisotropy and strongly reduced low-frequency optical conductivity, with small temperature dependence. Possible signatures of Dirac fermion excitations in the optical conductivity spectra are also analyzed and discussed. Our results demonstrate that small differences in the stoichiometry have a significant impact on the optical response of GdSb𝑥Te2−𝑥−𝛿 materials. |  |
Pichler, F.; Kuhlenkamp, C.; Knap, M. False Vacuum Decay in Flat-Band Ferromagnets: Role of Quantum Geometry and Chiral Edge States Journal Article Phys. Rev. Lett. 136, (2026), datadoi: 10.5281/zenodo.17924292. @article{pichlerFalseVacuumDecay2026,
title = {False Vacuum Decay in Flat-Band Ferromagnets: Role of Quantum Geometry and Chiral Edge States},
author = {F. Pichler and C. Kuhlenkamp and M. Knap},
url = {https://doi.org/10.1103/q7ss-pvcq},
doi = {10.1103/q7ss-pvcq},
issn = {1079-7114},
year = {2026},
date = {2026-04-15},
urldate = {2026-04-01},
journal = {Phys. Rev. Lett.},
volume = {136},
number = {15},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.17924292},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Liefferink, R.; Körber, L.; Gerlinger, K.; Pfau, B.; Büttner, F.; Mentink, J. H. Effective Theory of Ultrafast Skyrmion Nucleation Journal Article Phys. Rev. Lett. 136, 146705 (2026), datadoi: 10.34973/5168-bn56. @article{liefferinkEffectiveTheoryUltrafast2026,
title = {Effective Theory of Ultrafast Skyrmion Nucleation},
author = {R. Liefferink and L. Körber and K. Gerlinger and B. Pfau and F. Büttner and J. H. Mentink},
url = {https://link.aps.org/doi/10.1103/brnt-2m9l},
doi = {10.1103/brnt-2m9l},
issn = {0031-9007, 1079-7114},
year = {2026},
date = {2026-04-10},
urldate = {2026-04-10},
journal = {Phys. Rev. Lett.},
volume = {136},
number = {14},
pages = {146705},
note = {datadoi: 10.34973/5168-bn56},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
|  |
Ranaut, D.; Adroja, D. T.; Aouane, M.; Mukharjee, P. K.; Gegenwart, P.; Jaiswal-Nagar, D. Crystal field scheme and field-induced critical behavior in effective spin-1/2 NdVO4 Journal Article Phys. Rev. B 113, 144411 (2026). @article{ranautCrystalFieldScheme2026,
title = {Crystal field scheme and field-induced critical behavior in effective spin-1/2 NdVO_{4}},
author = {D. Ranaut and D. T. Adroja and M. Aouane and P. K. Mukharjee and P. Gegenwart and D. Jaiswal-Nagar},
url = {https://link.aps.org/doi/10.1103/c6v8-vx4h},
doi = {10.1103/c6v8-vx4h},
year = {2026},
date = {2026-04-07},
urldate = {2026-04-04},
journal = {Phys. Rev. B},
volume = {113},
number = {14},
pages = {144411},
publisher = {American Physical Society},
abstract = {Quantum fluctuations in low-spin (𝑆=1/2) systems make them potential materials to investigate various intriguing field-induced quantum phenomena. In this context, rare-earth (4𝑓)-based effective spin (𝐽eff=1/2) systems with localized magnetic moments and low energy scales offer an advantage of low critical fields and provide access to probe the complete magnetic phase diagram. Here, we present inelastic neutron scattering (INS) data to understand the crystal field (CF) scheme of the previously established 𝐽eff=1/2 antiferromagnet NdVO4, along with low-temperature magnetization and heat capacity measurements to construct the complete magnetic phase diagram. Our INS data validate the presence of the 𝐽eff=1/2 state at low temperatures with the ground and first excited CF state separated by an energy of 140 K. Furthermore, it yields a unique CF scheme where the excitation corresponding to the highest (fourth) CF state is observed via transitions involving the first and second excited states. Magnetic and heat capacity measurements yield the presence of a field-induced first-order spin-flop transition within the second-order antiferromagnetic (AFM) state. Magnetic phase diagrams constructed using the field-dependent magnetization and magnetic heat capacity reveal a continuous transformation from AFM to spin-flop state with a critical field of 𝐻sf∼1.4T. The presence of quantum fluctuations near 𝐻sf are evident from the V-shaped region in entropy contours indicating the presence of accumulated entropy.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
Quantum fluctuations in low-spin (𝑆=1/2) systems make them potential materials to investigate various intriguing field-induced quantum phenomena. In this context, rare-earth (4𝑓)-based effective spin (𝐽eff=1/2) systems with localized magnetic moments and low energy scales offer an advantage of low critical fields and provide access to probe the complete magnetic phase diagram. Here, we present inelastic neutron scattering (INS) data to understand the crystal field (CF) scheme of the previously established 𝐽eff=1/2 antiferromagnet NdVO4, along with low-temperature magnetization and heat capacity measurements to construct the complete magnetic phase diagram. Our INS data validate the presence of the 𝐽eff=1/2 state at low temperatures with the ground and first excited CF state separated by an energy of 140 K. Furthermore, it yields a unique CF scheme where the excitation corresponding to the highest (fourth) CF state is observed via transitions involving the first and second excited states. Magnetic and heat capacity measurements yield the presence of a field-induced first-order spin-flop transition within the second-order antiferromagnetic (AFM) state. Magnetic phase diagrams constructed using the field-dependent magnetization and magnetic heat capacity reveal a continuous transformation from AFM to spin-flop state with a critical field of 𝐻sf∼1.4T. The presence of quantum fluctuations near 𝐻sf are evident from the V-shaped region in entropy contours indicating the presence of accumulated entropy. |  |
Koraltan, S.; Sunny, J.; Karaman, T.; Peremadathil‐Pradeep, R.; Darwin, E.; Büttner, F.; Suess, D.; Hug, H. J.; Albrecht, M. Magnetic Force Microscopy Signatures of Higher‐Order Skyrmions and Antiskyrmions Journal Article Adv. Funct. Mater. 36, (2026). @article{koraltanMagneticForceMicroscopy2026,
title = {Magnetic Force Microscopy Signatures of Higher‐Order Skyrmions and Antiskyrmions},
author = {S. Koraltan and J. Sunny and T. Karaman and R. Peremadathil‐Pradeep and E. Darwin and F. Büttner and D. Suess and H. J. Hug and M. Albrecht},
url = {http://dx.doi.org/10.1002/adfm.202525716},
doi = {10.1002/adfm.202525716},
year = {2026},
date = {2026-03-13},
urldate = {2026-03-13},
journal = {Adv. Funct. Mater.},
volume = {36},
number = {41},
publisher = {Wiley},
abstract = {Higher-order skyrmions and antiskyrmions are topologically protected spin textures with integer topological charges beyond
±1, typically nucleating from vertical Bloch lines in domain walls. Until now, they have been reported only in ferromagnetic multilayers by Lorentz transmission electron microscopy (LTEM), which requires growth on ultrathin membranes and complicates their integration into spintronic devices. Moreover, LTEM often yields contrast patterns that are difficult to unambiguously assign to specific topological charges. Here, we demonstrate that magnetic force microscopy (MFM) operated under vacuum conditions provides a robust route to identify and distinguish higher-order spin textures in Co/Ni multilayers at room temperature. Supported by micromagnetic simulations, we show that MFM can resolve vertical Bloch lines as well as skyrmions and antiskyrmions with arbitrary charge. Our results establish advanced MFM as a powerful technique for the qualitative classification of complex spin textures, paving the way for their exploration and utilization in future skyrmionic device concepts.},
keywords = {A2, C2},
pubstate = {published},
tppubtype = {article}
}
Higher-order skyrmions and antiskyrmions are topologically protected spin textures with integer topological charges beyond
±1, typically nucleating from vertical Bloch lines in domain walls. Until now, they have been reported only in ferromagnetic multilayers by Lorentz transmission electron microscopy (LTEM), which requires growth on ultrathin membranes and complicates their integration into spintronic devices. Moreover, LTEM often yields contrast patterns that are difficult to unambiguously assign to specific topological charges. Here, we demonstrate that magnetic force microscopy (MFM) operated under vacuum conditions provides a robust route to identify and distinguish higher-order spin textures in Co/Ni multilayers at room temperature. Supported by micromagnetic simulations, we show that MFM can resolve vertical Bloch lines as well as skyrmions and antiskyrmions with arbitrary charge. Our results establish advanced MFM as a powerful technique for the qualitative classification of complex spin textures, paving the way for their exploration and utilization in future skyrmionic device concepts. |  |
Pichler, F.; Kuhlenkamp, C.; Knap, M.; Vishwanath, A. Microscopic mechanism of anyon superconductivity emerging from fractional Chern insulators Journal Article Newton 2, 100340 (2026), datadoi: 10.5281/zenodo.15594496. @article{pichlerMicroscopicMechanismAnyon2026,
title = {Microscopic mechanism of anyon superconductivity emerging from fractional Chern insulators},
author = {F. Pichler and C. Kuhlenkamp and M. Knap and A. Vishwanath},
url = {https://doi.org/10.1016/j.newton.2025.100340},
doi = {10.1016/j.newton.2025.100340},
issn = {2950-6360},
year = {2026},
date = {2026-03-02},
urldate = {2026-03-01},
journal = {Newton},
volume = {2},
number = {3},
pages = {100340},
publisher = {Elsevier BV},
note = {datadoi: 10.5281/zenodo.15594496},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Davenport, H.; Schindler, F.; Knolle, J. Berry curvature of low-energy excitons in rhombohedral graphene Journal Article Phys. Rev. B 113, 115102 (2026), datadoi: 10.5281/zenodo.16902666. @article{davenportBerryCurvatureLowenergy2026,
title = {Berry curvature of low-energy excitons in rhombohedral graphene},
author = {H. Davenport and F. Schindler and J. Knolle},
url = {https://link.aps.org/doi/10.1103/shrm-4swg},
doi = {10.1103/shrm-4swg},
year = {2026},
date = {2026-03-01},
journal = {Phys. Rev. B},
volume = {113},
number = {11},
pages = {115102},
publisher = {American Physical Society},
abstract = {We investigate low-energy excitons in rhombohedral pentalayer graphene encapsulated by hexagonal boron nitride (hBN/R5G/hBN), focusing on the regime at the experimental twist angle 𝜃=0.77° and with an applied electric field. We introduce a new low-energy two-band model of rhombohedral graphene that captures the band structure more accurately than previous models while keeping the number of parameters low. Using this model, we show that the centres of the exciton Wannier functions are displaced from the moiré unit cell origin by a quantized amount—they are instead localized at 𝐶3-symmetric points on the boundary. We also find that the exciton shift is electrically tunable: by varying the electric field strength, the exciton Wannier center can be exchanged between inequivalent corners of the moiré unit cell. Our results suggest the possibility of detecting excitonic corner or edge modes, as well as novel excitonic crystal defect responses in hBN/R5G/hBN. Lastly, we find that the excitons in hBN/R5G/hBN inherit excitonic Berry curvature from the underlying electronic bands, enriching their semiclassical transport properties. Our results position rhombohedral graphene as a compelling tunable platform for probing exciton topology in moiré materials.},
note = {datadoi: 10.5281/zenodo.16902666},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
We investigate low-energy excitons in rhombohedral pentalayer graphene encapsulated by hexagonal boron nitride (hBN/R5G/hBN), focusing on the regime at the experimental twist angle 𝜃=0.77° and with an applied electric field. We introduce a new low-energy two-band model of rhombohedral graphene that captures the band structure more accurately than previous models while keeping the number of parameters low. Using this model, we show that the centres of the exciton Wannier functions are displaced from the moiré unit cell origin by a quantized amount—they are instead localized at 𝐶3-symmetric points on the boundary. We also find that the exciton shift is electrically tunable: by varying the electric field strength, the exciton Wannier center can be exchanged between inequivalent corners of the moiré unit cell. Our results suggest the possibility of detecting excitonic corner or edge modes, as well as novel excitonic crystal defect responses in hBN/R5G/hBN. Lastly, we find that the excitons in hBN/R5G/hBN inherit excitonic Berry curvature from the underlying electronic bands, enriching their semiclassical transport properties. Our results position rhombohedral graphene as a compelling tunable platform for probing exciton topology in moiré materials. | |
Mangeolle, L.; Knolle, J. Extrinsic Contribution to Bosonic Thermal Hall Transport Journal Article Phys. Rev. X 16, 011048 (2026). @article{mangeolleExtrinsicContributionBosonic2026,
title = {Extrinsic Contribution to Bosonic Thermal Hall Transport},
author = {L. Mangeolle and J. Knolle},
url = {https://link.aps.org/doi/10.1103/grzx-v6sj},
doi = {10.1103/grzx-v6sj},
year = {2026},
date = {2026-03-01},
journal = {Phys. Rev. X},
volume = {16},
number = {1},
pages = {011048},
publisher = {American Physical Society},
abstract = {Bosonic excitations like phonons and magnons dominate the low-temperature transport of magnetic insulators. Similar to electronic Hall responses, the thermal Hall effect (THE) of charge-neutral bosons has been proposed as a powerful tool for probing topological properties of their wave functions. For example, the intrinsic contribution of the THE of a perfectly clean system is directly governed by the distribution of Berry curvature, and many experiments on topological magnon and phonon insulators have been interpreted in this way. However, disorder is inevitably present in any material, and its contribution to the THE has remained poorly understood. Here, we develop a rigorous kinetic theory of the extrinsic side-jump contribution to the THE of bosons. We show that the extrinsic THE is always relevant for bosonic systems and can be of the same order as the intrinsic one but sensitively depends on the type of local imperfection. We study different types of impurities and show that a THE can even arise as a pure impurity-induced effect in a system with a vanishing intrinsic contribution. As a side product, we also generalize existing results for the electronic anomalous Hall effect to general types of impurities beyond the standard assumption of local potential scattering. We discuss the importance of our results for the correct interpretation of THE measurements, for example, in the Kitaev magnet 𝛼−RuCl3, and provide a ready-to-use formula for comparison to experimental data.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Bosonic excitations like phonons and magnons dominate the low-temperature transport of magnetic insulators. Similar to electronic Hall responses, the thermal Hall effect (THE) of charge-neutral bosons has been proposed as a powerful tool for probing topological properties of their wave functions. For example, the intrinsic contribution of the THE of a perfectly clean system is directly governed by the distribution of Berry curvature, and many experiments on topological magnon and phonon insulators have been interpreted in this way. However, disorder is inevitably present in any material, and its contribution to the THE has remained poorly understood. Here, we develop a rigorous kinetic theory of the extrinsic side-jump contribution to the THE of bosons. We show that the extrinsic THE is always relevant for bosonic systems and can be of the same order as the intrinsic one but sensitively depends on the type of local imperfection. We study different types of impurities and show that a THE can even arise as a pure impurity-induced effect in a system with a vanishing intrinsic contribution. As a side product, we also generalize existing results for the electronic anomalous Hall effect to general types of impurities beyond the standard assumption of local potential scattering. We discuss the importance of our results for the correct interpretation of THE measurements, for example, in the Kitaev magnet 𝛼−RuCl3, and provide a ready-to-use formula for comparison to experimental data. | |
Nakano, R.; Yamada, R.; Bouaziz, J.; Colling, M.; Gen, M.; Shoriki, K.; Okamura, Y.; Kikkawa, A.; Misawa, R.; Baral, P. R.; Kitou, S.; Nakamura, Y.; Ohsumi, H.; Tanaka, Y.; Sagayama, H.; Nakao, H.; Ishihara, Y.; Gautam, K.; Fabelo, O.; Taguchi, Y.; Takahashi, Y.; Tokunaga, M.; Arima, T.; Tokura, Y.; Arita, R.; Masell, J.; Hayami, S.; Hirschberger, M. Perfectly harmonic spin cycloid and multi-Q textures in the Weyl semimetal GdAlSi Journal Article Nat. Commun. 17, (2026), datadoi: 10.5281/zenodo.18228967. @article{nakanoPerfectlyHarmonicSpin2026,
title = {Perfectly harmonic spin cycloid and multi-Q textures in the Weyl semimetal GdAlSi},
author = {R. Nakano and R. Yamada and J. Bouaziz and M. Colling and M. Gen and K. Shoriki and Y. Okamura and A. Kikkawa and R. Misawa and P. R. Baral and S. Kitou and Y. Nakamura and H. Ohsumi and Y. Tanaka and H. Sagayama and H. Nakao and Y. Ishihara and K. Gautam and O. Fabelo and Y. Taguchi and Y. Takahashi and M. Tokunaga and T. Arima and Y. Tokura and R. Arita and J. Masell and S. Hayami and M. Hirschberger},
url = {http://dx.doi.org/10.1038/s41467-026-69452-7},
doi = {10.1038/s41467-026-69452-7},
issn = {2041-1723},
year = {2026},
date = {2026-02-23},
urldate = {2026-02-01},
journal = {Nat. Commun.},
volume = {17},
number = {1},
publisher = {Springer Science and Business Media LLC},
abstract = {A fundamental question in condensed matter physics concerns how topological electronic states are influenced by many-body correlations, and magnetic Weyl semimetals represent an important material platform to address this problem. However, the magnetic structures realized in these materials are limited, and in particular, no clear example of an undistorted helimagnetic state has been definitively identified. Here, we report clear evidence of a harmonic helimagnetic cycloid with an incommensurate magnetic propagation vector Q in the Weyl semimetal GdAlSi via resonant elastic X-ray scattering, including rigorous polarization analysis. This cycloidal structure is consistent with the Dzyaloshinskii–Moriya interaction prescribed by the polar crystal structure of GdAlSi. Upon applying a magnetic field, the cycloid undergoes a transition to a novel multi-Q state. This field-induced, noncoplanar texture is consistent with our numerical spin model, which incorporates the Dzyaloshinskii–Moriya interaction and, crucially, anisotropic exchange interactions. The perfectly harmonic Weyl helimagnet GdAlSi serves as a prototypical platform to study electronic correlation effects in periodically modulated Weyl semimetals.},
note = {datadoi: 10.5281/zenodo.18228967},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
A fundamental question in condensed matter physics concerns how topological electronic states are influenced by many-body correlations, and magnetic Weyl semimetals represent an important material platform to address this problem. However, the magnetic structures realized in these materials are limited, and in particular, no clear example of an undistorted helimagnetic state has been definitively identified. Here, we report clear evidence of a harmonic helimagnetic cycloid with an incommensurate magnetic propagation vector Q in the Weyl semimetal GdAlSi via resonant elastic X-ray scattering, including rigorous polarization analysis. This cycloidal structure is consistent with the Dzyaloshinskii–Moriya interaction prescribed by the polar crystal structure of GdAlSi. Upon applying a magnetic field, the cycloid undergoes a transition to a novel multi-Q state. This field-induced, noncoplanar texture is consistent with our numerical spin model, which incorporates the Dzyaloshinskii–Moriya interaction and, crucially, anisotropic exchange interactions. The perfectly harmonic Weyl helimagnet GdAlSi serves as a prototypical platform to study electronic correlation effects in periodically modulated Weyl semimetals. |  |
Yamaguchi, D.; Mokhtari, P.; Yamada, R.; Kikkawa, A.; Taguchi, Y.; Tokura, Y.; Hirschberger, M. Topological thermal Hall effect and nondissipative transport of the nanometric skyrmion lattice in Gd2PdSi3 Journal Article PNAS Nexus 5, (2026). @article{yamaguchiTopologicalThermalHall2026,
title = {Topological thermal Hall effect and nondissipative transport of the nanometric skyrmion lattice in Gd_{2}PdSi_{3}},
author = {D. Yamaguchi and P. Mokhtari and R. Yamada and A. Kikkawa and Y. Taguchi and Y. Tokura and M. Hirschberger},
url = {http://dx.doi.org/10.1093/pnasnexus/pgag041},
doi = {10.1093/pnasnexus/pgag041},
issn = {2752-6542},
year = {2026},
date = {2026-02-23},
urldate = {2026-02-01},
journal = {PNAS Nexus},
volume = {5},
number = {3},
publisher = {Oxford University Press (OUP)},
abstract = {We report the first observation of a topological thermal Hall effect (tTHE) of electrons moving through a magnetic skyrmion lattice (SkL) of short period, where the skyrmion diameter is only a few nanometers. In the hexagonal intermetallic Gd2PdSi3, we observe a characteristic anomaly in the magnetic field dependence of the thermal Hall conductivity κxy, which scales well with the anomaly in the electrical Hall conductivity σxy and is closely related to the topological winding number of the SkL ground state. The relative magnitude of entropy and charge currents, defined as the Lorenz ratio ∼κxy/(σxyT), is consistent with a nondissipative, or intrinsic, mechanism for the topological Hall effect. We stress that the Berry phase in momentum space (k-space) causes such a nondissipative Hall transport, independent of the carrier relaxation time.},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
We report the first observation of a topological thermal Hall effect (tTHE) of electrons moving through a magnetic skyrmion lattice (SkL) of short period, where the skyrmion diameter is only a few nanometers. In the hexagonal intermetallic Gd2PdSi3, we observe a characteristic anomaly in the magnetic field dependence of the thermal Hall conductivity κxy, which scales well with the anomaly in the electrical Hall conductivity σxy and is closely related to the topological winding number of the SkL ground state. The relative magnitude of entropy and charge currents, defined as the Lorenz ratio ∼κxy/(σxyT), is consistent with a nondissipative, or intrinsic, mechanism for the topological Hall effect. We stress that the Berry phase in momentum space (k-space) causes such a nondissipative Hall transport, independent of the carrier relaxation time. |  |
Shao, J.; Kronseder, M.; Guo, J.; Mangold, M.; Pan, D.; Meier, T. N. G.; Zhao, W.; Zhao, J.; Back, C. H.; Chen, L. Electric-field tunable anisotropic g-Factor induced by spin pumping Journal Article Nano Letters 26, 2853–2860 (2026). @article{shaoElectricfieldTunableAnisotropic2026,
title = {Electric-field tunable anisotropic g-Factor induced by spin pumping},
author = {J. Shao and M. Kronseder and J. Guo and M. Mangold and D. Pan and T. N. G. Meier and W. Zhao and J. Zhao and C. H. Back and L. Chen},
url = {http://dx.doi.org/10.1021/acs.nanolett.5c05536},
doi = {10.1021/acs.nanolett.5c05536},
issn = {1530-6992},
year = {2026},
date = {2026-02-20},
urldate = {2026-02-01},
journal = {Nano Letters},
volume = {26},
number = {8},
pages = {2853–2860},
publisher = {American Chemical Society (ACS)},
abstract = {Spin pumping, a well-established phenomenon where the precessing magnetization of a ferromagnet (FM) injects a pure spin current into an adjacent nonmagnetic layer, is characteristically identified by the enhancement of magnetic damping in the FM. Theoretical work has also suggested that spin pumping can affect the Landé g-factoranother key parameter of ferromagnetic materials besides the magnetic damping. However, experimental evidence of this effect has remained limited. Here, we demonstrate that spin pumping can lead to significant modulation of the g-factor in a Py/AlOx/STO two-dimensional electron gas (2DEG) system with strong spin–orbit interaction. Specifically, we observe an anisotropic g-factor with 2-fold symmetry below the onset temperature of the 2DEG, and furthermore this anisotropy can be tuned when applying an external electric field. This work uncovers a previously overlooked effect and offers new possibilities for controlling magnetization dynamics in systems with a reduced dimension.},
keywords = {A2},
pubstate = {published},
tppubtype = {article}
}
Spin pumping, a well-established phenomenon where the precessing magnetization of a ferromagnet (FM) injects a pure spin current into an adjacent nonmagnetic layer, is characteristically identified by the enhancement of magnetic damping in the FM. Theoretical work has also suggested that spin pumping can affect the Landé g-factoranother key parameter of ferromagnetic materials besides the magnetic damping. However, experimental evidence of this effect has remained limited. Here, we demonstrate that spin pumping can lead to significant modulation of the g-factor in a Py/AlOx/STO two-dimensional electron gas (2DEG) system with strong spin–orbit interaction. Specifically, we observe an anisotropic g-factor with 2-fold symmetry below the onset temperature of the 2DEG, and furthermore this anisotropy can be tuned when applying an external electric field. This work uncovers a previously overlooked effect and offers new possibilities for controlling magnetization dynamics in systems with a reduced dimension. |  |
Schilberth, F.; Kondákor, M.; Ukolov, D.; Pawbake, A.; Vasin, K.; Ercem, O.; Prodan, L.; Tsurkan, V.; Tsirlin, A. A.; Faugeras, C.; Lemmens, P.; Penc, K.; Kézsmárki, I.; Bordács, S.; Deisenhofer, J. Optical phonons as a testing ground for spin group symmetries Journal Article npj Quantum Mater. 11, 26 (2026), datadoi: 10.5281/zenodo.16751739. @article{schilberthOpticalPhononsTesting2025,
title = {Optical phonons as a testing ground for spin group symmetries},
author = {F. Schilberth and M. Kondákor and D. Ukolov and A. Pawbake and K. Vasin and O. Ercem and L. Prodan and V. Tsurkan and A. A. Tsirlin and C. Faugeras and P. Lemmens and K. Penc and I. Kézsmárki and S. Bordács and J. Deisenhofer},
url = {https://doi.org/10.1038/s41535-026-00857-9},
doi = {0.1038/s41535-026-00857-9},
year = {2026},
date = {2026-02-17},
urldate = {2026-02-01},
journal = {npj Quantum Mater.},
volume = {11},
pages = {26},
abstract = {Lattice vibrations are highly sensitive to crystal symmetries and their changes across phase transitions. The latter can modify irreducible (co)representations and corresponding infrared and Raman selection rules of phonons. This concept is established for relativistic magnetic point groups, simultaneously transforming spatial and spin coordinates. However, in altermagnets described by non-relativistic spin groups with disjunct symmetry operations for both vector spaces, the phonon selection rules have remained unexplored. Here, we present a detailed study of the infrared- and Raman-active modes in the collinear antiferromagnet and altermagnet candidate Co2Mo3O8. Comparing to ab initio calculations accurately capturing the eigenfrequencies, we identify all expected phonon modes at room temperature and deduce their selection rules using both symmetry approaches. Importantly, we observe the change of selection rules upon antiferromagnetic ordering, agreeing with the relativistic symmetry approach, while the spin group formalism predicts no changes. Therefore, optical phonons sensing the symmetry of the magnetic order can reveal if relevant magnon-phonon coupling is compatible with the spin-group approach or not.},
note = {datadoi: 10.5281/zenodo.16751739},
keywords = {B1, C4},
pubstate = {published},
tppubtype = {article}
}
Lattice vibrations are highly sensitive to crystal symmetries and their changes across phase transitions. The latter can modify irreducible (co)representations and corresponding infrared and Raman selection rules of phonons. This concept is established for relativistic magnetic point groups, simultaneously transforming spatial and spin coordinates. However, in altermagnets described by non-relativistic spin groups with disjunct symmetry operations for both vector spaces, the phonon selection rules have remained unexplored. Here, we present a detailed study of the infrared- and Raman-active modes in the collinear antiferromagnet and altermagnet candidate Co2Mo3O8. Comparing to ab initio calculations accurately capturing the eigenfrequencies, we identify all expected phonon modes at room temperature and deduce their selection rules using both symmetry approaches. Importantly, we observe the change of selection rules upon antiferromagnetic ordering, agreeing with the relativistic symmetry approach, while the spin group formalism predicts no changes. Therefore, optical phonons sensing the symmetry of the magnetic order can reveal if relevant magnon-phonon coupling is compatible with the spin-group approach or not. |  |
Küchler, R.; Panja, S. N.; Wirth, S.; Gegenwart, P. High-resolution capacitance dilatometry of microscopically thin samples using a miniature dilatometer Journal Article Rev. Sci. Instrum. 97, 025209 (2026). @article{kuchlerHighresolutionCapacitanceDilatometry2026,
title = {High-resolution capacitance dilatometry of microscopically thin samples using a miniature dilatometer},
author = {R. Küchler and S. N. Panja and S. Wirth and P. Gegenwart},
url = {https://doi.org/10.1063/5.0300507},
doi = {10.1063/5.0300507},
issn = {0034-6748},
year = {2026},
date = {2026-02-12},
urldate = {2026-02-01},
journal = {Rev. Sci. Instrum.},
volume = {97},
number = {2},
pages = {025209},
abstract = {We present a novel application of our high-resolution capacitance dilatometer, specifically engineered for the precise characterization of quantum materials. These materials, which often appear as ultrathin, platelet-shaped crystals, are known for exotic phenomena such as superconductivity, topological order, and quantum spin liquid. However, these crystals seldom reach macroscopic dimensions, making them unsuitable for conventional dilatometry techniques. By introducing a modified sample-mounting configuration, our design enables high-resolution measurements of thermal expansion and magnetostriction along in-plane crystallographic directions in samples with thicknesses well below 500 μm. Validation measurements using a Quantum Design PPMS system confirm reliable performance for a 300 μm-thick silver platelet, relatively hard ferromagnetic EuB6 single crystals down to 50 μm, and a 40 μm-thin, soft AgCrS2 single crystal. This advancement significantly broadens the applicability of capacitance dilatometry, providing a powerful platform for investigating emergent phenomena in reduced-dimensional quantum systems.},
keywords = {B1, B3},
pubstate = {published},
tppubtype = {article}
}
We present a novel application of our high-resolution capacitance dilatometer, specifically engineered for the precise characterization of quantum materials. These materials, which often appear as ultrathin, platelet-shaped crystals, are known for exotic phenomena such as superconductivity, topological order, and quantum spin liquid. However, these crystals seldom reach macroscopic dimensions, making them unsuitable for conventional dilatometry techniques. By introducing a modified sample-mounting configuration, our design enables high-resolution measurements of thermal expansion and magnetostriction along in-plane crystallographic directions in samples with thicknesses well below 500 μm. Validation measurements using a Quantum Design PPMS system confirm reliable performance for a 300 μm-thick silver platelet, relatively hard ferromagnetic EuB6 single crystals down to 50 μm, and a 40 μm-thin, soft AgCrS2 single crystal. This advancement significantly broadens the applicability of capacitance dilatometry, providing a powerful platform for investigating emergent phenomena in reduced-dimensional quantum systems. |  |
Ohanyan, V.; Amiraghyan, L.; Sekania, M.; Kollar, M. Electric-field driven flat bands in the distorted sawtooth chain via the Katsura–Nagaosa–Balatsky mechanism Journal Article Z. Naturforsch. A 81, 289 (2026). @article{ohanyanElectricfieldDrivenFlat2026,
title = {Electric-field driven flat bands in the distorted sawtooth chain via the Katsura–Nagaosa–Balatsky mechanism},
author = {V. Ohanyan and L. Amiraghyan and M. Sekania and M. Kollar},
url = {https://doi.org/10.1515/zna-2025-0381},
doi = {doi:10.1515/zna-2025-0381},
year = {2026},
date = {2026-02-10},
urldate = {2026-02-01},
journal = {Z. Naturforsch. A},
volume = {81},
number = {4},
pages = {289},
abstract = {We investigate flat magnonic bands in a generalized sawtooth-chain model in which three sets of exchange parameters (symmetric Heisenberg exchange, axial Ising anisotropy, and antisymmetric Dzyaloshinskii–Moriya (DM) exchange) are assigned independently to each side of the triangular plaquette. If the effective Dzyaloshinskii–Moriya (DM) interaction parameters are generated via the Katsura–Nagaosa–Balatsky (KNB) mechanism of magnetoelectricity, they become explicit functions of the electric-field magnitude and direction, as well as of the lattice geometry, which in the present case is characterized by two bond angles. We focus on the situation in which these two angles are unequal, corresponding to a distortion of the triangular plaquette. Several electric-field–induced flat-band scenarios in the distorted sawtooth chain are analyzed, and expressions are derived for the electric-field strength required to drive the one-magnon excitations into a flat-band regime when the field is aligned along the lattice bonds. The saturation field and its dependence on the distortion angle are also examined. Finally, we establish a mapping between the flat-band solutions for a general DM interaction and its specific KNB-induced form.},
keywords = {C4},
pubstate = {published},
tppubtype = {article}
}
We investigate flat magnonic bands in a generalized sawtooth-chain model in which three sets of exchange parameters (symmetric Heisenberg exchange, axial Ising anisotropy, and antisymmetric Dzyaloshinskii–Moriya (DM) exchange) are assigned independently to each side of the triangular plaquette. If the effective Dzyaloshinskii–Moriya (DM) interaction parameters are generated via the Katsura–Nagaosa–Balatsky (KNB) mechanism of magnetoelectricity, they become explicit functions of the electric-field magnitude and direction, as well as of the lattice geometry, which in the present case is characterized by two bond angles. We focus on the situation in which these two angles are unequal, corresponding to a distortion of the triangular plaquette. Several electric-field–induced flat-band scenarios in the distorted sawtooth chain are analyzed, and expressions are derived for the electric-field strength required to drive the one-magnon excitations into a flat-band regime when the field is aligned along the lattice bonds. The saturation field and its dependence on the distortion angle are also examined. Finally, we establish a mapping between the flat-band solutions for a general DM interaction and its specific KNB-induced form. |  |
Gaggl, T.; Misawa, R.; Kriener, M.; Tanaka, Y.; Yamada, R.; Hirschberger, M. Bulk superconductivity in the kagome metal YRu3B2 Journal Article Phys. Scr. 101, 055912 (2026), datadoi: (10.5281/zenodo.18276372). @article{gagglBulkSuperconductivityKagome2026,
title = {Bulk superconductivity in the kagome metal YRu_{3}B_{2}},
author = {T. Gaggl and R. Misawa and M. Kriener and Y. Tanaka and R. Yamada and M. Hirschberger},
url = {https://doi.org/10.1088/1402-4896/ae3c65},
doi = {10.1088/1402-4896/ae3c65},
year = {2026},
date = {2026-02-05},
urldate = {2026-02-01},
journal = {Phys. Scr.},
volume = {101},
number = {5},
pages = {055912},
abstract = {Materials with a kagome lattice have been heavily studied for their exotic electronic band structure, geometrical frustration, high-temperature charge-order transitions, and unconventional electron-phonon coupling. In LaRu3Si2, it was proposed that electronic flat bands conspire with the characteristic phonon spectrum of the kagome lattice to drive enhanced superconductivity at Tc = 6.8 K. Here, we report bulk superconductivity in the structural analogue YRu3B2, which hosts a pristine kagome lattice. We observe a superconducting transition at Tc = 0.7 K through magnetization, resistivity, and heat-capacity measurements in this novel kagome metal.},
note = {datadoi: (10.5281/zenodo.18276372)},
keywords = {B5, C1},
pubstate = {published},
tppubtype = {article}
}
Materials with a kagome lattice have been heavily studied for their exotic electronic band structure, geometrical frustration, high-temperature charge-order transitions, and unconventional electron-phonon coupling. In LaRu3Si2, it was proposed that electronic flat bands conspire with the characteristic phonon spectrum of the kagome lattice to drive enhanced superconductivity at Tc = 6.8 K. Here, we report bulk superconductivity in the structural analogue YRu3B2, which hosts a pristine kagome lattice. We observe a superconducting transition at Tc = 0.7 K through magnetization, resistivity, and heat-capacity measurements in this novel kagome metal. |  |
Weber, T.; Heinsdorf, N.; Stekiel, M.; Steffens, P.; Schnyder, A. P.; Pfleiderer, C. Nonreciprocal zone boundary magnon propagation in Cu2OSeO3 Journal Article Phys. Rev. B 113, L020414 (2026), datadoi: 10.5281/zenodo.16600991. @article{weberNonreciprocalZoneBoundary2026,
title = {Nonreciprocal zone boundary magnon propagation in Cu_{2}OSeO_{3}},
author = {T. Weber and N. Heinsdorf and M. Stekiel and P. Steffens and A. P. Schnyder and C. Pfleiderer},
url = {https://link.aps.org/doi/10.1103/q77j-5g59},
doi = {10.1103/q77j-5g59},
year = {2026},
date = {2026-01-29},
urldate = {2026-01-29},
journal = {Phys. Rev. B},
volume = {113},
number = {2},
pages = {L020414},
publisher = {American Physical Society},
abstract = {Inelastic neutron scattering in the chiral magnet Cu2OSeO3 reveals strong nonreciprocal effects on magnon propagation at the boundary of the nuclear Brillouin zone. The nonreciprocal response is strongest at a central position between the zone corner and the edge midpoint. We explain these results using an effective linear spin-wave model. While directional effects in chiral magnets have so far only been known to exist at low momenta close to the center of the Brillouin zone, the present study shows that nonreciprocity persists at the highest possible reduced momenta. The observed magnons show very little damping within the limits of our experimental resolution, making them of great interest for the fundamental research on compact, high-frequency magnonic applications.},
note = {datadoi: 10.5281/zenodo.16600991},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
Inelastic neutron scattering in the chiral magnet Cu2OSeO3 reveals strong nonreciprocal effects on magnon propagation at the boundary of the nuclear Brillouin zone. The nonreciprocal response is strongest at a central position between the zone corner and the edge midpoint. We explain these results using an effective linear spin-wave model. While directional effects in chiral magnets have so far only been known to exist at low momenta close to the center of the Brillouin zone, the present study shows that nonreciprocity persists at the highest possible reduced momenta. The observed magnons show very little damping within the limits of our experimental resolution, making them of great interest for the fundamental research on compact, high-frequency magnonic applications. |  |
Gammon-Smith, A.; Knap, M.; Pollmann, F. Simulating topological order on quantum processors Journal Article Nat. Rev. Phys. 8, 160–170 (2026). @article{gammon-smithSimulatingTopologicalOrder2026,
title = {Simulating topological order on quantum processors},
author = {A. Gammon-Smith and M. Knap and F. Pollmann},
url = {https://doi.org/10.1038/s42254-025-00911-8},
doi = {10.1038/s42254-025-00911-8},
issn = {2522-5820},
year = {2026},
date = {2026-01-26},
urldate = {2026-01-01},
journal = {Nat. Rev. Phys.},
volume = {8},
number = {3},
pages = {160–170},
publisher = {Springer Science and Business Media LLC},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Magar, A.; Somesh, K.; Saravanan, M. P.; Sichelschmidt, J.; Skourski, Y.; Telling, M. T. F.; Ginga, V. A.; Tsirlin, A. A.; Nath, R. Proximate spin-liquid behavior in the double trillium lattice antiferromagnet K2Co2(SO4)3 Journal Article Phys. Rev. B 113, L020409 (2026). @article{magarProximateSpinliquidBehavior2025,
title = {Proximate spin-liquid behavior in the double trillium lattice antiferromagnet K_{2}Co_{2}(SO_{4})_{3}},
author = {A. Magar and K. Somesh and M. P. Saravanan and J. Sichelschmidt and Y. Skourski and M. T. F. Telling and V. A. Ginga and A. A. Tsirlin and R. Nath},
url = {https://doi.org/10.1103/m8mj-slvl},
doi = {10.1103/m8mj-slvl},
year = {2026},
date = {2026-01-16},
urldate = {2026-01-01},
journal = {Phys. Rev. B},
volume = {113},
number = {2},
pages = {L020409},
abstract = {We report proximate quantum spin liquid behavior in K2Co2 (SO4)3 with the magnetic Co2+ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder x-ray diffraction experiments reveal a structural phase transition at 𝑇_t≃125K from high-temperature cubic to low-temperature monoclinic phase with the threefold superstructure. Magnetization and heat capacity consistently show the formation of the 𝐽eff=1/2 state of Co2+ below 50 K. In zero field, K2Co2(SO4)3 shows signatures of static magnetic order formed below 𝑇*≃0.6K, but muon spin relaxation experiments reveal a large fluctuating component that persists down to at least 50 mK, reminiscent of quantum spin liquid (QSL). Static order is completely suppressed in the small magnetic field of ∼1T, and low-temperature heat capacity demonstrates the 𝑇2 behavior above this field, another fingerprint of QSL. Ab initio calculations show a competition of several antiferromagnetic couplings that render K2Co2(SO4)3 a promising pseudospin-1/2 material for studying quantum magnetism in the double trillium lattice geometry.},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
We report proximate quantum spin liquid behavior in K2Co2 (SO4)3 with the magnetic Co2+ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder x-ray diffraction experiments reveal a structural phase transition at 𝑇_t≃125K from high-temperature cubic to low-temperature monoclinic phase with the threefold superstructure. Magnetization and heat capacity consistently show the formation of the 𝐽eff=1/2 state of Co2+ below 50 K. In zero field, K2Co2(SO4)3 shows signatures of static magnetic order formed below 𝑇*≃0.6K, but muon spin relaxation experiments reveal a large fluctuating component that persists down to at least 50 mK, reminiscent of quantum spin liquid (QSL). Static order is completely suppressed in the small magnetic field of ∼1T, and low-temperature heat capacity demonstrates the 𝑇2 behavior above this field, another fingerprint of QSL. Ab initio calculations show a competition of several antiferromagnetic couplings that render K2Co2(SO4)3 a promising pseudospin-1/2 material for studying quantum magnetism in the double trillium lattice geometry. |  |
Yamada, R.; Kurebayashi, D.; Fujishiro, Y.; Okumura, S.; Nakamura, D.; Yasin, F. S.; Nakajima, T.; Yokouchi, T.; Kikkawa, A.; Taguchi, Y.; Tokura, Y.; Tretiakov, O. A.; Hirschberger, M. Emergent electric field induced by dissipative sliding dynamics of domain walls in a Weyl magnet Journal Article Nat. Phys. 22, 239–244 (2026), datadoi: (10.5281/zenodo.17188494). @article{yamadaEmergentElectricField2026,
title = {Emergent electric field induced by dissipative sliding dynamics of domain walls in a Weyl magnet},
author = {R. Yamada and D. Kurebayashi and Y. Fujishiro and S. Okumura and D. Nakamura and F. S. Yasin and T. Nakajima and T. Yokouchi and A. Kikkawa and Y. Taguchi and Y. Tokura and O. A. Tretiakov and M. Hirschberger},
url = {https://doi.org/10.1038/s41567-025-03124-z},
doi = {10.1038/s41567-025-03124-z},
year = {2026},
date = {2026-01-15},
urldate = {2026-01-01},
journal = {Nat. Phys.},
volume = {22},
number = {2},
pages = {239–244},
abstract = {The dynamic motion of topological defects in magnets induces an emergent electric field, as exemplified by the continuous flow of skyrmion vortices. However, the electrodynamics underlying this emergent field remains poorly understood. In this context, magnetic domain walls—one-dimensional topological defects with two collective modes, sliding and spin-tilt—offer a promising platform for exploration. Here we demonstrate that the dissipative motion of domain walls under oscillatory current excitation generates an emergent electric field. We image domain patterns and quantify the domain-wall length under applied magnetic fields in mesoscopic devices based on the magnetic Weyl semimetal NdAlSi. These devices exhibit exceptionally strong domain-wall scattering and a pronounced emergent electric field, as observed in the imaginary component of the complex impedance. Spin dynamics simulations reveal that domain-wall sliding dominates over spin-tilting, in which the phase delay of the domain-wall motion with respect to the driving force impacts the emergent electric field. Our findings establish domain-wall dynamics as a platform for studying emergent electromagnetic fields and motivate further investigations of the coupled motion of magnetic solitons and conduction electrons.},
note = {datadoi: (10.5281/zenodo.17188494)},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
The dynamic motion of topological defects in magnets induces an emergent electric field, as exemplified by the continuous flow of skyrmion vortices. However, the electrodynamics underlying this emergent field remains poorly understood. In this context, magnetic domain walls—one-dimensional topological defects with two collective modes, sliding and spin-tilt—offer a promising platform for exploration. Here we demonstrate that the dissipative motion of domain walls under oscillatory current excitation generates an emergent electric field. We image domain patterns and quantify the domain-wall length under applied magnetic fields in mesoscopic devices based on the magnetic Weyl semimetal NdAlSi. These devices exhibit exceptionally strong domain-wall scattering and a pronounced emergent electric field, as observed in the imaginary component of the complex impedance. Spin dynamics simulations reveal that domain-wall sliding dominates over spin-tilting, in which the phase delay of the domain-wall motion with respect to the driving force impacts the emergent electric field. Our findings establish domain-wall dynamics as a platform for studying emergent electromagnetic fields and motivate further investigations of the coupled motion of magnetic solitons and conduction electrons. |  |
Khodaeva, U. E.; Kovrizhin, D. L.; Knolle, J. Quantum critical dynamical response of the twisted Kitaev spin chain Journal Article Phys. Rev. B 113, 045120 (2026), datadoi: 10.5281/zenodo.15722856. @article{khodaevaQuantumCriticalDynamical2026,
title = {Quantum critical dynamical response of the twisted Kitaev spin chain},
author = {U. E. Khodaeva and D. L. Kovrizhin and J. Knolle},
url = {https://link.aps.org/doi/10.1103/884v-7tqh},
doi = {10.1103/884v-7tqh},
year = {2026},
date = {2026-01-12},
urldate = {2026-01-01},
journal = {Phys. Rev. B},
volume = {113},
number = {4},
pages = {045120},
publisher = {American Physical Society},
abstract = {The dynamical structure factor of the transverse field Ising model (TFIM) shows universal power-law divergence at its quantum critical point, signatures of which have been arguably observed in inelastic neutron scattering studies of quantum spin chain materials, for example CoNb2O6. However, it has recently been suggested that its microscopic description is better captured in terms of a twisted Kitaev spin chain (TKSC) with bond-anisotropic couplings. Here, we present exact results for the dynamical structure factor of the TKSC across its quantum critical point, analyzing both the universal low-frequency response and the non-universal high-energy features. In addition, we explore extensions of the model including broken glide symmetry as well as the case of random, and incommensurate magnetic fields. Notably, in the latter case, the fermionic excitations exhibit a localization-delocalization transition, which is manifest in the dynamical response as a distinct signature at finite frequency. We discuss the relevance of these features for the observation of quantum critical response in experiments.},
note = {datadoi: 10.5281/zenodo.15722856},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
The dynamical structure factor of the transverse field Ising model (TFIM) shows universal power-law divergence at its quantum critical point, signatures of which have been arguably observed in inelastic neutron scattering studies of quantum spin chain materials, for example CoNb2O6. However, it has recently been suggested that its microscopic description is better captured in terms of a twisted Kitaev spin chain (TKSC) with bond-anisotropic couplings. Here, we present exact results for the dynamical structure factor of the TKSC across its quantum critical point, analyzing both the universal low-frequency response and the non-universal high-energy features. In addition, we explore extensions of the model including broken glide symmetry as well as the case of random, and incommensurate magnetic fields. Notably, in the latter case, the fermionic excitations exhibit a localization-delocalization transition, which is manifest in the dynamical response as a distinct signature at finite frequency. We discuss the relevance of these features for the observation of quantum critical response in experiments. |  |
Winkler, M.; Prodan, L.; Tsurkan, V.; Lunkenheimer, P.; Kézsmárki, I.; Ghara, S. Strong magnetocapacitance anomaly signals the onset of the magnetoelectric Néel-type antiferromagnetic order in Co3O4 Journal Article Phys. Rev. B 113, 024409 (2026), datadoi: 10.5281/zenodo.17878913. @article{winklerStrongMagnetocapacitanceAnomaly2026,
title = {Strong magnetocapacitance anomaly signals the onset of the magnetoelectric Néel-type antiferromagnetic order in Co_{3}O_{4}},
author = {M. Winkler and L. Prodan and V. Tsurkan and P. Lunkenheimer and I. Kézsmárki and S. Ghara},
url = {https://link.aps.org/doi/10.1103/d9tp-h4wz},
doi = {10.1103/d9tp-h4wz},
issn = {2469-9950, 2469-9969},
year = {2026},
date = {2026-01-12},
urldate = {2026-01-12},
journal = {Phys. Rev. B},
volume = {113},
number = {2},
pages = {024409},
abstract = {The magnetoelectric antiferromagnet Co3O4 has recently been reported as a promising platform for isothermal electric manipulation of antiferromagnetic states. Here, we report a detailed study on magnetization, heat capacity, dielectric properties, and electric polarization in single crystals of Co3O4. Magnetization and heat capacity measurements affirm the occurrence of a Néel-type collinear antiferromagnetic ordering below its Néel temperature 𝑇N = 30 K, where the direction of the Néel vector can be rotated by weak fields. This magnetic ordering breaks the spatial inversion and time reversal symmetries and permits a strong linear magnetoelectric effect, leading to the emergence of field-induced electric polarization below 𝑇N, and is also manifested in a magnetic field-induced sharp 𝜆-like peak in the dielectric constant at 𝑇N. Notably, the corresponding magnetocapacitance reaches a maximum value as high as 110% close to 𝑇N. This magnetocapacitance exhibits a quadratic dependence on the strength of the applied magnetic field, which is discussed within the framework of a phenomenological Landau theory.},
note = {datadoi: 10.5281/zenodo.17878913},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
The magnetoelectric antiferromagnet Co3O4 has recently been reported as a promising platform for isothermal electric manipulation of antiferromagnetic states. Here, we report a detailed study on magnetization, heat capacity, dielectric properties, and electric polarization in single crystals of Co3O4. Magnetization and heat capacity measurements affirm the occurrence of a Néel-type collinear antiferromagnetic ordering below its Néel temperature 𝑇N = 30 K, where the direction of the Néel vector can be rotated by weak fields. This magnetic ordering breaks the spatial inversion and time reversal symmetries and permits a strong linear magnetoelectric effect, leading to the emergence of field-induced electric polarization below 𝑇N, and is also manifested in a magnetic field-induced sharp 𝜆-like peak in the dielectric constant at 𝑇N. Notably, the corresponding magnetocapacitance reaches a maximum value as high as 110% close to 𝑇N. This magnetocapacitance exhibits a quadratic dependence on the strength of the applied magnetic field, which is discussed within the framework of a phenomenological Landau theory. |  |
d'Ornellas, P.; Leeb, V.; Grushin, A. G.; Knolle, J. Altermagnetism without crystal symmetry Journal Article Phys. Rev. B 113, 024426 (2026), datadoi: https://github.com/dpreuo/alter_morph. @article{dornellasAltermagnetismCrystalSymmetry2026,
title = {Altermagnetism without crystal symmetry},
author = {P. d'Ornellas and V. Leeb and A. G. Grushin and J. Knolle},
url = {https://link.aps.org/doi/10.1103/zqnk-153f},
doi = {10.1103/zqnk-153f},
year = {2026},
date = {2026-01-01},
journal = {Phys. Rev. B},
volume = {113},
number = {2},
pages = {024426},
publisher = {American Physical Society},
abstract = {Altermagnetism is a collinear magnetic order in which opposite spin species are exchanged under a real-space rotation. Hence, the search for physical realizations has focused on crystalline solids with specific rotational symmetry. Here, we show that altermagnetism can also emerge in noncrystalline systems, such as amorphous solids, despite the lack of global rotational symmetries. We construct a minimal Hamiltonian with two directional orbitals per site on an amorphous lattice with interactions that are invariant under spin rotation. Altermagnetism then arises due to spontaneous symmetry breaking in the spin and orbital degrees of freedom around each atom, displaying a common point group symmetry. This form of altermagnetism exhibits anisotropic spin transport and spin spectral functions, both experimentally measurable. Our mechanism generalizes to any lattice and any altermagnetic order, opening the search for altermagnetic phenomena to noncrystalline systems.},
note = {datadoi: https://github.com/dpreuo/alter_morph},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Altermagnetism is a collinear magnetic order in which opposite spin species are exchanged under a real-space rotation. Hence, the search for physical realizations has focused on crystalline solids with specific rotational symmetry. Here, we show that altermagnetism can also emerge in noncrystalline systems, such as amorphous solids, despite the lack of global rotational symmetries. We construct a minimal Hamiltonian with two directional orbitals per site on an amorphous lattice with interactions that are invariant under spin rotation. Altermagnetism then arises due to spontaneous symmetry breaking in the spin and orbital degrees of freedom around each atom, displaying a common point group symmetry. This form of altermagnetism exhibits anisotropic spin transport and spin spectral functions, both experimentally measurable. Our mechanism generalizes to any lattice and any altermagnetic order, opening the search for altermagnetic phenomena to noncrystalline systems. | |
Davenport, H.; Knolle, J.; Schindler, F. Exciton Berryology Journal Article Phys. Rev. B 113, 045125 (2026). @article{davenportExcitonBerryology2026,
title = {Exciton Berryology},
author = {H. Davenport and J. Knolle and F. Schindler},
url = {https://link.aps.org/doi/10.1103/jtgq-vc7n},
doi = {10.1103/jtgq-vc7n},
year = {2026},
date = {2026-01-01},
journal = {Phys. Rev. B},
volume = {113},
number = {4},
pages = {045125},
publisher = {American Physical Society},
abstract = {In translationally invariant semiconductors that host exciton bound states, one can define an infinite number of possible exciton Berry connections. These correspond to the different ways in which a many-body exciton state, at fixed total momentum, can be decomposed into free electron and hole Bloch states that are entangled by an exciton envelope wave function. Inspired by the modern theory of polarization, we define an exciton projected position operator whose eigenvalues single out two unique choices of exciton Berry phase and associated Berry connection—one for electrons, and one for holes. We clarify the physical meaning of these exciton Berry phases and provide a discrete Wilson loop formulation that allows for their numerical calculation without a smooth gauge. As a corollary, we obtain a gauge-invariant expression for the exciton polarization at a given total momentum, i.e., the mean separation of the electron and hole within the exciton wave function. In the presence of crystalline inversion symmetry, the electron and hole exciton Berry phases are quantized to the same value and we derive how this value can be expressed in terms of inversion eigenvalues of the many-body exciton state. We then consider 𝐶2𝒯 symmetry, for which no symmetry eigenvalues are available as it is antiunitary, and confirm that the exciton Berry phase remains quantized and still diagnoses topologically distinct exciton bands. The notion of shift excitons, whose exciton Wannier states are displaced from those of the noninteracting bands by a quantized amount, can therefore be generalized beyond symmetry indicators.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
In translationally invariant semiconductors that host exciton bound states, one can define an infinite number of possible exciton Berry connections. These correspond to the different ways in which a many-body exciton state, at fixed total momentum, can be decomposed into free electron and hole Bloch states that are entangled by an exciton envelope wave function. Inspired by the modern theory of polarization, we define an exciton projected position operator whose eigenvalues single out two unique choices of exciton Berry phase and associated Berry connection—one for electrons, and one for holes. We clarify the physical meaning of these exciton Berry phases and provide a discrete Wilson loop formulation that allows for their numerical calculation without a smooth gauge. As a corollary, we obtain a gauge-invariant expression for the exciton polarization at a given total momentum, i.e., the mean separation of the electron and hole within the exciton wave function. In the presence of crystalline inversion symmetry, the electron and hole exciton Berry phases are quantized to the same value and we derive how this value can be expressed in terms of inversion eigenvalues of the many-body exciton state. We then consider 𝐶2𝒯 symmetry, for which no symmetry eigenvalues are available as it is antiunitary, and confirm that the exciton Berry phase remains quantized and still diagnoses topologically distinct exciton bands. The notion of shift excitons, whose exciton Wannier states are displaced from those of the noninteracting bands by a quantized amount, can therefore be generalized beyond symmetry indicators. | |
Upadhyay, P.; Suárez-Forero, D. G.; Huang, T. -S.; Mehrabad, M. J.; Gao, B.; Sarkar, S.; Session, D.; Watanabe, K.; Taniguchi, T.; Zhou, Y.; Knap, M.; Hafezi, M. Giant enhancement of exciton diffusion near an electronic Mott insulator Journal Article Science 391, 394–398 (2026), datadoi: 10.5061/dryad.3r2280gv7. @article{upadhyayGiantEnhancementExciton2026,
title = {Giant enhancement of exciton diffusion near an electronic Mott insulator},
author = {P. Upadhyay and D. G. Suárez-Forero and T. -S. Huang and M. J. Mehrabad and B. Gao and S. Sarkar and D. Session and K. Watanabe and T. Taniguchi and Y. Zhou and M. Knap and M. Hafezi},
url = {https://doi.org/10.1126/science.ads5266},
doi = {10.1126/science.ads5266},
issn = {1095-9203},
year = {2026},
date = {2026-01-01},
urldate = {2026-01-01},
journal = {Science},
volume = {391},
number = {6783},
pages = {394–398},
publisher = {American Association for the Advancement of Science (AAAS)},
note = {datadoi: 10.5061/dryad.3r2280gv7},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Krey, O.; Menner, M.; Peter, S.; Schleicher, M.; Thurner-Irmler, J. „Der andere Magnetismus“ – Konzeption und Erprobung eines School_Lab-Bausteins mit Gamification-Elementen Book Section In: Wenzel, A.; Schmäing, T. (Ed.): Außerschulisches lernen in der naturwissenschaftlichen bildung: Eine multiperspektivische betrachtung, 35–61 Springer Fachmedien Wiesbaden, Wiesbaden, (2026), ISBN: 978-3-658-50864-7. @incollection{Krey2026,
title = {„Der andere Magnetismus“ – Konzeption und Erprobung eines School_Lab-Bausteins mit Gamification-Elementen},
author = {O. Krey and M. Menner and S. Peter and M. Schleicher and J. Thurner-Irmler},
editor = {A. Wenzel and T. Schmäing},
url = {https://doi.org/10.1007/978-3-658-50864-7_3},
doi = {10.1007/978-3-658-50864-7_3},
isbn = {978-3-658-50864-7},
year = {2026},
date = {2026-09-02},
urldate = {2026-09-01},
booktitle = {Außerschulisches lernen in der naturwissenschaftlichen bildung: Eine multiperspektivische betrachtung},
pages = {35–61},
publisher = {Springer Fachmedien Wiesbaden},
address = {Wiesbaden},
abstract = {Die Auseinandersetzung mit aktuellen Quantenthemen erfordert eine frühzeitige, verständliche Heranführung von Schüler*innen an abstrakte physikalische Konzepte. Gamification wird dabei in der MINT-Bildung häufig als Ansatz diskutiert, um (situationales) Interesse zu wecken und Lernprozesse bei komplexen oder als abstrakt wahrgenommenen Inhalten zu unterstützen. Vor diesem Hintergrund wurde das außerschulische Programm “Der andere Magnetismus” entwickelt, in welchem Magnetismusarten als fachliche Grundlage für Quantenmaterialien experimentell erschlossen werden sollen. Zur Untersuchung der Wirkung von Gamification v. a. auf situationales Interesse wurde das Angebot in einer gamifizierten (g) und nicht-gamifizierten (ng) Variante durchgeführt und in einer Pilotstudie verglichen (Ng = 27},
keywords = {WIKO},
pubstate = {published},
tppubtype = {incollection}
}
Die Auseinandersetzung mit aktuellen Quantenthemen erfordert eine frühzeitige, verständliche Heranführung von Schüler*innen an abstrakte physikalische Konzepte. Gamification wird dabei in der MINT-Bildung häufig als Ansatz diskutiert, um (situationales) Interesse zu wecken und Lernprozesse bei komplexen oder als abstrakt wahrgenommenen Inhalten zu unterstützen. Vor diesem Hintergrund wurde das außerschulische Programm “Der andere Magnetismus” entwickelt, in welchem Magnetismusarten als fachliche Grundlage für Quantenmaterialien experimentell erschlossen werden sollen. Zur Untersuchung der Wirkung von Gamification v. a. auf situationales Interesse wurde das Angebot in einer gamifizierten (g) und nicht-gamifizierten (ng) Variante durchgeführt und in einer Pilotstudie verglichen (Ng = 27 | |
Pazmino, E. I.; Feng, S.; Dhakal, R.; Rousochatzakis, I.; Winter, S. M.; Knolle, J.; Tsirlin, A. A. Beyond Kitaev exchange: Γ'-driven magnetism in Ag3LiRh2O6 Unpublished (2026), arXiv:2610.19770. @unpublished{pazminoKitaevExchangeGammadriven2026,
title = {Beyond Kitaev exchange: Γ'-driven magnetism in Ag_{3}LiRh_{2}O_{6}},
author = {E. I. Pazmino and S. Feng and R. Dhakal and I. Rousochatzakis and S. M. Winter and J. Knolle and A. A. Tsirlin},
url = {https://arxiv.org/abs/2610.19770},
doi = {10.48550/arXiv.2610.19770},
year = {2026},
date = {2026-10-14},
urldate = {2026-10-14},
abstract = {In Kitaev magnets, frustration arises from bond-dependent spin anisotropic interactions, which can potentially realize sought-after quantum spin liquid phases. However, material realizations with dominating Kitaev exchange are scarce and the broad parameter space of extended Kitaev models remains largely unexplored experimentally. Here, we use density-functional theory, cluster many-body, spin-wave, and density-matrix renormalization calculations to show that the recently discovered honeycomb rhodate Ag3LiRh2O6 hosts an off-diagonal exchange Γ′1 that is second in magnitude only to the ferromagnetic Kitaev exchange K1. This combination of K1 and Γ′1 explains key experimental observations, an unusually high magnetic ordering temperature of 94 K at ambient pressure and its rapid decrease under hydrostatic pressure as Ag3LiRh2O6 evolves from ferromagnetic toward zigzag order within the honeycomb planes. Our spin-wave calculations further predict an unusual topology of the magnon bands arising from the Γ′1 term in the spin Hamiltonian of the honeycomb layer. We show that the large trigonal splitting of t2g states enhances Γ′1, the hitherto underappreciated term in Kitaev magnets, and opens the way to new interesting regimes of the extended Kitaev model.},
note = {arXiv:2610.19770},
keywords = {B1, B6},
pubstate = {published},
tppubtype = {unpublished}
}
In Kitaev magnets, frustration arises from bond-dependent spin anisotropic interactions, which can potentially realize sought-after quantum spin liquid phases. However, material realizations with dominating Kitaev exchange are scarce and the broad parameter space of extended Kitaev models remains largely unexplored experimentally. Here, we use density-functional theory, cluster many-body, spin-wave, and density-matrix renormalization calculations to show that the recently discovered honeycomb rhodate Ag3LiRh2O6 hosts an off-diagonal exchange Γ′1 that is second in magnitude only to the ferromagnetic Kitaev exchange K1. This combination of K1 and Γ′1 explains key experimental observations, an unusually high magnetic ordering temperature of 94 K at ambient pressure and its rapid decrease under hydrostatic pressure as Ag3LiRh2O6 evolves from ferromagnetic toward zigzag order within the honeycomb planes. Our spin-wave calculations further predict an unusual topology of the magnon bands arising from the Γ′1 term in the spin Hamiltonian of the honeycomb layer. We show that the large trigonal splitting of t2g states enhances Γ′1, the hitherto underappreciated term in Kitaev magnets, and opens the way to new interesting regimes of the extended Kitaev model. |  |
Que, X.; He, Q.; Zhou, L.; Prodan, L.; Tsurkan, V.; Kézsmárki, I.; Takagi, H.; Huang, D. Tunable flat band on the surface of a rhombohedral kagome ferromagnet Unpublished (2026), arXiv.2609.19857. @unpublished{que2026tunableflatbandsurface,
title = {Tunable flat band on the surface of a rhombohedral kagome ferromagnet},
author = {X. Que and Q. He and L. Zhou and L. Prodan and V. Tsurkan and I. Kézsmárki and H. Takagi and D. Huang},
url = {https://arxiv.org/abs/2609.19857},
doi = {10.48550/arXiv.2609.19857},
year = {2026},
date = {2026-09-17},
urldate = {2026-09-17},
abstract = {A central goal in the exploration of kagome-based materials is the realization of a flat band that has meV bandwidth and lies close to the Fermi energy. The prevailing assumption is that band flattening originates from destructive hopping processes on the kagome lattice. We perform scanning tunneling microscopy (STM) on the layered kagome ferromagnet Fe3Sn2 and show that it indeed hosts a flat band near the Fermi energy, which is manifested as a sharp peak in the differential tunneling conductance. First-principles slab calculations reveal, however, that this band is flattened not by the destructive interference of intralayer hopping, but by interlayer hopping between rhombohedral-stacked kagome planes in Fe3Sn2, and is confined to the surface layer. This surface band, forming in the vicinity of the Brillouin zone corners K¯ and K′¯, exhibits rich magnetic-field dependence, including fine structure due to valley-symmetry breaking by rotated Fe moments, as well as a persistent diamagnetic shift associated with orbital magnetic moments, all reproduced by our calculations. Our results, highlighting the crucial role of layer stacking on the band structure of kagome magnets, demonstrate experimentally an alternative mechanism of generating magnetically tunable flat bands in atomically thin volumes of topological magnets.},
note = {arXiv.2609.19857},
keywords = {A1, A3},
pubstate = {published},
tppubtype = {unpublished}
}
A central goal in the exploration of kagome-based materials is the realization of a flat band that has meV bandwidth and lies close to the Fermi energy. The prevailing assumption is that band flattening originates from destructive hopping processes on the kagome lattice. We perform scanning tunneling microscopy (STM) on the layered kagome ferromagnet Fe3Sn2 and show that it indeed hosts a flat band near the Fermi energy, which is manifested as a sharp peak in the differential tunneling conductance. First-principles slab calculations reveal, however, that this band is flattened not by the destructive interference of intralayer hopping, but by interlayer hopping between rhombohedral-stacked kagome planes in Fe3Sn2, and is confined to the surface layer. This surface band, forming in the vicinity of the Brillouin zone corners K¯ and K′¯, exhibits rich magnetic-field dependence, including fine structure due to valley-symmetry breaking by rotated Fe moments, as well as a persistent diamagnetic shift associated with orbital magnetic moments, all reproduced by our calculations. Our results, highlighting the crucial role of layer stacking on the band structure of kagome magnets, demonstrate experimentally an alternative mechanism of generating magnetically tunable flat bands in atomically thin volumes of topological magnets. |  |
Jarc, G.; Tartaglia, G.; Gabriele, F.; Forte, F.; Guarino, A.; Montanaro, A.; Rigoni, E. M.; Khatiwada, N.; Lincetto, C.; Bartolini, G.; Mastropasqua, A.; Mathengattil, S. Y.; Malvestuto, M.; Waqee-Ur-Rehman, M.; Fittipaldi, R.; Deisenhofer, J.; Tsirlin, A. A.; Vecchione, A.; Cuoco, M.; Fausti, D. Raman signatures of a non-reciprocal magnetic phase transition in Ca2RuO4 Unpublished (2026), arXiv.2609.07565. @unpublished{jarc2026ramansignaturesnonreciprocalmagnetic,
title = {Raman signatures of a non-reciprocal magnetic phase transition in Ca_{2}RuO_{4}},
author = {G. Jarc and G. Tartaglia and F. Gabriele and F. Forte and A. Guarino and A. Montanaro and E. M. Rigoni and N. Khatiwada and C. Lincetto and G. Bartolini and A. Mastropasqua and S. Y. Mathengattil and M. Malvestuto and M. Waqee-Ur-Rehman and R. Fittipaldi and J. Deisenhofer and A. A. Tsirlin and A. Vecchione and M. Cuoco and D. Fausti},
url = {https://arxiv.org/abs/2609.07565},
doi = {10.48550/arXiv.2609.07565},
year = {2026},
date = {2026-09-07},
urldate = {2026-09-01},
abstract = {The magnetic behavior of Ca2RuO4 represents a unique puzzle due to the interplay of strong electronic correlations, magneto-elastic interactions, and large spin-orbit coupling. At low temperatures, an anomalous Mott insulating state emerges, characterized by a complex antiferromagnetic order with a collective amplitude excitation of the magnetic moment which has been discussed in analogy with the Higgs mode. We report here evidence of a magnetic first-order phase transition driven by an out-of-plane magnetic field along the crystallographic c-axis of Ca2RuO4. Raman measurements in magnetic field reveal the emergence of mode of magnetic origin and a concomitant modification of the coupling between a phonon and the Higgs amplitude mode. Both the Raman features are characterized by a non-reciprocal hysteresis in magnetic field. Surprisingly, the observed phase transition does not affect the Raman scattering from the in-plane magnons, indicating that the dipolar antiferromagnetic order is preserved. This is consistent with the onset of a new quadrupolar field-controlled state, whose fluctuations structure can trigger an hybridization between the lattice and the magnetic Higgs mode resulting in the observed Raman features.},
note = {arXiv.2609.07565},
keywords = {A1, B1, C4},
pubstate = {published},
tppubtype = {unpublished}
}
The magnetic behavior of Ca2RuO4 represents a unique puzzle due to the interplay of strong electronic correlations, magneto-elastic interactions, and large spin-orbit coupling. At low temperatures, an anomalous Mott insulating state emerges, characterized by a complex antiferromagnetic order with a collective amplitude excitation of the magnetic moment which has been discussed in analogy with the Higgs mode. We report here evidence of a magnetic first-order phase transition driven by an out-of-plane magnetic field along the crystallographic c-axis of Ca2RuO4. Raman measurements in magnetic field reveal the emergence of mode of magnetic origin and a concomitant modification of the coupling between a phonon and the Higgs amplitude mode. Both the Raman features are characterized by a non-reciprocal hysteresis in magnetic field. Surprisingly, the observed phase transition does not affect the Raman scattering from the in-plane magnons, indicating that the dipolar antiferromagnetic order is preserved. This is consistent with the onset of a new quadrupolar field-controlled state, whose fluctuations structure can trigger an hybridization between the lattice and the magnetic Higgs mode resulting in the observed Raman features. |  |
Misawa, R.; Oiwa, R.; Kitou, S.; Miki, T.; Ezawa, M.; Yun, W.; Yamada, R.; Koyama, C.; Velamazán, J. A. Rodríguez; Kolincio, K. K.; Qureshi, N.; Zhakina, Elina; Nakamura, Y.; Masell, J.; Belopolski, I.; Arima, T.; Nomura, Y.; Hayami, S.; Hirschberger, M. Observation of g-wave altermagnetic multipole Unpublished (2026), arXiv:2609.01969. @unpublished{misawaObservationGwaveAltermagnetic2026-09-022026,
title = {Observation of g-wave altermagnetic multipole},
author = {R. Misawa and R. Oiwa and S. Kitou and T. Miki and M. Ezawa and W. Yun and R. Yamada and C. Koyama and J. A. Rodríguez Velamazán and K. K. Kolincio and N. Qureshi and Elina Zhakina and Y. Nakamura and J. Masell and I. Belopolski and T. Arima and Y. Nomura and S. Hayami and M. Hirschberger},
url = {https://arxiv.org/abs/2609.01969},
doi = {10.48550/arXiv.2609.01969},
year = {2026},
date = {2026-09-02},
urldate = {2026-09-01},
abstract = {Over the past few years, altermagnets have emerged as a new class of collinear magnets with broken time-reversal symmetry, offering novel opportunities for spintronics beyond conventional magnets. Rather than from net magnetization, as in ferromagnets, the unconventional time-reversal symmetry breaking of altermagnets originates from antiferroic magnetic dipoles locked to higher-order multipoles. Here we report the direct visualization of a g-wave altermagnetic multipole in the canonical altermagnet CrSb. Combining high-energy synchrotron X-ray diffraction with valence electron density (VED) analysis, we uncover a pronounced directional anisotropy of the VED distribution alternating between Cr sublattices. This evidences the antiferroic order of electric hexadecapoles predicted in g-wave altermagnets. Its coexistence with antiferroic magnetic dipoles induces ferroic magnetic multipoles, as probed by polarized neutron diffraction. We further identify a microscopic model of altermagnetism that directly relates the g-wave multipole and the g-wave spin splitting. Through direct observation and quantification of multipoles, this study provides a real-space fingerprint of altermagnetism and establishes a general probe of hidden multipole order in quantum materials.},
note = {arXiv:2609.01969},
keywords = {B5},
pubstate = {published},
tppubtype = {unpublished}
}
Over the past few years, altermagnets have emerged as a new class of collinear magnets with broken time-reversal symmetry, offering novel opportunities for spintronics beyond conventional magnets. Rather than from net magnetization, as in ferromagnets, the unconventional time-reversal symmetry breaking of altermagnets originates from antiferroic magnetic dipoles locked to higher-order multipoles. Here we report the direct visualization of a g-wave altermagnetic multipole in the canonical altermagnet CrSb. Combining high-energy synchrotron X-ray diffraction with valence electron density (VED) analysis, we uncover a pronounced directional anisotropy of the VED distribution alternating between Cr sublattices. This evidences the antiferroic order of electric hexadecapoles predicted in g-wave altermagnets. Its coexistence with antiferroic magnetic dipoles induces ferroic magnetic multipoles, as probed by polarized neutron diffraction. We further identify a microscopic model of altermagnetism that directly relates the g-wave multipole and the g-wave spin splitting. Through direct observation and quantification of multipoles, this study provides a real-space fingerprint of altermagnetism and establishes a general probe of hidden multipole order in quantum materials. |  |
Guo, J.; Brizolla, G. M. S.; Rao, P.; Shao, J.; Huang, X. H.; Meier, T. N. G.; Xu, T.; Ji, P.; Finley, J.; Fabian, J.; Knolle, J.; Back, C.; Chen, L. Electric-current control of anomalous Hall effect Unpublished (2026), arXiv: 2601.03744. @unpublished{guoElectriccurrentControlAnomalous2026,
title = {Electric-current control of anomalous Hall effect},
author = {J. Guo and G. M. S. Brizolla and P. Rao and J. Shao and X. H. Huang and T. N. G. Meier and T. Xu and P. Ji and J. Finley and J. Fabian and J. Knolle and C. Back and L. Chen},
url = {https://arxiv.org/abs/2601.03744},
doi = {10.48550/arXiv.2601.03744},
year = {2026},
date = {2026-08-26},
urldate = {2026-08-01},
abstract = {We demonstrate robust and reversible electric-current control of the anomalous Hall effect (AHE) in a two-dimensional WTe2/Fe3GeTe2 (FGT) stack. Applying a current through Td-WTe2 leads to a giant modulation of the AHE of the adjacent FGT layer, with the relative change of the AHE conductivity exceeding 180},
note = {arXiv: 2601.03744},
keywords = {A2, B6, C6},
pubstate = {published},
tppubtype = {unpublished}
}
We demonstrate robust and reversible electric-current control of the anomalous Hall effect (AHE) in a two-dimensional WTe2/Fe3GeTe2 (FGT) stack. Applying a current through Td-WTe2 leads to a giant modulation of the AHE of the adjacent FGT layer, with the relative change of the AHE conductivity exceeding 180 |  |
Chmeruk, A.; Jones, D.; Chioncel, L. Disorder-induced conducting edges on Kagomé lattice Unpublished (2026), arXiv: 2608.24472. @unpublished{chmeruk2026disorderinducedconductingedgeskagome,
title = {Disorder-induced conducting edges on Kagomé lattice},
author = {A. Chmeruk and D. Jones and L. Chioncel},
url = {https://arxiv.org/abs/2608.24472},
doi = {10.48550/arXiv.2608.24472},
year = {2026},
date = {2026-08-25},
urldate = {2026-08-01},
abstract = {Within a cluster extension of the coherent potential approximation, disorder averaging generates a non-local self-energy that renormalizes both diagonal and off-diagonal hopping terms of the non-interacting Kagome-lattice Hamiltonian. These renormalizations (of both nearest- and next-nearest-neighbor hopping amplitudes) drive the system between two topologically trivial insulating states through an intermediate gapless phase characterized by conducting edge modes over a broad range of impurity concentrations. Our results demonstrate that multiple-scattering effects alone can generate emergent effective spin-orbit interactions and qualitatively modify the edge spectrum of disordered Kagome systems.},
note = {arXiv: 2608.24472},
keywords = {A5},
pubstate = {published},
tppubtype = {unpublished}
}
Within a cluster extension of the coherent potential approximation, disorder averaging generates a non-local self-energy that renormalizes both diagonal and off-diagonal hopping terms of the non-interacting Kagome-lattice Hamiltonian. These renormalizations (of both nearest- and next-nearest-neighbor hopping amplitudes) drive the system between two topologically trivial insulating states through an intermediate gapless phase characterized by conducting edge modes over a broad range of impurity concentrations. Our results demonstrate that multiple-scattering effects alone can generate emergent effective spin-orbit interactions and qualitatively modify the edge spectrum of disordered Kagome systems. |  |
Labh, A.; Colman, R. H.; Šebesta, J.; Oefele, N.; Lhotel, E.; B., Adam; Steffens, P.; Zaharko, O.; Manuel, P.; Kibalin, I.; Gegenwart, P.; Legut, D.; Jochum, J. K.; Tsirlin, A. A.; Čermák, P. Ultralow-field triplon condensation in a spin-ladder magnet Unpublished (2026), arXiv.2608.21316. @unpublished{labh2026ultralowfieldtriploncondensationspinladder,
title = {Ultralow-field triplon condensation in a spin-ladder magnet},
author = {A. Labh and R. H. Colman and J. Šebesta and N. Oefele and E. Lhotel and Adam B. and P. Steffens and O. Zaharko and P. Manuel and I. Kibalin and P. Gegenwart and D. Legut and J. K. Jochum and A. A. Tsirlin and P. Čermák},
url = {https://arxiv.org/abs/2608.21316},
doi = {10.48550/arXiv.2608.21316},
year = {2026},
date = {2026-08-21},
urldate = {2026-08-01},
abstract = {We realise the first ultralow-field Bose-Einstein condensation of triplons in a spin-ladder magnet, uncovering a quantum critical point at only μ0Hc1=0.17 T in Henmilite (Ca2Cu(OH)4[B(OH)4]2). Unlike dimer magnets, a ladder retains extended one-dimensional correlations in its gapped parent state, making this limit strongly fluctuation dominated. Thermodynamic, magnetoelastic, μSR, and neutron-diffraction measurements overturn the previous assignment of zero-field antiferromagnetic order, establishing a quantum-disordered coupled-ladder parent state with persistent low-energy dynamics. The weak low-temperature anomaly instead marks a gap-controlled crossover from the correlated ladder regime into the activated quantum-disordered state. These measurements further reveal an exceptionally asymmetric ordered dome extending to μ0Hc2≃8.2 T. Quantum Monte Carlo simulations for the relevant spin Hamiltonian place Henmilite just on the gapped side of the zero-field ladder-ordering instability, naturally accounting for the strong separation between the exchange and residual-gap scales and the tiny critical field. Our findings extend ultralow-field triplon condensation beyond the dimer paradigm and establish Henmilite as a platform for controlled tuning across quantum criticality in a fluctuation-dominated spin ladder.},
note = {arXiv.2608.21316},
keywords = {B1, B3},
pubstate = {published},
tppubtype = {unpublished}
}
We realise the first ultralow-field Bose-Einstein condensation of triplons in a spin-ladder magnet, uncovering a quantum critical point at only μ0Hc1=0.17 T in Henmilite (Ca2Cu(OH)4[B(OH)4]2). Unlike dimer magnets, a ladder retains extended one-dimensional correlations in its gapped parent state, making this limit strongly fluctuation dominated. Thermodynamic, magnetoelastic, μSR, and neutron-diffraction measurements overturn the previous assignment of zero-field antiferromagnetic order, establishing a quantum-disordered coupled-ladder parent state with persistent low-energy dynamics. The weak low-temperature anomaly instead marks a gap-controlled crossover from the correlated ladder regime into the activated quantum-disordered state. These measurements further reveal an exceptionally asymmetric ordered dome extending to μ0Hc2≃8.2 T. Quantum Monte Carlo simulations for the relevant spin Hamiltonian place Henmilite just on the gapped side of the zero-field ladder-ordering instability, naturally accounting for the strong separation between the exchange and residual-gap scales and the tiny critical field. Our findings extend ultralow-field triplon condensation beyond the dimer paradigm and establish Henmilite as a platform for controlled tuning across quantum criticality in a fluctuation-dominated spin ladder. |  |
Östlin, A.; Titvinidze, I.; Kollar, M.; Jones, D.; Chioncel, L. Analytical results of typical medium theory for the bethe lattice with cauchy disorder Unpublished (2026), arXiv: 2608.03770. @unpublished{östlin2026analyticalresultstypicalmedium,
title = {Analytical results of typical medium theory for the bethe lattice with cauchy disorder},
author = {A. Östlin and I. Titvinidze and M. Kollar and D. Jones and L. Chioncel},
url = {https://arxiv.org/abs/2608.03770},
doi = {10.48550/arXiv.2608.03770},
year = {2026},
date = {2026-08-04},
urldate = {2026-08-01},
abstract = {We present a combined numerical and analytically tractable realization of the typical medium theory (TMT) for Anderson localization on the infinite-connectivity Bethe lattice with Cauchy-distributed on-site disorder. Exploiting the special properties of the Cauchy distribution and the Bethe lattice, we derive an analytical expression for the typical density of states (TDOS) and obtain a simplified TMT self-consistency scheme. We show that the TDOS at the band center decreases linearly with disorder strength and vanishes at the critical disorder Wc=D/2. The resulting ω–W phase diagram reveals the continuous collapse of the mobility edge and the disappearance of extended states.},
note = {arXiv: 2608.03770},
keywords = {A5},
pubstate = {published},
tppubtype = {unpublished}
}
We present a combined numerical and analytically tractable realization of the typical medium theory (TMT) for Anderson localization on the infinite-connectivity Bethe lattice with Cauchy-distributed on-site disorder. Exploiting the special properties of the Cauchy distribution and the Bethe lattice, we derive an analytical expression for the typical density of states (TDOS) and obtain a simplified TMT self-consistency scheme. We show that the TDOS at the band center decreases linearly with disorder strength and vanishes at the critical disorder Wc=D/2. The resulting ω–W phase diagram reveals the continuous collapse of the mobility edge and the disappearance of extended states. |  |
Schilberth, F.; Vasin, K.; Knauft, M.; Kondákor, M.; Vuckovic, M.; Herrmann, N.; Penc, K.; Minola, M.; Keimer, B.; Martinez, V. A.; Panda, K.; Sirenko, A. A.; Prodan, L.; Tsurkan, V.; Tsirlin, A. A.; Kézsmárki, I.; Deisenhofer, J. Magnetic circular dichroism of THz modes and selection rules of Raman-active optical phonons in the polar altermagnet candidate Mn2Mo3O8 Unpublished (2026), arXiv:2608.01062. @unpublished{schilberth_magnetic_2026,
title = {Magnetic circular dichroism of THz modes and selection rules of Raman-active optical phonons in the polar altermagnet candidate Mn_{2}Mo_{3}O_{8}},
author = {F. Schilberth and K. Vasin and M. Knauft and M. Kondákor and M. Vuckovic and N. Herrmann and K. Penc and M. Minola and B. Keimer and V. A. Martinez and K. Panda and A. A. Sirenko and L. Prodan and V. Tsurkan and A. A. Tsirlin and I. Kézsmárki and J. Deisenhofer},
url = {https://arxiv.org/abs/2608.01062},
doi = {10.48550/arXiv.2608.01062},
year = {2026},
date = {2026-08-02},
urldate = {2026-08-01},
note = {arXiv:2608.01062},
keywords = {A1, B2, B3, C4},
pubstate = {published},
tppubtype = {unpublished}
}
|  |
Calonge-Martínez, L.; Rao, P.; Mila, F.; Knolle, J. Topological Triplons in the Pinwheel Valence Bond Solid on the Kagome Lattice Unpublished (2026), arXiv.2606.09823
datadoi: 10.5281/zenodo.20917613. @unpublished{calonge-martinezTopologicalTriplonsPinwheel2026,
title = {Topological Triplons in the Pinwheel Valence Bond Solid on the Kagome Lattice},
author = {L. Calonge-Martínez and P. Rao and F. Mila and J. Knolle},
url = {https://doi.org/10.48550/arXiv.2606.09823},
doi = {10.48550/ARXIV.2606.09823},
year = {2026},
date = {2026-07-06},
urldate = {2026-07-01},
abstract = {We investigate the triplon excitations of the pinwheel valence-bond-solid phase on the deformed kagome lattice compound Rb2Cu3SnF12. Using bond-operator mean-field theory, we compute the triplon band structure, dynamical structure factor, Berry curvatures and the associated thermal Hall response. We show that the presence of Dzyaloshinskii-Moriya interactions and an external magnetic field are key for endowing triplon bands with nontrivial Chern numbers. We find good qualitative agreement of the low-energy dynamical structure factor with neutron-scattering experiments. An applied magnetic field can isolate the lowest triplon Chern band leading to a tunable thermal Hall conductivity for accessible temperature and field regimes. Our results establish the deformed kagome pinwheel valence-bond solid as a promising platform for topological triplon physics and for observing the associated thermal Hall effect.},
note = {arXiv.2606.09823
datadoi: 10.5281/zenodo.20917613},
keywords = {},
pubstate = {published},
tppubtype = {unpublished}
}
We investigate the triplon excitations of the pinwheel valence-bond-solid phase on the deformed kagome lattice compound Rb2Cu3SnF12. Using bond-operator mean-field theory, we compute the triplon band structure, dynamical structure factor, Berry curvatures and the associated thermal Hall response. We show that the presence of Dzyaloshinskii-Moriya interactions and an external magnetic field are key for endowing triplon bands with nontrivial Chern numbers. We find good qualitative agreement of the low-energy dynamical structure factor with neutron-scattering experiments. An applied magnetic field can isolate the lowest triplon Chern band leading to a tunable thermal Hall conductivity for accessible temperature and field regimes. Our results establish the deformed kagome pinwheel valence-bond solid as a promising platform for topological triplon physics and for observing the associated thermal Hall effect. | |
Wiener, T.; Brunner, L.; Heyl, M. Universal symmetry-breaking dynamics at continuous phase transitions: Evidence for a new dynamical critical exponent Unpublished (2026), arXiv: 2605.07753
datadoi: 10.5281/zenodo.18862010. @unpublished{wiener2026universalsymmetrybreakingdynamicscontinuous,
title = {Universal symmetry-breaking dynamics at continuous phase transitions: Evidence for a new dynamical critical exponent},
author = {T. Wiener and L. Brunner and M. Heyl},
url = {https://arxiv.org/abs/2605.07753},
doi = {10.48550/arXiv.2605.07753},
year = {2026},
date = {2026-07-03},
urldate = {2026-07-01},
abstract = {Uncovering and understanding universal dynamics in matter far from equilibrium remains a key challenge. In this work, we identify a so far unrecognized form of universal behavior that emerges after a sudden symmetry-breaking quench at continuous phase transitions. Our key observation is that the order-parameter fluctuations in Ising models exhibit a compelling temporal collapse across a wide range of system sizes and quench strengths, indicative of an emergent single-variable scaling form. This phenomenon can be explained by introducing a so far unknown dynamical critical exponent for the underlying continuous phase transition. We find evidence for a lower critical effective dimension of this universal regime: it is observed in the 2D quantum and 3D and 4D classical Ising models, but not in the 1D quantum or 2D classical cases. Our results suggest that our observed universal far-from-equilibrium scaling may extend beyond the Ising models studied here and could more broadly characterize systems with non-conserved order parameters, opening new avenues for exploring universal dynamics both theoretically and in current experimental platforms.},
note = {arXiv: 2605.07753
datadoi: 10.5281/zenodo.18862010},
keywords = {B6},
pubstate = {published},
tppubtype = {unpublished}
}
Uncovering and understanding universal dynamics in matter far from equilibrium remains a key challenge. In this work, we identify a so far unrecognized form of universal behavior that emerges after a sudden symmetry-breaking quench at continuous phase transitions. Our key observation is that the order-parameter fluctuations in Ising models exhibit a compelling temporal collapse across a wide range of system sizes and quench strengths, indicative of an emergent single-variable scaling form. This phenomenon can be explained by introducing a so far unknown dynamical critical exponent for the underlying continuous phase transition. We find evidence for a lower critical effective dimension of this universal regime: it is observed in the 2D quantum and 3D and 4D classical Ising models, but not in the 1D quantum or 2D classical cases. Our results suggest that our observed universal far-from-equilibrium scaling may extend beyond the Ising models studied here and could more broadly characterize systems with non-conserved order parameters, opening new avenues for exploring universal dynamics both theoretically and in current experimental platforms. |  |
Magar, A.; Sebastian, S. J.; Ding, Q. -P.; Skourski, Y.; Tsirlin, A. A.; Furukawa, Y.; Nath, R. Ground-state properties of the S=3/2 anisotropic triangular lattice antiferromagnet Na3Cr(PO4)2 Unpublished (2026), arXiv: 2606.17658. @unpublished{magar2026groundstatepropertiess32anisotropic,
title = {Ground-state properties of the S=3/2 anisotropic triangular lattice antiferromagnet Na_{3}Cr(PO_{4})_{2}},
author = {A. Magar and S. J. Sebastian and Q. -P. Ding and Y. Skourski and A. A. Tsirlin and Y. Furukawa and R. Nath},
url = {https://arxiv.org/abs/2606.17658},
doi = {10.48550/arXiv.2606.17658},
year = {2026},
date = {2026-06-16},
urldate = {2026-06-01},
abstract = {We report the crystal structure and magnetic properties of a S=3/2 anisotropic triangular lattice compound Na3Cr(PO4)2 employing single-crystal and powder x-ray diffraction, magnetization, heat capacity, and 31P nuclear magnetic resonance (NMR) experiments, supported by the band structure calculations. Magnetic susceptibility exhibits a broad maximum around 3.5 K, indicating the presence of a short-range antiferromagnetic order, typical of a low-dimensional spin system. Magnetization and heat capacity manifest an antiferromagnetic long-range ordering at around TN≃2.6 K. This was further confirmed by the drastic NMR line broadening and a peak in the nuclear spin-lattice and spin-spin relaxation rates. The isothermal magnetization data exhibit a field-induced spin-flop transition at around μ0HSF≃1.7 T reminiscent of an anisotropic two-dimensional magnet, before saturating above μ0Hsat≃4.5 T. The saturation field was further upheld by the field-dependent NMR relaxation measurements at low temperatures. The 31P NMR spectral shape confirms the commensurate antiferromagnetic nature of the ordering below TN. textbackslashtextitAb initio calculations reveal a significant deformation of the triangular spin lattice, resulting in triangles with two antiferromagnetic couplings of similar strength and a much weaker coupling along the third side of the triangle.},
note = {arXiv: 2606.17658},
keywords = {B1},
pubstate = {published},
tppubtype = {unpublished}
}
We report the crystal structure and magnetic properties of a S=3/2 anisotropic triangular lattice compound Na3Cr(PO4)2 employing single-crystal and powder x-ray diffraction, magnetization, heat capacity, and 31P nuclear magnetic resonance (NMR) experiments, supported by the band structure calculations. Magnetic susceptibility exhibits a broad maximum around 3.5 K, indicating the presence of a short-range antiferromagnetic order, typical of a low-dimensional spin system. Magnetization and heat capacity manifest an antiferromagnetic long-range ordering at around TN≃2.6 K. This was further confirmed by the drastic NMR line broadening and a peak in the nuclear spin-lattice and spin-spin relaxation rates. The isothermal magnetization data exhibit a field-induced spin-flop transition at around μ0HSF≃1.7 T reminiscent of an anisotropic two-dimensional magnet, before saturating above μ0Hsat≃4.5 T. The saturation field was further upheld by the field-dependent NMR relaxation measurements at low temperatures. The 31P NMR spectral shape confirms the commensurate antiferromagnetic nature of the ordering below TN. textbackslashtextitAb initio calculations reveal a significant deformation of the triangular spin lattice, resulting in triangles with two antiferromagnetic couplings of similar strength and a much weaker coupling along the third side of the triangle. |  |
Nakano, R.; Yamada, R.; Utesov, O. I.; Gen, M.; Kikkawa, A.; Sagayama, H.; Nakao, H.; Tokunaga, M.; Arima, T.; Tokura, Y.; Kim, S. K.; Hirschberger, M. Frustration of harmonic and solitonic helimagnetism on the body-centered tetragonal lattice of GdAlSi Unpublished (2026), arXiv:2605.07294. @unpublished{nakano2026frustrationharmonicsolitonichelimagnetism,
title = {Frustration of harmonic and solitonic helimagnetism on the body-centered tetragonal lattice of GdAlSi},
author = {R. Nakano and R. Yamada and O. I. Utesov and M. Gen and A. Kikkawa and H. Sagayama and H. Nakao and M. Tokunaga and T. Arima and Y. Tokura and S. K. Kim and M. Hirschberger},
url = {https://arxiv.org/abs/2605.07294},
doi = {10.48550/arXiv.2605.07294},
year = {2026},
date = {2026-05-20},
urldate = {2026-05-01},
abstract = {The triangular lattice antiferromagnet (TLAF) with nearest-neighbor exchange interaction is a model platform in the field of frustrated magnetism. Here, anharmonic (`up-up-down') and harmonic (`120 degree') magnetic states compete, because the fundamental helimagnetic wave and its higher harmonic are degenerate in energy. We show that a body-centered tetragonal lattice (BCTL) can realize a similar frustration of harmonic and anharmonic helimagnetic states, and that the tetragonal magnetic Weyl semimetal GdAlSi realizes this scenario. In an applied magnetic field, resonant elastic X-ray scattering reveals a competition of harmonic cycloidal and solitonic double-Q states, well consistent with mean-field calculations. Our work provides a new paradigm for frustration physics in BCTL materials.},
note = {arXiv:2605.07294},
keywords = {B5},
pubstate = {published},
tppubtype = {unpublished}
}
The triangular lattice antiferromagnet (TLAF) with nearest-neighbor exchange interaction is a model platform in the field of frustrated magnetism. Here, anharmonic (`up-up-down') and harmonic (`120 degree') magnetic states compete, because the fundamental helimagnetic wave and its higher harmonic are degenerate in energy. We show that a body-centered tetragonal lattice (BCTL) can realize a similar frustration of harmonic and anharmonic helimagnetic states, and that the tetragonal magnetic Weyl semimetal GdAlSi realizes this scenario. In an applied magnetic field, resonant elastic X-ray scattering reveals a competition of harmonic cycloidal and solitonic double-Q states, well consistent with mean-field calculations. Our work provides a new paradigm for frustration physics in BCTL materials. |  |
Leone, L.; Dutta, A.; Heyl, M.; Prati, E.; Torta, P. Solving classical and quantum spin glasses with deep boltzmann quantum states Unpublished (2026), arXiv.2605.15899. @unpublished{leone2026solvingclassicalquantumspin,
title = {Solving classical and quantum spin glasses with deep boltzmann quantum states},
author = {L. Leone and A. Dutta and M. Heyl and E. Prati and P. Torta},
url = {https://doi.org/10.48550/arXiv.2605.15899},
doi = {10.48550/arXiv.2605.15899},
year = {2026},
date = {2026-05-15},
urldate = {2026-05-15},
abstract = {Variational neural network models have achieved remarkable success in solving ground-state problems of quantum many-body systems. However, addressing classical and quantum spin glasses remains challenging, as disorder and energy frustration give rise to an exponentially large number of local energy minima separated by high-energy barriers, hindering the efficiency of conventional Metropolis-based Monte Carlo methods. To bridge this gap, we introduce Deep Boltzmann Quantum States, a class of neural quantum states inspired by deep Boltzmann machines that inherit efficient block Gibbs sampling. We also propose two key advances in the training algorithm. Firstly, we combine natural-gradient updates with state-of-the-art stochastic optimizers. Secondly, we gradually tune the hardness of the problem Hamiltonian by interpolating from an easy to a hard regime, without the need to closely approximate the instantaneous adiabatic state at intermediate times. We match the exact solution or the best available estimate for several instances of classical and quantum Ising spin-glass models with infinite-range interactions and hundreds of spins. We also solve instances of the NP-hard Job Shop Scheduling Problem exceeding the current limitations of quantum annealing hardware. To summarize, deep neural architectures with efficient global update rules and trained within an annealing-like scheme, provide a powerful framework for solving real-world hard combinatorial optimization and for investigating disordered quantum many-body systems.},
note = {arXiv.2605.15899},
keywords = {C4},
pubstate = {published},
tppubtype = {unpublished}
}
Variational neural network models have achieved remarkable success in solving ground-state problems of quantum many-body systems. However, addressing classical and quantum spin glasses remains challenging, as disorder and energy frustration give rise to an exponentially large number of local energy minima separated by high-energy barriers, hindering the efficiency of conventional Metropolis-based Monte Carlo methods. To bridge this gap, we introduce Deep Boltzmann Quantum States, a class of neural quantum states inspired by deep Boltzmann machines that inherit efficient block Gibbs sampling. We also propose two key advances in the training algorithm. Firstly, we combine natural-gradient updates with state-of-the-art stochastic optimizers. Secondly, we gradually tune the hardness of the problem Hamiltonian by interpolating from an easy to a hard regime, without the need to closely approximate the instantaneous adiabatic state at intermediate times. We match the exact solution or the best available estimate for several instances of classical and quantum Ising spin-glass models with infinite-range interactions and hundreds of spins. We also solve instances of the NP-hard Job Shop Scheduling Problem exceeding the current limitations of quantum annealing hardware. To summarize, deep neural architectures with efficient global update rules and trained within an annealing-like scheme, provide a powerful framework for solving real-world hard combinatorial optimization and for investigating disordered quantum many-body systems. |  |
Mukharjee, P. K.; Erdmann, S.; Kalaivanan, R.; Sankar, R.; Choi, K. -Y.; Tsirlin, A. A.; Gegenwart, P. Thermodynamic signatures of a field-induced ordered intermediate phase in Na2Co2TeO6 Unpublished (2026), arXiv:2605.15829,
datadoi: 10.5281/zenodo.19597935. @unpublished{mukharjee2026thermodynamicsignaturesfieldinducedordered,
title = {Thermodynamic signatures of a field-induced ordered intermediate phase in Na_{2}Co_{2}TeO_{6}},
author = {P. K. Mukharjee and S. Erdmann and R. Kalaivanan and R. Sankar and K. -Y. Choi and A. A. Tsirlin and P. Gegenwart},
url = {https://arxiv.org/abs/2605.15829},
doi = {10.48550/arXiv.2605.15829},
year = {2026},
date = {2026-05-15},
urldate = {2026-05-15},
note = {arXiv:2605.15829,
datadoi: 10.5281/zenodo.19597935},
keywords = {B1},
pubstate = {published},
tppubtype = {unpublished}
}
|  |
Koller, E.; Leeb, V.; Perkins, N. B.; Knolle, J. Raman Circular Dichroism and Quantum Geometry of Chiral Quantum Spin Liquids Unpublished (2026), arXiv.2503.14091
datadoi: 10.5281/zenodo.20414987. @unpublished{kollerRamanCircularDichroism2025,
title = {Raman Circular Dichroism and Quantum Geometry of Chiral Quantum Spin Liquids},
author = {E. Koller and V. Leeb and N. B. Perkins and J. Knolle},
url = {https://arxiv.org/abs/2503.14091},
doi = {10.48550/ARXIV.2503.14091},
year = {2026},
date = {2026-05-01},
urldate = {2026-10-01},
abstract = {We show that the quantum geometry of fractionalized spin excitations in Mott-insulating quantum spin liquids (QSL) gives rise to a finite Raman circular dichroism (RCD) signal. We demonstrate the equivalence between the Loudon-Fleury framework and the light-matter coupling approach for effective spinon bands. Using the latter, we derive an analytical decomposition of the RCD into different contributions of the quantum geometry. This reveals the sensitivity of the RCD to the underlying structure of the wave functions and the handedness of the excitations, rather than a nonzero Chern number of spinon excitations. To illustrate this, we apply our approach to two examples, the Kitaev honeycomb model in a magnetic field and a chiral $U(1)$ QSL on the triangular lattice, and discuss its experimental relevance for candidate materials.},
note = {arXiv.2503.14091
datadoi: 10.5281/zenodo.20414987},
keywords = {},
pubstate = {published},
tppubtype = {unpublished}
}
We show that the quantum geometry of fractionalized spin excitations in Mott-insulating quantum spin liquids (QSL) gives rise to a finite Raman circular dichroism (RCD) signal. We demonstrate the equivalence between the Loudon-Fleury framework and the light-matter coupling approach for effective spinon bands. Using the latter, we derive an analytical decomposition of the RCD into different contributions of the quantum geometry. This reveals the sensitivity of the RCD to the underlying structure of the wave functions and the handedness of the excitations, rather than a nonzero Chern number of spinon excitations. To illustrate this, we apply our approach to two examples, the Kitaev honeycomb model in a magnetic field and a chiral $U(1)$ QSL on the triangular lattice, and discuss its experimental relevance for candidate materials. | |
Prodan, L.; Sourd, J.; Zherlitsyn, S.; Chioncel, L. Magnetoelastic signatures of the conical state and charge density waves in antiferromagnetic FeGe Unpublished (2026), arXiv: 2603.05734. @unpublished{prodan2026magnetoelasticsignaturesconicalstate,
title = {Magnetoelastic signatures of the conical state and charge density waves in antiferromagnetic FeGe},
author = {L. Prodan and J. Sourd and S. Zherlitsyn and L. Chioncel},
url = {https://arxiv.org/abs/2603.05734},
doi = {10.48550/arXiv.2603.05734},
year = {2026},
date = {2026-04-12},
urldate = {2026-04-01},
abstract = {Kagome systems host intertwined spin, charge, and lattice degrees of freedom that drive emergent collective states. Here, we identify two distinct energy scales in the noncollinear kagome magnet FeGe: a field-tunable magnetic fluctuation channel at ∼35textasciitildeK associated with the conical state, and a field-independent channel at ∼100textasciitildeK linked to charge-density-wave fluctuations. Ultrasound measurements provide direct access to the exchange-renormalized magnetic stiffness, whose softening governs the acoustic anomaly and follows a symmetry-constrained quadratic field dependence. We further predict a linear temperature dependence of neutron diffraction intensities at fixed field and a quadratic field suppression at fixed temperature. These results identify magnetic stiffness as a key control parameter of spin-lattice dynamics and establish ultrasound as a sensitive probe of coupled collective modes.},
note = {arXiv: 2603.05734},
keywords = {A1, A5},
pubstate = {published},
tppubtype = {unpublished}
}
Kagome systems host intertwined spin, charge, and lattice degrees of freedom that drive emergent collective states. Here, we identify two distinct energy scales in the noncollinear kagome magnet FeGe: a field-tunable magnetic fluctuation channel at ∼35textasciitildeK associated with the conical state, and a field-independent channel at ∼100textasciitildeK linked to charge-density-wave fluctuations. Ultrasound measurements provide direct access to the exchange-renormalized magnetic stiffness, whose softening governs the acoustic anomaly and follows a symmetry-constrained quadratic field dependence. We further predict a linear temperature dependence of neutron diffraction intensities at fixed field and a quadratic field suppression at fixed temperature. These results identify magnetic stiffness as a key control parameter of spin-lattice dynamics and establish ultrasound as a sensitive probe of coupled collective modes. |  |
Guo, J.; Rao, P.; Huang, X.; Xu, T.; Guo, Y.; Shao, J.; Sun, C.; Orekhov, A.; Meier, T. N. G.; Knolle, J.; Back, C. H.; Chen, L. Current-tunable room temperature ferromagnetism and current-driven phase transitions Unpublished (2026), arXiv:2603.27298. @unpublished{guoCurrenttunableRoomTemperature2026-03-282026,
title = {Current-tunable room temperature ferromagnetism and current-driven phase transitions},
author = {J. Guo and P. Rao and X. Huang and T. Xu and Y. Guo and J. Shao and C. Sun and A. Orekhov and T. N. G. Meier and J. Knolle and C. H. Back and L. Chen},
url = {https://arxiv.org/abs/2603.27298},
doi = {10.48550/arxiv2603.27298},
year = {2026},
date = {2026-03-28},
urldate = {2026-03-01},
publisher = {arXiv},
abstract = {It is generally assumed that the application of a charge-current in ferromagnetic metals suppresses their ferromagnetic order through trivial Joule heating. Here, we demonstrate that a charge current can instead enhance magnetic ordering. Using a WTe2/Fe3Ge2Te (FGT) stack as a model system, we show that a charge current flowing in WTe2 controls the ferromagnetic properties and magnetic phase transition of the adjacent FGT via a current-induced effective magnetic-field arising from orbital magnetization. Remarkably, the charge current drives a substantial enhancement of the Curie temperature, boosting it well above room temperature. Furthermore, we show that the charge-current enables controlled tuning of the phase transitions in FGT, which confirms the scaling behaviour of a ferromagnet-paramagnet phase transition. This work provides a pathway for integrating two-dimensional ferromagnets into spintronic functionalities at technologically relevant temperatures and for exploring novel current-driven phenomena in ferromagnetic systems.},
note = {arXiv:2603.27298},
keywords = {A2, B6, C6},
pubstate = {published},
tppubtype = {unpublished}
}
It is generally assumed that the application of a charge-current in ferromagnetic metals suppresses their ferromagnetic order through trivial Joule heating. Here, we demonstrate that a charge current can instead enhance magnetic ordering. Using a WTe2/Fe3Ge2Te (FGT) stack as a model system, we show that a charge current flowing in WTe2 controls the ferromagnetic properties and magnetic phase transition of the adjacent FGT via a current-induced effective magnetic-field arising from orbital magnetization. Remarkably, the charge current drives a substantial enhancement of the Curie temperature, boosting it well above room temperature. Furthermore, we show that the charge-current enables controlled tuning of the phase transitions in FGT, which confirms the scaling behaviour of a ferromagnet-paramagnet phase transition. This work provides a pathway for integrating two-dimensional ferromagnets into spintronic functionalities at technologically relevant temperatures and for exploring novel current-driven phenomena in ferromagnetic systems. |  |
Misawa, R.; Kitou, S.; Sun, J. -P.; Yu, Y.; Koyama, C.; Nakamura, Y.; Arima, T.; Cheng, J. -G.; Hirschberger, M. Polar, checkerboard charge order in bilayer nickelate La3Ni2O7 Unpublished (2026), arXiv:2603.25119. @unpublished{misawaPolarCheckerboardCharge2026-03-262026,
title = {Polar, checkerboard charge order in bilayer nickelate La_{3}Ni_{2}O_{7}},
author = {R. Misawa and S. Kitou and J. -P. Sun and Y. Yu and C. Koyama and Y. Nakamura and T. Arima and J. -G. Cheng and M. Hirschberger},
url = {https://arxiv.org/abs/2603.25119},
doi = {10.48550/arXiv.2603.25119},
year = {2026},
date = {2026-03-26},
urldate = {2026-03-01},
abstract = {Competing charge and spin orders are central to uncovering the nature of unconventional superconductivity. Here we utilize synchrotron X-ray diffraction on a high-quality single crystal to reveal the charge order of La3Ni2O7 at ambient pressure, which competes with the high-temperature superconducting phase under pressure. Enabled by the high synchrotron photon flux and a large dynamic range, we resolve faint reflections – nearly four orders of magnitude weaker than the main Bragg reflections – that were overlooked in prior diffraction studies. This observation evidences a broken glide-mirror symmetry, leading to a polar crystal structure, rather than the widely used centrosymmetric structure model. The polarity is induced by checkerboard charge order on nickel sites in combination with octahedral tilting, reminiscent of bilayer manganese oxides. Our results provide a foundation for understanding phase competition and the mechanism of pressure-induced superconductivity in bilayer nickelates.},
note = {arXiv:2603.25119},
keywords = {B5},
pubstate = {published},
tppubtype = {unpublished}
}
Competing charge and spin orders are central to uncovering the nature of unconventional superconductivity. Here we utilize synchrotron X-ray diffraction on a high-quality single crystal to reveal the charge order of La3Ni2O7 at ambient pressure, which competes with the high-temperature superconducting phase under pressure. Enabled by the high synchrotron photon flux and a large dynamic range, we resolve faint reflections – nearly four orders of magnitude weaker than the main Bragg reflections – that were overlooked in prior diffraction studies. This observation evidences a broken glide-mirror symmetry, leading to a polar crystal structure, rather than the widely used centrosymmetric structure model. The polarity is induced by checkerboard charge order on nickel sites in combination with octahedral tilting, reminiscent of bilayer manganese oxides. Our results provide a foundation for understanding phase competition and the mechanism of pressure-induced superconductivity in bilayer nickelates. |  |
2025
|
Klinger, M.; Treu, T.; Kreisberger, F.; Heil, C.; Klinger, A.; Jesche, A.; Gegenwart, P. Sub-1 K Adiabatic Demagnetization Refrigeration with Rare-Earth Borates Ba3XB9O18 and Ba3XB3O9, X = (Yb, Gd) Journal Article Appl. Sci. 16, 290 (2025), datadoi: 10.5281/zenodo.17855051. @article{klingerSub1AdiabaticDemagnetization2026,
title = {Sub-1 K Adiabatic Demagnetization Refrigeration with Rare-Earth Borates Ba_{3}XB_{9}O_{18} and Ba_{3}XB_{3}O_{9}, X = (Yb, Gd)},
author = {M. Klinger and T. Treu and F. Kreisberger and C. Heil and A. Klinger and A. Jesche and P. Gegenwart},
url = {https://doi.org/10.3390/app16010290},
doi = {10.3390/app16010290},
year = {2025},
date = {2025-12-27},
urldate = {2026-01-01},
journal = {Appl. Sci.},
volume = {16},
number = {1},
pages = {290},
abstract = {Adiabatic demagnetization refrigeration (ADR) is regaining relevance for refrigeration to temperatures below 1 K as global helium-3 supply is increasingly strained. While ADR at these temperatures is long established with paramagnetic hydrated salts, more recently, frustrated rare-earth oxides were found to offer higher entropy densities and practical advantages, since they do not degrade under heating or evacuation. We report structural, magnetic, and thermodynamic properties of the rare-earth borates Ba3XB9O18 and Ba3XB3O9 with X = (Yb, Gd). Except for Ba3GdB9O18, which orders at 108 mK, the three other materials remain paramagnetic down to their lowest measured temperatures. ADR performance starting at 2 K in a field of 5 T is analyzed and compared to literature.},
note = {datadoi: 10.5281/zenodo.17855051},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
Adiabatic demagnetization refrigeration (ADR) is regaining relevance for refrigeration to temperatures below 1 K as global helium-3 supply is increasingly strained. While ADR at these temperatures is long established with paramagnetic hydrated salts, more recently, frustrated rare-earth oxides were found to offer higher entropy densities and practical advantages, since they do not degrade under heating or evacuation. We report structural, magnetic, and thermodynamic properties of the rare-earth borates Ba3XB9O18 and Ba3XB3O9 with X = (Yb, Gd). Except for Ba3GdB9O18, which orders at 108 mK, the three other materials remain paramagnetic down to their lowest measured temperatures. ADR performance starting at 2 K in a field of 5 T is analyzed and compared to literature. |  |
Neehus, A.; Rosch, A.; Knolle, J.; Seifert, U. F. P. Projectively Implemented Altermagnetism in an Exactly Solvable Quantum Spin Liquid Journal Article Phys. Rev. Lett. 135, 256504 (2025), datadoi: 10.5281/zenodo.15231830. @article{neehusProjectivelyImplementedAltermagnetism2025,
title = {Projectively Implemented Altermagnetism in an Exactly Solvable Quantum Spin Liquid},
author = {A. Neehus and A. Rosch and J. Knolle and U. F. P. Seifert},
url = {https://link.aps.org/doi/10.1103/cnk8-vnxg},
doi = {10.1103/cnk8-vnxg},
year = {2025},
date = {2025-12-19},
urldate = {2025-12-01},
journal = {Phys. Rev. Lett.},
volume = {135},
number = {25},
pages = {256504},
publisher = {American Physical Society},
abstract = {Altermagnets are a new class of symmetry-compensated magnets with large spin splittings. Here, we show that the notion of altermagnetism extends beyond the realm of Landau-type order: we study exactly solvable ℤ2 quantum spin(-orbital) liquids (QSLs), which simultaneously support magnetic long-range order as well as fractionalization and ℤ2 topological order. Our symmetry analysis reveals that in this model three distinct types of “fractionalized altermagnets (AM*)” emerge, which can be distinguished by their residual symmetries. Importantly, the fractionalized excitations of these states carry an emergent ℤ2 gauge charge, which implies that they transform projectively under symmetry operations. Consequently, we show that “altermagnetic spin splittings” are now encoded in a momentum-dependent particle-hole asymmetry of the fermionic parton bands. We discuss consequences for experimental observables such as dynamical spin structure factors and (nonlinear) thermal and spin transport.},
note = {datadoi: 10.5281/zenodo.15231830},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Altermagnets are a new class of symmetry-compensated magnets with large spin splittings. Here, we show that the notion of altermagnetism extends beyond the realm of Landau-type order: we study exactly solvable ℤ2 quantum spin(-orbital) liquids (QSLs), which simultaneously support magnetic long-range order as well as fractionalization and ℤ2 topological order. Our symmetry analysis reveals that in this model three distinct types of “fractionalized altermagnets (AM*)” emerge, which can be distinguished by their residual symmetries. Importantly, the fractionalized excitations of these states carry an emergent ℤ2 gauge charge, which implies that they transform projectively under symmetry operations. Consequently, we show that “altermagnetic spin splittings” are now encoded in a momentum-dependent particle-hole asymmetry of the fermionic parton bands. We discuss consequences for experimental observables such as dynamical spin structure factors and (nonlinear) thermal and spin transport. |  |
Shiotani, T.; Waki, T.; Tabata, Y.; Nakamura, H.; Kézsmárki, I. Near-room-temperature compensated itinerant pyrochlore ferrimagnets, RInCo4 ( R = Dy − Tm ) Journal Article Phy. Rev. Mater. 9, 124411 (2025). @article{shiotaniNearroomtemperatureCompensatedItinerant2025,
title = {Near-room-temperature compensated itinerant pyrochlore ferrimagnets, RInCo_{4} ( R = Dy − Tm )},
author = {T. Shiotani and T. Waki and Y. Tabata and H. Nakamura and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/xgkd-6jv1},
doi = {10.1103/xgkd-6jv1},
issn = {2475-9953},
year = {2025},
date = {2025-12-17},
urldate = {2025-12-17},
journal = {Phy. Rev. Mater.},
volume = {9},
number = {12},
pages = {124411},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
|  |
Zhou, S.; Litzius, K.; Büttner, F.; Caretta, L. Statistical Signatures of Topology and Chirality in the Annihilation Field Distributions of Magnetic Thin Films Journal Article Adv. Funct. Mater. 36, (2025). @article{zhouStatisticalSignaturesTopology2025,
title = {Statistical Signatures of Topology and Chirality in the Annihilation Field Distributions of Magnetic Thin Films},
author = {S. Zhou and K. Litzius and F. Büttner and L. Caretta},
url = {http://dx.doi.org/10.1002/adfm.202526052},
doi = {10.1002/adfm.202526052},
year = {2025},
date = {2025-12-17},
urldate = {2025-12-01},
journal = {Adv. Funct. Mater.},
volume = {36},
number = {19},
publisher = {Wiley},
abstract = {Magnetic skyrmions are winding spin textures whose proposed stability underpins their promise for next-generation spintronic devices. While this topological stabilization is widely theorized to suppress collapse and disorder-driven annihilation, direct experimental validation has remained challenging, often requiring complex imaging techniques or indirect electrical probes. Here, a simple and general method is introduced to probe skyrmion topology statistically by analyzing annihilation field distributions in large skyrmion bubble arrays using wide-field Kerr microscopy. By systematically applying in-plane (IP) magnetic fields, the skyrmion topology is continuously tuned, enabling transitions from topologically nontrivial to trivial states. It is found that this topological transition drives a clear shift in annihilation behavior: from broad, thermally activated distributions (stochastic collapse) to narrow, sharply defined distributions (deterministic collapse), confirmed by micromagnetic simulations. This direct correlation between topological state and statistical stability provides a new route for chirality detection and skyrmion state control. This method enables accessible identification of skyrmion topology and opens new possibilities for device concepts: deterministic collapse for synchronized skyrmion deletion in memory, and topology-tunable stochasticity for probabilistic computing and random bit generation.},
keywords = {A4, C2},
pubstate = {published},
tppubtype = {article}
}
Magnetic skyrmions are winding spin textures whose proposed stability underpins their promise for next-generation spintronic devices. While this topological stabilization is widely theorized to suppress collapse and disorder-driven annihilation, direct experimental validation has remained challenging, often requiring complex imaging techniques or indirect electrical probes. Here, a simple and general method is introduced to probe skyrmion topology statistically by analyzing annihilation field distributions in large skyrmion bubble arrays using wide-field Kerr microscopy. By systematically applying in-plane (IP) magnetic fields, the skyrmion topology is continuously tuned, enabling transitions from topologically nontrivial to trivial states. It is found that this topological transition drives a clear shift in annihilation behavior: from broad, thermally activated distributions (stochastic collapse) to narrow, sharply defined distributions (deterministic collapse), confirmed by micromagnetic simulations. This direct correlation between topological state and statistical stability provides a new route for chirality detection and skyrmion state control. This method enables accessible identification of skyrmion topology and opens new possibilities for device concepts: deterministic collapse for synchronized skyrmion deletion in memory, and topology-tunable stochasticity for probabilistic computing and random bit generation. |  |
Rao, P.; Knolle, J.; Classen, L. Van Hove singularities and competing instabilities in an altermagnetic metal Journal Article Phys. Rev. B 112, 235140 (2025), datadoi: 10.5281/zenodo.17868124. @article{zfk4-rxh1,
title = {Van Hove singularities and competing instabilities in an altermagnetic metal},
author = {P. Rao and J. Knolle and L. Classen},
url = {https://link.aps.org/doi/10.1103/zfk4-rxh1},
doi = {10.1103/zfk4-rxh1},
year = {2025},
date = {2025-12-15},
urldate = {2025-12-15},
journal = {Phys. Rev. B},
volume = {112},
number = {23},
pages = {235140},
abstract = {Van Hove (VH) singularities in the single-particle band spectrum are important for interaction-driven quantum phases. Whereas VH points are usually spin-degenerate, in newly proposed altermagnets VH singularities can become spin-dependent, due to momentum-dependent spin polarization of the Fermi surfaces arising from combined rotation and time-reversal symmetry. We consider two altermagnetic models (𝑑𝑥2−𝑦2- and 𝑑𝑥𝑦-wave) on a square lattice with spin-polarized VH points, and study their stable fixed-point solutions indicating interaction-induced instabilities using parquet renormalization group. For both models, we find new stable fixed-point solutions of the renormalization group equations which are not connected to the solution in the spin-degenerate limit. This implies that on the square lattice, the system with VH singularities is unstable with respect to altermagnetic perturbations. The leading instability for the 𝑑𝑥2−𝑦2 model is real transverse spin density wave. For the 𝑑𝑥𝑦-wave model, it is found to be real transverse spin density wave at large altermagnetic splitting. At small altermagnetic splitting both imaginary charge density wave and real longitudinal spin density waves are dominant.},
note = {datadoi: 10.5281/zenodo.17868124},
keywords = {A6, B6},
pubstate = {published},
tppubtype = {article}
}
Van Hove (VH) singularities in the single-particle band spectrum are important for interaction-driven quantum phases. Whereas VH points are usually spin-degenerate, in newly proposed altermagnets VH singularities can become spin-dependent, due to momentum-dependent spin polarization of the Fermi surfaces arising from combined rotation and time-reversal symmetry. We consider two altermagnetic models (𝑑𝑥2−𝑦2- and 𝑑𝑥𝑦-wave) on a square lattice with spin-polarized VH points, and study their stable fixed-point solutions indicating interaction-induced instabilities using parquet renormalization group. For both models, we find new stable fixed-point solutions of the renormalization group equations which are not connected to the solution in the spin-degenerate limit. This implies that on the square lattice, the system with VH singularities is unstable with respect to altermagnetic perturbations. The leading instability for the 𝑑𝑥2−𝑦2 model is real transverse spin density wave. For the 𝑑𝑥𝑦-wave model, it is found to be real transverse spin density wave at large altermagnetic splitting. At small altermagnetic splitting both imaginary charge density wave and real longitudinal spin density waves are dominant. |  |
Song, W.; Liu, G.; Deng, H.; Yang, T.; Li, Y.; Yan, X. -Y.; Liao, R.; Wang, Q.; Xu, J.; Yan, C.; Zhao, Y.; Qin, H.; Wang, D.; Jing, W.; Shen, D.; Nakayama, K.; Sato, T.; Setty, C.; Wu, D.; Song, B.; Ying, T.; Tian, Z.; Sakai, A.; Nakatsuji, S.; Kumar, H.; Kuntscher, C. A.; Wang, Z.; Xue, Q. -K.; Yin, J. -X. Many-body electronic structure in the pyrochlore superconductor CsBi2 and spin-liquid candidate Pr2Ir2O7 Journal Article Phys. Rev. B 112, 245131 (2025). @article{song_many-body_2025,
title = {Many-body electronic structure in the pyrochlore superconductor CsBi_{2} and spin-liquid candidate Pr_{2}Ir_{2}O_{7}},
author = {W. Song and G. Liu and H. Deng and T. Yang and Y. Li and X. -Y. Yan and R. Liao and Q. Wang and J. Xu and C. Yan and Y. Zhao and H. Qin and D. Wang and W. Jing and D. Shen and K. Nakayama and T. Sato and C. Setty and D. Wu and B. Song and T. Ying and Z. Tian and A. Sakai and S. Nakatsuji and H. Kumar and C. A. Kuntscher and Z. Wang and Q. -K. Xue and J. -X. Yin},
url = {https://link.aps.org/doi/10.1103/6jq5-fgxl},
doi = {10.1103/6jq5-fgxl},
year = {2025},
date = {2025-12-12},
urldate = {2025-12-12},
journal = {Phys. Rev. B},
volume = {112},
number = {24},
pages = {245131},
abstract = {The pyrochlore lattice materials can exhibit geometrical frustration, while the related many-body electronic states remain elusive. In this work, we performed scanning tunneling microscopy measurements on the pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7 at 0.3 K. For the first time, we obtained atomically resolved images of their (111) surfaces, revealing a hexagonal lattice or a kagome lattice. Tunneling spectroscopy in CsBi2 reveals a nearly fully opened superconductivity gap. The ratio of 2Δ/𝑘_𝐵𝑇_C=4.7 suggests relatively strong coupling superconductivity, as compared with that in kagome superconductors 𝐴V3Sb5 (𝐴 = K, Rb, Cs). In contrast to the previous study categorizing CsBi2 as a type-I superconductor, the applied magnetic field induces a hexagonal vortex lattice in which each vortex core exhibits an intriguing threefold symmetry state. In Pr2Ir2O7, we observed a spatially homogeneous Kondo-lattice resonance, which is compared with that in the kagome Kondo-lattice material CsCr6Sb6. We further discover that the Kondo resonance exhibits a spatial modulation with threefold symmetry, and the applied magnetic field induces a Zeeman splitting of the Kondo resonance with intriguing atomic site dependence. We discuss the relations of these many-body electronic phenomena with the pyrochlore lattice geometry and its charge or spin frustration. Our systematic observations offer atomic-scale insights into the many-body electronic structures of the geometrically frustrated pyrochlore superconductors and spin liquids.},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
The pyrochlore lattice materials can exhibit geometrical frustration, while the related many-body electronic states remain elusive. In this work, we performed scanning tunneling microscopy measurements on the pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7 at 0.3 K. For the first time, we obtained atomically resolved images of their (111) surfaces, revealing a hexagonal lattice or a kagome lattice. Tunneling spectroscopy in CsBi2 reveals a nearly fully opened superconductivity gap. The ratio of 2Δ/𝑘_𝐵𝑇_C=4.7 suggests relatively strong coupling superconductivity, as compared with that in kagome superconductors 𝐴V3Sb5 (𝐴 = K, Rb, Cs). In contrast to the previous study categorizing CsBi2 as a type-I superconductor, the applied magnetic field induces a hexagonal vortex lattice in which each vortex core exhibits an intriguing threefold symmetry state. In Pr2Ir2O7, we observed a spatially homogeneous Kondo-lattice resonance, which is compared with that in the kagome Kondo-lattice material CsCr6Sb6. We further discover that the Kondo resonance exhibits a spatial modulation with threefold symmetry, and the applied magnetic field induces a Zeeman splitting of the Kondo resonance with intriguing atomic site dependence. We discuss the relations of these many-body electronic phenomena with the pyrochlore lattice geometry and its charge or spin frustration. Our systematic observations offer atomic-scale insights into the many-body electronic structures of the geometrically frustrated pyrochlore superconductors and spin liquids. |  |
Grumbach, J.; Sourd, J.; Deeb, M.; Miyata, A.; Suwa, H.; Gottschall, T.; Hauspurg, A.; Chattopadhyay, S.; Rotter, M.; Granovsky, S.; Prodan, L.; Tsurkan, V.; Zherlitsyn, S.; Doerr, M.; Wosnitza, J. Contrasting magnetic behavior in MnSc2X4 (X = S, Se) spinel compounds investigated by magnetoelastic studies Journal Article Phys. Rev. B 112, 214415 (2025). @article{479d-4jvy,
title = {Contrasting magnetic behavior in MnSc_{2}X_{4} (X = S, Se) spinel compounds investigated by magnetoelastic studies},
author = {J. Grumbach and J. Sourd and M. Deeb and A. Miyata and H. Suwa and T. Gottschall and A. Hauspurg and S. Chattopadhyay and M. Rotter and S. Granovsky and L. Prodan and V. Tsurkan and S. Zherlitsyn and M. Doerr and J. Wosnitza},
url = {https://link.aps.org/doi/10.1103/479d-4jvy},
doi = {10.1103/479d-4jvy},
year = {2025},
date = {2025-12-08},
urldate = {2025-12-01},
journal = {Phys. Rev. B},
volume = {112},
number = {21},
pages = {214415},
abstract = {The spinel compounds MnSc2𝑋4 are highly frustrated and candidate materials for vortex-like 3 q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic (𝐻,𝑇) phase diagram for MnSc2S4 from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated MnSc2Se4, having a larger distance between the magnetic Mn3+ ions using the same methods. Unlike in MnSc2S4, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
The spinel compounds MnSc2𝑋4 are highly frustrated and candidate materials for vortex-like 3 q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic (𝐻,𝑇) phase diagram for MnSc2S4 from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated MnSc2Se4, having a larger distance between the magnetic Mn3+ ions using the same methods. Unlike in MnSc2S4, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well. |  |
Ferrari, F.; Willsher, J.; Seifert, U. F. P.; Valentí, R.; Knolle, J. Stability of algebraic spin liquids coupled to quantum phonons Journal Article Phys. Rev. Res. 7, L042053 (2025), datadoi: 10.5281/zenodo.14039384. @article{ferrariStabilityAlgebraicSpin2025,
title = {Stability of algebraic spin liquids coupled to quantum phonons},
author = {F. Ferrari and J. Willsher and U. F. P. Seifert and R. Valentí and J. Knolle},
url = {https://link.aps.org/doi/10.1103/9wnn-w8bg},
doi = {10.1103/9wnn-w8bg},
year = {2025},
date = {2025-12-05},
urldate = {2025-12-01},
journal = {Phys. Rev. Res.},
volume = {7},
number = {4},
pages = {L042053},
publisher = {American Physical Society},
abstract = {Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the 𝐽1−𝐽2 antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model’s stability under spin-lattice coupling with dynamical quantum phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ansätze inspired by the low-energy DSL’s conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering.},
note = {datadoi: 10.5281/zenodo.14039384},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the 𝐽1−𝐽2 antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model’s stability under spin-lattice coupling with dynamical quantum phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ansätze inspired by the low-energy DSL’s conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering. |  |
Misawa, R.; Kitou, S.; Yamada, R.; Gaggl, T.; Nakano, R.; Shibata, Y.; Okamura, Y.; Kriener, M.; Baral, P. R.; Nakamura, Y.; Ōnuki, Y.; Takahashi, Y.; Arima, T.; Jovanovic, M.; Schoop, L. M.; Hirschberger, M. Successive orthorhombic distortions in kagome metals by molecular orbital formation Journal Article Adv. Mater. e13015 (2025). @article{misawaSuccessiveOrthorhombicDistortions2025,
title = {Successive orthorhombic distortions in kagome metals by molecular orbital formation},
author = {R. Misawa and S. Kitou and R. Yamada and T. Gaggl and R. Nakano and Y. Shibata and Y. Okamura and M. Kriener and P. R. Baral and Y. Nakamura and Y. Ōnuki and Y. Takahashi and T. Arima and M. Jovanovic and L. M. Schoop and M. Hirschberger},
url = {https://advanced.onlinelibrary.wiley.com/doi/abs/10.1002/adma.202513015},
doi = {10.1002/adma.202513015},
year = {2025},
date = {2025-12-05},
urldate = {2025-12-01},
journal = {Adv. Mater.},
pages = {e13015},
abstract = {Abstract The kagome lattice, with its inherent frustration, hosts a plethora of exotic phenomena, including the emergence of 3q charge-density-wave order. The high rotational symmetry required to realize such an unconventional charge order is broken in many kagome materials by orthorhombic distortions at high temperature, the origin of which remains much less examined despite their ubiquity. In this study, synchrotron X-ray diffraction reveals a structural phase transition from a parent hexagonal structure to an orthorhombic groundstate, mediated by a critical regime with diffuse scattering in the prototypical kagome metals RRu3Si2 (R = Nd, Pr). Structural analysis uncovers partially ordered bonds between kagome layers in the orthorhombic phases. Accordingly, a short-range correlated dimer model on the kagome layers reproduces the diffuse scattering, with the short-range order arising from competing structures induced by the geometrical frustration of the kagome lattice. The observations point to molecular orbital formation between Ru $4d_zˆ2$ orbitals as the driving force behind the transition, consistent with ab initio calculations. A framework based on electronegativity and a tolerance factor is proposed to evaluate the stability of the hexagonal phase in various kagome metals, guiding the design of highly symmetric materials.},
keywords = {B5, C1},
pubstate = {published},
tppubtype = {article}
}
Abstract The kagome lattice, with its inherent frustration, hosts a plethora of exotic phenomena, including the emergence of 3q charge-density-wave order. The high rotational symmetry required to realize such an unconventional charge order is broken in many kagome materials by orthorhombic distortions at high temperature, the origin of which remains much less examined despite their ubiquity. In this study, synchrotron X-ray diffraction reveals a structural phase transition from a parent hexagonal structure to an orthorhombic groundstate, mediated by a critical regime with diffuse scattering in the prototypical kagome metals RRu3Si2 (R = Nd, Pr). Structural analysis uncovers partially ordered bonds between kagome layers in the orthorhombic phases. Accordingly, a short-range correlated dimer model on the kagome layers reproduces the diffuse scattering, with the short-range order arising from competing structures induced by the geometrical frustration of the kagome lattice. The observations point to molecular orbital formation between Ru $4d_zˆ2$ orbitals as the driving force behind the transition, consistent with ab initio calculations. A framework based on electronegativity and a tolerance factor is proposed to evaluate the stability of the hexagonal phase in various kagome metals, guiding the design of highly symmetric materials. |  |
Romen, A.; Knolle, J.; Knap, M. Fractionalized prethermalization in the one-dimensional Hubbard model Journal Article Phys. Rev. B 112, 195124 (2025), datadoi: 10.5281/zenodo.17343675. @article{romenFractionalizedPrethermalizationOnedimensional2025,
title = {Fractionalized prethermalization in the one-dimensional Hubbard model},
author = {A. Romen and J. Knolle and M. Knap},
url = {https://doi.org/10.1103/qlky-lzx6},
doi = {10.1103/qlky-lzx6},
year = {2025},
date = {2025-11-20},
urldate = {2025-11-20},
journal = {Phys. Rev. B},
volume = {112},
number = {19},
pages = {195124},
abstract = {Prethermalization phenomena in driven systems are generally understood via a local Floquet Hamiltonian obtained from a high-frequency expansion. Remarkably, recently it has been shown that a driven Kitaev spin liquid with fractionalized excitations can realize a quasistationary state that is not captured by this paradigm. Instead distinct types of fractionalized excitations are characterized by vastly different temperatures—a phenomenon dubbed . In our work, we analyze fractionalized prethermalization in a driven one-dimensional Hubbard model at strong coupling which hosts spin-charge fractionalization. At intermediate frequencies quasisteady states emerge which are characterized by a low spin and high charge temperature with lifetimes set by two competing processes: the lifetime of the quasiparticles determined by Fermi's Golden rule and the exponentially long lifetime of a Floquet prethermal plateau. We classify drives into three categories, each giving rise to distinct (fractional) prethermalization dynamics. Resorting to a time-dependent variant of the Schrieffer-Wolff transformation, we systematically analyze how these drive categories are linked to the underlying driven Hubbard model, thereby providing a general understanding of the emergent thermalization dynamics. We discuss routes toward an experimental realization of this phenomenon in quantum simulation platforms.},
note = {datadoi: 10.5281/zenodo.17343675},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Prethermalization phenomena in driven systems are generally understood via a local Floquet Hamiltonian obtained from a high-frequency expansion. Remarkably, recently it has been shown that a driven Kitaev spin liquid with fractionalized excitations can realize a quasistationary state that is not captured by this paradigm. Instead distinct types of fractionalized excitations are characterized by vastly different temperatures—a phenomenon dubbed . In our work, we analyze fractionalized prethermalization in a driven one-dimensional Hubbard model at strong coupling which hosts spin-charge fractionalization. At intermediate frequencies quasisteady states emerge which are characterized by a low spin and high charge temperature with lifetimes set by two competing processes: the lifetime of the quasiparticles determined by Fermi's Golden rule and the exponentially long lifetime of a Floquet prethermal plateau. We classify drives into three categories, each giving rise to distinct (fractional) prethermalization dynamics. Resorting to a time-dependent variant of the Schrieffer-Wolff transformation, we systematically analyze how these drive categories are linked to the underlying driven Hubbard model, thereby providing a general understanding of the emergent thermalization dynamics. We discuss routes toward an experimental realization of this phenomenon in quantum simulation platforms. |  |
Wu, Y.; Dai, Z.; Anand, S.; Lin, S. -H.; Yang, Q.; Wang, L.; Pollmann, F.; Zaletel, M. P. Alternating and Gaussian Fermionic Isometric Tensor Network States Journal Article PRX Quantum 6, 040324 (2025). @article{wu_alternating_2025,
title = {Alternating and Gaussian Fermionic Isometric Tensor Network States},
author = {Y. Wu and Z. Dai and S. Anand and S. -H. Lin and Q. Yang and L. Wang and F. Pollmann and M. P. Zaletel},
url = {https://link.aps.org/doi/10.1103/8ypw-c8t4},
doi = {10.1103/8ypw-c8t4},
year = {2025},
date = {2025-11-05},
urldate = {2025-11-01},
journal = {PRX Quantum},
volume = {6},
number = {4},
pages = {040324},
abstract = {Isometric tensor networks in two dimensions enable efficient and accurate study of quantum many-body states, yet the effect of the isometric restriction on the represented quantum states is not fully understood. We address this question in two main contributions. First, we introduce an improved variant of isometric tensor network states (isoTNS) in two dimensions, where the isometric arrows on the columns of the network alternate between pointing upward and downward; hence the name alternating isometric tensor network states. Second, we introduce a numerical tool—the isometric Gaussian fermionic TNS (isoGfTNS)—that incorporates isometric constraints into the framework of Gaussian fermionic tensor network states. We demonstrate in numerous ways that alternating isoTNSs represent many-body ground states of two-dimensional quantum systems significantly better than the original isoTNSs. First, we show that the entanglement in an isoTNS is mediated along the isometric arrows and that alternating isoTNSs mediate entanglement more efficiently than conventional isoTNSs. Second, alternating isoTNSs correspond to a deeper, and thus more representative, sequential-circuit construction of depth 𝒪(𝐿𝑥 ⋅𝐿𝑦) compared to the original isoTNSs of depth 𝒪(𝐿𝑥 +𝐿𝑦). Third, using the Gaussian framework and gradient-based energy minimization, we provide numerical evidence of better bond-dimension scaling and variational energy of alternating isoGfTNSs for ground states of various free-fermionic models, including the Fermi surface, the band insulator, and the 𝑝𝑥 +𝑖𝑝𝑦 mean-field superconductor. Finally, benchmarking on the transverse-field Ising model, we demonstrate that an alternating isoTNS provides substantially improved performance and stability relative to the original isoTNS for the ground-state search algorithm in interacting systems.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Isometric tensor networks in two dimensions enable efficient and accurate study of quantum many-body states, yet the effect of the isometric restriction on the represented quantum states is not fully understood. We address this question in two main contributions. First, we introduce an improved variant of isometric tensor network states (isoTNS) in two dimensions, where the isometric arrows on the columns of the network alternate between pointing upward and downward; hence the name alternating isometric tensor network states. Second, we introduce a numerical tool—the isometric Gaussian fermionic TNS (isoGfTNS)—that incorporates isometric constraints into the framework of Gaussian fermionic tensor network states. We demonstrate in numerous ways that alternating isoTNSs represent many-body ground states of two-dimensional quantum systems significantly better than the original isoTNSs. First, we show that the entanglement in an isoTNS is mediated along the isometric arrows and that alternating isoTNSs mediate entanglement more efficiently than conventional isoTNSs. Second, alternating isoTNSs correspond to a deeper, and thus more representative, sequential-circuit construction of depth 𝒪(𝐿𝑥 ⋅𝐿𝑦) compared to the original isoTNSs of depth 𝒪(𝐿𝑥 +𝐿𝑦). Third, using the Gaussian framework and gradient-based energy minimization, we provide numerical evidence of better bond-dimension scaling and variational energy of alternating isoGfTNSs for ground states of various free-fermionic models, including the Fermi surface, the band insulator, and the 𝑝𝑥 +𝑖𝑝𝑦 mean-field superconductor. Finally, benchmarking on the transverse-field Ising model, we demonstrate that an alternating isoTNS provides substantially improved performance and stability relative to the original isoTNS for the ground-state search algorithm in interacting systems. |  |
Tsirlin, A. A.; Uykur, E. Beyond Kagome: p‐Bands in Kagome Metals Journal Article Adv. Quantum Technol. 8, e2500336 (2025), datadoi: 10.5281/zenodo.15724593. @article{tsirlinKagomePBandsKagome2025,
title = {Beyond Kagome: p‐Bands in Kagome Metals},
author = {A. A. Tsirlin and E. Uykur},
url = {https://advanced.onlinelibrary.wiley.com/doi/10.1002/qute.202500336},
doi = {10.1002/qute.202500336},
issn = {2511-9044, 2511-9044},
year = {2025},
date = {2025-11-01},
urldate = {2025-07-01},
journal = {Adv. Quantum Technol.},
volume = {8},
number = {11},
pages = {e2500336},
abstract = {Recent studies on quantum materials where transition‐metal atoms give rise to ‐bands typical of kagome metals are reviewed. Using examples from several material families – , FeGe, , and – it is argued that ‐bands contributed by elements beyond the kagome network play a crucial role in the electronic instabilities, including the charge‐density waves and superconductivity in kagome metals.},
note = {datadoi: 10.5281/zenodo.15724593},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Recent studies on quantum materials where transition‐metal atoms give rise to ‐bands typical of kagome metals are reviewed. Using examples from several material families – , FeGe, , and – it is argued that ‐bands contributed by elements beyond the kagome network play a crucial role in the electronic instabilities, including the charge‐density waves and superconductivity in kagome metals. | |
Tang, N.; Tripathi, R.; Shimura, Y.; Takabatake, T.; Adroja, D. A.; Gegenwart, P. Quantum Griffiths phase in the kagome Kondo lattice CeRh0.9Pd0.1Sn Journal Article Phys. Rev. B 112, 155151 (2025), datadoi: 10.5281/zenodo.16284216. @article{tangQuantumGriffithsPhase2025,
title = {Quantum Griffiths phase in the kagome Kondo lattice CeRh_{0.9}Pd_{0.1}Sn},
author = {N. Tang and R. Tripathi and Y. Shimura and T. Takabatake and D. A. Adroja and P. Gegenwart},
url = {https://link.aps.org/doi/10.1103/8lf7-j26n},
doi = {10.1103/8lf7-j26n},
issn = {2469-9950, 2469-9969},
year = {2025},
date = {2025-10-23},
urldate = {2025-10-01},
journal = {Phys. Rev. B},
volume = {112},
number = {15},
pages = {155151},
abstract = {CeRhSn is a valence fluctuating heavy-fermion metal with a twisted Ce-kagome lattice, displaying zero-field quantum criticality, previously associated with geometrical frustration. The partial substitution of Rh by Pd in CeRh1−𝑥Pd𝑥Sn enlarges the unit-cell volume, suppresses valence fluctuations, decreases the Kondo temperature, and stabilizes a possible long-range antiferromagnetic (AFM) ordered ground state with 𝑇𝑁=0.8 K at 𝑥=0.5. Previous thermodynamic and spectroscopic measurements for 𝑥=0.1 suggested a quantum critical spin liquid. We report low-temperature dilatometry and magnetization measurements on CeRh0.9Pd0.1Sn and compare with published low-𝑇 specific heat data. The absence of a Grüneisen parameter divergence excludes a conventional quantum criticality scenario. Instead, the weak power-law divergences signal non-Fermi-liquid (NFL) behavior, according to a disorder-driven quantum Griffiths phase scenario. At low temperatures, a negative thermal expansion is found in fields above approximately 0.5 T and the NFL scaling breaks down, probably due to the polarization of AFM correlations.},
note = {datadoi: 10.5281/zenodo.16284216},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
CeRhSn is a valence fluctuating heavy-fermion metal with a twisted Ce-kagome lattice, displaying zero-field quantum criticality, previously associated with geometrical frustration. The partial substitution of Rh by Pd in CeRh1−𝑥Pd𝑥Sn enlarges the unit-cell volume, suppresses valence fluctuations, decreases the Kondo temperature, and stabilizes a possible long-range antiferromagnetic (AFM) ordered ground state with 𝑇𝑁=0.8 K at 𝑥=0.5. Previous thermodynamic and spectroscopic measurements for 𝑥=0.1 suggested a quantum critical spin liquid. We report low-temperature dilatometry and magnetization measurements on CeRh0.9Pd0.1Sn and compare with published low-𝑇 specific heat data. The absence of a Grüneisen parameter divergence excludes a conventional quantum criticality scenario. Instead, the weak power-law divergences signal non-Fermi-liquid (NFL) behavior, according to a disorder-driven quantum Griffiths phase scenario. At low temperatures, a negative thermal expansion is found in fields above approximately 0.5 T and the NFL scaling breaks down, probably due to the polarization of AFM correlations. | |
Yamada, R.; Birch, M. T.; Baral, P. R.; Okumura, S.; Nakano, R.; Gao, S.; Ezawa, M.; Nomoto, T.; Masell, J.; Ishihara, Y.; Kolincio, K. K.; Belopolski, I.; Sagayama, H.; Nakao, H.; Ohishi, K.; Ohhara, T.; Kiyanagi, R.; Nakajima, T.; Tokura, Y.; Arima, T.; Motome, Y.; Hirschmann, M. M.; Hirschberger, M. A metallic p-wave magnet with commensurate spin helix Journal Article Nature 646, 837 (2025), datadoi: (10.5281/zenodo.17035625). @article{yamadaMetallicPwaveMagnet2025,
title = {A metallic p-wave magnet with commensurate spin helix},
author = {R. Yamada and M. T. Birch and P. R. Baral and S. Okumura and R. Nakano and S. Gao and M. Ezawa and T. Nomoto and J. Masell and Y. Ishihara and K. K. Kolincio and I. Belopolski and H. Sagayama and H. Nakao and K. Ohishi and T. Ohhara and R. Kiyanagi and T. Nakajima and Y. Tokura and T. Arima and Y. Motome and M. M. Hirschmann and M. Hirschberger},
url = {https://doi.org/10.1038/s41586-025-09633-4},
doi = {10.1038/s41586-025-09633-4},
year = {2025},
date = {2025-10-22},
urldate = {2025-10-01},
journal = {Nature},
volume = {646},
number = {8086},
pages = {837},
abstract = {Antiferromagnetic states with a spin-split electronic structure give rise to spintronic, magnonic and electronic phenomena despite (near-)zero net magnetization [1–7]. The simplest odd-parity spin splitting—p wave—was originally proposed to emerge from a collective instability in interacting electron systems [8–12]. Recent theory has identified a distinct route to realize p-wave spin-split electronic bands without strong correlations [13,14], termed p-wave magnetism. Here we demonstrate an experimental realization of a metallic p-wave magnet. The odd-parity spin splitting of delocalized conduction electrons arises from their coupling to an antiferromagnetic texture of localized magnetic moments: a coplanar spin helix whose magnetic period is an even multiple of the chemical unit cell, as revealed by X-ray scattering experiments. This texture breaks space-inversion symmetry but approximately preserves time-reversal symmetry up to a half-unit-cell translation—thereby fulfilling the symmetry conditions for p-wave magnetism. Consistent with theoretical predictions, our p-wave magnet shows a characteristic anisotropy in the electronic conductivity [13–15]. Relativistic spin–orbit coupling and a tiny spontaneous net magnetization further break time-reversal symmetry, resulting in a giant anomalous Hall effect (Hall conductivity >600 S cm−1, Hall angle >3%), for an antiferromagnet. Our model calculations show that the spin-nodal planes found in the electronic structure of p-wave magnets are readily gapped by a small perturbation to induce the anomalous Hall effect. We establish metallic p-wave magnets as an ideal platform to explore the functionality of spin-split electronic states in magnets, superconductors, and in spintronic devices.},
note = {datadoi: (10.5281/zenodo.17035625)},
keywords = {B5},
pubstate = {published},
tppubtype = {article}
}
Antiferromagnetic states with a spin-split electronic structure give rise to spintronic, magnonic and electronic phenomena despite (near-)zero net magnetization [1–7]. The simplest odd-parity spin splitting—p wave—was originally proposed to emerge from a collective instability in interacting electron systems [8–12]. Recent theory has identified a distinct route to realize p-wave spin-split electronic bands without strong correlations [13,14], termed p-wave magnetism. Here we demonstrate an experimental realization of a metallic p-wave magnet. The odd-parity spin splitting of delocalized conduction electrons arises from their coupling to an antiferromagnetic texture of localized magnetic moments: a coplanar spin helix whose magnetic period is an even multiple of the chemical unit cell, as revealed by X-ray scattering experiments. This texture breaks space-inversion symmetry but approximately preserves time-reversal symmetry up to a half-unit-cell translation—thereby fulfilling the symmetry conditions for p-wave magnetism. Consistent with theoretical predictions, our p-wave magnet shows a characteristic anisotropy in the electronic conductivity [13–15]. Relativistic spin–orbit coupling and a tiny spontaneous net magnetization further break time-reversal symmetry, resulting in a giant anomalous Hall effect (Hall conductivity >600 S cm−1, Hall angle >3%), for an antiferromagnet. Our model calculations show that the spin-nodal planes found in the electronic structure of p-wave magnets are readily gapped by a small perturbation to induce the anomalous Hall effect. We establish metallic p-wave magnets as an ideal platform to explore the functionality of spin-split electronic states in magnets, superconductors, and in spintronic devices. |  |
Nandi, S.; Jawale, M.; Bachhar, S.; Kumar, Rahul; Schuller, M.; Bag, R.; Wilkinson, J.; Sichelschmidt, J.; Sundaresan, A.; Haravifard, S.; Büttgen, N.; Mahajan, A. V. Observation of a gapped phase in the one-dimensional S = 1/2 Heisenberg antiferromagnetic chain Cu(Ampy)ClBr Journal Article Phys. Rev. B 112, 134437 (2025). @article{nandi_observationof_2025,
title = {Observation of a gapped phase in the one-dimensional S = 1/2 Heisenberg antiferromagnetic chain Cu(Ampy)ClBr},
author = {S. Nandi and M. Jawale and S. Bachhar and Rahul Kumar and M. Schuller and R. Bag and J. Wilkinson and J. Sichelschmidt and A. Sundaresan and S. Haravifard and N. Büttgen and A. V. Mahajan},
url = {https://link.aps.org/doi/10.1103/mkdv-8m61},
doi = {10.1103/mkdv-8m61},
year = {2025},
date = {2025-10-22},
urldate = {2025-10-22},
journal = {Phys. Rev. B},
volume = {112},
number = {13},
pages = {134437},
abstract = {Spin-1/2 Heisenberg antiferromagnetic frustrated spin-chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is tuned. We present a comprehensive investigation of the structural, magnetic, and thermodynamics properties of the spin-1/2 compound, Cu(Ampy)ClBr(Ampy=C6H8N2=2 -(aminomethyl)pyridine) via x-ray diffraction, magnetization, specific heat, 1H nuclear magnetic resonance (NMR), electron spin resonance, and muon spin relaxation (𝜇SR) techniques. The crystal structure features an anisotropic triangular chain lattice of magnetic Cu2+ ions. Our bulk and local probe experiments detect neither long-range magnetic ordering nor spin freezing down to 0.06 K despite the presence of moderate antiferromagnetic interaction between Cu2+ spins as reflected by a Curie-Weiss temperature of about −9 K from the bulk susceptibility data. A broad maximum is observed at about 9 K in magnetic susceptibility and specific-heat data, indicating the onset of short-range spin correlations. At low temperatures, the zero-field magnetic specific heat and the 1H NMR spin-lattice relaxation rate follow an exponential temperature dependence, indicating the presence of gapped magnetic excitations. Furthermore, persistent spin dynamics down to 0.088 K observed by zero-field 𝜇SR evidences lack of any static magnetism.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
Spin-1/2 Heisenberg antiferromagnetic frustrated spin-chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is tuned. We present a comprehensive investigation of the structural, magnetic, and thermodynamics properties of the spin-1/2 compound, Cu(Ampy)ClBr(Ampy=C6H8N2=2 -(aminomethyl)pyridine) via x-ray diffraction, magnetization, specific heat, 1H nuclear magnetic resonance (NMR), electron spin resonance, and muon spin relaxation (𝜇SR) techniques. The crystal structure features an anisotropic triangular chain lattice of magnetic Cu2+ ions. Our bulk and local probe experiments detect neither long-range magnetic ordering nor spin freezing down to 0.06 K despite the presence of moderate antiferromagnetic interaction between Cu2+ spins as reflected by a Curie-Weiss temperature of about −9 K from the bulk susceptibility data. A broad maximum is observed at about 9 K in magnetic susceptibility and specific-heat data, indicating the onset of short-range spin correlations. At low temperatures, the zero-field magnetic specific heat and the 1H NMR spin-lattice relaxation rate follow an exponential temperature dependence, indicating the presence of gapped magnetic excitations. Furthermore, persistent spin dynamics down to 0.088 K observed by zero-field 𝜇SR evidences lack of any static magnetism. |  |
Kovács, A.; Weber, J. T.; Charilaou, M.; Kong, D.; Prodan, L.; Tsurkan, V.; Schröder, A.; Kiselev, N. S.; Kézsmárki, I.; Dunin-Borkowski, R. E.; Tavabi, A. H.; Schäfer, S. All-optical stochastic switching of magnetisation textures in Fe3Sn2 Journal Article Commun. Mater. 6, 223 (2025). @article{kovacs_all-optical_2025,
title = {All-optical stochastic switching of magnetisation textures in Fe_{3}Sn_{2}},
author = {A. Kovács and J. T. Weber and M. Charilaou and D. Kong and L. Prodan and V. Tsurkan and A. Schröder and N. S. Kiselev and I. Kézsmárki and R. E. Dunin-Borkowski and A. H. Tavabi and S. Schäfer},
url = {https://doi.org/10.1038/s43246-025-00974-1},
doi = {10.1038/s43246-025-00974-1},
year = {2025},
date = {2025-10-14},
urldate = {2025-10-01},
journal = {Commun. Mater.},
volume = {6},
number = {1},
pages = {223},
abstract = {The all-optical control of magnetisation at room temperature broadens the scope of applications of spin degrees-of-freedom in data storage, spintronics, and quantum computing. Topological magnetic spin structures, such as skyrmions, are of particular interest due to their particle-like properties, small size and inherent stability. Controlling skyrmion states without strong magnetic fields or large current densities would create new possibilities for their application. In this work, we utilize femtosecond optical pulses to alter the helicity of the spin configuration in dipolar skyrmions formed in the kagome magnet Fe3Sn2 in the absence of an external magnetic field and at room temperature. In situ Lorentz transmission electron microscopy is used to visualise the light-induced stochastic switching process of chiral Néel caps, while the internal Bloch component of the dipolar skyrmions remains unchanged. In addition to this switching process, we observe the interconversion between type I skyrmionic and type II bubble configurations depending on the external magnetic field and illumination conditions. To corroborate the spin states and the light-induced magnetisation dynamics, micromagnetic modelling and simulations of the resulting electron phase shift maps are conducted to elucidate the spin rearrangement induced by individual femtosecond optical pulses.},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
The all-optical control of magnetisation at room temperature broadens the scope of applications of spin degrees-of-freedom in data storage, spintronics, and quantum computing. Topological magnetic spin structures, such as skyrmions, are of particular interest due to their particle-like properties, small size and inherent stability. Controlling skyrmion states without strong magnetic fields or large current densities would create new possibilities for their application. In this work, we utilize femtosecond optical pulses to alter the helicity of the spin configuration in dipolar skyrmions formed in the kagome magnet Fe3Sn2 in the absence of an external magnetic field and at room temperature. In situ Lorentz transmission electron microscopy is used to visualise the light-induced stochastic switching process of chiral Néel caps, while the internal Bloch component of the dipolar skyrmions remains unchanged. In addition to this switching process, we observe the interconversion between type I skyrmionic and type II bubble configurations depending on the external magnetic field and illumination conditions. To corroborate the spin states and the light-induced magnetisation dynamics, micromagnetic modelling and simulations of the resulting electron phase shift maps are conducted to elucidate the spin rearrangement induced by individual femtosecond optical pulses. |  |
Isbrandt, G.; Pollmann, F.; Knap, M. Anisotropic spin ice on a breathing pyrochlore lattice Journal Article Phys. Rev. B 112, 165110 (2025), datadoi: 10.5281/zenodo.14931247. @article{isbrandtAnisotropicSpinIce2025,
title = {Anisotropic spin ice on a breathing pyrochlore lattice},
author = {G. Isbrandt and F. Pollmann and M. Knap},
url = {https://link.aps.org/doi/10.1103/gyf7-nm5v},
doi = {10.1103/gyf7-nm5v},
year = {2025},
date = {2025-10-07},
urldate = {2025-10-01},
journal = {Phys. Rev. B},
volume = {112},
number = {16},
pages = {165110},
abstract = {Spin ice systems represent a prime example of constrained spin systems and exhibit rich low-energy physics. In this study, we explore how introducing a tunable anisotropic spin coupling to the conventional Ising spin ice Hamiltonian on the breathing pyrochlore lattice affects the ground state properties of the system. Significant changes are observed in the ground state structure, reflected in the spin structure factor and in a reduction of residual entropy at low temperatures. We theoretically uncover a rich phase diagram by varying the anisotropy and demonstrate how this modification reduces the ground state degeneracy across different phases. Numerical simulations reveal that, at sufficiently low temperatures, the system either undergoes a crossover into a constrained spin ice manifold, characterized by an entropy density that drops below the Pauling entropy of conventional spin ice, or a phase transition into a symmetry-broken state, depending on the perturbations. Additionally, we compute the spin structure factors for the anisotropic model and compare these results to analytical predictions from a self-consistent Gaussian approximation, finding good agreement. This work develops the understanding of spin ice in anisotropic limits, which may be experimentally realized by strain, providing, among others, key signatures in entropy and specific heat.},
note = {datadoi: 10.5281/zenodo.14931247},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
Spin ice systems represent a prime example of constrained spin systems and exhibit rich low-energy physics. In this study, we explore how introducing a tunable anisotropic spin coupling to the conventional Ising spin ice Hamiltonian on the breathing pyrochlore lattice affects the ground state properties of the system. Significant changes are observed in the ground state structure, reflected in the spin structure factor and in a reduction of residual entropy at low temperatures. We theoretically uncover a rich phase diagram by varying the anisotropy and demonstrate how this modification reduces the ground state degeneracy across different phases. Numerical simulations reveal that, at sufficiently low temperatures, the system either undergoes a crossover into a constrained spin ice manifold, characterized by an entropy density that drops below the Pauling entropy of conventional spin ice, or a phase transition into a symmetry-broken state, depending on the perturbations. Additionally, we compute the spin structure factors for the anisotropic model and compare these results to analytical predictions from a self-consistent Gaussian approximation, finding good agreement. This work develops the understanding of spin ice in anisotropic limits, which may be experimentally realized by strain, providing, among others, key signatures in entropy and specific heat. |  |
Rao, P.; Knolle, J. Order-by-disorder in magnets with frustrated spin interactions—classical and large-S limits via the spin functional integral Journal Article J. Phys.: Condens. Matter 37, 405802 (2025). @article{rao_order-by-disorder_2025,
title = {Order-by-disorder in magnets with frustrated spin interactions—classical and large-S limits via the spin functional integral},
author = {P. Rao and J. Knolle},
url = {https://doi.org/10.1088/1361-648X/ae0bdf},
doi = {10.1088/1361-648X/ae0bdf},
year = {2025},
date = {2025-10-07},
urldate = {2025-10-01},
journal = {J. Phys.: Condens. Matter},
volume = {37},
number = {40},
pages = {405802},
abstract = {We investigate spin systems with extensive degeneracies in the classical ground states due to anisotropic frustrated spin interactions, where the degeneracy is not protected by symmetry. Using spin functional integration, we study the lifting of the degeneracies by fluctuations called order-by-disorder (ObD), and the associated gap in the spin-wave spectrum. It is shown that ObD corresponds to gradient-dependent anisotropic interactions of the pseudo-Goldstone modes, which vanish for a classical uniform spin configuration. Fluctuations generate a gradient-independent effective potential which determines the ground state and the pseudo-Goldstone gap. Furthermore, we recover previous predictions for the pseudo-Goldstone gap in type-I and II ObD with two-spin interactions in the large spin-S limit or the classical small temperature limit, by computing the gap explicitly for the type-II cubic compass model and the type-I square compass model. We show that these two limits correspond to the one-loop approximation for the effective potential. We also discuss other types of order by disorder due to m-spin interactions where m > 2.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
We investigate spin systems with extensive degeneracies in the classical ground states due to anisotropic frustrated spin interactions, where the degeneracy is not protected by symmetry. Using spin functional integration, we study the lifting of the degeneracies by fluctuations called order-by-disorder (ObD), and the associated gap in the spin-wave spectrum. It is shown that ObD corresponds to gradient-dependent anisotropic interactions of the pseudo-Goldstone modes, which vanish for a classical uniform spin configuration. Fluctuations generate a gradient-independent effective potential which determines the ground state and the pseudo-Goldstone gap. Furthermore, we recover previous predictions for the pseudo-Goldstone gap in type-I and II ObD with two-spin interactions in the large spin-S limit or the classical small temperature limit, by computing the gap explicitly for the type-II cubic compass model and the type-I square compass model. We show that these two limits correspond to the one-loop approximation for the effective potential. We also discuss other types of order by disorder due to m-spin interactions where m > 2. |  |
Heinsdorf, N.; Joshi, D. G.; Katsura, H.; Schnyder, A. P. Fate of Bosonic Topological Edge Modes in the Presence of Many-Body Interactions Journal Article Phys. Rev. Lett. 135, 146702 (2025). @article{heinsdorf_fate_2025,
title = {Fate of Bosonic Topological Edge Modes in the Presence of Many-Body Interactions},
author = {N. Heinsdorf and D. G. Joshi and H. Katsura and A. P. Schnyder},
url = {https://link.aps.org/doi/10.1103/1pty-fvpf},
doi = {10.1103/1pty-fvpf},
year = {2025},
date = {2025-10-03},
urldate = {2025-10-01},
journal = {Phys. Rev. Lett.},
volume = {135},
number = {14},
pages = {146702},
abstract = {Many magnetic materials are predicted to exhibit bosonic topological edge modes in their excitation spectra, because of the nontrivial topology of their magnon, triplon, or other quasiparticle band structures. However, there is a discrepancy between theory prediction and experimental observation, which suggests some underlying mechanism that intrinsically suppresses the expected experimental signatures, like the thermal Hall current. Many-body interactions that are not accounted for in the noninteracting quasiparticle picture are most often identified as the reason for the absence of the topological edge modes. Here we report persistent bosonic edge modes at the boundaries of a ladder quantum paramagnet with gapped triplon excitations in the presence of the full many-body interaction. We use tensor network methods to resolve topological edge modes in the time-dependent spin-spin correlations and the dynamical structure factor, which is directly accessible experimentally. We further show that signatures of these edge modes survive even when the noninteracting quasiparticle theory breaks down; we discuss the topological phase diagram of the model, demonstrate the fractionalization of its low-lying excitations, and propose potential material candidates.},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
Many magnetic materials are predicted to exhibit bosonic topological edge modes in their excitation spectra, because of the nontrivial topology of their magnon, triplon, or other quasiparticle band structures. However, there is a discrepancy between theory prediction and experimental observation, which suggests some underlying mechanism that intrinsically suppresses the expected experimental signatures, like the thermal Hall current. Many-body interactions that are not accounted for in the noninteracting quasiparticle picture are most often identified as the reason for the absence of the topological edge modes. Here we report persistent bosonic edge modes at the boundaries of a ladder quantum paramagnet with gapped triplon excitations in the presence of the full many-body interaction. We use tensor network methods to resolve topological edge modes in the time-dependent spin-spin correlations and the dynamical structure factor, which is directly accessible experimentally. We further show that signatures of these edge modes survive even when the noninteracting quasiparticle theory breaks down; we discuss the topological phase diagram of the model, demonstrate the fractionalization of its low-lying excitations, and propose potential material candidates. |  |
Ginga, V. A.; Shen, B.; Uykur, E.; Giordano, N.; Gegenwart, P.; Tsirlin, A. A. Pressure-tuned spin chains in brochantite, Cu4SO4(OH)6 Journal Article Phys. Rev. Mater. 9, 094412 (2025). @article{ginga_pressure-tuned_2025,
title = {Pressure-tuned spin chains in brochantite, Cu_{4}SO_{4}(OH)_{6}},
author = {V. A. Ginga and B. Shen and E. Uykur and N. Giordano and P. Gegenwart and A. A. Tsirlin},
url = {https://link.aps.org/doi/10.1103/g459-sxb7},
doi = {10.1103/g459-sxb7},
year = {2025},
date = {2025-09-24},
urldate = {2025-09-01},
journal = {Phys. Rev. Mater.},
volume = {9},
number = {9},
pages = {094412},
abstract = {Using high-pressure single-crystal x-ray diffraction combined with thermodynamic measurements and density-functional calculations, we uncover the microscopic magnetic model of the mineral brochantite, Cu4SO4(OH)6, and its evolution upon compression. The formation of antiferromagnetic spin chains with the effective intrachain coupling of 𝐽≃100K is attributed to the occurrence of longer Cu–Cu distances and larger Cu–O–Cu bond angles between the structural chains within the layers of the brochantite structure. These zigzag spin chains are additionally stabilized by ferromagnetic couplings 𝐽2 between second neighbors and moderately frustrated by several antiferromagnetic couplings that manifest themselves in the reduced Néel temperature of the material. Pressure tuning of the brochantite structure keeps its monoclinic symmetry unchanged and leads to the growth of antiferromagnetic 𝐽 with the rate of 3.2 K/GPa, although this trend is primarily caused by the enhanced ferromagnetic couplings 𝐽2. Our results show that the nature of magnetic couplings in brochantite and in other layered Cu2+ minerals is controlled by the size of the lattice translation along their structural chains and by the extent of the layer buckling.},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Using high-pressure single-crystal x-ray diffraction combined with thermodynamic measurements and density-functional calculations, we uncover the microscopic magnetic model of the mineral brochantite, Cu4SO4(OH)6, and its evolution upon compression. The formation of antiferromagnetic spin chains with the effective intrachain coupling of 𝐽≃100K is attributed to the occurrence of longer Cu–Cu distances and larger Cu–O–Cu bond angles between the structural chains within the layers of the brochantite structure. These zigzag spin chains are additionally stabilized by ferromagnetic couplings 𝐽2 between second neighbors and moderately frustrated by several antiferromagnetic couplings that manifest themselves in the reduced Néel temperature of the material. Pressure tuning of the brochantite structure keeps its monoclinic symmetry unchanged and leads to the growth of antiferromagnetic 𝐽 with the rate of 3.2 K/GPa, although this trend is primarily caused by the enhanced ferromagnetic couplings 𝐽2. Our results show that the nature of magnetic couplings in brochantite and in other layered Cu2+ minerals is controlled by the size of the lattice translation along their structural chains and by the extent of the layer buckling. |  |
Seidov, Z. Y.; Yatsyk, I. V.; Shestakov, A. V.; Ovchinnikov, A. S.; Vagizov, F. G.; Shustov, V. A.; Badelin, A. G.; Karpasyuk, V. K.; Najafzade, M. J.; Ibrahimov, I. N.; von Nidda, H. -A. Krug; Eremina, R. M. Griffiths phase and magnetocaloric effect in ferromagnetic La0.7Sr0.3Mn0.9Fe0.1−xZnxO3 (x = 0.05, 0.075 and 0.1) Journal Article J. Alloys Compd. 1040, 182887 (2025). @article{seidov_griffiths_2025,
title = {Griffiths phase and magnetocaloric effect in ferromagnetic La_{0.7}Sr_{0.3}Mn_{0.9}Fe_{0.1−x}Zn_{x}O_{3} (x = 0.05, 0.075 and 0.1)},
author = {Z. Y. Seidov and I. V. Yatsyk and A. V. Shestakov and A. S. Ovchinnikov and F. G. Vagizov and V. A. Shustov and A. G. Badelin and V. K. Karpasyuk and M. J. Najafzade and I. N. Ibrahimov and H. -A. Krug von Nidda and R. M. Eremina},
url = {https://www.sciencedirect.com/science/article/pii/S0925838825044482},
doi = {https://doi.org/10.1016/j.jallcom.2025.182887},
issn = {0925-8388},
year = {2025},
date = {2025-09-23},
urldate = {2025-09-01},
journal = {J. Alloys Compd.},
volume = {1040},
pages = {182887},
abstract = {The polycrystalline La0.7Sr0.3Mn0.9Fe0.1−xZnxO3 (x= 0.05, 0.075 and 0.1) have been investigated by means of electron spin resonance (ESR), magnetic susceptibility, magnetization, and Mössbauer measurements. Mössbauer studies for x = 0.05 indicate that Fe in these compounds is in the trivalent high-spin state. All compounds exhibits a paramagnetic to ferromagnetic transition at the Curie temperature TC. The Curie temperature TC decreases on increasing Zn content according to 278, 193 and 166 K for x = 0.05, 0.075 and 0.1, respectively. The existence of a Griffiths like phase is experimentally detected by means of magnetic susceptibility and ESR measurements and corroborated by theoretical modeling. We also observed a magnetocaloric effect with a maximum magnetic entropy change (textbarΔSMmaxtextbar) value occurring close to the Curie temperature TC, corresponding to textbarΔSMmaxtextbar = 2.9, 2.6 and 2.68 J/(kg K) under magnetic field change (ΔH) of 50 kOe for x = 0.05, 0.075 and 0.1, respectively. The relative cooling power values were found to vary between 0.25 and 0.31 kJ/kg.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
The polycrystalline La0.7Sr0.3Mn0.9Fe0.1−xZnxO3 (x= 0.05, 0.075 and 0.1) have been investigated by means of electron spin resonance (ESR), magnetic susceptibility, magnetization, and Mössbauer measurements. Mössbauer studies for x = 0.05 indicate that Fe in these compounds is in the trivalent high-spin state. All compounds exhibits a paramagnetic to ferromagnetic transition at the Curie temperature TC. The Curie temperature TC decreases on increasing Zn content according to 278, 193 and 166 K for x = 0.05, 0.075 and 0.1, respectively. The existence of a Griffiths like phase is experimentally detected by means of magnetic susceptibility and ESR measurements and corroborated by theoretical modeling. We also observed a magnetocaloric effect with a maximum magnetic entropy change (textbarΔSMmaxtextbar) value occurring close to the Curie temperature TC, corresponding to textbarΔSMmaxtextbar = 2.9, 2.6 and 2.68 J/(kg K) under magnetic field change (ΔH) of 50 kOe for x = 0.05, 0.075 and 0.1, respectively. The relative cooling power values were found to vary between 0.25 and 0.31 kJ/kg. |  |
Ghara, S.; Winkler, M.; Schmid, S. W.; Prodan, L.; Geirhos, K.; Tsurkan, V.; Ge, Wenbo; Wu, Weida; Halbritter, A.; Krohns, S.; Kézsmárki, I. Nonvolatile electric control of antiferromagnetic states on nanosecond timescales Journal Article Phys. Rev. Lett. 135, 126704 (2025), datadoi: 10.5281/zenodo.16949831. @article{gharaNonvolatileElectricControl2025,
title = {Nonvolatile electric control of antiferromagnetic states on nanosecond timescales},
author = {S. Ghara and M. Winkler and S. W. Schmid and L. Prodan and K. Geirhos and V. Tsurkan and Wenbo Ge and Weida Wu and A. Halbritter and S. Krohns and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/yzrk-h3rz},
doi = {10.1103/yzrk-h3rz},
year = {2025},
date = {2025-09-18},
urldate = {2025-09-18},
journal = {Phys. Rev. Lett.},
volume = {135},
number = {12},
pages = {126704},
abstract = {Electrical manipulation of antiferromagnetic (AFM) states, a cornerstone of AFM spintronics, is a great challenge, requiring novel material platforms. Here we report the full control over AFM states by voltage pulses in the insulating Co3O4 spinel well below its Néel temperature. We show that the strong linear magnetoelectric effect is fully governed by the orientation of the Néel vector. As a unique feature of Co3O4, the magnetoelectric energy can easily overcome the weak magnetocrystalline anisotropy; thus, the Néel vector can be manipulated on demand, either rotated smoothly or reversed suddenly, by combined electric and magnetic fields. We achieve the nonvolatile switching within a few tens of nanoseconds between time-reversed AFM states in macroscopic volumes by voltage pulses. These observations render quasicubic antiferromagnets, like Co3O4, an ideal platform for the ultrafast (picosecond to nanosecond) manipulation of microscopic AFM domains and may pave the way for the realization of AFM spintronic devices.},
note = {datadoi: 10.5281/zenodo.16949831},
keywords = {A4, C2},
pubstate = {published},
tppubtype = {article}
}
Electrical manipulation of antiferromagnetic (AFM) states, a cornerstone of AFM spintronics, is a great challenge, requiring novel material platforms. Here we report the full control over AFM states by voltage pulses in the insulating Co3O4 spinel well below its Néel temperature. We show that the strong linear magnetoelectric effect is fully governed by the orientation of the Néel vector. As a unique feature of Co3O4, the magnetoelectric energy can easily overcome the weak magnetocrystalline anisotropy; thus, the Néel vector can be manipulated on demand, either rotated smoothly or reversed suddenly, by combined electric and magnetic fields. We achieve the nonvolatile switching within a few tens of nanoseconds between time-reversed AFM states in macroscopic volumes by voltage pulses. These observations render quasicubic antiferromagnets, like Co3O4, an ideal platform for the ultrafast (picosecond to nanosecond) manipulation of microscopic AFM domains and may pave the way for the realization of AFM spintronic devices. |  |
Wang, Z.; Cui, X.; Treu, T.; Guo, J.; Liu, X.; Klinger, M.; Heil, C.; Ma, N.; Sheng, X.; Deng, Z.; Lu, X.; Wang, X.; Li, W.; Gegenwart, P.; Jin, C.; Zhao, K. Antiferromagnetic ordering and critical behavior induced giant magnetocaloric effect in distorted kagome lattice Gd3BWO9 Journal Article Phys. Rev. Mater. 9, 094407 (2025). @article{wang_antiferromagnetic_2025,
title = {Antiferromagnetic ordering and critical behavior induced giant magnetocaloric effect in distorted kagome lattice Gd_{3}BWO_{9}},
author = {Z. Wang and X. Cui and T. Treu and J. Guo and X. Liu and M. Klinger and C. Heil and N. Ma and X. Sheng and Z. Deng and X. Lu and X. Wang and W. Li and P. Gegenwart and C. Jin and K. Zhao},
url = {https://link.aps.org/doi/10.1103/7l6y-hdw5},
doi = {10.1103/7l6y-hdw5},
year = {2025},
date = {2025-09-16},
urldate = {2025-09-01},
journal = {Phys. Rev. Mater.},
volume = {9},
number = {9},
pages = {094407},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
|  |
Neehus, A.; Pollmann, F.; Knolle, J. Genuine Topological Anderson Insulator from Impurity Induced Chirality Reversal Journal Article Phys. Rev. Lett. 135, 126604 (2025). @article{neehus_genuine_2025,
title = {Genuine Topological Anderson Insulator from Impurity Induced Chirality Reversal},
author = {A. Neehus and F. Pollmann and J. Knolle},
url = {https://link.aps.org/doi/10.1103/7p8y-2mp6},
doi = {10.1103/7p8y-2mp6},
year = {2025},
date = {2025-09-16},
urldate = {2025-09-01},
journal = {Phys. Rev. Lett.},
volume = {135},
number = {12},
pages = {126604},
abstract = {We investigate a model of Dirac fermions with mass impurities that open a global topological gap even in the dilute limit. Surprisingly, we find that the chirality of this mass term, i.e., the sign of the Chern number, can be reversed by tuning the magnitude of the single-impurity scattering. Consequently, the disorder induces a phase disconnected from the simple clean limit of the topological insulator, which is achieved via an impurity resonance inducing additional bands with Chern number 2. Thus, we call this impurity induced phase a genuine topological Anderson insulator. In seeming contradiction to the expectation that mass disorder is an irrelevant perturbation to the Dirac semimetal, the tricritical point separating these two Chern insulating phases and a thermal metal phase is located at zero impurity density and connected to the appearance of a zero energy bound state in the continuum that corresponds to a perfectly resonant mass impurity. Our conclusions based on the 𝑇
-matrix expansion are substantiated by large scale Chebyshev-polynomial Green’s function numerics. We discuss possible experimental platforms.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
We investigate a model of Dirac fermions with mass impurities that open a global topological gap even in the dilute limit. Surprisingly, we find that the chirality of this mass term, i.e., the sign of the Chern number, can be reversed by tuning the magnitude of the single-impurity scattering. Consequently, the disorder induces a phase disconnected from the simple clean limit of the topological insulator, which is achieved via an impurity resonance inducing additional bands with Chern number 2. Thus, we call this impurity induced phase a genuine topological Anderson insulator. In seeming contradiction to the expectation that mass disorder is an irrelevant perturbation to the Dirac semimetal, the tricritical point separating these two Chern insulating phases and a thermal metal phase is located at zero impurity density and connected to the appearance of a zero energy bound state in the continuum that corresponds to a perfectly resonant mass impurity. Our conclusions based on the 𝑇
-matrix expansion are substantiated by large scale Chebyshev-polynomial Green’s function numerics. We discuss possible experimental platforms. | |
Ferreira-Carvalho, M. M.; Rößler, S.; Chang, C. F.; Hu, Z.; Valvidares, S. M.; Gargiani, P.; Haverkort, M. W.; Mukharjee, P. K.; Gegenwart, P.; Tsirlin, A. A.; Tjeng, L. H. Trigonal distortion in the Kitaev candidate honeycomb magnet BaCo2(AsO4)2 Journal Article Phys. Rev. B 112, 125135 (2025), datadoi: 10.17617/3.PZLFIH. @article{ferreira-carvalhoTrigonalDistortionKitaev2025,
title = {Trigonal distortion in the Kitaev candidate honeycomb magnet BaCo_{2}(AsO_{4})_{2}},
author = {M. M. Ferreira-Carvalho and S. Rößler and C. F. Chang and Z. Hu and S. M. Valvidares and P. Gargiani and M. W. Haverkort and P. K. Mukharjee and P. Gegenwart and A. A. Tsirlin and L. H. Tjeng},
url = {https://link.aps.org/doi/10.1103/2sdd-pyx1},
doi = {10.1103/2sdd-pyx1},
year = {2025},
date = {2025-09-16},
urldate = {2025-09-01},
journal = {Phys. Rev. B},
volume = {112},
number = {12},
pages = {125135},
abstract = {We conducted x-ray absorption (XAS) and magnetic circular dichroism (XMCD) measurements at the Co 𝐿2,3 edges on single crystals of the Kitaev candidate honeycomb lattice compound BaCo2(AsO4)2. The measurements employed the inverse partial fluorescence yield technique, which is ideal for acquiring reliable x-ray absorption spectra from highly insulating samples, enabling precise quantitative analysis. Our experimental results revealed a significant linear dichroic signal, indicating strong trigonal distortion in the CoO6 octahedra in BaCo2(AsO4)2. We performed a detailed analysis of the experimental XAS and XMCD spectra using a full-multiplet configuration-interaction cluster model. This analysis unveiled that the 𝑡2𝑔 hole density is predominantly localized in the 𝑎1𝑔 orbital. Through XMCD sum rules and theoretical calculations, we quantified both the spin and orbital magnetic moments. Our study demonstrates that the local electronic structure of the CoO6 octahedra displays an effective trigonal distortion of approximately −0.114 eV. This distortion is larger than the Co 3𝑑 spin-orbit coupling constant, emphasizing the crucial impact of local structural distortions on the electronic and magnetic properties of BaCo2(AsO4)2.},
note = {datadoi: 10.17617/3.PZLFIH},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
We conducted x-ray absorption (XAS) and magnetic circular dichroism (XMCD) measurements at the Co 𝐿2,3 edges on single crystals of the Kitaev candidate honeycomb lattice compound BaCo2(AsO4)2. The measurements employed the inverse partial fluorescence yield technique, which is ideal for acquiring reliable x-ray absorption spectra from highly insulating samples, enabling precise quantitative analysis. Our experimental results revealed a significant linear dichroic signal, indicating strong trigonal distortion in the CoO6 octahedra in BaCo2(AsO4)2. We performed a detailed analysis of the experimental XAS and XMCD spectra using a full-multiplet configuration-interaction cluster model. This analysis unveiled that the 𝑡2𝑔 hole density is predominantly localized in the 𝑎1𝑔 orbital. Through XMCD sum rules and theoretical calculations, we quantified both the spin and orbital magnetic moments. Our study demonstrates that the local electronic structure of the CoO6 octahedra displays an effective trigonal distortion of approximately −0.114 eV. This distortion is larger than the Co 3𝑑 spin-orbit coupling constant, emphasizing the crucial impact of local structural distortions on the electronic and magnetic properties of BaCo2(AsO4)2. |  |
Will, M.; Cochran, T. A.; Rosenberg, E.; Jobst, B.; Eassa, N. M.; Roushan, P.; Knap, M.; Gammon-Smith, A.; Pollmann, F. Probing non-equilibrium topological order on a quantum processor Journal Article Nature 645, 348 (2025), datadoi: (10.5281/zenodo.15837492). @article{willProbingNonequilibriumTopological2025,
title = {Probing non-equilibrium topological order on a quantum processor},
author = {M. Will and T. A. Cochran and E. Rosenberg and B. Jobst and N. M. Eassa and P. Roushan and M. Knap and A. Gammon-Smith and F. Pollmann},
url = {https://doi.org/10.1038/s41586-025-09456-3},
doi = {10.1038/s41586-025-09456-3},
year = {2025},
date = {2025-09-10},
urldate = {2025-09-01},
journal = {Nature},
volume = {645},
number = {8080},
pages = {348},
abstract = {Out-of-equilibrium phases in many-body systems constitute a new paradigm in quantum matter—they exhibit dynamical properties that may otherwise be forbidden by equilibrium thermodynamics. Among these non-equilibrium phases are periodically driven (Floquet) systems1–5, which are generically difficult to simulate classically because of their high entanglement. Here we realize a Floquet topologically ordered state theoretically proposed in ref. 6, on an array of superconducting qubits. We image the characteristic dynamics of its chiral edge modes and characterize its emergent anyonic excitations. Devising an interferometric algorithm allows us to introduce and measure a bulk topological invariant to probe the dynamical transmutation of anyons for system sizes up to 58 qubits. Our work demonstrates that quantum processors can provide key insights into the thus-far largely unexplored landscape of highly entangled non-equilibrium phases of matter.},
note = {datadoi: (10.5281/zenodo.15837492)},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
Out-of-equilibrium phases in many-body systems constitute a new paradigm in quantum matter—they exhibit dynamical properties that may otherwise be forbidden by equilibrium thermodynamics. Among these non-equilibrium phases are periodically driven (Floquet) systems1–5, which are generically difficult to simulate classically because of their high entanglement. Here we realize a Floquet topologically ordered state theoretically proposed in ref. 6, on an array of superconducting qubits. We image the characteristic dynamics of its chiral edge modes and characterize its emergent anyonic excitations. Devising an interferometric algorithm allows us to introduce and measure a bulk topological invariant to probe the dynamical transmutation of anyons for system sizes up to 58 qubits. Our work demonstrates that quantum processors can provide key insights into the thus-far largely unexplored landscape of highly entangled non-equilibrium phases of matter. |  |
Birnkammer, S.; Knap, M.; Knolle, J.; Mook, A.; Bastianello, A. Scattering theory of chiral edge modes in topological magnon insulators Journal Article Phys. Rev. B 112, 094417 (2025), datadoi: 10.5281/zenodo.13895647. @article{birnkammerScatteringTheoryChiral2025,
title = {Scattering theory of chiral edge modes in topological magnon insulators},
author = {S. Birnkammer and M. Knap and J. Knolle and A. Mook and A. Bastianello},
url = {https://link.aps.org/doi/10.1103/btt2-mp62},
doi = {10.1103/btt2-mp62},
year = {2025},
date = {2025-09-09},
urldate = {2025-09-09},
journal = {Phys. Rev. B},
volume = {112},
number = {9},
pages = {094417},
abstract = {Topological magnon insulators exhibit robust edge modes with chiral properties similar to quantum Hall edge states. However, due to their strong localization at the edges, interactions between these chiral edge magnons can be significant, as we show in a model of coupled magnon-conserving spin chains in an electric field gradient. The chiral edge modes remain edge-localized and do not scatter into the bulk, and we characterize their scattering phase: for strongly localized edge modes, we observe significant deviation from the bare scattering phase. This renormalization of edge scattering can be attributed to bound bulk modes resonating with the chiral edge magnons in the spirit of Feshbach resonances in atomic physics. We argue that the scattering dynamics can be probed experimentally with a real-time measurement protocol using inelastic scanning tunneling spectroscopy. Our results show that interaction among magnons can be encoded in an effective edge model of reduced dimensionality, where the interactions with the bulk renormalize the effective couplings. Our work introduces a systematic way to determine the many-body effective theory for edge states in topological magnon insulators.},
note = {datadoi: 10.5281/zenodo.13895647},
keywords = {B6, C5, C6},
pubstate = {published},
tppubtype = {article}
}
Topological magnon insulators exhibit robust edge modes with chiral properties similar to quantum Hall edge states. However, due to their strong localization at the edges, interactions between these chiral edge magnons can be significant, as we show in a model of coupled magnon-conserving spin chains in an electric field gradient. The chiral edge modes remain edge-localized and do not scatter into the bulk, and we characterize their scattering phase: for strongly localized edge modes, we observe significant deviation from the bare scattering phase. This renormalization of edge scattering can be attributed to bound bulk modes resonating with the chiral edge magnons in the spirit of Feshbach resonances in atomic physics. We argue that the scattering dynamics can be probed experimentally with a real-time measurement protocol using inelastic scanning tunneling spectroscopy. Our results show that interaction among magnons can be encoded in an effective edge model of reduced dimensionality, where the interactions with the bulk renormalize the effective couplings. Our work introduces a systematic way to determine the many-body effective theory for edge states in topological magnon insulators. |  |
Wiedmann, R.; Alpin, K.; Hirschmann, M. M.; Schnyder, A. P. Quantum geometry and low-frequency optical conductivity of nodal planes Journal Article Phys. Rev. B 112, 125102 (2025), datadoi: 10.5281/zenodo.16900403. @article{wiedmannQuantumGeometryLowfrequency2025,
title = {Quantum geometry and low-frequency optical conductivity of nodal planes},
author = {R. Wiedmann and K. Alpin and M. M. Hirschmann and A. P. Schnyder},
url = {https://link.aps.org/doi/10.1103/2f4l-tz7p},
doi = {10.1103/2f4l-tz7p},
issn = {2469-9950, 2469-9969},
year = {2025},
date = {2025-09-02},
urldate = {2025-09-01},
journal = {Phys. Rev. B},
volume = {112},
number = {12},
pages = {125102},
abstract = {Nodal planes, two-dimensional symmetry-enforced band crossings, can carry a topological charge, similar to Weyl points. While the transport properties of Weyl points are well understood, those of nodal planes remain largely unexplored. These properties are influenced not only by the Berry curvature, but also by other quantum geometric quantities. In this work we study the quantum geometry, specifically the Berry curvature and quantum metric, and the linear optical conductivity of topological nodal planes. We introduce a low-energy model and investigate its low-frequency optical responses to determine the unique signatures of nodal planes. By comparing these findings to the optical response in a tight-binding model with a topological nodal plane, we observe consistent low-frequency behavior with a cubic power law. This paves the way for the experimental detection of nodal planes through optical conductivity measurements for which we suggest suitable materials, most promisingly the material group 𝑋Mo3S3 (𝑋= Rb, K, Cs).},
note = {datadoi: 10.5281/zenodo.16900403},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
Nodal planes, two-dimensional symmetry-enforced band crossings, can carry a topological charge, similar to Weyl points. While the transport properties of Weyl points are well understood, those of nodal planes remain largely unexplored. These properties are influenced not only by the Berry curvature, but also by other quantum geometric quantities. In this work we study the quantum geometry, specifically the Berry curvature and quantum metric, and the linear optical conductivity of topological nodal planes. We introduce a low-energy model and investigate its low-frequency optical responses to determine the unique signatures of nodal planes. By comparing these findings to the optical response in a tight-binding model with a topological nodal plane, we observe consistent low-frequency behavior with a cubic power law. This paves the way for the experimental detection of nodal planes through optical conductivity measurements for which we suggest suitable materials, most promisingly the material group 𝑋Mo3S3 (𝑋= Rb, K, Cs). |  |
Huber, N.; Volkau, I.; Engelhardt, A.; Sheikin, I.; Bauer, A.; Pfleiderer, C.; Wilde, M. A. Fermi surface and magnetic breakdown in PdGa Journal Article Phys. Rev. B 112, 085116 (2025), datadoi: 10.5281/zenodo.15770032. @article{huberFermiSurfaceMagnetic2025,
title = {Fermi surface and magnetic breakdown in PdGa},
author = {N. Huber and I. Volkau and A. Engelhardt and I. Sheikin and A. Bauer and C. Pfleiderer and M. A. Wilde},
url = {https://link.aps.org/doi/10.1103/kwgt-cryz},
doi = {10.1103/kwgt-cryz},
year = {2025},
date = {2025-08-08},
urldate = {2025-08-08},
journal = {Phys. Rev. B},
volume = {112},
number = {8},
pages = {085116},
abstract = {We study the electronic structure of the chiral semimetal PdGa by means of the de Haas–van Alphen and Shubnikov–de Haas effect. We find that the Fermi surface of PdGa comprises multiple pockets split by spin-orbit coupling. We compare our experimental findings with the band structure calculated ab initio. We demonstrate that the quantum oscillation spectra can be fully understood by considering topological nodal plane degeneracies at the Brillouin zone boundary and magnetic breakdown between individual Fermi-surface pockets. Expanding traditional analysis methods, we explicitly calculate magnetic breakdown frequencies and cyclotron masses while taking into account that extremal breakdown trajectories may reside away from the planes of the single-band orbits. We further analyze high-frequency contributions arising from breakdown trajectories involving multiple revolutions around the Fermi surface which are distinct from conventional harmonic frequencies. Our results highlight the existence of gaps induced by spin-orbit coupling throughout the band structure of PdGa, the relevance of nodal planes on the Brillouin zone boundary, and the necessity for a comprehensive analysis of magnetic breakdown.},
note = {datadoi: 10.5281/zenodo.15770032},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
We study the electronic structure of the chiral semimetal PdGa by means of the de Haas–van Alphen and Shubnikov–de Haas effect. We find that the Fermi surface of PdGa comprises multiple pockets split by spin-orbit coupling. We compare our experimental findings with the band structure calculated ab initio. We demonstrate that the quantum oscillation spectra can be fully understood by considering topological nodal plane degeneracies at the Brillouin zone boundary and magnetic breakdown between individual Fermi-surface pockets. Expanding traditional analysis methods, we explicitly calculate magnetic breakdown frequencies and cyclotron masses while taking into account that extremal breakdown trajectories may reside away from the planes of the single-band orbits. We further analyze high-frequency contributions arising from breakdown trajectories involving multiple revolutions around the Fermi surface which are distinct from conventional harmonic frequencies. Our results highlight the existence of gaps induced by spin-orbit coupling throughout the band structure of PdGa, the relevance of nodal planes on the Brillouin zone boundary, and the necessity for a comprehensive analysis of magnetic breakdown. |  |
Rao, P.; Moessner, R.; Knolle, J. Dynamical response theory of interacting Majorana fermions and its application to generic Kitaev quantum spin liquids in a field Journal Article Phys. Rev. B 112, 024440 (2025), datadoi: (10.5281/zenodo.15125435). @article{raoDynamicalResponseTheory2025,
title = {Dynamical response theory of interacting Majorana fermions and its application to generic Kitaev quantum spin liquids in a field},
author = {P. Rao and R. Moessner and J. Knolle},
url = {https://link.aps.org/doi/10.1103/f4b4-h1yr},
doi = {10.1103/f4b4-h1yr},
year = {2025},
date = {2025-07-28},
urldate = {2025-07-01},
journal = {Phys. Rev. B},
volume = {112},
number = {2},
pages = {024440},
abstract = {Motivated by the appearance of Majorana fermions in a broad range of correlated and topological electronic systems, we develop a general method to compute the dynamical response of interacting Majorana fermions in the random-phase approximation (RPA). This can be applied self-consistently on top of Majorana mean-field theory backgrounds, thereby in particular providing a powerful tool to analyze generic behavior in the vicinity of (various heavily studied) exactly soluble models. Prime examples are quantum spin liquids (QSL) with emergent Majorana excitations, with the celebrated exact solution of Kitaev. We employ the RPA to study in considerable detail phase structure and dynamics of the extended Kitaev honeycomb 𝐾𝐽Γ model, with and without an applied field. First, we benchmark our method with Kitaev's exactly soluble model, finding a remarkable agreement. The interactions between Majorana fermions even turn out to mimic the effect of local ℤ2 flux excitations, which we explain analytically. Second, we show how small non-Kitaev couplings 𝐽 and Γ induce Majorana bound states, resulting in sharp features in the dynamical structure factor in the presence of fractionalization: such “spinon excitons” naturally appear, and can coexist and interact with the broad Majorana continuum. Third, for increasing couplings or field, our theory predicts instabilities of the Kitaev QSL (KQSL) triggered by the condensation of the sharp modes. From the high-symmetry momenta of the condensation we can deduce which magnetically ordered phases surround the KQSL, in good agreement with previous finite-size numerics. We discuss implications for experiments and the broad range of applicability of our method to other QSL and Majorana systems.},
note = {datadoi: (10.5281/zenodo.15125435)},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Motivated by the appearance of Majorana fermions in a broad range of correlated and topological electronic systems, we develop a general method to compute the dynamical response of interacting Majorana fermions in the random-phase approximation (RPA). This can be applied self-consistently on top of Majorana mean-field theory backgrounds, thereby in particular providing a powerful tool to analyze generic behavior in the vicinity of (various heavily studied) exactly soluble models. Prime examples are quantum spin liquids (QSL) with emergent Majorana excitations, with the celebrated exact solution of Kitaev. We employ the RPA to study in considerable detail phase structure and dynamics of the extended Kitaev honeycomb 𝐾𝐽Γ model, with and without an applied field. First, we benchmark our method with Kitaev's exactly soluble model, finding a remarkable agreement. The interactions between Majorana fermions even turn out to mimic the effect of local ℤ2 flux excitations, which we explain analytically. Second, we show how small non-Kitaev couplings 𝐽 and Γ induce Majorana bound states, resulting in sharp features in the dynamical structure factor in the presence of fractionalization: such “spinon excitons” naturally appear, and can coexist and interact with the broad Majorana continuum. Third, for increasing couplings or field, our theory predicts instabilities of the Kitaev QSL (KQSL) triggered by the condensation of the sharp modes. From the high-symmetry momenta of the condensation we can deduce which magnetically ordered phases surround the KQSL, in good agreement with previous finite-size numerics. We discuss implications for experiments and the broad range of applicability of our method to other QSL and Majorana systems. |  |
Papaefstathiou, I.; Malz, D.; Cirac, J. I.; Bañuls, M. C. Efficient tensor network simulation of multiemitter non-Markovian systems Journal Article Phys. Rev. A 112, 013721 (2025), datadoi: (10.5281/zenodo.15764360). @article{papaefstathiouEfficientTensorNetwork2025,
title = {Efficient tensor network simulation of multiemitter non-Markovian systems},
author = {I. Papaefstathiou and D. Malz and J. I. Cirac and M. C. Bañuls},
url = {https://link.aps.org/doi/10.1103/hmbj-lg7p},
doi = {10.1103/hmbj-lg7p},
year = {2025},
date = {2025-07-24},
urldate = {2025-07-01},
journal = {Phys. Rev. A},
volume = {112},
number = {1},
pages = {013721},
note = {datadoi: (10.5281/zenodo.15764360)},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
|  |
Xu, W. -T.; Knap, M.; Pollmann, F. Tensor-Network Study of the Roughening Transition in a (2+1)D ℤ2 Lattice Gauge Theory with Matter Journal Article Phys. Rev. Lett. 135, (2025), datadoi: 10.5281/zenodo.15324471. @article{xuTensorNetworkStudyRoughening2025,
title = {Tensor-Network Study of the Roughening Transition in a (2+1)D ℤ_{2} Lattice Gauge Theory with Matter},
author = {W. -T. Xu and M. Knap and F. Pollmann},
url = {https://doi.org/10.1103/3lxj-dx76},
doi = {10.1103/3lxj-dx76},
issn = {1079-7114},
year = {2025},
date = {2025-07-17},
urldate = {2025-07-01},
journal = {Phys. Rev. Lett.},
volume = {135},
number = {3},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.15324471},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Schilberth, F.; Jiang, M. -C.; Mardelé, F. Le; Papp, L. B.; Mohelsky, I.; Kassem, M. A.; Tabata, Y.; Waki, T.; Nakamura, H.; Guo, G. -Y.; Orlita, M.; Arita, R.; Kézsmárki, I.; Bordács, S. Generation of a nodal line and Weyl points by magnetization reorientation in Co3Sn2S2 Journal Article npj Quantum Mater. 10, 67 (2025), datadoi: 10.5281/zenodo.15354906. @article{schilberthGenerationNodalLine2025,
title = {Generation of a nodal line and Weyl points by magnetization reorientation in Co_{3}Sn_{2}S_{2}},
author = {F. Schilberth and M. -C. Jiang and F. Le Mardelé and L. B. Papp and I. Mohelsky and M. A. Kassem and Y. Tabata and T. Waki and H. Nakamura and G. -Y. Guo and M. Orlita and R. Arita and I. Kézsmárki and S. Bordács},
url = {https://doi.org/10.1038/s41535-025-00785-0},
doi = {10.1038/s41535-025-00785-0},
year = {2025},
date = {2025-07-01},
urldate = {2025-07-01},
journal = {npj Quantum Mater.},
volume = {10},
number = {1},
pages = {67},
abstract = {Topological magnets exhibit fascinating physics like topologically protected surface states and anomalous transport. Although these states and phenomena are expected to strongly depend on the magnetic order, their experimental manipulation has been scarcely studied. Here, we demonstrate the magnetic field control of the topological band structure in Co3Sn2S2 by magneto-optical spectroscopy. We resolve a magnetic field-induced redshift of the nodal loop resonance as the magnetization is rotated into the kagome plane. Our material-specific theory, capturing the observed field-induced spectral reconstruction, reveals the emergence of a gapless nodal loop for one of the in-plane magnetization directions. The calculations show that the additionally created Weyl points for in-plane fields marginally contribute to the optical response. These findings demonstrate that breaking underlying crystal symmetries with external fields provides an efficient way to manipulate topological band features. Moreover, our results highlight the potential of low-energy magneto-optical spectroscopy in probing variations of quantum geometry.},
note = {datadoi: 10.5281/zenodo.15354906},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
Topological magnets exhibit fascinating physics like topologically protected surface states and anomalous transport. Although these states and phenomena are expected to strongly depend on the magnetic order, their experimental manipulation has been scarcely studied. Here, we demonstrate the magnetic field control of the topological band structure in Co3Sn2S2 by magneto-optical spectroscopy. We resolve a magnetic field-induced redshift of the nodal loop resonance as the magnetization is rotated into the kagome plane. Our material-specific theory, capturing the observed field-induced spectral reconstruction, reveals the emergence of a gapless nodal loop for one of the in-plane magnetization directions. The calculations show that the additionally created Weyl points for in-plane fields marginally contribute to the optical response. These findings demonstrate that breaking underlying crystal symmetries with external fields provides an efficient way to manipulate topological band features. Moreover, our results highlight the potential of low-energy magneto-optical spectroscopy in probing variations of quantum geometry. |  |
Sharma, S.; Chioncel, L.; Marco, I. Di Exploring strong electronic correlations in the breathing kagome metal Fe3Sn Journal Article Phys. Rev. B 111, 235127 (2025), datadoi: 10.24435/materialscloud:t7-7p. @article{sharmaExploringStrongElectronic2025,
title = {Exploring strong electronic correlations in the breathing kagome metal Fe_{3}Sn},
author = {S. Sharma and L. Chioncel and I. Di Marco},
url = {https://link.aps.org/doi/10.1103/xmmr-mfv4},
doi = {10.1103/xmmr-mfv4},
year = {2025},
date = {2025-06-16},
urldate = {2025-06-01},
journal = {Phys. Rev. B},
volume = {111},
number = {23},
pages = {235127},
abstract = {Kagome metals have emerged as pivotal materials in condensed matter physics due to their unique geometric arrangement and intriguing electronic properties. Understanding the origin of magnetism in these materials, particularly in iron-rich Fe-Sn binary compounds such as Fe3Sn, holds a significant importance, as they represent potential candidates for permanent magnets with a high Curie temperature and a strong magnetic anisotropy. In the present study, we employ density functional theory and dynamical mean-field theory to analyze the electronic structure and magnetic properties of Fe3Sn. Our investigation reveals the presence of several nearly flat bands and Weyl nodes at low excitation energies. The inclusion of local correlation effects is shown to push these features even closer to the Fermi energy, which may be important for their manipulation via external stimuli. Regarding magnetism, the Hubbard-like interaction leads to an increase of orbital polarization at the expenses of a minor reduction of the spin moment. The magnetic anisotropy energy exhibits a strong dependence on the particular choice of the Coulomb interaction parameters. Additionally, our detailed analysis of the interatomic exchange interactions indicates a significant contribution from the antisymmetric exchange, i.e., the Dzyaloshinskii-Moriya interaction, which showcases the existence of magnetic chirality in the system. Overall, our investigation highlights a strong interplay between the flat bands near the Fermi level, the local Coulomb interaction, and the triangular geometry of the lattice, which plays a crucial role in driving the magnetic properties of this material.},
note = {datadoi: 10.24435/materialscloud:t7-7p},
keywords = {A5},
pubstate = {published},
tppubtype = {article}
}
Kagome metals have emerged as pivotal materials in condensed matter physics due to their unique geometric arrangement and intriguing electronic properties. Understanding the origin of magnetism in these materials, particularly in iron-rich Fe-Sn binary compounds such as Fe3Sn, holds a significant importance, as they represent potential candidates for permanent magnets with a high Curie temperature and a strong magnetic anisotropy. In the present study, we employ density functional theory and dynamical mean-field theory to analyze the electronic structure and magnetic properties of Fe3Sn. Our investigation reveals the presence of several nearly flat bands and Weyl nodes at low excitation energies. The inclusion of local correlation effects is shown to push these features even closer to the Fermi energy, which may be important for their manipulation via external stimuli. Regarding magnetism, the Hubbard-like interaction leads to an increase of orbital polarization at the expenses of a minor reduction of the spin moment. The magnetic anisotropy energy exhibits a strong dependence on the particular choice of the Coulomb interaction parameters. Additionally, our detailed analysis of the interatomic exchange interactions indicates a significant contribution from the antisymmetric exchange, i.e., the Dzyaloshinskii-Moriya interaction, which showcases the existence of magnetic chirality in the system. Overall, our investigation highlights a strong interplay between the flat bands near the Fermi level, the local Coulomb interaction, and the triangular geometry of the lattice, which plays a crucial role in driving the magnetic properties of this material. |  |
Natori, W.; Yang, Y.; Jin, H. -K.; Knolle, J.; Perkins, N. B. Ferrimagnetic Kitaev spin liquids in mixed spin-1/2 and spin-3/2 honeycomb magnets Journal Article Phys. Rev. B 111, 214411 (2025). @article{natori_ferrimagnetic_2025,
title = {Ferrimagnetic Kitaev spin liquids in mixed spin-1/2 and spin-3/2 honeycomb magnets},
author = {W. Natori and Y. Yang and H. -K. Jin and J. Knolle and N. B. Perkins},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.214411},
doi = {10.1103/PhysRevB.111.214411},
year = {2025},
date = {2025-06-04},
urldate = {2025-06-01},
journal = {Phys. Rev. B},
volume = {111},
number = {21},
pages = {214411},
abstract = {We explore the phase diagram of a mixed-spin Kitaev model, where spin-1/2 and spin-3/2 ions form a staggered pattern on a honeycomb lattice. Enabled by an exact mapping of local conserved flux operators onto 𝑍2 gauge fields, we perform a parton mean-field theory for the model with a single-ion anisotropy. The phase diagram contains four types of quantum spin liquids distinguished by quadrupolar parameters. These analytical results are quantitatively confirmed by state-of-the-art DMRG simulations. We also explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr0.5Ru0.5Cl3. By developing a superexchange theory specifically for this mixed-spin system, we identify the conditions under which dominant Kitaev-like interactions emerge. Our findings highlight the importance of spin-orbital couplings and quadrupolar order parameters in stabilizing exotic phases, providing a foundation for exploring mixed-spin Kitaev magnets.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
We explore the phase diagram of a mixed-spin Kitaev model, where spin-1/2 and spin-3/2 ions form a staggered pattern on a honeycomb lattice. Enabled by an exact mapping of local conserved flux operators onto 𝑍2 gauge fields, we perform a parton mean-field theory for the model with a single-ion anisotropy. The phase diagram contains four types of quantum spin liquids distinguished by quadrupolar parameters. These analytical results are quantitatively confirmed by state-of-the-art DMRG simulations. We also explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr0.5Ru0.5Cl3. By developing a superexchange theory specifically for this mixed-spin system, we identify the conditions under which dominant Kitaev-like interactions emerge. Our findings highlight the importance of spin-orbital couplings and quadrupolar order parameters in stabilizing exotic phases, providing a foundation for exploring mixed-spin Kitaev magnets. |  |
Parshukov, K.; Wiedmann, R.; Schnyder, A. P. Topological crossings in two-dimensional altermagnets: Symmetry classification and topological responses Journal Article Phys. Rev. B 111, 224406 (2025), datadoi: 10.5281/zenodo.16279046. @article{parshukovTopologicalCrossingsTwodimensional2025,
title = {Topological crossings in two-dimensional altermagnets: Symmetry classification and topological responses},
author = {K. Parshukov and R. Wiedmann and A. P. Schnyder},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.224406},
doi = {10.1103/PhysRevB.111.224406},
year = {2025},
date = {2025-06-04},
urldate = {2025-06-01},
journal = {Phys. Rev. B},
volume = {111},
number = {22},
pages = {224406},
abstract = {We study the symmetry requirements for topologically protected spin-polarized Dirac points in 2D altermagnets. The topology is characterized by a quantized 𝜋-Berry phase and the degeneracy is protected by spin-space group symmetries. Gapped phases with finite Chern and/or spin/chirality Chern numbers emerge under different symmetry-breaking mass terms. We investigate the surface and transport properties of these gapped phases using representative electronic tight-binding and magnonic linear spin-wave models. In particular, we calculate the electronic and magnonic Hall currents and discuss implications for experiments.},
note = {datadoi: 10.5281/zenodo.16279046},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
We study the symmetry requirements for topologically protected spin-polarized Dirac points in 2D altermagnets. The topology is characterized by a quantized 𝜋-Berry phase and the degeneracy is protected by spin-space group symmetries. Gapped phases with finite Chern and/or spin/chirality Chern numbers emerge under different symmetry-breaking mass terms. We investigate the surface and transport properties of these gapped phases using representative electronic tight-binding and magnonic linear spin-wave models. In particular, we calculate the electronic and magnonic Hall currents and discuss implications for experiments. |  |
Cochran, T. A.; Jobst, B.; Rosenberg, E.; Lensky, Y. D.; Gyawali, G.; Eassa, N.; Will, M.; Szasz, A.; Abanin, D.; Acharya, R.; Beni, L. Aghababaie; Andersen, T. I.; Ansmann, M.; Arute, F.; Arya, K.; Asfaw, A.; Atalaya, J.; Babbush, R.; Ballard, B.; Bardin, J. C.; Bengtsson, A.; Bilmes, A.; Bourassa, A.; Bovaird, J.; Broughton, M.; Browne, D. A.; Buchea, B.; Buckley, B. B.; Burger, T.; Burkett, B.; Bushnell, N.; Cabrera, A.; Campero, J.; Chang, H. -S.; Chen, Z.; Chiaro, B.; Claes, J.; Cleland, A. Y.; Cogan, J.; Collins, R.; Conner, P.; Courtney, W.; Crook, A. L.; Curtin, B.; Das, S.; Demura, S.; Lorenzo, L. De; Paolo, A. Di; Donohoe, P.; Drozdov, I.; Dunsworth, A.; Eickbusch, A.; Elbag, A. Moshe; Elzouka, M.; Erickson, C.; Ferreira, V. S.; Burgos, L. Flores; Forati, E.; Fowler, A. G.; Foxen, B.; Ganjam, S.; Gasca, R.; Genois, É.; Giang, W.; Gilboa, D.; Gosula, R.; Dau, A. Grajales; Graumann, D.; Greene, A.; Gross, J. A.; Habegger, S.; Hansen, M.; Harrigan, M. P.; Harrington, S. D.; Heu, P.; Higgott, O.; Hilton, J.; Huang, H. -Y.; Huff, A.; Huggins, W.; Jeffrey, E.; Jiang, Z.; Jones, C.; Joshi, C.; Juhas, P.; Kafri, D.; Kang, H.; Karamlou, A. H.; Kechedzhi, K.; Khaire, T.; Khattar, T.; Khezri, M.; Kim, S.; Klimov, P.; Kobrin, B.; Korotkov, A.; Kostritsa, F.; Kreikebaum, J.; Kurilovich, V.; Landhuis, D.; Lange-Dei, T.; Langley, B.; Lau, K. -M.; Ledford, J.; Lee, K.; Lester, B.; Guevel, L. Le; Li, W.; Lill, A. T.; Livingston, W.; Locharla, A.; Lundahl, D.; Lunt, A.; Madhuk, S.; Maloney, A.; Mandrà, S.; Martin, L.; Martin, O.; Maxfield, C.; McClean, J.; McEwen, M.; Meeks, S.; Megrant, A.; Miao, K.; Molavi, R.; Molina, S.; Montazeri, S.; Movassagh, R.; Neill, C.; Newman, M.; Nguyen, A.; Nguyen, M.; Ni, C. -H.; Ottosson, K.; Pizzuto, A.; Potter, R.; Pritchard, O.; Quintana, C.; Ramachandran, G.; Reagor, M.; Rhodes, D.; Roberts, G.; Sankaragomathi, K.; Satzinger, K.; Schurkus, H.; Shearn, M.; Shorter, A.; Shutty, N.; Shvarts, V.; Sivak, V.; Small, S.; Smith, W. C.; Springer, S.; Sterling, G.; Suchard, J.; Sztein, A.; Thor, D.; Torunbalci, M.; Vaishnav, A.; Vargas, J.; Vdovichev, S.; Vidal, G.; Heidweiller, C. Vollgraff; Waltman, S.; Wang, S. X.; Ware, B.; White, T.; Wong, K.; Woo, B. W. K.; Xing, C.; Yao, Z. Jamie; Yeh, P.; Ying, B.; Yoo, J.; Yosri, N.; Young, G.; Zalcman, A.; Zhang, Y.; Zhu, N.; Zobrist, N.; Boixo, S.; Kelly, J.; Lucero, E.; Chen, Y.; Smelyanskiy, V.; Neven, H.; Gammon-Smith, A.; Pollmann, F.; Knap, M.; Roushan, P. Visualizing dynamics of charges and strings in (2 + 1)D lattice gauge theories Journal Article Nature 642, 315 (2025). @article{cochran_visualizing_2025,
title = {Visualizing dynamics of charges and strings in (2 + 1)D lattice gauge theories},
author = {T. A. Cochran and B. Jobst and E. Rosenberg and Y. D. Lensky and G. Gyawali and N. Eassa and M. Will and A. Szasz and D. Abanin and R. Acharya and L. Aghababaie Beni and T. I. Andersen and M. Ansmann and F. Arute and K. Arya and A. Asfaw and J. Atalaya and R. Babbush and B. Ballard and J. C. Bardin and A. Bengtsson and A. Bilmes and A. Bourassa and J. Bovaird and M. Broughton and D. A. Browne and B. Buchea and B. B. Buckley and T. Burger and B. Burkett and N. Bushnell and A. Cabrera and J. Campero and H. -S. Chang and Z. Chen and B. Chiaro and J. Claes and A. Y. Cleland and J. Cogan and R. Collins and P. Conner and W. Courtney and A. L. Crook and B. Curtin and S. Das and S. Demura and L. De Lorenzo and A. Di Paolo and P. Donohoe and I. Drozdov and A. Dunsworth and A. Eickbusch and A. Moshe Elbag and M. Elzouka and C. Erickson and V. S. Ferreira and L. Flores Burgos and E. Forati and A. G. Fowler and B. Foxen and S. Ganjam and R. Gasca and É. Genois and W. Giang and D. Gilboa and R. Gosula and A. Grajales Dau and D. Graumann and A. Greene and J. A. Gross and S. Habegger and M. Hansen and M. P. Harrigan and S. D. Harrington and P. Heu and O. Higgott and J. Hilton and H. -Y. Huang and A. Huff and W. Huggins and E. Jeffrey and Z. Jiang and C. Jones and C. Joshi and P. Juhas and D. Kafri and H. Kang and A. H. Karamlou and K. Kechedzhi and T. Khaire and T. Khattar and M. Khezri and S. Kim and P. Klimov and B. Kobrin and A. Korotkov and F. Kostritsa and J. Kreikebaum and V. Kurilovich and D. Landhuis and T. Lange-Dei and B. Langley and K. -M. Lau and J. Ledford and K. Lee and B. Lester and L. Le Guevel and W. Li and A. T. Lill and W. Livingston and A. Locharla and D. Lundahl and A. Lunt and S. Madhuk and A. Maloney and S. Mandrà and L. Martin and O. Martin and C. Maxfield and J. McClean and M. McEwen and S. Meeks and A. Megrant and K. Miao and R. Molavi and S. Molina and S. Montazeri and R. Movassagh and C. Neill and M. Newman and A. Nguyen and M. Nguyen and C. -H. Ni and K. Ottosson and A. Pizzuto and R. Potter and O. Pritchard and C. Quintana and G. Ramachandran and M. Reagor and D. Rhodes and G. Roberts and K. Sankaragomathi and K. Satzinger and H. Schurkus and M. Shearn and A. Shorter and N. Shutty and V. Shvarts and V. Sivak and S. Small and W. C. Smith and S. Springer and G. Sterling and J. Suchard and A. Sztein and D. Thor and M. Torunbalci and A. Vaishnav and J. Vargas and S. Vdovichev and G. Vidal and C. Vollgraff Heidweiller and S. Waltman and S. X. Wang and B. Ware and T. White and K. Wong and B. W. K. Woo and C. Xing and Z. Jamie Yao and P. Yeh and B. Ying and J. Yoo and N. Yosri and G. Young and A. Zalcman and Y. Zhang and N. Zhu and N. Zobrist and S. Boixo and J. Kelly and E. Lucero and Y. Chen and V. Smelyanskiy and H. Neven and A. Gammon-Smith and F. Pollmann and M. Knap and P. Roushan},
url = {https://doi.org/10.1038/s41586-025-08999-9},
doi = {10.1038/s41586-025-08999-9},
year = {2025},
date = {2025-06-04},
urldate = {2025-06-01},
journal = {Nature},
volume = {642},
number = {8067},
pages = {315},
abstract = {Lattice gauge theories (LGTs)1–4 can be used to understand a wide range of phenomena, from elementary particle scattering in high-energy physics to effective descriptions of many-body interactions in materials5–7. Studying dynamical properties of emergent phases can be challenging, as it requires solving many-body problems that are generally beyond perturbative limits8–10. Here we investigate the dynamics of local excitations in a $$textbackslashmathbbZ_2$$LGT using a two-dimensional lattice of superconducting qubits. We first construct a simple variational circuit that prepares low-energy states that have a large overlap with the ground state; then we create charge excitations with local gates and simulate their quantum dynamics by means of a discretized time evolution. As the electric field coupling constant is increased, our measurements show signatures of transitioning from deconfined to confined dynamics. For confined excitations, the electric field induces a tension in the string connecting them. Our method allows us to experimentally image string dynamics in a (2+1)D LGT, from which we uncover two distinct regimes inside the confining phase: for weak confinement, the string fluctuates strongly in the transverse direction, whereas for strong confinement, transverse fluctuations are effectively frozen11,12. We also demonstrate a resonance condition at which dynamical string breaking is facilitated. Our LGT implementation on a quantum processor presents a new set of techniques for investigating emergent excitations and string dynamics.},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
Lattice gauge theories (LGTs)1–4 can be used to understand a wide range of phenomena, from elementary particle scattering in high-energy physics to effective descriptions of many-body interactions in materials5–7. Studying dynamical properties of emergent phases can be challenging, as it requires solving many-body problems that are generally beyond perturbative limits8–10. Here we investigate the dynamics of local excitations in a $$textbackslashmathbbZ_2$$LGT using a two-dimensional lattice of superconducting qubits. We first construct a simple variational circuit that prepares low-energy states that have a large overlap with the ground state; then we create charge excitations with local gates and simulate their quantum dynamics by means of a discretized time evolution. As the electric field coupling constant is increased, our measurements show signatures of transitioning from deconfined to confined dynamics. For confined excitations, the electric field induces a tension in the string connecting them. Our method allows us to experimentally image string dynamics in a (2+1)D LGT, from which we uncover two distinct regimes inside the confining phase: for weak confinement, the string fluctuates strongly in the transverse direction, whereas for strong confinement, transverse fluctuations are effectively frozen11,12. We also demonstrate a resonance condition at which dynamical string breaking is facilitated. Our LGT implementation on a quantum processor presents a new set of techniques for investigating emergent excitations and string dynamics. |  |
Prodan, L.; Evans, D. M.; Sukhanov, A. S.; Nikitin, S. E.; Tsirlin, A. A.; Puntigam, L.; Rahn, M. C.; Chioncel, L.; Tsurkan, V.; Kézsmárki, I. Easy-cone state mediating the spin reorientation in the topological kagome magnet Fe3Sn2 Journal Article Phys. Rev. B 111, 184442 (2025), datadoi: (10.5281/zenodo.15367272). @article{prodanEasyconeStateMediating2025,
title = {Easy-cone state mediating the spin reorientation in the topological kagome magnet Fe_{3}Sn_{2}},
author = {L. Prodan and D. M. Evans and A. S. Sukhanov and S. E. Nikitin and A. A. Tsirlin and L. Puntigam and M. C. Rahn and L. Chioncel and V. Tsurkan and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.184442},
doi = {10.1103/PhysRevB.111.184442},
year = {2025},
date = {2025-05-30},
urldate = {2025-05-01},
journal = {Phys. Rev. B},
volume = {111},
number = {18},
pages = {184442},
abstract = {We investigated temperature-driven spin reorientation (SR) in the itinerant kagome magnet Fe3Sn2 using high-resolution synchrotron x-ray diffraction, neutron diffraction, magnetometry, and magnetic force microscopy (MFM), further supported by phenomenological analysis. Our study reveals a crossover from the state with easy-plane anisotropy to the high-temperature state with uniaxial easy-axis anisotropy taking place between ∼40 and 130 K through an intermediate easy-cone (or tilted spin) state. This state, induced by the interplay between the anisotropy constants 𝐾1 and 𝐾2, is clearly manifested in the thermal evolution of the magnetic structure factor, which reveals a gradual change of the SR angle 𝜃 between 40 and 130 K. We also found that the SR is accompanied by a magnetoelastic effect. Zero-field MFM images across the SR range show a transformation in surface magnetic patterns from a dendritic structure at 120 K to domain-wall-dominated MFM contrast at 40 K. Our analysis suggests that the SR and associated microstructural transformations are the results of competing first- and second-order anisotropy constants.},
note = {datadoi: (10.5281/zenodo.15367272)},
keywords = {A4, B1},
pubstate = {published},
tppubtype = {article}
}
We investigated temperature-driven spin reorientation (SR) in the itinerant kagome magnet Fe3Sn2 using high-resolution synchrotron x-ray diffraction, neutron diffraction, magnetometry, and magnetic force microscopy (MFM), further supported by phenomenological analysis. Our study reveals a crossover from the state with easy-plane anisotropy to the high-temperature state with uniaxial easy-axis anisotropy taking place between ∼40 and 130 K through an intermediate easy-cone (or tilted spin) state. This state, induced by the interplay between the anisotropy constants 𝐾1 and 𝐾2, is clearly manifested in the thermal evolution of the magnetic structure factor, which reveals a gradual change of the SR angle 𝜃 between 40 and 130 K. We also found that the SR is accompanied by a magnetoelastic effect. Zero-field MFM images across the SR range show a transformation in surface magnetic patterns from a dendritic structure at 120 K to domain-wall-dominated MFM contrast at 40 K. Our analysis suggests that the SR and associated microstructural transformations are the results of competing first- and second-order anisotropy constants. |  |
Sakrikar, P.; Shen, B.; Poldi, Eduardo H. T.; Bahrami, F.; Hu, X.; Kenney, E. M.; Wang, Q.; Fruhling, K. W.; Wang, C.; Gupta, R.; Khasanov, R.; Luetkens, H.; Calder, S. A.; Aczel, A. A.; Fabbris, G.; Hemley, R. J.; Plumb, K. W.; Ran, Y.; Gegenwart, P.; Tsirlin, A. A.; Haskel, D.; Graf, M. J.; Tafti, F. Pressure tuning of competing interactions on a honeycomb lattice Journal Article Nat. Commun. 16, 4712 (2025), datadoi: 10.18126/4gwk-2m53. @article{sakrikarPressureTuningCompeting2025,
title = {Pressure tuning of competing interactions on a honeycomb lattice},
author = {P. Sakrikar and B. Shen and Eduardo H. T. Poldi and F. Bahrami and X. Hu and E. M. Kenney and Q. Wang and K. W. Fruhling and C. Wang and R. Gupta and R. Khasanov and H. Luetkens and S. A. Calder and A. A. Aczel and G. Fabbris and R. J. Hemley and K. W. Plumb and Y. Ran and P. Gegenwart and A. A. Tsirlin and D. Haskel and M. J. Graf and F. Tafti},
url = {https://doi.org/10.1038/s41467-025-59897-7},
doi = {10.1038/s41467-025-59897-7},
year = {2025},
date = {2025-05-21},
urldate = {2025-05-01},
journal = {Nat. Commun.},
volume = {16},
number = {1},
pages = {4712},
abstract = {Exchange interactions are mediated via orbital overlaps across chemical bonds. Thus, modifying the bond angles by physical pressure or strain can tune the relative strength of competing interactions. Here we present a remarkable case of such tuning between the Heisenberg (J) and Kitaev (K) exchange, which respectively establish magnetically ordered and spin liquid phases on a honeycomb lattice. We observe a rapid suppression of the Néel temperature (TN) with pressure in Ag3LiRh2O6, a spin-1/2 honeycomb lattice with both J and K couplings. Using a combined analysis of x-ray data and first-principles calculations, we find that pressure modifies the bond angles in a way that increases the ∣K/J∣ ratio and thereby suppresses TN. Consistent with this picture, we observe a spontaneous onset of muon spin relaxation (μSR) oscillations below TN at low pressure, whereas in the high pressure phase, oscillations appear only when T < TN/2. Unlike other candidate Kitaev materials, Ag3LiRh2O6is tuned toward a quantum critical point by pressure while avoiding a structural dimerization in the relevant pressure range.},
note = {datadoi: 10.18126/4gwk-2m53},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Exchange interactions are mediated via orbital overlaps across chemical bonds. Thus, modifying the bond angles by physical pressure or strain can tune the relative strength of competing interactions. Here we present a remarkable case of such tuning between the Heisenberg (J) and Kitaev (K) exchange, which respectively establish magnetically ordered and spin liquid phases on a honeycomb lattice. We observe a rapid suppression of the Néel temperature (TN) with pressure in Ag3LiRh2O6, a spin-1/2 honeycomb lattice with both J and K couplings. Using a combined analysis of x-ray data and first-principles calculations, we find that pressure modifies the bond angles in a way that increases the ∣K/J∣ ratio and thereby suppresses TN. Consistent with this picture, we observe a spontaneous onset of muon spin relaxation (μSR) oscillations below TN at low pressure, whereas in the high pressure phase, oscillations appear only when T < TN/2. Unlike other candidate Kitaev materials, Ag3LiRh2O6is tuned toward a quantum critical point by pressure while avoiding a structural dimerization in the relevant pressure range. |  |
Xu, W. -T.; Pollmann, F.; Knap, M. Critical behavior of Fredenhagen-Marcu string order parameters at topological phase transitions with emergent higher-form symmetries Journal Article npj Quantum Inf. 11, 74 (2025), datadoi: (10.5281/zenodo.10494399). @article{xuCriticalBehaviorFredenhagenMarcu2025,
title = {Critical behavior of Fredenhagen-Marcu string order parameters at topological phase transitions with emergent higher-form symmetries},
author = {W. -T. Xu and F. Pollmann and M. Knap},
url = {https://doi.org/10.1038/s41534-025-01030-z},
doi = {10.1038/s41534-025-01030-z},
year = {2025},
date = {2025-05-09},
urldate = {2025-05-09},
journal = {npj Quantum Inf.},
volume = {11},
number = {1},
pages = {74},
abstract = {A nonlocal string order parameter detecting topological order and deconfinement has been proposed by Fredenhagen and Marcu (FM). However, due to the lack of exact internal symmetries for lattice models and the nonlinear dependence of the FM string order parameter on ground states, it is a priori not guaranteed that it is a genuine order parameter for topological phase transitions. In this work, we find that the FM string order parameter exhibits universal scaling behavior near critical points of charge condensation transitions, by directly evaluating the FM string order parameter in the infinite string-length limit using infinite Projected Entangled Pair States (iPEPS) for the toric code in a magnetic field. Our results thus demonstrate that the FM string order parameter represents a quantitatively well-behaved order parameter. We find that only in the presence of an emergent 1-form symmetry the corresponding FM string order parameter can faithfully detect topological transitions.},
note = {datadoi: (10.5281/zenodo.10494399)},
keywords = {B6, C5, C6},
pubstate = {published},
tppubtype = {article}
}
A nonlocal string order parameter detecting topological order and deconfinement has been proposed by Fredenhagen and Marcu (FM). However, due to the lack of exact internal symmetries for lattice models and the nonlinear dependence of the FM string order parameter on ground states, it is a priori not guaranteed that it is a genuine order parameter for topological phase transitions. In this work, we find that the FM string order parameter exhibits universal scaling behavior near critical points of charge condensation transitions, by directly evaluating the FM string order parameter in the infinite string-length limit using infinite Projected Entangled Pair States (iPEPS) for the toric code in a magnetic field. Our results thus demonstrate that the FM string order parameter represents a quantitatively well-behaved order parameter. We find that only in the presence of an emergent 1-form symmetry the corresponding FM string order parameter can faithfully detect topological transitions. |  |
Szaller, D.; Prodan, L.; Geirhos, K.; Felea, V.; Skourski, Y.; Gorbunov, D.; Förster, T.; Helm, T.; Nomura, T.; Miyata, A.; Zherlitsyn, S.; Wosnitza, J.; Tsirlin, A. A.; Tsurkan, V.; Kézsmárki, I. Coexistence of antiferromagnetism and ferrimagnetism in adjacent honeycomb layers Journal Article Phys. Rev. B 111, 184404 (2025). @article{szaller_coexistence_2025,
title = {Coexistence of antiferromagnetism and ferrimagnetism in adjacent honeycomb layers},
author = {D. Szaller and L. Prodan and K. Geirhos and V. Felea and Y. Skourski and D. Gorbunov and T. Förster and T. Helm and T. Nomura and A. Miyata and S. Zherlitsyn and J. Wosnitza and A. A. Tsirlin and V. Tsurkan and I. Kézsmárki},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.184404},
doi = {10.1103/PhysRevB.111.184404},
year = {2025},
date = {2025-05-02},
urldate = {2025-05-02},
journal = {Phys. Rev. B},
volume = {111},
number = {18},
pages = {184404},
abstract = {Ferro-/ferri- and antiferromagnetically ordered phases are typically exclusive in nature, thus, their coexistence in atomic-scale proximity is expected only in heterostructures. Breaking this paradigm and broadening the range of unconventional magnetic states, we report here on the observation of a new, atomic-scale hybrid spin state. This ordering is stabilized in three-dimensional crystals of the polar antiferromagnet Co2Mo3O8 by magnetic fields applied perpendicular to the Co honeycomb layers and possesses a spontaneous in-plane ferromagnetic moment. Our microscopic spin model, capturing the observed field dependence of the longitudinal and transverse magnetization as well as the magnetoelectric/elastic properties, reveals that this novel spin state is composed of an alternating stacking of antiferromagnetic and ferrimagnetic honeycomb layers. The strong intralayer and the weak interlayer exchange couplings together with competing anisotropies at octahedral and tetrahedral Co sites are identified as the key ingredients to stabilize antiferromagnetic and ferrimagnetic layers in such close proximity. We show that the proper balance of magnetic interactions can extend the stability range of this hybrid phase down to zero magnetic field. The possibility to realize a layer-by-layer stacking of such distinct spin orders via suitable combinations of microscopic interactions opens a new dimension toward the nanoscale engineering of magnetic states.},
keywords = {B1, C2},
pubstate = {published},
tppubtype = {article}
}
Ferro-/ferri- and antiferromagnetically ordered phases are typically exclusive in nature, thus, their coexistence in atomic-scale proximity is expected only in heterostructures. Breaking this paradigm and broadening the range of unconventional magnetic states, we report here on the observation of a new, atomic-scale hybrid spin state. This ordering is stabilized in three-dimensional crystals of the polar antiferromagnet Co2Mo3O8 by magnetic fields applied perpendicular to the Co honeycomb layers and possesses a spontaneous in-plane ferromagnetic moment. Our microscopic spin model, capturing the observed field dependence of the longitudinal and transverse magnetization as well as the magnetoelectric/elastic properties, reveals that this novel spin state is composed of an alternating stacking of antiferromagnetic and ferrimagnetic honeycomb layers. The strong intralayer and the weak interlayer exchange couplings together with competing anisotropies at octahedral and tetrahedral Co sites are identified as the key ingredients to stabilize antiferromagnetic and ferrimagnetic layers in such close proximity. We show that the proper balance of magnetic interactions can extend the stability range of this hybrid phase down to zero magnetic field. The possibility to realize a layer-by-layer stacking of such distinct spin orders via suitable combinations of microscopic interactions opens a new dimension toward the nanoscale engineering of magnetic states. |  |
Zerba, C.; Seidel, A.; Pollmann, F.; Knap, M. Emergent Fracton Hydrodynamics of Ultracold Atoms in Partially Filled Landau Levels Journal Article PRX Quantum 6, 020321 (2025), datadoi: 10.5281/zenodo.13897004. @article{zerbaEmergentFractonHydrodynamics2025,
title = {Emergent Fracton Hydrodynamics of Ultracold Atoms in Partially Filled Landau Levels},
author = {C. Zerba and A. Seidel and F. Pollmann and M. Knap},
url = {https://link.aps.org/doi/10.1103/PRXQuantum.6.020321},
doi = {10.1103/PRXQuantum.6.020321},
year = {2025},
date = {2025-04-30},
urldate = {2025-04-01},
journal = {PRX Quantum},
volume = {6},
number = {2},
pages = {020321},
abstract = {The realization of synthetic gauge fields for charge neutral ultracold atoms and the simulation of quantum Hall physics have witnessed remarkable experimental progress. Here, we establish key signatures of fractional quantum Hall systems in their nonequilibrium quantum dynamics. We show that in the lowest Landau level the system generically relaxes subdiffusively. The slow relaxation is understood from emergent conservation laws of the total charge and the associated dipole moment that arises from the effective Hamiltonian projected onto the lowest Landau level, leading to subdiffusive fracton hydrodynamics. We discuss the prospect of rotating quantum gases as well as ultracold atoms in optical lattices for observing this unconventional relaxation dynamics.},
note = {datadoi: 10.5281/zenodo.13897004},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
The realization of synthetic gauge fields for charge neutral ultracold atoms and the simulation of quantum Hall physics have witnessed remarkable experimental progress. Here, we establish key signatures of fractional quantum Hall systems in their nonequilibrium quantum dynamics. We show that in the lowest Landau level the system generically relaxes subdiffusively. The slow relaxation is understood from emergent conservation laws of the total charge and the associated dipole moment that arises from the effective Hamiltonian projected onto the lowest Landau level, leading to subdiffusive fracton hydrodynamics. We discuss the prospect of rotating quantum gases as well as ultracold atoms in optical lattices for observing this unconventional relaxation dynamics. |  |
Kern, L. -M.; Kuchkin, V. M.; Deinhart, V.; Klose, C.; Sidiropoulos, T.; Auer, M.; Gaebel, S.; Gerlinger, K.; Battistelli, R.; Wittrock, S.; Karaman, T.; Schneider, M.; Günther, C. M.; Engel, D.; Will, I.; Wintz, S.; Weigand, M.; Büttner, F.; Höflich, K.; Eisebitt, S.; Pfau, B. Controlled Formation of Skyrmion Bags Journal Article Adv. Mater. 2501250 (2025), (contributed). @article{kern_controlled_2025,
title = {Controlled Formation of Skyrmion Bags},
author = {L. -M. Kern and V. M. Kuchkin and V. Deinhart and C. Klose and T. Sidiropoulos and M. Auer and S. Gaebel and K. Gerlinger and R. Battistelli and S. Wittrock and T. Karaman and M. Schneider and C. M. Günther and D. Engel and I. Will and S. Wintz and M. Weigand and F. Büttner and K. Höflich and S. Eisebitt and B. Pfau},
url = {https://advanced.onlinelibrary.wiley.com/doi/abs/10.1002/adma.202501250},
doi = {10.1002/adma.202501250},
year = {2025},
date = {2025-04-28},
urldate = {2025-04-01},
journal = {Adv. Mater.},
pages = {2501250},
abstract = {Abstract Topologically non-trivial magnetic solitons are complex spin textures with a distinct single-particle nature. Although magnetic skyrmions, especially those with unity topological charge, have attracted substantial interest due to their potential applications, more complex topological textures remain largely theoretical. In this work, the stabilization of isolated higher-order skyrmion bags beyond the prototypical π-skyrmion in ferromagnetic thin films is experimentally demonstrate, which has posed considerable challenges to date. Specifically, controlled generation of skyrmionium (2π-skyrmion), target skyrmion (3π-skyrmion), and skyrmion bags (with variable topological charge) are achieved through the introduction of artificially engineered anisotropy defects via local ion irradiation. They act as preferential sites for the field- or laser-induced nucleation of skyrmion bags. Remarkably, ultrafast laser pulses achieve a substantially higher conversion rate transforming skyrmions into higher-order skyrmion bags compared to their formation driven by magnetic fields. High-resolution x-ray imaging enables direct observation of the resulting skyrmion bags. Complementary micromagnetic simulations reveal the pivotal role of defect geometry–particularly diameter–in stabilizing closed-loop domain textures. The findings not only broaden the experimental horizon for skyrmion research, but also suggest strategies for exploiting complex topological spin textures within a unified material platform for practical applications.},
note = {(contributed)},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
Abstract Topologically non-trivial magnetic solitons are complex spin textures with a distinct single-particle nature. Although magnetic skyrmions, especially those with unity topological charge, have attracted substantial interest due to their potential applications, more complex topological textures remain largely theoretical. In this work, the stabilization of isolated higher-order skyrmion bags beyond the prototypical π-skyrmion in ferromagnetic thin films is experimentally demonstrate, which has posed considerable challenges to date. Specifically, controlled generation of skyrmionium (2π-skyrmion), target skyrmion (3π-skyrmion), and skyrmion bags (with variable topological charge) are achieved through the introduction of artificially engineered anisotropy defects via local ion irradiation. They act as preferential sites for the field- or laser-induced nucleation of skyrmion bags. Remarkably, ultrafast laser pulses achieve a substantially higher conversion rate transforming skyrmions into higher-order skyrmion bags compared to their formation driven by magnetic fields. High-resolution x-ray imaging enables direct observation of the resulting skyrmion bags. Complementary micromagnetic simulations reveal the pivotal role of defect geometry–particularly diameter–in stabilizing closed-loop domain textures. The findings not only broaden the experimental horizon for skyrmion research, but also suggest strategies for exploiting complex topological spin textures within a unified material platform for practical applications. |  |
Metternich, D.; Litzius, K.; Wintz, S.; Gerlinger, K.; Petz, S.; Engel, D.; Sidiropoulos, T.; Battistelli, R.; Steinbach, F.; Weigand, M.; Wittrock, S.; Schmising, C. Korff; Büttner, F. Defects in magnetic domain walls after single-shot all-optical switching Journal Article Struct. Dyn. 12, 024504 (2025), datadoi: (10.5281/zenodo.14499566). @article{metternichDefectsMagneticDomain2025,
title = {Defects in magnetic domain walls after single-shot all-optical switching},
author = {D. Metternich and K. Litzius and S. Wintz and K. Gerlinger and S. Petz and D. Engel and T. Sidiropoulos and R. Battistelli and F. Steinbach and M. Weigand and S. Wittrock and C. Korff Schmising and F. Büttner},
url = {https://doi.org/10.1063/4.0000287},
doi = {10.1063/4.0000287},
year = {2025},
date = {2025-04-18},
urldate = {2025-04-01},
journal = {Struct. Dyn.},
volume = {12},
number = {2},
pages = {024504},
abstract = {Helicity-independent all-optical switching (HI-AOS) is the fastest known way to switch the magnetic order parameter. While the switching process of extended areas is well understood, the formation of domain walls enclosing switched areas remains less explored. Here, we study domain walls around all-optically nucleated magnetic domains using x-ray vector spin imaging and observe a high density of vertical Bloch line defects. Surprisingly, the defect density appears to be independent of optical pulse parameters, significantly varies between materials, and is only slightly higher than in domain walls generated by field cycling. A possible explanation is given by time-resolved Kerr microscopy, which reveals that magnetic domains considerably expand after the initial AOS process. During this expansion, and likewise during field cycling, domain walls propagate at speeds above the Walker breakdown. Micromagnetic simulations suggest that at such speeds, domain walls accumulate defects when moving over magnetic pinning sites, explaining similar defect densities after two very different switching processes. The slightly larger defect density after AOS compared to field-induced switching indicates that some defects are created already when the domain wall comes into existence. Our work shows that engineered low-pinning materials are a key ingredient to uncover the intrinsic dynamics of domain wall formation during ultrafast all-optical switching.},
note = {datadoi: (10.5281/zenodo.14499566)},
keywords = {C2},
pubstate = {published},
tppubtype = {article}
}
Helicity-independent all-optical switching (HI-AOS) is the fastest known way to switch the magnetic order parameter. While the switching process of extended areas is well understood, the formation of domain walls enclosing switched areas remains less explored. Here, we study domain walls around all-optically nucleated magnetic domains using x-ray vector spin imaging and observe a high density of vertical Bloch line defects. Surprisingly, the defect density appears to be independent of optical pulse parameters, significantly varies between materials, and is only slightly higher than in domain walls generated by field cycling. A possible explanation is given by time-resolved Kerr microscopy, which reveals that magnetic domains considerably expand after the initial AOS process. During this expansion, and likewise during field cycling, domain walls propagate at speeds above the Walker breakdown. Micromagnetic simulations suggest that at such speeds, domain walls accumulate defects when moving over magnetic pinning sites, explaining similar defect densities after two very different switching processes. The slightly larger defect density after AOS compared to field-induced switching indicates that some defects are created already when the domain wall comes into existence. Our work shows that engineered low-pinning materials are a key ingredient to uncover the intrinsic dynamics of domain wall formation during ultrafast all-optical switching. |  |
Mangeolle, L.; Knolle, J. Anomalous Quantum Oscillations from Boson-Mediated Interband Scattering Journal Article Phys. Rev. Lett. 134, 146502 (2025). @article{mangeolle_anomalous_2025-1,
title = {Anomalous Quantum Oscillations from Boson-Mediated Interband Scattering},
author = {L. Mangeolle and J. Knolle},
url = {https://link.aps.org/doi/10.1103/PhysRevLett.134.146502},
doi = {10.1103/PhysRevLett.134.146502},
year = {2025},
date = {2025-04-09},
urldate = {2025-04-01},
journal = {Phys. Rev. Lett.},
volume = {134},
number = {14},
pages = {146502},
abstract = {Quantum oscillations (QOs) in metals refer to the periodic variation of thermodynamic and transport properties as a function of inverse applied magnetic field. QO frequencies are normally associated with semiclassical trajectories of Fermi surface orbits, but recent experiments challenge the canonical description. We develop a theory of composite frequency quantum oscillations (CFQOs) in two-dimensional Fermi liquids with several Fermi surfaces and interband scattering mediated by a dynamical boson, e.g., phonons or spin fluctuations. Specifically, we show that CFQOs arise from oscillations in the fermionic self-energy with anomalous frequency splitting and distinct strongly non-Lifshitz–Kosevich temperature dependences. Our theory goes beyond the framework of semiclassical Fermi surface trajectories highlighting the role of interaction effects. We provide experimental predictions and discuss the effect of nonequilibrium boson occupation in driven systems.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Quantum oscillations (QOs) in metals refer to the periodic variation of thermodynamic and transport properties as a function of inverse applied magnetic field. QO frequencies are normally associated with semiclassical trajectories of Fermi surface orbits, but recent experiments challenge the canonical description. We develop a theory of composite frequency quantum oscillations (CFQOs) in two-dimensional Fermi liquids with several Fermi surfaces and interband scattering mediated by a dynamical boson, e.g., phonons or spin fluctuations. Specifically, we show that CFQOs arise from oscillations in the fermionic self-energy with anomalous frequency splitting and distinct strongly non-Lifshitz–Kosevich temperature dependences. Our theory goes beyond the framework of semiclassical Fermi surface trajectories highlighting the role of interaction effects. We provide experimental predictions and discuss the effect of nonequilibrium boson occupation in driven systems. |  |
Hua, N.; Breitner, F.; Jesche, A.; Huang, S. -W.; Rüegg, C.; Gegenwart, P. Structural and magnetic properties of β-Li2IrO3 after grazing-angle focused ion beam thinning Journal Article Acta Crystallogr. B 81, 202 (2025). @article{hua_structural_2025,
title = {Structural and magnetic properties of β-Li_{2}IrO_{3} after grazing-angle focused ion beam thinning},
author = {N. Hua and F. Breitner and A. Jesche and S. -W. Huang and C. Rüegg and P. Gegenwart},
url = {https://doi.org/10.1107/S2052520625000587},
doi = {10.1107/S2052520625000587},
year = {2025},
date = {2025-04-01},
urldate = {2025-04-01},
journal = {Acta Crystallogr. B},
volume = {81},
number = {2},
pages = {202},
abstract = {Manipulating the size and orientation of quantum materials is often used to tune emergent phenomena, but precise control of these parameters is also necessary from an experimental point of view. Various synthesis techniques already exist, such as epitaxial thin film growth and chemical etching, that are capable of producing specific sample dimensions with high precision. However, certain materials exist as single crystals that are often difficult to manipulate, thereby limiting their studies to a certain subset of experimental techniques. One particular class of these materials includes lithium and sodium iridates, which are promising candidates for hosting a Kitaev quantum spin liquid state. Here a controlled method of using a focused ion beam at grazing incidence to reduce the size of a β-Li_2IrO_3 single crystal to a thickness of 1–2𝜇m is presented. Subsequent X-ray diffraction measurements show the lattice remains intact, albeit with a larger mosaic spread. The integrity of the magnetic order is also preserved as the temperature dependent magnetic diffraction peak follows the same trend as its bulk counterpart with a transition temperature at textitT = 37.5K. Our study demonstrates a technique that opens up the possibility of nonequilibrium experiments where submicron thin samples are often essential.},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Manipulating the size and orientation of quantum materials is often used to tune emergent phenomena, but precise control of these parameters is also necessary from an experimental point of view. Various synthesis techniques already exist, such as epitaxial thin film growth and chemical etching, that are capable of producing specific sample dimensions with high precision. However, certain materials exist as single crystals that are often difficult to manipulate, thereby limiting their studies to a certain subset of experimental techniques. One particular class of these materials includes lithium and sodium iridates, which are promising candidates for hosting a Kitaev quantum spin liquid state. Here a controlled method of using a focused ion beam at grazing incidence to reduce the size of a β-Li_2IrO_3 single crystal to a thickness of 1–2𝜇m is presented. Subsequent X-ray diffraction measurements show the lattice remains intact, albeit with a larger mosaic spread. The integrity of the magnetic order is also preserved as the temperature dependent magnetic diffraction peak follows the same trend as its bulk counterpart with a transition temperature at textitT = 37.5K. Our study demonstrates a technique that opens up the possibility of nonequilibrium experiments where submicron thin samples are often essential. |  |
Vivanco, F. J.; Schuckert, A.; Huang, S.; Schumacher, G. L.; Assumpção, G. G. T.; Ji, Y.; Chen, J.; Knap, M.; Navon, N. The strongly driven Fermi polaron Journal Article Nat. Phys. 21, 564 (2025), datadoi: 10.1038/s41567-025-02799-8. @article{vivancoStronglyDrivenFermi2025,
title = {The strongly driven Fermi polaron},
author = {F. J. Vivanco and A. Schuckert and S. Huang and G. L. Schumacher and G. G. T. Assumpção and Y. Ji and J. Chen and M. Knap and N. Navon},
url = {https://doi.org/10.1038/s41567-025-02799-8},
doi = {10.1038/s41567-025-02799-8},
year = {2025},
date = {2025-04-01},
urldate = {2025-04-01},
journal = {Nat. Phys.},
volume = {21},
number = {4},
pages = {564},
abstract = {Quasiparticles are emergent excitations of matter that underlie much of our understanding of quantum many-body systems. Therefore, the prospect of controlling their properties has both fundamental and practical implications. However, in solid-state materials, it is often challenging to understand how quasiparticles are modified by external fields due to their complex interplay with other collective excitations. Here we demonstrate the manipulation of Fermi polarons—quasiparticles formed by impurities interacting with a Fermi gas—in a homogeneous atomic gas using fast radio-frequency control. Exploiting two internal states of the impurity species, we develop a steady-state spectroscopy, from which we extract the energy of the driven polaron. By varying the drive Rabi frequency, we measure the decay rate and the quasiparticle residue of the polaron in the weak-drive limit. At large Rabi frequencies, we observe signs that the drive causes a hybridization of the driven polaron with an incoherent background, leading to the breakdown of a description in terms of textbook quasiparticles. Our experiment establishes the driven Fermi polaron as a promising platform for studying controllable quasiparticles in strongly driven quantum matter and calls for a controlled theoretical framework to describe the dynamics of this strongly interacting quantum system.},
note = {datadoi: 10.1038/s41567-025-02799-8},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Quasiparticles are emergent excitations of matter that underlie much of our understanding of quantum many-body systems. Therefore, the prospect of controlling their properties has both fundamental and practical implications. However, in solid-state materials, it is often challenging to understand how quasiparticles are modified by external fields due to their complex interplay with other collective excitations. Here we demonstrate the manipulation of Fermi polarons—quasiparticles formed by impurities interacting with a Fermi gas—in a homogeneous atomic gas using fast radio-frequency control. Exploiting two internal states of the impurity species, we develop a steady-state spectroscopy, from which we extract the energy of the driven polaron. By varying the drive Rabi frequency, we measure the decay rate and the quasiparticle residue of the polaron in the weak-drive limit. At large Rabi frequencies, we observe signs that the drive causes a hybridization of the driven polaron with an incoherent background, leading to the breakdown of a description in terms of textbook quasiparticles. Our experiment establishes the driven Fermi polaron as a promising platform for studying controllable quasiparticles in strongly driven quantum matter and calls for a controlled theoretical framework to describe the dynamics of this strongly interacting quantum system. |  |
Uykur, E.; Janson, O.; Ginga, V. A.; Schmidt, M.; Giordano, N.; Tsirlin, A. A. Tunable Dirac nodal line in orthorhombic RuO2 Journal Article Phys. Rev. B 111, 134114 (2025), datdoi: 10.14278/rodare.3261. @article{uykurTunableDiracNodal2025,
title = {Tunable Dirac nodal line in orthorhombic RuO_{2}},
author = {E. Uykur and O. Janson and V. A. Ginga and M. Schmidt and N. Giordano and A. A. Tsirlin},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.134114},
doi = {10.1103/PhysRevB.111.134114},
year = {2025},
date = {2025-04-01},
urldate = {2025-04-01},
journal = {Phys. Rev. B},
volume = {111},
number = {13},
pages = {134114},
abstract = {The pressure evolution of RuO2 is studied using single-crystal x-ray diffraction in a diamond anvil cell, combined with ab initio band-structure calculations. The tetragonal rutile structure transforms into the orthorhombic CaCl2-type structure above 13 GPa under quasihydrostatic pressure conditions. This second-order transition is ferroelastic in nature and accompanied by tilts of the RuO6 octahedra. Orthorhombic RuO2 is expected to be a paramagnetic metal, similar to ambient-pressure RuO2. It shows the increased 𝑡2𝑔−𝑒𝑔 crystal-field splitting that is responsible for the pressure-induced color change. It further features the Dirac nodal line that shifts across the Fermi level upon compression.},
note = {datdoi: 10.14278/rodare.3261},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
The pressure evolution of RuO2 is studied using single-crystal x-ray diffraction in a diamond anvil cell, combined with ab initio band-structure calculations. The tetragonal rutile structure transforms into the orthorhombic CaCl2-type structure above 13 GPa under quasihydrostatic pressure conditions. This second-order transition is ferroelastic in nature and accompanied by tilts of the RuO6 octahedra. Orthorhombic RuO2 is expected to be a paramagnetic metal, similar to ambient-pressure RuO2. It shows the increased 𝑡2𝑔−𝑒𝑔 crystal-field splitting that is responsible for the pressure-induced color change. It further features the Dirac nodal line that shifts across the Fermi level upon compression. |  |
Halloran, T.; Wang, Y.; Plumb, K. W.; Stone, M. B.; Winn, B.; Graves-Brook, M. K.; Rodriguez-Rivera, J. A.; Qui, Y.; Chauhan, P.; Knolle, J.; Moessner, R.; Armitage, N. P.; Takayama, T.; Takagi, H.; Broholm, C. Continuum of magnetic excitations in the Kitaev honeycomb iridate D3LiIr2O6 Journal Article npj Quantum Mater. 10, 35 (2025). @article{halloran_continuum_2025,
title = {Continuum of magnetic excitations in the Kitaev honeycomb iridate D_{3}LiIr_{2}O_{6}},
author = {T. Halloran and Y. Wang and K. W. Plumb and M. B. Stone and B. Winn and M. K. Graves-Brook and J. A. Rodriguez-Rivera and Y. Qui and P. Chauhan and J. Knolle and R. Moessner and N. P. Armitage and T. Takayama and H. Takagi and C. Broholm},
url = {https://www.nature.com/articles/s41535-025-00748-5},
doi = {10.1038/s41535-025-00748-5},
year = {2025},
date = {2025-03-29},
urldate = {2025-03-29},
journal = {npj Quantum Mater.},
volume = {10},
pages = {35},
abstract = {Inelastic neutron scattering (INS) measurements of powder D3LiIr2O6 reveal low energy magnetic excitations with a scattering cross-section that is broad in ∣Q∣ and energy transfer. The magnetic nature of the excitation spectrum is demonstrated by longitudinally polarized neutron scattering. The total magnetic moment of 1.8(4)μB/Ir inferred from the observed magnetic scattering cross-section is consistent with the effective moment inferred from magnetic susceptibility data and expectations for the Jeff = 1/2 single ion state. The rise in the dynamic correlation function S(Q, ω) for ℏω < 5 meV can be described by a simple model assuming nearest-neighbor anisotropic spin exchange, such as that found in the Kitaev model. Exchange disorder associated with the D site likely plays an important role in stabilizing the low T quantum fluctuating state.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Inelastic neutron scattering (INS) measurements of powder D3LiIr2O6 reveal low energy magnetic excitations with a scattering cross-section that is broad in ∣Q∣ and energy transfer. The magnetic nature of the excitation spectrum is demonstrated by longitudinally polarized neutron scattering. The total magnetic moment of 1.8(4)μB/Ir inferred from the observed magnetic scattering cross-section is consistent with the effective moment inferred from magnetic susceptibility data and expectations for the Jeff = 1/2 single ion state. The rise in the dynamic correlation function S(Q, ω) for ℏω < 5 meV can be described by a simple model assuming nearest-neighbor anisotropic spin exchange, such as that found in the Kitaev model. Exchange disorder associated with the D site likely plays an important role in stabilizing the low T quantum fluctuating state. | |
Que, X.; He, Q.; Zhou, L.; Lei, S.; Schoop, L.; Huang, D.; Takagi, H. Visualizing the internal structure of the charge-density-wave state in CeSbTe Journal Article Nat. Commun. 16, 3053 (2025), datadoi: 10.6084/m9.figshare.27255576. @article{queVisualizingInternalStructure2025,
title = {Visualizing the internal structure of the charge-density-wave state in CeSbTe},
author = {X. Que and Q. He and L. Zhou and S. Lei and L. Schoop and D. Huang and H. Takagi},
url = {https://doi.org/10.1038/s41467-025-58417-x},
doi = {10.1038/s41467-025-58417-x},
year = {2025},
date = {2025-03-28},
urldate = {2025-03-01},
journal = {Nat. Commun.},
volume = {16},
number = {1},
pages = {3053},
abstract = {The collective reorganization of electrons into a charge density wave has long served as a textbook example of an ordered phase in condensed matter physics. Two-dimensional square lattices with p electrons are well-suited to the realization of charge density waves, due to the anisotropy of the p orbitals and the resulting one dimensionality of the electronic structure. In spite of a long history of study of charge density waves in square-lattice systems, few reports have recognized the significance of a hidden orbital degree of freedom. The degeneracy of px and py electrons may give rise to orbital patterns in real space that endow the charge density wave with additional broken symmetries or unusual order parameters. Here, we use scanning tunneling microscopy to visualize the internal structure of the charge-density-wave state of CeSbTe, which contains Sb square lattices with 5p electrons. We image atomic-sized, anisotropic lobes of charge density with periodically modulating anisotropy, which we interpret in terms of a superposition of px and py bond density waves. Our results support the fact that delocalized p orbitals can reorganize into emergent electronic states of matter.},
note = {datadoi: 10.6084/m9.figshare.27255576},
keywords = {A3},
pubstate = {published},
tppubtype = {article}
}
The collective reorganization of electrons into a charge density wave has long served as a textbook example of an ordered phase in condensed matter physics. Two-dimensional square lattices with p electrons are well-suited to the realization of charge density waves, due to the anisotropy of the p orbitals and the resulting one dimensionality of the electronic structure. In spite of a long history of study of charge density waves in square-lattice systems, few reports have recognized the significance of a hidden orbital degree of freedom. The degeneracy of px and py electrons may give rise to orbital patterns in real space that endow the charge density wave with additional broken symmetries or unusual order parameters. Here, we use scanning tunneling microscopy to visualize the internal structure of the charge-density-wave state of CeSbTe, which contains Sb square lattices with 5p electrons. We image atomic-sized, anisotropic lobes of charge density with periodically modulating anisotropy, which we interpret in terms of a superposition of px and py bond density waves. Our results support the fact that delocalized p orbitals can reorganize into emergent electronic states of matter. |  |
Zerba, C.; Kuhlenkamp, C.; Mangeolle, L.; Knap, M. Tuning Transport in Solid-State Bose-Fermi Mixtures by Feshbach Resonances Journal Article Phys. Rev. Lett. 134, (2025), datadoi: 10.5281/zenodo.13842074. @article{zerbaTuningTransportSolidState2025,
title = {Tuning Transport in Solid-State Bose-Fermi Mixtures by Feshbach Resonances},
author = {C. Zerba and C. Kuhlenkamp and L. Mangeolle and M. Knap},
url = {https://doi.org/10.1103/PhysRevLett.134.126502},
doi = {10.1103/physrevlett.134.126502},
issn = {1079-7114},
year = {2025},
date = {2025-03-26},
urldate = {2025-03-01},
journal = {Phys. Rev. Lett.},
volume = {134},
number = {12},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.13842074},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Li, Y.; Pollmann, F.; Read, N.; Sala, P. Highly Entangled Stationary States from Strong Symmetries Journal Article Phys. Rev. X 15, 011068 (2025), datdoi: 10.5281/zenodo.13292265. @article{liHighlyEntangledStationary2025,
title = {Highly Entangled Stationary States from Strong Symmetries},
author = {Y. Li and F. Pollmann and N. Read and P. Sala},
url = {https://link.aps.org/doi/10.1103/PhysRevX.15.011068},
doi = {10.1103/PhysRevX.15.011068},
year = {2025},
date = {2025-03-21},
urldate = {2025-03-01},
journal = {Phys. Rev. X},
volume = {15},
number = {1},
pages = {011068},
abstract = {We find that the presence of strong non-Abelian symmetries can lead to highly entangled stationary states even for unital quantum channels. We derive exact expressions for the bipartite logarithmic negativity, Rényi negativities, and operator space entanglement for stationary states restricted to one symmetric subspace, with focus on the trivial subspace. We prove that these apply to open quantum evolutions whose commutants, characterizing all strongly conserved quantities, correspond to either the universal enveloping algebra of a Lie algebra or the Read-Saleur commutants. The latter provides an example of quantum fragmentation, whose dimension is exponentially large in system size. We find a general upper bound for all these quantities given by the logarithm of the dimension of the commutant on the smaller bipartition of the chain. As Abelian examples, we show that strong U(1) symmetries and classical fragmentation lead to separable stationary states in any symmetric subspace. In contrast, for non-Abelian SU(𝑁)
symmetries, both logarithmic and Rényi negativities scale logarithmically with system size. Finally, we prove that, while Rényi negativities with 𝑛 >2 scale logarithmically with system size, the logarithmic negativity (as well as generalized Rényi negativities with 𝑛 <2) exhibits a volume-law scaling for the Read-Saleur commutants. Our derivations rely on the commutant possessing a Hopf algebra structure in the limit of infinitely large systems and, hence, also apply to finite groups and quantum groups.},
note = {datdoi: 10.5281/zenodo.13292265},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
We find that the presence of strong non-Abelian symmetries can lead to highly entangled stationary states even for unital quantum channels. We derive exact expressions for the bipartite logarithmic negativity, Rényi negativities, and operator space entanglement for stationary states restricted to one symmetric subspace, with focus on the trivial subspace. We prove that these apply to open quantum evolutions whose commutants, characterizing all strongly conserved quantities, correspond to either the universal enveloping algebra of a Lie algebra or the Read-Saleur commutants. The latter provides an example of quantum fragmentation, whose dimension is exponentially large in system size. We find a general upper bound for all these quantities given by the logarithm of the dimension of the commutant on the smaller bipartition of the chain. As Abelian examples, we show that strong U(1) symmetries and classical fragmentation lead to separable stationary states in any symmetric subspace. In contrast, for non-Abelian SU(𝑁)
symmetries, both logarithmic and Rényi negativities scale logarithmically with system size. Finally, we prove that, while Rényi negativities with 𝑛 >2 scale logarithmically with system size, the logarithmic negativity (as well as generalized Rényi negativities with 𝑛 <2) exhibits a volume-law scaling for the Read-Saleur commutants. Our derivations rely on the commutant possessing a Hopf algebra structure in the limit of infinitely large systems and, hence, also apply to finite groups and quantum groups. |  |
Hayashida, S.; Gretarsson, H.; Puphal, P.; Isobe, M.; Goering, E.; Matsumoto, Y.; Nuss, J.; Takagi, H.; Hepting, M.; Keimer, B. Magnetic ground state of the dimer-based hexagonal perovskite Ba3ZnRu2O9 Journal Article Phys. Rev. B 111, 104418 (2025), datadoi: 10.5281/zenodo.14115503. @article{hayashidaMagneticGroundState2025,
title = {Magnetic ground state of the dimer-based hexagonal perovskite Ba_{3}ZnRu_{2}O_{9}},
author = {S. Hayashida and H. Gretarsson and P. Puphal and M. Isobe and E. Goering and Y. Matsumoto and J. Nuss and H. Takagi and M. Hepting and B. Keimer},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.104418},
doi = {10.1103/PhysRevB.111.104418},
year = {2025},
date = {2025-03-13},
urldate = {2025-03-01},
journal = {Phys. Rev. B},
volume = {111},
number = {10},
pages = {104418},
abstract = {We investigate the magnetic ground state of single crystals of the ruthenium-dimer-based hexagonal perovskite Ba3ZnRu2O9 using magnetic susceptibility and resonant inelastic x-ray scattering (RIXS) measurements. While a previous study on powder samples exhibited intriguing magnetic behavior, questions about whether the spin state within a Ru2O9 dimer is a conventional 𝑆=3/2 dimer or an orbital-selective 𝑆=1 dimer were raised. The RIXS spectra reveal magnetic excitations from Hund's intraionic multiplet and intradimer spin-triplet transitions. The observed transition energies of the Hund's intraionic multiplets align with the 𝑆=3/2 ground state, contrasting with the theoretically proposed orbital-selective 𝑆=1 dimer state. High-temperature magnetic susceptibility analysis confirms the realization of the spin 𝑆=3/2 dimer state, and the extracted intradimer coupling is consistent with the spin-triplet transition energy observed in the RIXS spectra. These results highlights the ability of “spectroscopic fingerprinting” by RIXS to determine the magnetic ground states of complex materials.},
note = {datadoi: 10.5281/zenodo.14115503},
keywords = {B2},
pubstate = {published},
tppubtype = {article}
}
We investigate the magnetic ground state of single crystals of the ruthenium-dimer-based hexagonal perovskite Ba3ZnRu2O9 using magnetic susceptibility and resonant inelastic x-ray scattering (RIXS) measurements. While a previous study on powder samples exhibited intriguing magnetic behavior, questions about whether the spin state within a Ru2O9 dimer is a conventional 𝑆=3/2 dimer or an orbital-selective 𝑆=1 dimer were raised. The RIXS spectra reveal magnetic excitations from Hund's intraionic multiplet and intradimer spin-triplet transitions. The observed transition energies of the Hund's intraionic multiplets align with the 𝑆=3/2 ground state, contrasting with the theoretically proposed orbital-selective 𝑆=1 dimer state. High-temperature magnetic susceptibility analysis confirms the realization of the spin 𝑆=3/2 dimer state, and the extracted intradimer coupling is consistent with the spin-triplet transition energy observed in the RIXS spectra. These results highlights the ability of “spectroscopic fingerprinting” by RIXS to determine the magnetic ground states of complex materials. |  |
Telang, P.; Treu, T.; Klinger, M.; Tsirlin, A. A.; Gegenwart, P.; Jesche, A. Adiabatic demagnetization refrigeration with antiferromagnetically ordered NaGdP2O7 Journal Article Phys. Rev. B 111, 064431 (2025), datadoi: 10.5281/zenodo.14697906. @article{telangAdiabaticDemagnetizationRefrigeration2025,
title = {Adiabatic demagnetization refrigeration with antiferromagnetically ordered NaGdP_{2}O_{7}},
author = {P. Telang and T. Treu and M. Klinger and A. A. Tsirlin and P. Gegenwart and A. Jesche},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.064431},
doi = {10.1103/PhysRevB.111.064431},
year = {2025},
date = {2025-02-28},
urldate = {2025-02-01},
journal = {Phys. Rev. B},
volume = {111},
number = {6},
pages = {064431},
abstract = {We present a comprehensive study of the structural, magnetic, and thermodynamic properties, as well as the adiabatic demagnetization refrigeration (ADR) performance of NaGdP2O7. Although NaGdP2O7 exhibits antiferromagnetic ordering at a Néel temperature of 𝑇N=570mK in zero field, ADR experiments achieved a minimum temperature of 220 mK starting from 𝑇=2K under an applied magnetic field of 𝜇0𝐻=5T. The warm-up time back to 𝑇=2K exceeds 60 hours with 9 hours below 𝑇=400mK underscoring the potential of NaGdP2O7 as an efficient precooling stage in double-stage ADR systems. We show that the spin lattice of NaGdP2O7 can be seen as a network of ferromagnetic spin chains with antiferromagnetic interchain couplings and also investigate the influence of antiferromagnetic ordering on the magnetic entropy. We find that the temperature dependence of the entropy plays a more dominant role than its magnetic field dependence in the magnetically ordered state.},
note = {datadoi: 10.5281/zenodo.14697906},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
We present a comprehensive study of the structural, magnetic, and thermodynamic properties, as well as the adiabatic demagnetization refrigeration (ADR) performance of NaGdP2O7. Although NaGdP2O7 exhibits antiferromagnetic ordering at a Néel temperature of 𝑇N=570mK in zero field, ADR experiments achieved a minimum temperature of 220 mK starting from 𝑇=2K under an applied magnetic field of 𝜇0𝐻=5T. The warm-up time back to 𝑇=2K exceeds 60 hours with 9 hours below 𝑇=400mK underscoring the potential of NaGdP2O7 as an efficient precooling stage in double-stage ADR systems. We show that the spin lattice of NaGdP2O7 can be seen as a network of ferromagnetic spin chains with antiferromagnetic interchain couplings and also investigate the influence of antiferromagnetic ordering on the magnetic entropy. We find that the temperature dependence of the entropy plays a more dominant role than its magnetic field dependence in the magnetically ordered state. |  |
Gotovko, S. K.; Ivanova, A. G.; Kudimkina, P. S.; Bush, A. A.; Kozlov, V. I.; Hemmida, M.; von Nidda, H. -A. Krug; Svistov, L. E. Low-frequency dynamics of LiCu3O3: An antiferromagnet on a strongly depleted square lattice Journal Article Phys. Rev. B 111, 064430 (2025). @article{gotovko_low-frequency_2025,
title = {Low-frequency dynamics of LiCu_{3}O_{3}: An antiferromagnet on a strongly depleted square lattice},
author = {S. K. Gotovko and A. G. Ivanova and P. S. Kudimkina and A. A. Bush and V. I. Kozlov and M. Hemmida and H. -A. Krug von Nidda and L. E. Svistov},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.064430},
doi = {10.1103/PhysRevB.111.064430},
year = {2025},
date = {2025-02-28},
urldate = {2025-02-01},
journal = {Phys. Rev. B},
volume = {111},
number = {6},
pages = {064430},
abstract = {We present the study of low-frequency dynamics of LiCu3O3 —an antiferromagnet on a strongly depleted square lattice. The crystal structure contains two types of square planes with different Li+ → Cu2+ substitution rates (20% and 40%). Recent nuclear magnetic resonance (NMR), magnetization measurements and neutron scattering experiments revealed the occurrence of antiferromagnetic order at Tc1=123K and the change of the magnetic state at Tc2≈30K. Electron spin resonance (ESR) intensity measurements confirmed that at Tc1=123K a magnetic phase transition of only a part of the sample occurs, while the rest of the sample remains paramagnetic. Supposedly, the order occurs in the magnetic planes with higher concentrations of magnetic ions. The ratio of ESR intensity values before and after the transition is in agreement with this suggestion. In the studied frequency and temperature range (18–140GHz, 30–300K) only one electron paramagnetic resonance (EPR) branch was observed. At temperatures T<30K, the ESR branch acquires a gap which gradually increases with temperature decrease. The behavior of the observed gap in the magnetic resonance spectra indicates that this gap is, in fact, a pseudogap of exchange nature associated with finite-sized clusters of magnetic ions.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
We present the study of low-frequency dynamics of LiCu3O3 —an antiferromagnet on a strongly depleted square lattice. The crystal structure contains two types of square planes with different Li+ → Cu2+ substitution rates (20% and 40%). Recent nuclear magnetic resonance (NMR), magnetization measurements and neutron scattering experiments revealed the occurrence of antiferromagnetic order at Tc1=123K and the change of the magnetic state at Tc2≈30K. Electron spin resonance (ESR) intensity measurements confirmed that at Tc1=123K a magnetic phase transition of only a part of the sample occurs, while the rest of the sample remains paramagnetic. Supposedly, the order occurs in the magnetic planes with higher concentrations of magnetic ions. The ratio of ESR intensity values before and after the transition is in agreement with this suggestion. In the studied frequency and temperature range (18–140GHz, 30–300K) only one electron paramagnetic resonance (EPR) branch was observed. At temperatures T<30K, the ESR branch acquires a gap which gradually increases with temperature decrease. The behavior of the observed gap in the magnetic resonance spectra indicates that this gap is, in fact, a pseudogap of exchange nature associated with finite-sized clusters of magnetic ions. |  |
Leeb, V.; Huber, N.; Pfleiderer, C.; Knolle, J.; Wilde, M. A. A Field Guide to Non-Onsager Quantum Oscillations in Metals Journal Article Adv. Phys. Res. 4, 2400134 (2025). @article{leeb_field_2025,
title = {A Field Guide to Non-Onsager Quantum Oscillations in Metals},
author = {V. Leeb and N. Huber and C. Pfleiderer and J. Knolle and M. A. Wilde},
url = {https://doi.org/10.1002/apxr.202400134},
doi = {10.1002/apxr.202400134},
year = {2025},
date = {2025-02-25},
urldate = {2025-02-25},
journal = {Adv. Phys. Res.},
volume = {4},
number = {4},
pages = {2400134},
abstract = {Abstract Quantum oscillation (QO) measurements constitute a powerful method to measure the Fermi surface (FS) properties of metals. The observation of QOs is usually taken as strong evidence for the existence of extremal cross-sectional areas of the FS according to the famous Onsager relation. Here, mechanisms that generate QO frequencies that defy the Onsager relation are reviewed and material candidates are discussed. These include magnetic breakdown, magnetic interaction, chemical potential oscillations, and Stark quantum interference, most of which lead to signals occurring at combinations of ?parent? Onsager frequencies. A special emphasis is put on the recently discovered mechanism of quasi-particle lifetime oscillations (QPLOs). This work aims to provide a field guide that allows, on the one hand, to distinguish such non-Onsager QOs from conventional QOs arising from extremal cross sections and, on the other hand, to distinguish the various non-Onsager mechanisms from each other. A practical classification of non-Onsager QOs is given in terms of the prerequisites for their occurrence and their characteristics. It is shown that, in particular, the recently discovered QPLOs may pose significant challenges for the interpretation of QO spectra, as they may occur quite generically as frequency differences in multi-orbit systems, without the necessity of visible ?parent? frequencies in the spectrum, owing to a strongly suppressed temperature dephasing of QPLOs. An extensive list of material candidates is presented where QPLOs may represent an alternative explanation for the observation of unexpected QO frequencies.},
keywords = {A6, B6, C1},
pubstate = {published},
tppubtype = {article}
}
Abstract Quantum oscillation (QO) measurements constitute a powerful method to measure the Fermi surface (FS) properties of metals. The observation of QOs is usually taken as strong evidence for the existence of extremal cross-sectional areas of the FS according to the famous Onsager relation. Here, mechanisms that generate QO frequencies that defy the Onsager relation are reviewed and material candidates are discussed. These include magnetic breakdown, magnetic interaction, chemical potential oscillations, and Stark quantum interference, most of which lead to signals occurring at combinations of ?parent? Onsager frequencies. A special emphasis is put on the recently discovered mechanism of quasi-particle lifetime oscillations (QPLOs). This work aims to provide a field guide that allows, on the one hand, to distinguish such non-Onsager QOs from conventional QOs arising from extremal cross sections and, on the other hand, to distinguish the various non-Onsager mechanisms from each other. A practical classification of non-Onsager QOs is given in terms of the prerequisites for their occurrence and their characteristics. It is shown that, in particular, the recently discovered QPLOs may pose significant challenges for the interpretation of QO spectra, as they may occur quite generically as frequency differences in multi-orbit systems, without the necessity of visible ?parent? frequencies in the spectrum, owing to a strongly suppressed temperature dephasing of QPLOs. An extensive list of material candidates is presented where QPLOs may represent an alternative explanation for the observation of unexpected QO frequencies. |  |
Kong, D.; Kovács, A.; Charilaou, M.; Altthaler, M.; Prodan, L.; Tsurkan, V.; Meier, D.; Han, X.; Kézsmárki, I.; Dunin-Borkowski, R. E. Strain Engineering of Magnetic Anisotropy in the Kagome Magnet Fe3Sn2 Journal Article ACS Nano 19, 8142–8151 (2025). @article{kong_strain_2025,
title = {Strain Engineering of Magnetic Anisotropy in the Kagome Magnet Fe_{3}Sn_{2}},
author = {D. Kong and A. Kovács and M. Charilaou and M. Altthaler and L. Prodan and V. Tsurkan and D. Meier and X. Han and I. Kézsmárki and R. E. Dunin-Borkowski},
url = {https://doi.org/10.1021/acsnano.4c16603},
doi = {10.1021/acsnano.4c16603},
year = {2025},
date = {2025-02-24},
urldate = {2025-03-01},
journal = {ACS Nano},
volume = {19},
number = {8},
pages = {8142–8151},
abstract = {The ability to control magnetism with strain offers innovative pathways for the modulation of magnetic domain configurations and for the manipulation of magnetic states in materials on the nanoscale. Although the effect of strain on magnetic domains has been recognized since the early work of C. Kittel, detailed local observations have been elusive. Here, we use mechanical strain to achieve reversible control of magnetic textures in a kagome-type Fe3Sn2 ferromagnet without the use of an external electric current or magnetic field in situ in a transmission electron microscope at room temperature. We use Fresnel defocus imaging, off-axis electron holography and micromagnetic simulations to show that tensile strain modifies the structures of dipolar skyrmions and switches the magnetization between out-of-plane and in-plane configurations. We also present quantitative measurements of magnetic domain wall structures and their transformations as a function of strain. Our results demonstrate the fundamental importance of anisotropy effects and their interplay with magnetoelastic and magnetocrystalline energies, providing opportunities for the development of strain-controlled devices for spintronic applications.},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
The ability to control magnetism with strain offers innovative pathways for the modulation of magnetic domain configurations and for the manipulation of magnetic states in materials on the nanoscale. Although the effect of strain on magnetic domains has been recognized since the early work of C. Kittel, detailed local observations have been elusive. Here, we use mechanical strain to achieve reversible control of magnetic textures in a kagome-type Fe3Sn2 ferromagnet without the use of an external electric current or magnetic field in situ in a transmission electron microscope at room temperature. We use Fresnel defocus imaging, off-axis electron holography and micromagnetic simulations to show that tensile strain modifies the structures of dipolar skyrmions and switches the magnetization between out-of-plane and in-plane configurations. We also present quantitative measurements of magnetic domain wall structures and their transformations as a function of strain. Our results demonstrate the fundamental importance of anisotropy effects and their interplay with magnetoelastic and magnetocrystalline energies, providing opportunities for the development of strain-controlled devices for spintronic applications. |  |
Zahn, M.; Müller, A. M.; Kelley, K. P.; Neumayer, S.; Kalinin, S. V.; Kézsmarki, I.; Fiebig, M.; Lottermoser, T.; Domingo, N.; Meier, D.; Schultheiß, J. Reversible long-range domain wall motion in an improper ferroelectric Journal Article Nat. Commun. 16, 1781 (2025), datadoi: 10.5281/zenodo.14624857. @article{zahnReversibleLongrangeDomain2025,
title = {Reversible long-range domain wall motion in an improper ferroelectric},
author = {M. Zahn and A. M. Müller and K. P. Kelley and S. Neumayer and S. V. Kalinin and I. Kézsmarki and M. Fiebig and T. Lottermoser and N. Domingo and D. Meier and J. Schultheiß},
url = {https://doi.org/10.1038/s41467-025-57062-8},
doi = {10.1038/s41467-025-57062-8},
year = {2025},
date = {2025-02-19},
urldate = {2025-02-01},
journal = {Nat. Commun.},
volume = {16},
number = {1},
pages = {1781},
abstract = {Reversible ferroelectric domain wall movements beyond the 10 nm range associated with Rayleigh behavior are usually restricted to specific defect-engineered systems. Here, we demonstrate that such long-range movements naturally occur in the improper ferroelectric ErMnO3 during electric-field-cycling. We study the electric-field-driven motion of domain walls, showing that they readily return to their initial position after having traveled distances exceeding 250 nm. By applying switching spectroscopy band-excitation piezoresponse force microscopy, we track the domain wall movement with nanometric spatial precision and analyze the local switching behavior. Phase field simulations show that the reversible long-range motion is intrinsic to the hexagonal manganites, linking it to their improper ferroelectricity and topologically protected structural vortex lines, which serve as anchor point for the ferroelectric domain walls. Our results give new insight into the local dynamics of domain walls in improper ferroelectrics and demonstrate the possibility to reversibly displace domain walls over much larger distances than commonly expected for ferroelectric systems in their pristine state, ensuring predictable device behavior for applications such as tunable capacitors or sensors.},
note = {datadoi: 10.5281/zenodo.14624857},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
Reversible ferroelectric domain wall movements beyond the 10 nm range associated with Rayleigh behavior are usually restricted to specific defect-engineered systems. Here, we demonstrate that such long-range movements naturally occur in the improper ferroelectric ErMnO3 during electric-field-cycling. We study the electric-field-driven motion of domain walls, showing that they readily return to their initial position after having traveled distances exceeding 250 nm. By applying switching spectroscopy band-excitation piezoresponse force microscopy, we track the domain wall movement with nanometric spatial precision and analyze the local switching behavior. Phase field simulations show that the reversible long-range motion is intrinsic to the hexagonal manganites, linking it to their improper ferroelectricity and topologically protected structural vortex lines, which serve as anchor point for the ferroelectric domain walls. Our results give new insight into the local dynamics of domain walls in improper ferroelectrics and demonstrate the possibility to reversibly displace domain walls over much larger distances than commonly expected for ferroelectric systems in their pristine state, ensuring predictable device behavior for applications such as tunable capacitors or sensors. |  |
Aqeel, A.; Kronseder, M.; Vlietstra, N.; Huebl, H.; Heuver, J. A.; Noheda, B.; Herrero-Martín, J.; Pellegrin, E.; Vasili, H. B.; Mostovoy, M.; Back, C. Spin Hall magnetoresistance and spin Seebeck effect in Pt textbarCoCr2O4 heterostructures Journal Article Sci. Technol. Adv. Mater. 26, 2457320 (2025). @article{aqeelSpinHallMagnetoresistance2025,
title = {Spin Hall magnetoresistance and spin Seebeck effect in Pt textbarCoCr_{2}O_{4} heterostructures},
author = {A. Aqeel and M. Kronseder and N. Vlietstra and H. Huebl and J. A. Heuver and B. Noheda and J. Herrero-Martín and E. Pellegrin and H. B. Vasili and M. Mostovoy and C. Back},
url = {https://doi.org/10.1080/14686996.2025.2457320},
doi = {10.1080/14686996.2025.2457320},
year = {2025},
date = {2025-02-12},
urldate = {2025-12-01},
journal = {Sci. Technol. Adv. Mater.},
volume = {26},
number = {1},
pages = {2457320},
abstract = {This study delves into spin current-induced phenomena, such as spin-Hall magnetoresistance and the spin Seebeck effect within Pt films deposited on a noncollinear magnet, CoCr 2O 4 (CCO), particularly at low temperatures. Detailed investigation of the angular dependencies of spin Hall magnetoresistance (SMR) and spin Seebeck effect (SSE) was carried out. The temperature-dependent behavior of both SMR and SSE signals exhibits a discernible variation correlated with different magnetic phases of CCO. To distinguish the contributions arising from magnetic proximity effects, we conducted X-ray magnetic dichroism (XMCD) at the Pt-M 3 edge. XMCD data from Pt/CCO heterostructures suggest that any magnetic moment associated with Pt, if present, is below the detection limit. This supports the notion that the observed signals primarily stem from SMR and SSE. This study offers insights into spin-current-driven phenomena, paving the way for potential spintronic applications. This study uniquely differentiates non-collinear magnetic phases in CoCr?O? using all-electrical SMR and SSE, validated by excluding proximity-induced magnetization via XMCD, advancing spintronic detection techniques.},
keywords = {A2, B4, C3},
pubstate = {published},
tppubtype = {article}
}
This study delves into spin current-induced phenomena, such as spin-Hall magnetoresistance and the spin Seebeck effect within Pt films deposited on a noncollinear magnet, CoCr 2O 4 (CCO), particularly at low temperatures. Detailed investigation of the angular dependencies of spin Hall magnetoresistance (SMR) and spin Seebeck effect (SSE) was carried out. The temperature-dependent behavior of both SMR and SSE signals exhibits a discernible variation correlated with different magnetic phases of CCO. To distinguish the contributions arising from magnetic proximity effects, we conducted X-ray magnetic dichroism (XMCD) at the Pt-M 3 edge. XMCD data from Pt/CCO heterostructures suggest that any magnetic moment associated with Pt, if present, is below the detection limit. This supports the notion that the observed signals primarily stem from SMR and SSE. This study offers insights into spin-current-driven phenomena, paving the way for potential spintronic applications. This study uniquely differentiates non-collinear magnetic phases in CoCr?O? using all-electrical SMR and SSE, validated by excluding proximity-induced magnetization via XMCD, advancing spintronic detection techniques. |  |
Pichler, F.; Kadow, W.; Kuhlenkamp, C.; Knap, M. Single-particle spectral function of fractional quantum anomalous Hall states Journal Article Phys. Rev. B 111, (2025), datadoi: 10.5281/zenodo.13692026. @article{pichlerSingleparticleSpectralFunction2025,
title = {Single-particle spectral function of fractional quantum anomalous Hall states},
author = {F. Pichler and W. Kadow and C. Kuhlenkamp and M. Knap},
url = {https://doi.org/10.1103/PhysRevB.111.075108},
doi = {10.1103/physrevb.111.075108},
issn = {2469-9969},
year = {2025},
date = {2025-02-04},
urldate = {2025-02-01},
journal = {Phys. Rev. B},
volume = {111},
number = {7},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.13692026},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Wenzel, M.; Uykur, E.; Rößler, S.; Schmidt, M.; Janson, O.; Tiwari, A.; Dressel, M.; Tsirlin, A. A. Fermi-liquid behavior of nonaltermagnetic RuO2 Journal Article Phys. Rev. B 111, L041115 (2025). @article{wenzel_fermi-liquid_2025,
title = {Fermi-liquid behavior of nonaltermagnetic RuO_{2}},
author = {M. Wenzel and E. Uykur and S. Rößler and M. Schmidt and O. Janson and A. Tiwari and M. Dressel and A. A. Tsirlin},
url = {https://link.aps.org/doi/10.1103/PhysRevB.111.L041115},
doi = {10.1103/PhysRevB.111.L041115},
year = {2025},
date = {2025-01-28},
urldate = {2025-01-28},
journal = {Phys. Rev. B},
volume = {111},
number = {4},
pages = {L041115},
abstract = {The presence of magnetism in potentially altermagnetic RuO2 has been a subject of intense debate. Using broadband infrared spectroscopy combined with density-functional band-structure calculations, we show that the optical conductivity of RuO2, the bulk probe of its electronic structure, is best described by a nonmagnetic model. The sharp Pauli edge demonstrates the presence of a Dirac nodal line lying 45 meV below the Fermi level. An excellent match between the experimental and ab initio plasma frequencies underpins the weakness of electronic correlations. The intraband part of the optical conductivity indicates Fermi-liquid behavior with two distinct scattering rates below 150 K. Fermi-liquid theory also accounts for the temperature-dependent magnetic susceptibility of RuO2 and allows a consistent description of this material as a paramagnetic metal.},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
The presence of magnetism in potentially altermagnetic RuO2 has been a subject of intense debate. Using broadband infrared spectroscopy combined with density-functional band-structure calculations, we show that the optical conductivity of RuO2, the bulk probe of its electronic structure, is best described by a nonmagnetic model. The sharp Pauli edge demonstrates the presence of a Dirac nodal line lying 45 meV below the Fermi level. An excellent match between the experimental and ab initio plasma frequencies underpins the weakness of electronic correlations. The intraband part of the optical conductivity indicates Fermi-liquid behavior with two distinct scattering rates below 150 K. Fermi-liquid theory also accounts for the temperature-dependent magnetic susceptibility of RuO2 and allows a consistent description of this material as a paramagnetic metal. |  |
Shen, B.; Pazmino, E. Insuasti; Dhakal, R.; Freund, F.; Gegenwart, P.; Winter, S. M.; Tsirlin, A. A. Pressure-dependent magnetism of the Kitaev candidate Li2RhO3 Journal Article npj Quantum Mater. 10, 9 (2025), datadoi: 10.5281/zenodo.13784958. @article{shenPressuredependentMagnetismKitaev2025,
title = {Pressure-dependent magnetism of the Kitaev candidate Li_{2}RhO_{3}},
author = {B. Shen and E. Insuasti Pazmino and R. Dhakal and F. Freund and P. Gegenwart and S. M. Winter and A. A. Tsirlin},
url = {https://doi.org/10.1038/s41535-025-00730-1},
doi = {10.1038/s41535-025-00730-1},
year = {2025},
date = {2025-01-22},
urldate = {2025-01-01},
journal = {npj Quantum Mater.},
volume = {10},
number = {1},
pages = {9},
abstract = {We use magnetization measurements under pressure along with ab initio and cluster many-body calculations to investigate magnetism of the Kitaev candidate Li2RhO3. Hydrostatic compression leads to a decrease in the magnitude of the nearest-neighbor ferromagnetic Kitaev coupling K1 and the corresponding increase in the off-diagonal anisotropy Γ1, whereas the experimental Curie-Weiss temperature changes from negative to positive with the slope of +40 K/GPa. On the other hand, spin freezing persists up to at least 3.46 GPa with the almost constant freezing temperature of 5 K that does not follow the large changes in the exchange couplings and indicates the likely extrinsic origin of spin freezing. Magnetic frustration in Li2RhO3 is mainly related to the interplay between ferromagnetic K1 and antiferromagnetic Γ1, along with the weakness of the third-neighbor coupling J3 that would otherwise stabilize zigzag order. The small J3 distinguishes Li2RhO3 from other Kitaev candidates.},
note = {datadoi: 10.5281/zenodo.13784958},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
We use magnetization measurements under pressure along with ab initio and cluster many-body calculations to investigate magnetism of the Kitaev candidate Li2RhO3. Hydrostatic compression leads to a decrease in the magnitude of the nearest-neighbor ferromagnetic Kitaev coupling K1 and the corresponding increase in the off-diagonal anisotropy Γ1, whereas the experimental Curie-Weiss temperature changes from negative to positive with the slope of +40 K/GPa. On the other hand, spin freezing persists up to at least 3.46 GPa with the almost constant freezing temperature of 5 K that does not follow the large changes in the exchange couplings and indicates the likely extrinsic origin of spin freezing. Magnetic frustration in Li2RhO3 is mainly related to the interplay between ferromagnetic K1 and antiferromagnetic Γ1, along with the weakness of the third-neighbor coupling J3 that would otherwise stabilize zigzag order. The small J3 distinguishes Li2RhO3 from other Kitaev candidates. |  |
Papaefstathiou, I.; Knolle, J.; Bañuls, M. C. Real-time scattering in the lattice Schwinger model Journal Article Phys. Rev. D 111, 014504 (2025). @article{papaefstathiou_real-time_2025,
title = {Real-time scattering in the lattice Schwinger model},
author = {I. Papaefstathiou and J. Knolle and M. C. Bañuls},
url = {https://link.aps.org/doi/10.1103/PhysRevD.111.014504},
doi = {10.1103/PhysRevD.111.014504},
year = {2025},
date = {2025-01-15},
urldate = {2025-01-15},
journal = {Phys. Rev. D},
volume = {111},
number = {1},
pages = {014504},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Xu, W. -T.; Rakovszky, T.; Knap, M.; Pollmann, F. Entanglement Properties of Gauge Theories from Higher-Form Symmetries Journal Article Phys. Rev. X 15, 011001 (2025), datadoi: (10.5281/zenodo.14360829). @article{xuEntanglementPropertiesGauge2025,
title = {Entanglement Properties of Gauge Theories from Higher-Form Symmetries},
author = {W. -T. Xu and T. Rakovszky and M. Knap and F. Pollmann},
doi = {10.1103/PhysRevX.15.011001},
year = {2025},
date = {2025-01-02},
urldate = {2025-01-02},
journal = {Phys. Rev. X},
volume = {15},
number = {1},
pages = {011001},
abstract = {We explore the relationship between higher-form symmetries and entanglement properties in lattice gauge theories with discrete gauge groups, which can exhibit both topologically ordered phases and higher-form symmetry-protected topological (SPT) phases. Our study centers on a generalization of the Fradkin-Shenker model describing ℤ2 lattice gauge theory with matter, where the Gauss law constraint can be either emergent or exact. The phase diagram includes a topologically ordered deconfined phase and a nontrivial SPT phase protected by a 1-form and a 0-form symmetry, among others. We obtain the following key findings: First, the entanglement properties of the model depend on whether the 1-form symmetries and the Gauss law constraint are exact or emergent. For the emergent Gauss law, the entanglement spectrum (ES) of the nontrivial SPT phase exhibits degeneracies, which are robust at low energies against weak perturbations that explicitly break the exact 1-form symmetry. When the Gauss law and the 1-form symmetry are both exact, the ES degeneracy is extensive. This extensive degeneracy turns out to be fragile and can be removed completely by infinitesimal perturbations that explicitly break the exact 1-form symmetry while keeping the Gauss law exact. Second, we consider the ES in the topologically ordered phase where 1-form symmetries are spontaneously broken. In contrast to the ES of the nontrivial SPT phase, we find that spontaneous higher-form symmetry breaking removes “half” of the ES levels, leading to a nondegenerate ES in the topologically ordered phase, in general. Third, we derive a connection between spontaneous higher-form symmetry breaking and the topological entanglement entropy (TEE). Using this relation, we investigate the entanglement entropy that can be distilled in the deconfined phase of the original Fradkin-Shenker model using gauge-invariant measurements. We show that the TEE is robust against the measurement when the 1-form symmetry is emergent but it is fragile when the 1-form symmetry is exact. Our results demonstrate the advantage of higher-form symmetries for understanding entanglement properties of gauge theories.},
note = {datadoi: (10.5281/zenodo.14360829)},
keywords = {B6, C5, C6},
pubstate = {published},
tppubtype = {article}
}
We explore the relationship between higher-form symmetries and entanglement properties in lattice gauge theories with discrete gauge groups, which can exhibit both topologically ordered phases and higher-form symmetry-protected topological (SPT) phases. Our study centers on a generalization of the Fradkin-Shenker model describing ℤ2 lattice gauge theory with matter, where the Gauss law constraint can be either emergent or exact. The phase diagram includes a topologically ordered deconfined phase and a nontrivial SPT phase protected by a 1-form and a 0-form symmetry, among others. We obtain the following key findings: First, the entanglement properties of the model depend on whether the 1-form symmetries and the Gauss law constraint are exact or emergent. For the emergent Gauss law, the entanglement spectrum (ES) of the nontrivial SPT phase exhibits degeneracies, which are robust at low energies against weak perturbations that explicitly break the exact 1-form symmetry. When the Gauss law and the 1-form symmetry are both exact, the ES degeneracy is extensive. This extensive degeneracy turns out to be fragile and can be removed completely by infinitesimal perturbations that explicitly break the exact 1-form symmetry while keeping the Gauss law exact. Second, we consider the ES in the topologically ordered phase where 1-form symmetries are spontaneously broken. In contrast to the ES of the nontrivial SPT phase, we find that spontaneous higher-form symmetry breaking removes “half” of the ES levels, leading to a nondegenerate ES in the topologically ordered phase, in general. Third, we derive a connection between spontaneous higher-form symmetry breaking and the topological entanglement entropy (TEE). Using this relation, we investigate the entanglement entropy that can be distilled in the deconfined phase of the original Fradkin-Shenker model using gauge-invariant measurements. We show that the TEE is robust against the measurement when the 1-form symmetry is emergent but it is fragile when the 1-form symmetry is exact. Our results demonstrate the advantage of higher-form symmetries for understanding entanglement properties of gauge theories. |  |
Battistelli, R.; Körber, L.; Litzius, K.; Grelier, M.; Joy, K. P.; Schneider, M.; Wittrock, S.; Metternich, D.; Karaman, T.; Kern, L. -M.; Klose, C.; Finizio, S.; Fuchs, J.; Günther, C. M.; Butcher, T. A.; Prokeš, K.; Boltje, R.; Patra, M.; Wintz, S.; Weigand, M.; Petz, S.; Popescu, H.; Raabe, J.; Jaouen, N.; Eisebitt, S.; Cros, V.; Pfau, B.; Mentink, J. H.; Reyren, N.; Büttner, F. A fluctuation-free pathway for a topological magnetic phase transition Unpublished (2025), arXiv:2512.22947
datadoi: 10.5281/zenodo.18004538. @unpublished{battistelliFluctuationfreePathwayTopological2025,
title = {A fluctuation-free pathway for a topological magnetic phase transition},
author = {R. Battistelli and L. Körber and K. Litzius and M. Grelier and K. P. Joy and M. Schneider and S. Wittrock and D. Metternich and T. Karaman and L. -M. Kern and C. Klose and S. Finizio and J. Fuchs and C. M. Günther and T. A. Butcher and K. Prokeš and R. Boltje and M. Patra and S. Wintz and M. Weigand and S. Petz and H. Popescu and J. Raabe and N. Jaouen and S. Eisebitt and V. Cros and B. Pfau and J. H. Mentink and N. Reyren and F. Büttner},
url = {https://arxiv.org/abs/2512.22947},
doi = {10.48550/arXiv.2512.22947},
year = {2025},
date = {2025-12-28},
urldate = {2025-12-01},
abstract = {Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism.},
note = {arXiv:2512.22947
datadoi: 10.5281/zenodo.18004538},
keywords = {C2},
pubstate = {published},
tppubtype = {unpublished}
}
Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism. |  |
Metternich, D.; Schneider, M.; Mercurio, G.; Hegstad, T.; Möller, M.; Battistelli, R.; Klose, C.; Wittrock, S.; Patra, M. R.; Joy, K. P.; Deinhart, V.; Petz, S.; Prokes, K.; Wintz, S.; Weigand, M.; Engel, W. -D.; Sidiropoulos, T.; Will, I.; Eisebitt, S.; Carley, R. E.; Mercadier, L.; Schlappa, J.; Teichmann, M.; Scherz, A.; Zayko, S.; Sorokin, B. V.; Bagschik, K.; Ropers, C.; Mentink, J. H.; Pfau, B.; Büttner, F. Picosecond localization dynamics following ultrafast nanoscale magnetic switching Unpublished (2025), arXiv:2512.17643. @unpublished{metternichPicosecondLocalizationDynamics2025,
title = {Picosecond localization dynamics following ultrafast nanoscale magnetic switching},
author = {D. Metternich and M. Schneider and G. Mercurio and T. Hegstad and M. Möller and R. Battistelli and C. Klose and S. Wittrock and M. R. Patra and K. P. Joy and V. Deinhart and S. Petz and K. Prokes and S. Wintz and M. Weigand and W. -D. Engel and T. Sidiropoulos and I. Will and S. Eisebitt and R. E. Carley and L. Mercadier and J. Schlappa and M. Teichmann and A. Scherz and S. Zayko and B. V. Sorokin and K. Bagschik and C. Ropers and J. H. Mentink and B. Pfau and F. Büttner},
url = {https://arxiv.org/abs/2512.17643},
doi = {https://doi.org/10.48550/arXiv.2512.17643},
year = {2025},
date = {2025-12-19},
urldate = {2025-12-01},
abstract = {Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined. However, the physics of domain localization during such ultrafast phase transitions remains unresolved. Here, we use shot-resolved pump-probe resonant x-ray scattering together with a material featuring a periodically modulated magnetic anisotropy landscape to track, in real time, the laser-driven nucleation and localization of nanometer-scale spin textures. We find that nucleation and localization are two distinct processes. Nucleation occurs homogeneously via fluctuations at early times, whereas spatially periodic structures emerge only later and, under suitable conditions, localize in less than one nanosecond. Real-space simulations show that this localization is governed by strong lateral variations in spin-texture lifetimes. Our results demonstrate that ultrafast phase-transition dynamics fundamentally differ from conventional transitions, yet still can be controlled through moderate nanometer-scale tailoring of the energy landscape.},
note = {arXiv:2512.17643},
keywords = {C2},
pubstate = {published},
tppubtype = {unpublished}
}
Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined. However, the physics of domain localization during such ultrafast phase transitions remains unresolved. Here, we use shot-resolved pump-probe resonant x-ray scattering together with a material featuring a periodically modulated magnetic anisotropy landscape to track, in real time, the laser-driven nucleation and localization of nanometer-scale spin textures. We find that nucleation and localization are two distinct processes. Nucleation occurs homogeneously via fluctuations at early times, whereas spatially periodic structures emerge only later and, under suitable conditions, localize in less than one nanosecond. Real-space simulations show that this localization is governed by strong lateral variations in spin-texture lifetimes. Our results demonstrate that ultrafast phase-transition dynamics fundamentally differ from conventional transitions, yet still can be controlled through moderate nanometer-scale tailoring of the energy landscape. |  |
Schilberth, F.; DeFreitas, L.; Zhao, K.; LeMardelé, F.; Mohelsky, I.; Orlita, M.; Gegenwart, P.; Chen, H.; Kézsmárki, I.; Bordács, S. Large magnetoreflectance and optical anisotropy due to 4f flat bands in the frustrated kagome magnet HoAgGe Unpublished (2025), arXiv.2504.10274. @unpublished{schilberth_large_2025,
title = {Large magnetoreflectance and optical anisotropy due to 4f flat bands in the frustrated kagome magnet HoAgGe},
author = {F. Schilberth and L. DeFreitas and K. Zhao and F. LeMardelé and I. Mohelsky and M. Orlita and P. Gegenwart and H. Chen and I. Kézsmárki and S. Bordács},
url = {https://arxiv.org/abs/2504.10274},
doi = {10.48550/arXiv.2504.10274},
year = {2025},
date = {2025-04-01},
urldate = {2025-04-01},
abstract = {We report peculiar optical properties of the frustrated itinerant magnet HoAgGe, which exhibits multiple magnetically ordered states obeying the kagome spin-ice rule. The optical conductivity is surprisingly higher for light polarization perpendicular to the kagome plane, both for the free carrier response and the interband transitions. The latter ones have strong contributions from Ho 4f flat bands located near the Fermi level, as revealed by our textbackslashtextitab initio calculations, explaining the unusual anisotropy of the optical properties and the pronounced temperature dependence of the interband transitions for out–of–plane light polarization. The key role of Ho 4f states is further supported by the large variation of the reflectivity upon the metamagnetic transitions, that follows the field dependence of the magnetization, in contrast to that of the dc magnetotransport data. Such heavy-electron bands near the Fermi level offer an efficient way to control transport and optical properties.},
note = {arXiv.2504.10274},
keywords = {A1, B3},
pubstate = {published},
tppubtype = {unpublished}
}
We report peculiar optical properties of the frustrated itinerant magnet HoAgGe, which exhibits multiple magnetically ordered states obeying the kagome spin-ice rule. The optical conductivity is surprisingly higher for light polarization perpendicular to the kagome plane, both for the free carrier response and the interband transitions. The latter ones have strong contributions from Ho 4f flat bands located near the Fermi level, as revealed by our textbackslashtextitab initio calculations, explaining the unusual anisotropy of the optical properties and the pronounced temperature dependence of the interband transitions for out–of–plane light polarization. The key role of Ho 4f states is further supported by the large variation of the reflectivity upon the metamagnetic transitions, that follows the field dependence of the magnetization, in contrast to that of the dc magnetotransport data. Such heavy-electron bands near the Fermi level offer an efficient way to control transport and optical properties. |  |
Shen, B.; Du, F.; Breitner, F.; Ginga, V. A.; Uykur, E.; Tsirlin, A. A.; Gegenwart, P. Pressure-induced strange metal phase in a metallic kagome ferromagnet Unpublished (2025), arXiv:2503.09524,
datadoi: 10.5281/zenodo.14651315. @unpublished{shenPressureinducedStrangeMetal2025,
title = {Pressure-induced strange metal phase in a metallic kagome ferromagnet},
author = {B. Shen and F. Du and F. Breitner and V. A. Ginga and E. Uykur and A. A. Tsirlin and P. Gegenwart},
url = {https://arxiv.org/abs/2503.09524},
doi = {10.48550/arXiv.2503.09524},
year = {2025},
date = {2025-03-12},
urldate = {2025-03-01},
abstract = {Strange metallicity with T-linear electrical resistance preceding high-Tc superconductivity remains an enigmatic, yet crucial, signature of correlation physics. Using electrical transport and magnetization measurements up to 50 GPa, we show that such a strange-metal phase is formed in pressurized kagome ferromagnet CrNiAs. In contrast to other kagome materials, a linear suppression of the Curie temperature is found, with the ferromagnetic quantum critical point at pc=GPa. Remarkably, from pc up to the highest measured pressure, characteristic strange-metal behavior is observed, whereas magnetic field reinstates the Fermi liquid. Electronic structure calculations reveal robust weakly dispersive bands persisting unchanged beyond pc, possibly at the origin of the T-linear electrical resistance. This establishes pressurized kagome ferromagnets as an intriguing platform for strange-metal behavior.},
note = { arXiv:2503.09524,
datadoi: 10.5281/zenodo.14651315},
keywords = {B3},
pubstate = {published},
tppubtype = {unpublished}
}
Strange metallicity with T-linear electrical resistance preceding high-Tc superconductivity remains an enigmatic, yet crucial, signature of correlation physics. Using electrical transport and magnetization measurements up to 50 GPa, we show that such a strange-metal phase is formed in pressurized kagome ferromagnet CrNiAs. In contrast to other kagome materials, a linear suppression of the Curie temperature is found, with the ferromagnetic quantum critical point at pc=GPa. Remarkably, from pc up to the highest measured pressure, characteristic strange-metal behavior is observed, whereas magnetic field reinstates the Fermi liquid. Electronic structure calculations reveal robust weakly dispersive bands persisting unchanged beyond pc, possibly at the origin of the T-linear electrical resistance. This establishes pressurized kagome ferromagnets as an intriguing platform for strange-metal behavior. |  |
Scheuchenpflug, L.; Esser, S.; Gruhl, R.; Hirschberger, M.; Gegenwart, P. Current-linear emergent induction of pinned skyrmion textures in an oxide bilayer Unpublished (2025), arXiv:2503.10600. @unpublished{scheuchenpflug_current-linear_2025,
title = {Current-linear emergent induction of pinned skyrmion textures in an oxide bilayer},
author = {L. Scheuchenpflug and S. Esser and R. Gruhl and M. Hirschberger and P. Gegenwart},
url = {https://arxiv.org/abs/2503.10600},
doi = {10.48550/arXiv.2503.10600},
year = {2025},
date = {2025-03-01},
urldate = {2025-03-13},
abstract = {Emergent electromagnetic induction (EEMI) induced through current-driven spin dynamics was recently predicted and subsequently observed in helical spin magnets, opening a new direction in spintronics and paving the way towards further miniaturization of electronic circuit elements. In contrast to conventional inductors consisting of coil-like structures whose inductance shows a linear dependence on the cross-section , emergent inductors exhibit an inverse (textasciitildeAˆ-1) proportionality, favorable for the miniaturization of electrical devices. However, the expected current-linear response of the EEMI voltage has not been demonstrated. Magnetic skyrmions hold promise as a simple platform to study the conceptual foundations of EEMI from current-driven spin dynamics. We fabricated devices of thin film bilayers of ferromagnetic SrRuO3 and paramagnetic SrIrO3, which are known to host interfacial Néel skyrmions detected by the appearance of a topological Hall-effect (THE). A large, positive and current-linear inductive response is found to accompany the THE. In our experiment, the current-induced dynamics of pinned magnetic skyrmions creates a voltage both parallel and perpendicular to the applied electric current flow, corresponding to longitudinal and transverse induction, respectively. This is the first report of transverse EEMI, indicating an angle of 80° between skyrmion motion and the applied current. Our observation of current-linear longitudinal and transverse EEMI is a hallmark of pinned dynamics of magnetic skyrmion textures in oxide heterostructures.},
note = {arXiv:2503.10600},
keywords = {B5},
pubstate = {published},
tppubtype = {unpublished}
}
Emergent electromagnetic induction (EEMI) induced through current-driven spin dynamics was recently predicted and subsequently observed in helical spin magnets, opening a new direction in spintronics and paving the way towards further miniaturization of electronic circuit elements. In contrast to conventional inductors consisting of coil-like structures whose inductance shows a linear dependence on the cross-section , emergent inductors exhibit an inverse (textasciitildeAˆ-1) proportionality, favorable for the miniaturization of electrical devices. However, the expected current-linear response of the EEMI voltage has not been demonstrated. Magnetic skyrmions hold promise as a simple platform to study the conceptual foundations of EEMI from current-driven spin dynamics. We fabricated devices of thin film bilayers of ferromagnetic SrRuO3 and paramagnetic SrIrO3, which are known to host interfacial Néel skyrmions detected by the appearance of a topological Hall-effect (THE). A large, positive and current-linear inductive response is found to accompany the THE. In our experiment, the current-induced dynamics of pinned magnetic skyrmions creates a voltage both parallel and perpendicular to the applied electric current flow, corresponding to longitudinal and transverse induction, respectively. This is the first report of transverse EEMI, indicating an angle of 80° between skyrmion motion and the applied current. Our observation of current-linear longitudinal and transverse EEMI is a hallmark of pinned dynamics of magnetic skyrmion textures in oxide heterostructures. |  |
Tang, N.; Glamsch, S.; Aqeel, A.; Scheuchenpflug, L.; Schulze, M.; Liebald, C.; Rytz, D.; Guguschev, C.; Albrecht, M.; Gegenwart, P. Observation via spin Seebeck effect of macroscopic magnetic transport from emergent magnetic monopoles Unpublished (2025), arXiv:2509.18422. @unpublished{tang_observation_2025,
title = {Observation via spin Seebeck effect of macroscopic magnetic transport from emergent magnetic monopoles},
author = {N. Tang and S. Glamsch and A. Aqeel and L. Scheuchenpflug and M. Schulze and C. Liebald and D. Rytz and C. Guguschev and M. Albrecht and P. Gegenwart},
url = {https://arxiv.org/abs/2509.18422},
doi = {10.48550/arXiv.2509.18422},
year = {2025},
date = {2025-01-01},
urldate = {2025-09-22},
abstract = {Magnetic monopoles, elusive in high-energy physics, have been realised as emergent quasiparticles in solid-state systems, where their unique properties hold promise for novel spintronic applications. Magnetic monopoles have been invoked in diverse platforms, including skyrmion lattices, chiral magnets, soft ferromagnets, aritifical nanomagnets. Yet, a demonstration of their role in magnetic transport has remained elusive. Here, we report such an observation via the spin Seebeck effect in the bulk insulating pyrochlore oxide, spin ice Dy2Ti2O7. By applying a thermal gradient perpendicular to a [111]-oriented magnetic field, we detect a transverse spin Seebeck voltage marked by a dominant peak at the onset of monopole proliferation, accompanied by a secondary feature and frequency-dependent behavior. Our findings establish a direct link between monopole dynamics and magnetic transport in an insulating medium, establishing a new pathway for probing fractionalized excitations and advancing towards novel spintronic applications.},
note = {arXiv:2509.18422},
keywords = {A2, B5},
pubstate = {published},
tppubtype = {unpublished}
}
Magnetic monopoles, elusive in high-energy physics, have been realised as emergent quasiparticles in solid-state systems, where their unique properties hold promise for novel spintronic applications. Magnetic monopoles have been invoked in diverse platforms, including skyrmion lattices, chiral magnets, soft ferromagnets, aritifical nanomagnets. Yet, a demonstration of their role in magnetic transport has remained elusive. Here, we report such an observation via the spin Seebeck effect in the bulk insulating pyrochlore oxide, spin ice Dy2Ti2O7. By applying a thermal gradient perpendicular to a [111]-oriented magnetic field, we detect a transverse spin Seebeck voltage marked by a dominant peak at the onset of monopole proliferation, accompanied by a secondary feature and frequency-dependent behavior. Our findings establish a direct link between monopole dynamics and magnetic transport in an insulating medium, establishing a new pathway for probing fractionalized excitations and advancing towards novel spintronic applications. |  |
2024
|
Tang, N.; Gen, M.; Rotter, M.; Man, H.; Matsuhira, K.; Matsuo, A.; Kindo, K.; Ikeda, A.; Matsuda, Y.; Gegenwart, P.; Nakatsuji, S.; Kohama, Y. Crystal field magnetostriction of spin ice under ultrahigh magnetic fields Journal Article Phys. Rev. B 110, 214414 (2024). @article{tang_crystal_2024,
title = {Crystal field magnetostriction of spin ice under ultrahigh magnetic fields},
author = {N. Tang and M. Gen and M. Rotter and H. Man and K. Matsuhira and A. Matsuo and K. Kindo and A. Ikeda and Y. Matsuda and P. Gegenwart and S. Nakatsuji and Y. Kohama},
url = {https://link.aps.org/doi/10.1103/PhysRevB.110.214414},
doi = {10.1103/PhysRevB.110.214414},
year = {2024},
date = {2024-12-09},
urldate = {2024-12-01},
journal = {Phys. Rev. B},
volume = {110},
number = {21},
pages = {214414},
abstract = {We present a comprehensive study of the magnetoelastic properties of the Ising pyrochlore oxide Ho2Ti2O7, known as spin ice, by means of high-field magnetostriction measurements and numerical calculations. When a magnetic field is applied along the crystallographic ⟨111⟩ axis, the longitudinal magnetostriction exhibits a broad maximum in the low-field regime around 30 T, followed by a dramatic lattice contraction due to crystal-field (CF) level crossing at 𝐵cf∼65 T. The transverse magnetostriction exhibits a contrasting behavior, highlighting the anisotropic nature of the CF striction. By applying a magnetic field at varying sweep rates, we identify distinct timescales of spin dynamics that are relevant to monopole formation and annihilation, as well as CF-phonon dynamics. Our mean-field calculations, based on a point-charge model, successfully reproduce the overall magnetostriction behavior, revealing the competition between the exchange striction and CF striction. A signature of the CF level crossing is also observed through adiabatic magnetocaloric-effect measurements, consistent with our magnetostriction data.},
keywords = {B3, B5},
pubstate = {published},
tppubtype = {article}
}
We present a comprehensive study of the magnetoelastic properties of the Ising pyrochlore oxide Ho2Ti2O7, known as spin ice, by means of high-field magnetostriction measurements and numerical calculations. When a magnetic field is applied along the crystallographic ⟨111⟩ axis, the longitudinal magnetostriction exhibits a broad maximum in the low-field regime around 30 T, followed by a dramatic lattice contraction due to crystal-field (CF) level crossing at 𝐵cf∼65 T. The transverse magnetostriction exhibits a contrasting behavior, highlighting the anisotropic nature of the CF striction. By applying a magnetic field at varying sweep rates, we identify distinct timescales of spin dynamics that are relevant to monopole formation and annihilation, as well as CF-phonon dynamics. Our mean-field calculations, based on a point-charge model, successfully reproduce the overall magnetostriction behavior, revealing the competition between the exchange striction and CF striction. A signature of the CF level crossing is also observed through adiabatic magnetocaloric-effect measurements, consistent with our magnetostriction data. |  |
Winkler, M.; Geirhos, K.; Tyborowski, T.; Tóth, B.; Farkas, D. G.; White, J. S.; Ito, T.; Krohns, S.; Lunkenheimer, P.; Bordács, S.; Kézsmárki, I. Anisotropic magnetocapacitance of antiferromagnetic cycloids in BiFeO3 Journal Article Appl. Phys. Lett. 125, 252902 (2024), datadoi: 10.5281/zenodo.17855050. @article{winklerAnisotropicMagnetocapacitanceAntiferromagnetic2024,
title = {Anisotropic magnetocapacitance of antiferromagnetic cycloids in BiFeO_{3}},
author = {M. Winkler and K. Geirhos and T. Tyborowski and B. Tóth and D. G. Farkas and J. S. White and T. Ito and S. Krohns and P. Lunkenheimer and S. Bordács and I. Kézsmárki},
url = {https://doi.org/10.1063/5.0237659},
doi = {10.1063/5.0237659},
year = {2024},
date = {2024-12-01},
urldate = {2024-12-01},
journal = {Appl. Phys. Lett.},
volume = {125},
number = {25},
pages = {252902},
abstract = {Distinguishing different antiferromagnetic domains by electrical probes is a challenging task, which in itinerant compounds can be achieved, e.g., via the anisotropic magnetoresistance. Here, we demonstrate that in insulators, the anisotropic magnetocapacitance can be exploited for the same purpose. We studied the magnetic field dependence of the dielectric response in BiFeO3, one of the few room-temperature multiferroics. We observed a sizeable dielectric anisotropy upon the rotation of the modulation vector of the antiferromagnetic cycloid in the plane normal to the rhombohedral axis. Importantly, this anisotropy is characteristic of the cycloidal mono-domain state even in zero magnetic field, thus facilitating the determination of the antiferromagnetic domain population. This approach can be utilized to electrically distinguish between antiferromagnetic domains even in complex magnets, such as modulated spin structures, via the magnetodielectric coupling.},
note = {datadoi: 10.5281/zenodo.17855050},
keywords = {A4},
pubstate = {published},
tppubtype = {article}
}
Distinguishing different antiferromagnetic domains by electrical probes is a challenging task, which in itinerant compounds can be achieved, e.g., via the anisotropic magnetoresistance. Here, we demonstrate that in insulators, the anisotropic magnetocapacitance can be exploited for the same purpose. We studied the magnetic field dependence of the dielectric response in BiFeO3, one of the few room-temperature multiferroics. We observed a sizeable dielectric anisotropy upon the rotation of the modulation vector of the antiferromagnetic cycloid in the plane normal to the rhombohedral axis. Importantly, this anisotropy is characteristic of the cycloidal mono-domain state even in zero magnetic field, thus facilitating the determination of the antiferromagnetic domain population. This approach can be utilized to electrically distinguish between antiferromagnetic domains even in complex magnets, such as modulated spin structures, via the magnetodielectric coupling. |  |
Leeb, V.; Knolle, J. Numerical study of quantum oscillations of quasiparticle lifetime: Impurity spectroscopy and electric field and strain effects Journal Article Phys. Rev. B 110, 195143 (2024), datadoi: 10.5281/zenodo.13144810. @article{leebNumericalStudyQuantum2024,
title = {Numerical study of quantum oscillations of quasiparticle lifetime: Impurity spectroscopy and electric field and strain effects},
author = {V. Leeb and J. Knolle},
url = {https://link.aps.org/doi/10.1103/PhysRevB.110.195143},
doi = {10.1103/PhysRevB.110.195143},
year = {2024},
date = {2024-11-21},
urldate = {2024-11-01},
journal = {Phys. Rev. B},
volume = {110},
number = {19},
pages = {195143},
abstract = {Quantum oscillation (QO) measurements constitute one of the most powerful methods for determining the Fermi surface (FS) of metals, exploiting the famous Onsager relation between the FS area and the QO frequency. The recent observation of non-Onsager QOs with a frequency set by the difference of two FS orbits in a bulk three-dimensional metal can be understood as the QO of quasiparticle lifetime (QPL) due to interorbital scattering [N. Huber et al., Nature (London) 621, 276 (2023)]. QPL oscillations (QPLOs) generalize magnetointersubband oscillations known from coupled two-dimensional metals. They may provide a novel tool for extracting otherwise hard-to-measure intraband versus interband scattering times of quasiparticles. Here, we provide a numerical lattice study of QPLOs comparing transport and thermodynamic observables. We explore the effect of different imperfections like general impurities, Hall-effect-induced electric fields, various forms of strain from bending, and magnetic field inhomogeneities. We confirm the basic phenomenology of QPLOs as predicted in analytical calculations and identify additional nonperturbative features. Remarkably, we find that some imperfections can stabilize, or even enhance, non-Onsager QPLOs in contrast to standard QO frequencies. We discuss various avenues for identifying QPLOs in experiments and how to use their dependence on imperfections to extract material properties.},
note = {datadoi: 10.5281/zenodo.13144810},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Quantum oscillation (QO) measurements constitute one of the most powerful methods for determining the Fermi surface (FS) of metals, exploiting the famous Onsager relation between the FS area and the QO frequency. The recent observation of non-Onsager QOs with a frequency set by the difference of two FS orbits in a bulk three-dimensional metal can be understood as the QO of quasiparticle lifetime (QPL) due to interorbital scattering [N. Huber et al., Nature (London) 621, 276 (2023)]. QPL oscillations (QPLOs) generalize magnetointersubband oscillations known from coupled two-dimensional metals. They may provide a novel tool for extracting otherwise hard-to-measure intraband versus interband scattering times of quasiparticles. Here, we provide a numerical lattice study of QPLOs comparing transport and thermodynamic observables. We explore the effect of different imperfections like general impurities, Hall-effect-induced electric fields, various forms of strain from bending, and magnetic field inhomogeneities. We confirm the basic phenomenology of QPLOs as predicted in analytical calculations and identify additional nonperturbative features. Remarkably, we find that some imperfections can stabilize, or even enhance, non-Onsager QPLOs in contrast to standard QO frequencies. We discuss various avenues for identifying QPLOs in experiments and how to use their dependence on imperfections to extract material properties. | |
Abdeldaim, A. H.; Gretarsson, H.; Day, S. J.; Le, M. D.; Stenning, G. B. G.; Manuel, P.; Perry, R. S.; Tsirlin, A. A.; Nilsen, G. J.; Clark, L. Kitaev Interactions Through an Extended Superexchange Pathway in the jeff = 1/2 Ru3+ Honeycomb Magnet RuP3SiO11 Journal Article Nat. Commun. 15, 9778 (2024), datadoi: 10.5281/zenodo.13890183. @article{abdeldaimKitaevInteractionsExtended2024,
title = {Kitaev Interactions Through an Extended Superexchange Pathway in the j_{eff} = 1/2 Ru^{3+} Honeycomb Magnet RuP_{3}SiO_{11}},
author = {A. H. Abdeldaim and H. Gretarsson and S. J. Day and M. D. Le and G. B. G. Stenning and P. Manuel and R. S. Perry and A. A. Tsirlin and G. J. Nilsen and L. Clark},
doi = {10.1038/s41467-024-53900-3},
year = {2024},
date = {2024-11-15},
urldate = {2024-11-01},
journal = {Nat. Commun.},
volume = {15},
number = {1},
pages = {9778},
abstract = {Magnetic materials are composed of the simple building blocks of magnetic moments on a crystal lattice that interact via magnetic exchange. Yet from this simplicity emerges a remarkable diversity of magnetic states. Some reveal the deep quantum mechanical origins of magnetism, for example, quantum spin liquid (QSL) states in which magnetic moments remain disordered at low temperatures despite being strongly correlated through quantum entanglement. A promising theoretical model of a QSL is the Kitaev model, composed of unusual bond-dependent exchange interactions, but experimentally, this model is challenging to realise. Here we show that the material requirements for the Kitaev QSL survive an extended pseudo-edge-sharing superexchange pathway of Ru3+ octahedra within the honeycomb layers of the inorganic framework solid, RuP3SiO11. We confirm the requisite
state of Ru3+ in RuP3SiO11 and resolve the hierarchy of exchange interactions that provide experimental access to an unexplored region of the Kitaev model.},
note = {datadoi: 10.5281/zenodo.13890183},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Magnetic materials are composed of the simple building blocks of magnetic moments on a crystal lattice that interact via magnetic exchange. Yet from this simplicity emerges a remarkable diversity of magnetic states. Some reveal the deep quantum mechanical origins of magnetism, for example, quantum spin liquid (QSL) states in which magnetic moments remain disordered at low temperatures despite being strongly correlated through quantum entanglement. A promising theoretical model of a QSL is the Kitaev model, composed of unusual bond-dependent exchange interactions, but experimentally, this model is challenging to realise. Here we show that the material requirements for the Kitaev QSL survive an extended pseudo-edge-sharing superexchange pathway of Ru3+ octahedra within the honeycomb layers of the inorganic framework solid, RuP3SiO11. We confirm the requisite
state of Ru3+ in RuP3SiO11 and resolve the hierarchy of exchange interactions that provide experimental access to an unexplored region of the Kitaev model. |  |
Adler, D.; Wei, D.; Will, M.; Srakaew, K.; Agrawal, S.; Weckesser, P.; Moessner, R.; Pollmann, F.; Bloch, I.; Zeiher, J. Observation of Hilbert space fragmentation and fractonic excitations in 2D Journal Article Nature 636, 80 (2024), datadoi: 10.17617/3.FPKWEQ. @article{adlerObservationHilbertSpace2024,
title = {Observation of Hilbert space fragmentation and fractonic excitations in 2D},
author = {D. Adler and D. Wei and M. Will and K. Srakaew and S. Agrawal and P. Weckesser and R. Moessner and F. Pollmann and I. Bloch and J. Zeiher},
url = {https://doi.org/10.1038/s41586-024-08188-0},
doi = {10.1038/s41586-024-08188-0},
year = {2024},
date = {2024-11-13},
urldate = {2024-11-01},
journal = {Nature},
volume = {636},
number = {8041},
pages = {80},
abstract = {The relaxation behaviour of isolated quantum systems taken out of equilibrium is among the most intriguing questions in many-body physics1. Quantum systems out of equilibrium typically relax to thermal equilibrium states by scrambling local information and building up entanglement entropy. However, kinetic constraints in the Hamiltonian can lead to a breakdown of this fundamental paradigm owing to a fragmentation of the underlying Hilbert space into dynamically decoupled subsectors in which thermalization can be strongly suppressed2–5. Here we experimentally observe Hilbert space fragmentation in a two-dimensional tilted Bose–Hubbard model. Using quantum gas microscopy, we engineer a wide variety of initial states and find a rich set of manifestations of Hilbert space fragmentation involving bulk states, interfaces and defects, that is, two-, one- and zero-dimensional objects. Specifically, uniform initial states with equal particle number and energy differ strikingly in their relaxation dynamics. Inserting controlled defects on top of a global, non-thermalizing chequerboard state, we observe highly anisotropic, subdimensional dynamics, an immediate signature of their fractonic nature6–9. An interface between localized and thermalizing states in turn shows dynamics depending on its orientation. Our results mark the observation of Hilbert space fragmentation beyond one dimension, as well as the concomitant direct observation of fractons, and pave the way for in-depth studies of microscopic transport phenomena in constrained systems.},
note = {datadoi: 10.17617/3.FPKWEQ},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
The relaxation behaviour of isolated quantum systems taken out of equilibrium is among the most intriguing questions in many-body physics1. Quantum systems out of equilibrium typically relax to thermal equilibrium states by scrambling local information and building up entanglement entropy. However, kinetic constraints in the Hamiltonian can lead to a breakdown of this fundamental paradigm owing to a fragmentation of the underlying Hilbert space into dynamically decoupled subsectors in which thermalization can be strongly suppressed2–5. Here we experimentally observe Hilbert space fragmentation in a two-dimensional tilted Bose–Hubbard model. Using quantum gas microscopy, we engineer a wide variety of initial states and find a rich set of manifestations of Hilbert space fragmentation involving bulk states, interfaces and defects, that is, two-, one- and zero-dimensional objects. Specifically, uniform initial states with equal particle number and energy differ strikingly in their relaxation dynamics. Inserting controlled defects on top of a global, non-thermalizing chequerboard state, we observe highly anisotropic, subdimensional dynamics, an immediate signature of their fractonic nature6–9. An interface between localized and thermalizing states in turn shows dynamics depending on its orientation. Our results mark the observation of Hilbert space fragmentation beyond one dimension, as well as the concomitant direct observation of fractons, and pave the way for in-depth studies of microscopic transport phenomena in constrained systems. |  |
Kamenskyi, D.; Vasin, K.; Prodan, L.; Kutko, K.; Khrustalyov, V.; Pavlov, S. G.; Hübers, H. -W. Terahertz Resonant Emission by Optically Excited Infrared-Active Shear Phonons in KY(MoO4)2 Journal Article Adv. Sci. 12, 2407028 (2024). @article{kamenskyi_terahertz_2024,
title = {Terahertz Resonant Emission by Optically Excited Infrared-Active Shear Phonons in KY(MoO_{4})_{2}},
author = {D. Kamenskyi and K. Vasin and L. Prodan and K. Kutko and V. Khrustalyov and S. G. Pavlov and H. -W. Hübers},
url = {https://advanced.onlinelibrary.wiley.com/doi/abs/10.1002/advs.202407028},
doi = {10.1002/advs.202407028},
year = {2024},
date = {2024-11-13},
urldate = {2024-11-01},
journal = {Adv. Sci.},
volume = {12},
number = {2},
pages = {2407028},
abstract = {Abstract The generation of monochromatic electromagnetic radiation in the terahertz (THz) frequency range has remained a challenging task for many decades. Here, the emission of monochromatic sub-THz radiation by optical phonons in the dielectric material KY(MoO4)2 is demonstrated. The layered crystal structure of KY(MoO4)2 causes infrared-active shear lattice vibrations to have energies below 3.7 meV, corresponding to frequencies lower than 900 GHz where solid-state-based monochromatic radiation sources are rare. Directly excited by a 5 ps long broadband THz pulse, infrared-active optical vibrations in KY(MoO4)2 re-emit narrowband sub-THz radiation as a time-varying dipole for tens of picoseconds, which is exceptionally long for oscillators with frequencies below 1 THz. Such a long coherent emission allows for the detection of more than 50 periods of radiation with frequencies of 568 and 860 GHz. The remarkably long decay time together with the chemical stability of the employed material suggests a variety of possible applications in THz technology.},
keywords = {C4},
pubstate = {published},
tppubtype = {article}
}
Abstract The generation of monochromatic electromagnetic radiation in the terahertz (THz) frequency range has remained a challenging task for many decades. Here, the emission of monochromatic sub-THz radiation by optical phonons in the dielectric material KY(MoO4)2 is demonstrated. The layered crystal structure of KY(MoO4)2 causes infrared-active shear lattice vibrations to have energies below 3.7 meV, corresponding to frequencies lower than 900 GHz where solid-state-based monochromatic radiation sources are rare. Directly excited by a 5 ps long broadband THz pulse, infrared-active optical vibrations in KY(MoO4)2 re-emit narrowband sub-THz radiation as a time-varying dipole for tens of picoseconds, which is exceptionally long for oscillators with frequencies below 1 THz. Such a long coherent emission allows for the detection of more than 50 periods of radiation with frequencies of 568 and 860 GHz. The remarkably long decay time together with the chemical stability of the employed material suggests a variety of possible applications in THz technology. |  |
Langmann, J.; Eickerling, G.; Prodan, L.; Tsirlin, A. A.; Winkler, M.; Bordács, S.; Tsurkan, V.; Kézsmárki, I. Atomic-Scale Polar Helix in Inorganic Crystals Journal Article Chem. Mater. 36, 11180–11188 (2024). @article{langmann_atomic-scale_2024,
title = {Atomic-Scale Polar Helix in Inorganic Crystals},
author = {J. Langmann and G. Eickerling and L. Prodan and A. A. Tsirlin and M. Winkler and S. Bordács and V. Tsurkan and I. Kézsmárki},
url = {https://doi.org/10.1021/acs.chemmater.4c02060},
doi = {10.1021/acs.chemmater.4c02060},
year = {2024},
date = {2024-11-04},
urldate = {2024-11-01},
journal = {Chem. Mater.},
volume = {36},
number = {22},
pages = {11180–11188},
abstract = {Chiral structures, noncentrosymmetric objects with a given handedness, emerge on all scales in nature. The most well-known chiral form, the helix, has numerous materializations not only on the microscopic scale (DNA, cholesteric liquid crystals, and spin helices) but also on macroscopic and even cosmological scales. The ongoing quest for new types of chiral structures is fueled by a wide range of fascinating phenomena observed in chiral materials, such as nonreciprocal transport and optical processes, electro-optical effects, and chiral amplification and induction. Here, we report a novel route to chirality in antipolar GaTa4Se8 crystals, where the rotation of the electric polarization vector through the unit cell traces out a helix. The determination of atomic positions using X-ray diffraction combined with ab initio calculations reveals that quasi-molecular Ta4Se4 clusters distort upon a phase transition and evoke significant local electric polarization within structural layers of the unit cell. This polarization is found to rotate in 90° steps between neighboring layers, either clockwise or anticlockwise. A similar analysis performed on two archetypal chiral compounds, α-quartz and tellurium, implies that antipolar crystals with screw-axis symmetry may generally host atomic-scale polarization helices with emergent functionalities.},
keywords = {A4, B1},
pubstate = {published},
tppubtype = {article}
}
Chiral structures, noncentrosymmetric objects with a given handedness, emerge on all scales in nature. The most well-known chiral form, the helix, has numerous materializations not only on the microscopic scale (DNA, cholesteric liquid crystals, and spin helices) but also on macroscopic and even cosmological scales. The ongoing quest for new types of chiral structures is fueled by a wide range of fascinating phenomena observed in chiral materials, such as nonreciprocal transport and optical processes, electro-optical effects, and chiral amplification and induction. Here, we report a novel route to chirality in antipolar GaTa4Se8 crystals, where the rotation of the electric polarization vector through the unit cell traces out a helix. The determination of atomic positions using X-ray diffraction combined with ab initio calculations reveals that quasi-molecular Ta4Se4 clusters distort upon a phase transition and evoke significant local electric polarization within structural layers of the unit cell. This polarization is found to rotate in 90° steps between neighboring layers, either clockwise or anticlockwise. A similar analysis performed on two archetypal chiral compounds, α-quartz and tellurium, implies that antipolar crystals with screw-axis symmetry may generally host atomic-scale polarization helices with emergent functionalities. |  |
Jin, H. -K.; Knolle, J. Floquet Prethermal Order by Disorder Journal Article Phys. Rev. Research 6, L042033 (2024). @article{jin_floquet_2024,
title = {Floquet Prethermal Order by Disorder},
author = {H. -K. Jin and J. Knolle},
url = {https://journals.aps.org/prresearch/abstract/10.1103/PhysRevResearch.6.L042033},
doi = {10.1103/PhysRevResearch.6.L042033},
year = {2024},
date = {2024-11-04},
urldate = {2024-11-01},
journal = {Phys. Rev. Research},
volume = {6},
pages = {L042033},
abstract = {Frustrated magnets can have accidental ground state degeneracies which may be lifted by various forms of disorder, for example in the form of thermal or quantum fluctuations. This order by disorder (ObD) paradigm is well established in equilibrium and here is generalized to Floquet many-body systems. Investigating a periodically-driven XXZ-compass model on the square lattice, we show that in a prethermal regime, dynamical fluctuations induced by high-frequency drives select a discrete set of states out of a degenerate ground state manifold of the lowest order Floquet Hamiltonian chosen as initial states. Remarkably, prior to the ObD selection, an unusual fluctuating regime emerges leading to a prethermalization timescale scaling linearly with the drive frequency. We argue that prethermal ObD with its unusual approach to the selected states is a generic phenomenon of driven frustrated systems and confirm it in the paradigmatic $J_1-J_2$ XX model.},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
Frustrated magnets can have accidental ground state degeneracies which may be lifted by various forms of disorder, for example in the form of thermal or quantum fluctuations. This order by disorder (ObD) paradigm is well established in equilibrium and here is generalized to Floquet many-body systems. Investigating a periodically-driven XXZ-compass model on the square lattice, we show that in a prethermal regime, dynamical fluctuations induced by high-frequency drives select a discrete set of states out of a degenerate ground state manifold of the lowest order Floquet Hamiltonian chosen as initial states. Remarkably, prior to the ObD selection, an unusual fluctuating regime emerges leading to a prethermalization timescale scaling linearly with the drive frequency. We argue that prethermal ObD with its unusual approach to the selected states is a generic phenomenon of driven frustrated systems and confirm it in the paradigmatic $J_1-J_2$ XX model. |  |
Radhakrishnan, P.; Rabinovich, K. S.; Boris, A. V.; Fürsich, K.; Minola, M.; Christiani, G.; Logvenov, G.; Keimer, B.; Benckiser, E. Imprinted atomic displacements drive spin–orbital order in a vanadate perovskite Journal Article Nat. Phys. 21, 126 (2024), datadoi: 10.17617/3.YPXUG0. @article{radhakrishnanImprintedAtomicDisplacements2024,
title = {Imprinted atomic displacements drive spin–orbital order in a vanadate perovskite},
author = {P. Radhakrishnan and K. S. Rabinovich and A. V. Boris and K. Fürsich and M. Minola and G. Christiani and G. Logvenov and B. Keimer and E. Benckiser},
url = {https://doi.org/10.1038/s41567-024-02686-8},
doi = {10.1038/s41567-024-02686-8},
year = {2024},
date = {2024-10-29},
urldate = {2024-10-01},
journal = {Nat. Phys.},
volume = {21},
number = {1},
pages = {126},
abstract = {Perovskites with the generic composition ABO3 exhibit an enormous variety of quantum states, such as orbital order, magnetism and superconductivity. Their flexible and comparatively simple structure allows for straightforward chemical substitution and cube-on-cube combination of different compounds in atomically sharp epitaxial heterostructures. Many of the diverse physical properties of perovskites are determined by small deviations from the ideal cubic perovskite structure, which are challenging to control. Here we show that directional imprinting of atomic displacements in the antiferromagnetic Mott insulator YVO3 can be achieved by depositing epitaxial films on different facets of the same isostructural substrate. These facets were chosen such that other well-known control parameters, including lattice and polarity mismatch with the overlayer, remain nearly unchanged. We observe signatures of staggered orbital and magnetic order and demonstrate distinct spin–orbital ordering patterns on different facets. We attribute these results to the influence of specific octahedral rotation and cation displacement patterns, which are imprinted by the substrate facet, on the covalency of the bonds and the superexchange interactions in YVO3. Our results show that substrate-induced templating of lattice distortion patterns constitutes a pathway for materials design beyond established strain-engineering strategies.},
note = {datadoi: 10.17617/3.YPXUG0},
keywords = {B2},
pubstate = {published},
tppubtype = {article}
}
Perovskites with the generic composition ABO3 exhibit an enormous variety of quantum states, such as orbital order, magnetism and superconductivity. Their flexible and comparatively simple structure allows for straightforward chemical substitution and cube-on-cube combination of different compounds in atomically sharp epitaxial heterostructures. Many of the diverse physical properties of perovskites are determined by small deviations from the ideal cubic perovskite structure, which are challenging to control. Here we show that directional imprinting of atomic displacements in the antiferromagnetic Mott insulator YVO3 can be achieved by depositing epitaxial films on different facets of the same isostructural substrate. These facets were chosen such that other well-known control parameters, including lattice and polarity mismatch with the overlayer, remain nearly unchanged. We observe signatures of staggered orbital and magnetic order and demonstrate distinct spin–orbital ordering patterns on different facets. We attribute these results to the influence of specific octahedral rotation and cation displacement patterns, which are imprinted by the substrate facet, on the covalency of the bonds and the superexchange interactions in YVO3. Our results show that substrate-induced templating of lattice distortion patterns constitutes a pathway for materials design beyond established strain-engineering strategies. |  |
Shen, B.; Breitner, F.; Gegenwart, P.; Jesche, A. Strong Enhancement of Magnetic Coercivity Induced by Uniaxial Stress Journal Article Phys. Rev. Lett. 133, 186702 (2024), datadoi: 10.5281/zenodo.10972989. @article{shenStrongEnhancementMagnetic2024,
title = {Strong Enhancement of Magnetic Coercivity Induced by Uniaxial Stress},
author = {B. Shen and F. Breitner and P. Gegenwart and A. Jesche},
doi = {10.1103/PhysRevLett.133.186702},
year = {2024},
date = {2024-10-28},
urldate = {2024-10-01},
journal = {Phys. Rev. Lett.},
volume = {133},
number = {18},
pages = {186702},
abstract = {The performance of permanent magnets is intricately tied to their magnetic hysteresis loop. In this study, we investigate the heavy-fermion ferromagnet CeAgSb2 through magnetization measurements under uniaxial stress. We observe a 2400% increase in magnetic coercivity with just a modest stress of approximately 1 kbar. This effect persists even after pressure release, attributable to stress-induced defects that efficiently pin domain walls. Other magnetic properties such as ordering temperature and saturation moment exhibit only weak pressure dependencies and display full reversibility. Our findings offer a promising route for increasing coercive field strength and enhancing the energy product in ferromagnetic materials and are potentially applicable to a broad spectrum of commercial or emerging magnetic applications.},
note = {datadoi: 10.5281/zenodo.10972989},
keywords = {B1, B3},
pubstate = {published},
tppubtype = {article}
}
The performance of permanent magnets is intricately tied to their magnetic hysteresis loop. In this study, we investigate the heavy-fermion ferromagnet CeAgSb2 through magnetization measurements under uniaxial stress. We observe a 2400% increase in magnetic coercivity with just a modest stress of approximately 1 kbar. This effect persists even after pressure release, attributable to stress-induced defects that efficiently pin domain walls. Other magnetic properties such as ordering temperature and saturation moment exhibit only weak pressure dependencies and display full reversibility. Our findings offer a promising route for increasing coercive field strength and enhancing the energy product in ferromagnetic materials and are potentially applicable to a broad spectrum of commercial or emerging magnetic applications. |  |
Davenport, H.; Knolle, J.; Schindler, F. Interaction-Induced Crystalline Topology of Excitons Journal Article Phys. Rev. Lett. 133, 176601 (2024). @article{davenport_interaction-induced_2024,
title = {Interaction-Induced Crystalline Topology of Excitons},
author = {H. Davenport and J. Knolle and F. Schindler},
url = {https://link.aps.org/doi/10.1103/PhysRevLett.133.176601},
doi = {10.1103/PhysRevLett.133.176601},
year = {2024},
date = {2024-10-21},
urldate = {2024-10-01},
journal = {Phys. Rev. Lett.},
volume = {133},
number = {17},
pages = {176601},
abstract = {We apply the topological theory of symmetry indicators to interaction-induced exciton band structures in centrosymmetric semiconductors. Crucially, we distinguish between the topological invariants inherited from the underlying electron and hole bands and those that are intrinsic to the exciton wave function itself. Focusing on the latter, we show that there exists a class of exciton bands for which the maximally localized exciton Wannier states are shifted with respect to the electronic Wannier states by a quantized amount; we call these excitons shift excitons. Our analysis explains how the exciton spectrum can be topologically nontrivial and sustain exciton edge states in open boundary conditions even when the underlying noninteracting bands have a trivial atomic limit. We demonstrate the presence of shift excitons as the lowest energy neutral excitations of the Su-Schrieffer-Heeger model in its trivial phase when supplemented by local two-body interactions.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
We apply the topological theory of symmetry indicators to interaction-induced exciton band structures in centrosymmetric semiconductors. Crucially, we distinguish between the topological invariants inherited from the underlying electron and hole bands and those that are intrinsic to the exciton wave function itself. Focusing on the latter, we show that there exists a class of exciton bands for which the maximally localized exciton Wannier states are shifted with respect to the electronic Wannier states by a quantized amount; we call these excitons shift excitons. Our analysis explains how the exciton spectrum can be topologically nontrivial and sustain exciton edge states in open boundary conditions even when the underlying noninteracting bands have a trivial atomic limit. We demonstrate the presence of shift excitons as the lowest energy neutral excitations of the Su-Schrieffer-Heeger model in its trivial phase when supplemented by local two-body interactions. | |
Mukharjee, P. K.; Shen, B.; Erdmann, S.; Jesche, A.; Kaiser, J.; Baral, P. R.; Zaharko, O.; Gegenwart, P.; Tsirlin, A. A. Intermediate field-induced phase of the honeycomb magnet BaCo2(AsO4)2 Journal Article Phys. Rev. B 110, L140407 (2024), datadoi: 10.5281/zenodo.10721313. @article{mukharjeeIntermediateFieldinducedPhase2024a,
title = {Intermediate field-induced phase of the honeycomb magnet BaCo_{2}(AsO_{4})_{2}},
author = {P. K. Mukharjee and B. Shen and S. Erdmann and A. Jesche and J. Kaiser and P. R. Baral and O. Zaharko and P. Gegenwart and A. A. Tsirlin},
doi = {10.1103/PhysRevB.110.L140407},
year = {2024},
date = {2024-10-21},
urldate = {2024-10-01},
journal = {Phys. Rev. B},
volume = {110},
number = {14},
pages = {L140407},
abstract = {We use magnetometry, calorimetry, and high-resolution capacitive dilatometry, as well as single-crystal neutron diffraction to explore the temperature-field phase diagram of the anisotropic honeycomb magnet BaCo2(AsO4)2. Our data reveal four distinct ordered states observed for in-plane magnetic fields. Of particular interest is the narrow region between 0.51 and 0.54 T that separates the up-up-down order from the fully polarized state and coincides with the field range where signatures of the spin-liquid behavior have been reported. We show that magnetic Bragg peaks persist in this intermediate phase, thus ruling out its spin-liquid nature. However, the simultaneous nonmonotonic evolution of nuclear Bragg peaks suggests the involvement of the lattice, witnessed also in other regions of the phase diagram where large changes in the sample length are observed upon entering the magnetically ordered states. Our data highlight the importance of lattice effects in BaCo2(AsO4)2.},
note = {datadoi: 10.5281/zenodo.10721313},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
We use magnetometry, calorimetry, and high-resolution capacitive dilatometry, as well as single-crystal neutron diffraction to explore the temperature-field phase diagram of the anisotropic honeycomb magnet BaCo2(AsO4)2. Our data reveal four distinct ordered states observed for in-plane magnetic fields. Of particular interest is the narrow region between 0.51 and 0.54 T that separates the up-up-down order from the fully polarized state and coincides with the field range where signatures of the spin-liquid behavior have been reported. We show that magnetic Bragg peaks persist in this intermediate phase, thus ruling out its spin-liquid nature. However, the simultaneous nonmonotonic evolution of nuclear Bragg peaks suggests the involvement of the lattice, witnessed also in other regions of the phase diagram where large changes in the sample length are observed upon entering the magnetically ordered states. Our data highlight the importance of lattice effects in BaCo2(AsO4)2. |  |
Birnkammer, S.; Knolle, J.; Knap, M. Signatures of domain-wall confinement in Raman spectroscopy of Ising spin chains Journal Article Phys. Rev. B 110, 134408 (2024), datadoi: 10.5281/zenodo.8252835. @article{birnkammerSignaturesDomainwallConfinement2024a,
title = {Signatures of domain-wall confinement in Raman spectroscopy of Ising spin chains},
author = {S. Birnkammer and J. Knolle and M. Knap},
url = {https://link.aps.org/doi/10.1103/PhysRevB.110.134408},
doi = {10.1103/PhysRevB.110.134408},
year = {2024},
date = {2024-10-03},
urldate = {2024-10-01},
journal = {Phys. Rev. B},
volume = {110},
number = {13},
pages = {134408},
abstract = {Mesonic bound states of domain walls (DWs) can be stabilized in quasi-one-dimensional magnetic compounds. Here, we theoretically study the Raman light scattering response of a twisted Kitaev chain with tilted magnetic fields as a minimal model for confinement in CoNb2O6. By both numerical matrix product states and few-DW variational states, we show that confinement-induced bound states directly manifest themselves as sharp peaks in the Raman response. Remarkably, by tuning the polarization of the incident light field, we demonstrate that the Raman response offers insights into the intrinsic symmetry of the bound-state wave function.},
note = {datadoi: 10.5281/zenodo.8252835},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
Mesonic bound states of domain walls (DWs) can be stabilized in quasi-one-dimensional magnetic compounds. Here, we theoretically study the Raman light scattering response of a twisted Kitaev chain with tilted magnetic fields as a minimal model for confinement in CoNb2O6. By both numerical matrix product states and few-DW variational states, we show that confinement-induced bound states directly manifest themselves as sharp peaks in the Raman response. Remarkably, by tuning the polarization of the incident light field, we demonstrate that the Raman response offers insights into the intrinsic symmetry of the bound-state wave function. |  |
Säubert, S.; Franz, C.; Jochum, J. K.; Benka, G.; Bauer, A.; Shapiro, S. M.; Böni, P.; Pfleiderer, C. Evolution of spin dynamics during freezing in the spin-glass FexCr1-x Journal Article Phys. Rev. B 110, 094422 (2024). @article{saubert_evolution_2024,
title = {Evolution of spin dynamics during freezing in the spin-glass Fe_{x}Cr_{1-x}},
author = {S. Säubert and C. Franz and J. K. Jochum and G. Benka and A. Bauer and S. M. Shapiro and P. Böni and C. Pfleiderer},
doi = {10.1103/PhysRevB.110.094422},
year = {2024},
date = {2024-09-13},
urldate = {2024-09-13},
journal = {Phys. Rev. B},
volume = {110},
number = {9},
pages = {094422},
abstract = {In the iron–chromium system, Fe𝑥Cr1−𝑥, a wide dome of spin-glass behavior emerges when the ferromagnetism of iron is suppressed and the antiferromagnetism of chromium emerges as a function of increasing iron content 𝑥. As both, the high-temperature state and the characteristic cluster size vary as a function of 𝑥, different regimes of spin-glass behavior may be compared in a single, isostructural material system. Here, we report a study of the spin dynamics across the freezing process into the spin-glass state for different iron concentrations (𝑥=0.145, 0.175, 0.21) using modulation of intensity with zero effort (MIEZE) spectroscopy. In the parameter range studied, the relaxation process observed experimentally may be described well in terms of a stretched exponential. In the reentrant cluster-glass regime, 𝑥=0.145, this behavior persists up to high temperatures. In comparison, in the superparamagnetic regime, 𝑥=0.175 and 𝑥=0.21, a single relaxation time at elevated temperatures is observed. For all samples studied, the spin relaxation exhibits a momentum dependence consistent with a power law, providing evidence of a dispersive character of the spin relaxation.},
keywords = {C1, C3},
pubstate = {published},
tppubtype = {article}
}
In the iron–chromium system, Fe𝑥Cr1−𝑥, a wide dome of spin-glass behavior emerges when the ferromagnetism of iron is suppressed and the antiferromagnetism of chromium emerges as a function of increasing iron content 𝑥. As both, the high-temperature state and the characteristic cluster size vary as a function of 𝑥, different regimes of spin-glass behavior may be compared in a single, isostructural material system. Here, we report a study of the spin dynamics across the freezing process into the spin-glass state for different iron concentrations (𝑥=0.145, 0.175, 0.21) using modulation of intensity with zero effort (MIEZE) spectroscopy. In the parameter range studied, the relaxation process observed experimentally may be described well in terms of a stretched exponential. In the reentrant cluster-glass regime, 𝑥=0.145, this behavior persists up to high temperatures. In comparison, in the superparamagnetic regime, 𝑥=0.175 and 𝑥=0.21, a single relaxation time at elevated temperatures is observed. For all samples studied, the spin relaxation exhibits a momentum dependence consistent with a power law, providing evidence of a dispersive character of the spin relaxation. |  |
Hofmeier, D.; Willsher, J.; Seifert, U. F. P.; Knolle, J. Spin-Peierls instability of deconfined quantum critical points Journal Article Phys. Rev. B 110, 125130 (2024). @article{hofmeier_spin-peierls_2024,
title = {Spin-Peierls instability of deconfined quantum critical points},
author = {D. Hofmeier and J. Willsher and U. F. P. Seifert and J. Knolle},
url = {https://link.aps.org/doi/10.1103/PhysRevB.110.125130},
doi = {10.1103/PhysRevB.110.125130},
year = {2024},
date = {2024-09-13},
urldate = {2024-09-01},
journal = {Phys. Rev. B},
volume = {110},
number = {12},
pages = {125130},
abstract = {Deconfined quantum critical points (DQCPs) are putative phase transitions beyond the Landau paradigm with emergent fractionalized degrees of freedom. The original example of a DQCP is the spin-1/2 quantum antiferromagnet on the square lattice which features a second-order transition between valence bond solid (VBS) and Néel order. The VBS order breaks a lattice symmetry, and the corresponding VBS order parameter may couple to lattice distortion modes (phonons) at appropriate momenta. We investigate a field-theoretic description of the DQCP in the presence of such a spin-lattice coupling. We show that treating phonons as classical lattice distortions leads to a relevant monopole-phonon interaction inducing an instability towards a distorted lattice by an analogous mechanism to the spin-Peierls instability in one dimension. Consequently, there is a breakdown of the DQCP which generally becomes a strong first-order transition. Taking into account the full quantum nature of the phonons, we argue that the continuous DQCP persists above a critical phonon frequency. Lastly, we comment on the connection to general gapless, deconfined gauge theories.},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Deconfined quantum critical points (DQCPs) are putative phase transitions beyond the Landau paradigm with emergent fractionalized degrees of freedom. The original example of a DQCP is the spin-1/2 quantum antiferromagnet on the square lattice which features a second-order transition between valence bond solid (VBS) and Néel order. The VBS order breaks a lattice symmetry, and the corresponding VBS order parameter may couple to lattice distortion modes (phonons) at appropriate momenta. We investigate a field-theoretic description of the DQCP in the presence of such a spin-lattice coupling. We show that treating phonons as classical lattice distortions leads to a relevant monopole-phonon interaction inducing an instability towards a distorted lattice by an analogous mechanism to the spin-Peierls instability in one dimension. Consequently, there is a breakdown of the DQCP which generally becomes a strong first-order transition. Taking into account the full quantum nature of the phonons, we argue that the continuous DQCP persists above a critical phonon frequency. Lastly, we comment on the connection to general gapless, deconfined gauge theories. |  |
Prodan, L.; Chmeruk, A.; Chioncel, L.; Tsurkan, V.; Kézsmárki, I. Anisotropic charge transport in the easy-plane kagome ferromagnet Fe3Sn Journal Article Phys. Rev. B 110, 094407 (2024). @article{prodan_anisotropic_2024,
title = {Anisotropic charge transport in the easy-plane kagome ferromagnet Fe_{3}Sn},
author = {L. Prodan and A. Chmeruk and L. Chioncel and V. Tsurkan and I. Kézsmárki},
doi = {10.1103/PhysRevB.110.094407},
year = {2024},
date = {2024-09-05},
urldate = {2024-09-05},
journal = {Phys. Rev. B},
volume = {110},
number = {9},
pages = {094407},
abstract = {We report on the anisotropic electronic properties of the metallic kagome ferromagnet , as revealed by magnetotransport studies on single-crystalline samples and material-specific ab initio calculations. The longitudinal resistivity shows a remarkable anisotropy, where surprisingly the resistivity perpendicular to the kagome planes is about three times lower than the in-plane resistivity (𝜌𝑥𝑥). The ordinary Hall constants are negative for the magnetic field applied parallel to the 𝐇||𝐜 and positive for 𝐇||𝐚, indicating the coexistence of electron- and hole-like carriers at the Fermi surface. The anomalous Hall resistivity (𝜌𝐴𝑖𝑗) shows large values over a wide temperature range and exhibits a significant anisotropy ratio (𝜌𝑥𝑦/𝜌𝑧𝑦), with 𝜌𝑥𝑦 =8 µΩcm and 𝜌𝑧𝑦 =3.2 µΩcm at room temperature. Our study reveals that the anisotropy ratio scales almost linearly with the magnetocrystalline anisotropy constant (𝐾𝑢) over a broad temperature range (2 K ≤ T ≤ 300 K), indicating that spin-orbit coupling is the underlying mechanism driving both the anisotropic transport properties and the magnetocrystalline anisotropy energy. Material-specific ab initio calculations further demonstrate that the magnetic reconstruction of bands near the Fermi level, induced by the spin-orbit coupling, is predominantly responsible for the anisotropic behavior of the Berry curvature and, consequently, the large anomalous Hall effect observed in Fe3Sn. These results provide valuable insight into the complex interplay between charge transport and magnetism in kagome magnets, emphasizing the strong manifestation of spin-orbit coupling on kagome lattices.},
keywords = {A1, A5},
pubstate = {published},
tppubtype = {article}
}
We report on the anisotropic electronic properties of the metallic kagome ferromagnet , as revealed by magnetotransport studies on single-crystalline samples and material-specific ab initio calculations. The longitudinal resistivity shows a remarkable anisotropy, where surprisingly the resistivity perpendicular to the kagome planes is about three times lower than the in-plane resistivity (𝜌𝑥𝑥). The ordinary Hall constants are negative for the magnetic field applied parallel to the 𝐇||𝐜 and positive for 𝐇||𝐚, indicating the coexistence of electron- and hole-like carriers at the Fermi surface. The anomalous Hall resistivity (𝜌𝐴𝑖𝑗) shows large values over a wide temperature range and exhibits a significant anisotropy ratio (𝜌𝑥𝑦/𝜌𝑧𝑦), with 𝜌𝑥𝑦 =8 µΩcm and 𝜌𝑧𝑦 =3.2 µΩcm at room temperature. Our study reveals that the anisotropy ratio scales almost linearly with the magnetocrystalline anisotropy constant (𝐾𝑢) over a broad temperature range (2 K ≤ T ≤ 300 K), indicating that spin-orbit coupling is the underlying mechanism driving both the anisotropic transport properties and the magnetocrystalline anisotropy energy. Material-specific ab initio calculations further demonstrate that the magnetic reconstruction of bands near the Fermi level, induced by the spin-orbit coupling, is predominantly responsible for the anisotropic behavior of the Berry curvature and, consequently, the large anomalous Hall effect observed in Fe3Sn. These results provide valuable insight into the complex interplay between charge transport and magnetism in kagome magnets, emphasizing the strong manifestation of spin-orbit coupling on kagome lattices. |  |
Jin, H. -K.; Kadow, W.; Knap, M.; Knolle, J. Kinetic ferromagnetism and topological magnons of the hole-doped Kitaev spin liquid Journal Article npj Quantum Mater. 9, 65 (2024), datadoi: (10.5281/zenodo.8370778). @article{jinKineticFerromagnetismTopological2024,
title = {Kinetic ferromagnetism and topological magnons of the hole-doped Kitaev spin liquid},
author = {H. -K. Jin and W. Kadow and M. Knap and J. Knolle},
doi = {10.1038/s41535-024-00678-8},
year = {2024},
date = {2024-09-04},
urldate = {2024-09-01},
journal = {npj Quantum Mater.},
volume = {9},
number = {1},
pages = {65},
abstract = {We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange K the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group simulations on finite systems, we uncover that the introduction of a single hole, corresponding to ≈1% hole doping for the system size we consider, with a hopping strength of just t textasciitilde 0.28K is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic exchange Γ drives the polarization towards the [111] direction via a transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental implications for Kitaev candidate materials.},
note = {datadoi: (10.5281/zenodo.8370778)},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange K the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group simulations on finite systems, we uncover that the introduction of a single hole, corresponding to ≈1% hole doping for the system size we consider, with a hopping strength of just t textasciitilde 0.28K is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic exchange Γ drives the polarization towards the [111] direction via a transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental implications for Kitaev candidate materials. |  |
Chen, L.; Sun, Y.; Mankovsky, S.; Meier, T. N. G.; Kronseder, M.; Sun, C.; Orekhov, A.; Ebert, H.; Weiss, D.; Back, C. H. Signatures of magnetism control by flow of angular momentum Journal Article Nature 633, 548–553 (2024), datadoi: 10.17605/OSF.IO/RZMUJ. @article{chenSignaturesMagnetismControl2024,
title = {Signatures of magnetism control by flow of angular momentum},
author = {L. Chen and Y. Sun and S. Mankovsky and T. N. G. Meier and M. Kronseder and C. Sun and A. Orekhov and H. Ebert and D. Weiss and C. H. Back},
doi = {10.1038/s41586-024-07914-y},
issn = {1476-4687},
year = {2024},
date = {2024-09-04},
urldate = {2024-09-01},
journal = {Nature},
volume = {633},
number = {8030},
pages = {548–553},
abstract = {Exploring new strategies to manipulate the order parameter of magnetic materials by electrical means is of great importance not only for advancing our understanding of fundamental magnetism but also for unlocking potential applications. A well-established concept uses gate voltages to control magnetic properties by modulating the carrier population in a capacitor structure1–5. Here we show that, in Pt/Al/Fe/GaAs(001) multilayers, the application of an in-plane charge current in Pt leads to a shift in the ferromagnetic resonance field depending on the microwave frequency when the Fe film is sufficiently thin. The experimental observation is interpreted as a current-induced modification of the magnetocrystalline anisotropy ΔHA of Fe. We show that (1) ΔHA decreases with increasing Fe film thickness and is connected to the damping-like torque; and (2) ΔHA depends not only on the polarity of charge current but also on the magnetization direction, that is, ΔHA has an opposite sign when the magnetization direction is reversed. The symmetry of the modification is consistent with a current-induced spin6–8 and/or orbit9–13 accumulation, which, respectively, act on the spin and/or orbit component of the magnetization. In this study, as Pt is regarded as a typical spin current source6,14, the spin current can play a dominant part. The control of magnetism by a spin current results from the modified exchange splitting of the majority and minority spin bands, providing functionality that was previously unknown and could be useful in advanced spintronic devices.},
note = {datadoi: 10.17605/OSF.IO/RZMUJ},
keywords = {A2},
pubstate = {published},
tppubtype = {article}
}
Exploring new strategies to manipulate the order parameter of magnetic materials by electrical means is of great importance not only for advancing our understanding of fundamental magnetism but also for unlocking potential applications. A well-established concept uses gate voltages to control magnetic properties by modulating the carrier population in a capacitor structure1–5. Here we show that, in Pt/Al/Fe/GaAs(001) multilayers, the application of an in-plane charge current in Pt leads to a shift in the ferromagnetic resonance field depending on the microwave frequency when the Fe film is sufficiently thin. The experimental observation is interpreted as a current-induced modification of the magnetocrystalline anisotropy ΔHA of Fe. We show that (1) ΔHA decreases with increasing Fe film thickness and is connected to the damping-like torque; and (2) ΔHA depends not only on the polarity of charge current but also on the magnetization direction, that is, ΔHA has an opposite sign when the magnetization direction is reversed. The symmetry of the modification is consistent with a current-induced spin6–8 and/or orbit9–13 accumulation, which, respectively, act on the spin and/or orbit component of the magnetization. In this study, as Pt is regarded as a typical spin current source6,14, the spin current can play a dominant part. The control of magnetism by a spin current results from the modified exchange splitting of the majority and minority spin bands, providing functionality that was previously unknown and could be useful in advanced spintronic devices. |  |
Kirchner, N.; Choi, W.; Pollmann, F. Characterizing the entanglement of anyonic systems using the anyonic partial transpose Journal Article Phys. Rev. B 110, 085143 (2024), datadoi: 10.5281/zenodo.10825841. @article{kirchnerCharacterizingEntanglementAnyonic2024,
title = {Characterizing the entanglement of anyonic systems using the anyonic partial transpose},
author = {N. Kirchner and W. Choi and F. Pollmann},
doi = {10.1103/PhysRevB.110.085143},
year = {2024},
date = {2024-08-21},
urldate = {2024-08-01},
journal = {Phys. Rev. B},
volume = {110},
number = {8},
pages = {085143},
abstract = {Entanglement of mixed quantum states can be quantified using the partial transpose and its corresponding entanglement measure, the logarithmic negativity. Recently, the notion of partial transpose has been extended to systems of anyons, which are exotic quasiparticles whose exchange statistics go beyond the bosonic and fermionic cases. Studying the fundamental properties of this anyonic partial transpose, we first reveal that when applied to the special case of fermionic systems, it can be reduced to the fermionic partial transpose or its twisted variant depending on whether or not a boundary Majorana fermion is present. Focusing on ground state properties, we find that the anyonic partial transpose captures both the correct entanglement scaling for gapless systems, as predicted by conformal field theory, and the phase transition between a topologically trivial and a nontrivial phase. For non-Abelian anyons and the bipartition geometry, we find a rich multiplet structure in the eigenvalues of the partial transpose, the so-called negativity spectrum, and reveal the possibility of defining both a charge- and an imbalance-resolved negativity.},
note = {datadoi: 10.5281/zenodo.10825841},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Entanglement of mixed quantum states can be quantified using the partial transpose and its corresponding entanglement measure, the logarithmic negativity. Recently, the notion of partial transpose has been extended to systems of anyons, which are exotic quasiparticles whose exchange statistics go beyond the bosonic and fermionic cases. Studying the fundamental properties of this anyonic partial transpose, we first reveal that when applied to the special case of fermionic systems, it can be reduced to the fermionic partial transpose or its twisted variant depending on whether or not a boundary Majorana fermion is present. Focusing on ground state properties, we find that the anyonic partial transpose captures both the correct entanglement scaling for gapless systems, as predicted by conformal field theory, and the phase transition between a topologically trivial and a nontrivial phase. For non-Abelian anyons and the bipartition geometry, we find a rich multiplet structure in the eigenvalues of the partial transpose, the so-called negativity spectrum, and reveal the possibility of defining both a charge- and an imbalance-resolved negativity. |  |
Seifert, U. F. P.; Willsher, J.; Drescher, M.; Pollmann, F.; Knolle, J. Spin-Peierls instability of the U(1) Dirac spin liquid Journal Article Nat. Commun. 15, 7110 (2024), datadoi: 10.5281/zenodo.8246416. @article{seifertSpinPeierlsInstabilityU12024,
title = {Spin-Peierls instability of the U(1) Dirac spin liquid},
author = {U. F. P. Seifert and J. Willsher and M. Drescher and F. Pollmann and J. Knolle},
url = {https://doi.org/10.1038/s41467-024-51367-w},
doi = {10.1038/s41467-024-51367-w},
year = {2024},
date = {2024-08-19},
urldate = {2024-08-01},
journal = {Nat. Commun.},
volume = {15},
number = {1},
pages = {7110},
abstract = {Quantum fluctuations can inhibit long-range ordering in frustrated magnets and potentially lead to quantum spin liquid (QSL) phases. A prime example are gapless QSLs with emergent U(1) gauge fields, which have been understood to be described in terms of quantum electrodynamics in 2+1 dimension (QED3). Despite several promising candidate materials, however, a complicating factor for their realisation is the presence of other degrees of freedom. In particular lattice distortions can act to relieve magnetic frustration, precipitating conventionally ordered states. In this work, we use field-theoretic arguments as well as extensive numerical simulations to show that the U(1) Dirac QSL on the triangular and kagome lattices exhibits a weak-coupling instability due to the coupling of monopoles of the emergent gauge field to lattice distortions, leading to valence-bond solid ordering. This generalises the spin-Peierls instability of one-dimensional quantum critical spin chains to two-dimensional algebraic QSLs. We study static distortions as well as quantum-mechanical phonons. Even in regimes where the QSL is stable, the singular spin-lattice coupling leads to marked temperature-dependent corrections to the phonon spectrum, which provide salient experimental signatures of spin fractionalisation. We discuss the coupling of QSLs to the lattice as a general tool for their discovery and characterisation.},
note = {datadoi: 10.5281/zenodo.8246416},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Quantum fluctuations can inhibit long-range ordering in frustrated magnets and potentially lead to quantum spin liquid (QSL) phases. A prime example are gapless QSLs with emergent U(1) gauge fields, which have been understood to be described in terms of quantum electrodynamics in 2+1 dimension (QED3). Despite several promising candidate materials, however, a complicating factor for their realisation is the presence of other degrees of freedom. In particular lattice distortions can act to relieve magnetic frustration, precipitating conventionally ordered states. In this work, we use field-theoretic arguments as well as extensive numerical simulations to show that the U(1) Dirac QSL on the triangular and kagome lattices exhibits a weak-coupling instability due to the coupling of monopoles of the emergent gauge field to lattice distortions, leading to valence-bond solid ordering. This generalises the spin-Peierls instability of one-dimensional quantum critical spin chains to two-dimensional algebraic QSLs. We study static distortions as well as quantum-mechanical phonons. Even in regimes where the QSL is stable, the singular spin-lattice coupling leads to marked temperature-dependent corrections to the phonon spectrum, which provide salient experimental signatures of spin fractionalisation. We discuss the coupling of QSLs to the lattice as a general tool for their discovery and characterisation. |  |
Hemmida, M.; Masell, J.; Karube, K.; Ehlers, D.; von Nidda, H. -A. Krug; Tsurkan, V.; Tokura, Y.; Taguchi, Y.; Kézsmárki, I. Role of magnetic anisotropy in the antiskyrmion-host schreibersite magnets Journal Article Phys. Rev. B 110, 054416 (2024). @article{hemmida_role_2024,
title = {Role of magnetic anisotropy in the antiskyrmion-host schreibersite magnets},
author = {M. Hemmida and J. Masell and K. Karube and D. Ehlers and H. -A. Krug von Nidda and V. Tsurkan and Y. Tokura and Y. Taguchi and I. Kézsmárki},
doi = {10.1103/PhysRevB.110.054416},
year = {2024},
date = {2024-08-08},
urldate = {2024-08-08},
journal = {Phys. Rev. B},
volume = {110},
number = {5},
pages = {054416},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
|  |
Vasin, K. V.; Strinić, A.; Schilberth, F.; Reschke, S.; Prodan, L.; Tsurkan, V.; Nurmukhametov, A. R.; Eremin, M. V.; Kézsmárki, I.; Deisenhofer, J. Optical magnetoelectric effect in the polar honeycomb antiferromagnet Fe2Mo3O8 Journal Article Phys. Rev. B 110, 054401 (2024). @article{vasin_optical_2024,
title = {Optical magnetoelectric effect in the polar honeycomb antiferromagnet Fe_{2}Mo_{3}O_{8}},
author = {K. V. Vasin and A. Strinić and F. Schilberth and S. Reschke and L. Prodan and V. Tsurkan and A. R. Nurmukhametov and M. V. Eremin and I. Kézsmárki and J. Deisenhofer},
doi = {10.1103/PhysRevB.110.054401},
year = {2024},
date = {2024-08-01},
urldate = {2024-08-01},
journal = {Phys. Rev. B},
volume = {110},
number = {5},
pages = {054401},
abstract = {The lack of both time-reversal and spatial inversion symmetry in polar magnets is a prerequisite for the occurrence of optical magnetoelectric effects such as nonreciprocal directional dichroism, i.e., a difference in refractive index and absorption for two counter-propagating electromagnetic waves, which has the potential for the realization of optical diodes. In particular, antiferromagnetic materials with magnetic excitations in the THz range such as Fe2Mo3O8 are promising candidates for next-generation spintronic applications. In a combined experimental and theoretical effort we investigated the THz excitations of the polar honeycomb antiferromagnet Fe2Mo3O8 in external magnetic fields and their nonreciprocal directional dichroism, together with the temperature dependence of the electronic transitions in the mid- and near-infrared frequency range. Using an advanced single-ion approach for the Fe ions, we are able to describe optical excitations from the THz to the near-infrared frequency range quantitatively and model the observed nonreciprocal directional dichroism in the THz regime successfully.},
keywords = {A1, C4},
pubstate = {published},
tppubtype = {article}
}
The lack of both time-reversal and spatial inversion symmetry in polar magnets is a prerequisite for the occurrence of optical magnetoelectric effects such as nonreciprocal directional dichroism, i.e., a difference in refractive index and absorption for two counter-propagating electromagnetic waves, which has the potential for the realization of optical diodes. In particular, antiferromagnetic materials with magnetic excitations in the THz range such as Fe2Mo3O8 are promising candidates for next-generation spintronic applications. In a combined experimental and theoretical effort we investigated the THz excitations of the polar honeycomb antiferromagnet Fe2Mo3O8 in external magnetic fields and their nonreciprocal directional dichroism, together with the temperature dependence of the electronic transitions in the mid- and near-infrared frequency range. Using an advanced single-ion approach for the Fe ions, we are able to describe optical excitations from the THz to the near-infrared frequency range quantitatively and model the observed nonreciprocal directional dichroism in the THz regime successfully. |  |
Zerba, C.; Kuhlenkamp, C.; Imamoğlu, A.; Knap, M. Realizing topological superconductivity in tunable bose-fermi mixtures with transition metal dichalcogenide heterostructures Journal Article Phys. Rev. Lett. 133, 056902 (2024), datadoi: (10.5281/zenodo.10008122). @article{zerbaRealizingTopologicalSuperconductivity2024,
title = {Realizing topological superconductivity in tunable bose-fermi mixtures with transition metal dichalcogenide heterostructures},
author = {C. Zerba and C. Kuhlenkamp and A. Imamoğlu and M. Knap},
doi = {10.1103/PhysRevLett.133.056902},
year = {2024},
date = {2024-07-30},
urldate = {2024-07-30},
journal = {Phys. Rev. Lett.},
volume = {133},
number = {5},
pages = {056902},
abstract = {Heterostructures of two-dimensional transition metal dichalcogenides are emerging as a promising platform for investigating exotic correlated states of matter. Here, we propose to engineer Bose-Fermi mixtures in these systems by coupling interlayer excitons to doped charges in a trilayer structure. Their interactions are determined by the interlayer trion, whose spin-selective nature allows excitons to mediate an attractive interaction between charge carriers of only one spin species. Remarkably, we find that this causes the system to become unstable to topological 𝑝+𝑖𝑝 superconductivity at low temperatures. We then demonstrate a general mechanism to develop and control this unconventional state by tuning the trion binding energy using a solid-state Feshbach resonance.},
note = {datadoi: (10.5281/zenodo.10008122)},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Heterostructures of two-dimensional transition metal dichalcogenides are emerging as a promising platform for investigating exotic correlated states of matter. Here, we propose to engineer Bose-Fermi mixtures in these systems by coupling interlayer excitons to doped charges in a trilayer structure. Their interactions are determined by the interlayer trion, whose spin-selective nature allows excitons to mediate an attractive interaction between charge carriers of only one spin species. Remarkably, we find that this causes the system to become unstable to topological 𝑝+𝑖𝑝 superconductivity at low temperatures. We then demonstrate a general mechanism to develop and control this unconventional state by tuning the trion binding energy using a solid-state Feshbach resonance. |  |
Magnaterra, M.; Attig, J.; Peterlini, L.; Hermanns, M.; Upton, M. H.; Kim, Jungho; Prodan, L.; Tsurkan, V.; Kézsmárki, I.; Loosdrecht, P. H. M.; Grüninger, M. Quasimolecular Jtet = 3/2 Moments in the Cluster Mott Insulator GaTa4Se8 Journal Article Phys. Rev. Lett. 133, 046501 (2024). @article{magnaterra_quasimolecular_2024,
title = {Quasimolecular J_{tet} = 3/2 Moments in the Cluster Mott Insulator GaTa_{4}Se_{8}},
author = {M. Magnaterra and J. Attig and L. Peterlini and M. Hermanns and M. H. Upton and Jungho Kim and L. Prodan and V. Tsurkan and I. Kézsmárki and P. H. M. Loosdrecht and M. Grüninger},
doi = {10.1103/PhysRevLett.133.046501},
year = {2024},
date = {2024-07-22},
urldate = {2024-07-22},
journal = {Phys. Rev. Lett.},
volume = {133},
number = {4},
pages = {046501},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
|  |
Büttgen, N.; von Nidda, H. -A. Krug Magnetic resonance in quantum spin chains with competing exchange interactions Journal Article J. Phys. A: Math. Theor. 57, 313001 (2024). @article{buttgen_magnetic_2024,
title = {Magnetic resonance in quantum spin chains with competing exchange interactions},
author = {N. Büttgen and H. -A. Krug von Nidda},
doi = {10.1088/1751-8121/ad5e4c},
year = {2024},
date = {2024-07-18},
urldate = {2024-07-01},
journal = {J. Phys. A: Math. Theor.},
volume = {57},
number = {31},
pages = {313001},
abstract = {Based on a previous review on magnetic resonance in quantum spin chains (Krug von Nidda et al 2010 Eur. Phys. J. Spec. Top. 180 161–89) we report on further development in this field with special focus on transition–metal oxides and halogenides consisting of quasi one–dimensional spin systems, where both intra–and inter–chain exchange interaction may give rise to frustration effects and higher–order anisotropic exchange contributions like the Dzyaloshinskii–Moriya interaction become decisive for the formation of the magnetic ground state. Selected examples show how NMR and ESR contribute valuable information on the magnetic phases and exchange interactions involved: LiCuVO4 with competing nearest neighbour and next–nearest neighbour intra–chain exchange, LiCu2O2 with complex zig–zag chains, and Cs2CuCl4 where the chains form a triangular lattice with the inter–chain interaction weaker but of the same order of magnitude than the intra–chain interaction. The so called paper–chain compound Ba3Cu3In4O12, where each successive pair of CuO4 plaquettes is rotated by 90° with respect to its predecessor along the c–direction like in a paper–chain, provides an interesting topology of frustrated intra–chain exchange interactions. Finally, a few dimer systems are considered.},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
Based on a previous review on magnetic resonance in quantum spin chains (Krug von Nidda et al 2010 Eur. Phys. J. Spec. Top. 180 161–89) we report on further development in this field with special focus on transition–metal oxides and halogenides consisting of quasi one–dimensional spin systems, where both intra–and inter–chain exchange interaction may give rise to frustration effects and higher–order anisotropic exchange contributions like the Dzyaloshinskii–Moriya interaction become decisive for the formation of the magnetic ground state. Selected examples show how NMR and ESR contribute valuable information on the magnetic phases and exchange interactions involved: LiCuVO4 with competing nearest neighbour and next–nearest neighbour intra–chain exchange, LiCu2O2 with complex zig–zag chains, and Cs2CuCl4 where the chains form a triangular lattice with the inter–chain interaction weaker but of the same order of magnitude than the intra–chain interaction. The so called paper–chain compound Ba3Cu3In4O12, where each successive pair of CuO4 plaquettes is rotated by 90° with respect to its predecessor along the c–direction like in a paper–chain, provides an interesting topology of frustrated intra–chain exchange interactions. Finally, a few dimer systems are considered. |  |
Kumar, H.; Köpf, M.; Telang, P.; Bura, N.; Jesche, A.; Gegenwart, P.; Kuntscher, C. A. Optical conductivity of the metallic pyrochlore iridate Pr2Ir2O7: Influence of spin-orbit coupling and electronic correlations on the electronic structure Journal Article Phys. Rev. B 110, 035140 (2024). @article{kumar_optical_2024,
title = {Optical conductivity of the metallic pyrochlore iridate Pr_{2}Ir_{2}O_{7}: Influence of spin-orbit coupling and electronic correlations on the electronic structure},
author = {H. Kumar and M. Köpf and P. Telang and N. Bura and A. Jesche and P. Gegenwart and C. A. Kuntscher},
url = {https://link.aps.org/doi/10.1103/PhysRevB.110.035140},
doi = {10.1103/PhysRevB.110.035140},
year = {2024},
date = {2024-07-15},
urldate = {2024-07-15},
journal = {Phys. Rev. B},
volume = {110},
number = {3},
pages = {035140},
abstract = {The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single crystals of the pyrochlore iridate Pr2Ir2O7 and explored its magnetic, lattice dynamical, and electronic properties. While Raman spectroscopy data reveal six phonon modes confirming the cubic Fd‾3m crystal symmetry, dc magnetic susceptibility data show no anomalies and hence indicate the absence of magnetic phase transitions down to 2 K. Both temperature-dependent electric transport and optical conductivity data reveal the metallic character of Pr2Ir2O7. The optical conductivity spectrum contains a midinfrared absorption band, which becomes more pronounced with decreasing temperature due to spectral weight transfer from high to low energies. The presence of the midinfrared band hints at the importance of correlation physics. The optical response furthermore suggests that Pr2Ir2O7 is close to the Weyl semimetal phase.},
keywords = {A1, B3},
pubstate = {published},
tppubtype = {article}
}
The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single crystals of the pyrochlore iridate Pr2Ir2O7 and explored its magnetic, lattice dynamical, and electronic properties. While Raman spectroscopy data reveal six phonon modes confirming the cubic Fd‾3m crystal symmetry, dc magnetic susceptibility data show no anomalies and hence indicate the absence of magnetic phase transitions down to 2 K. Both temperature-dependent electric transport and optical conductivity data reveal the metallic character of Pr2Ir2O7. The optical conductivity spectrum contains a midinfrared absorption band, which becomes more pronounced with decreasing temperature due to spectral weight transfer from high to low energies. The presence of the midinfrared band hints at the importance of correlation physics. The optical response furthermore suggests that Pr2Ir2O7 is close to the Weyl semimetal phase. |  |
Kalin, J.; Sievers, S.; Schumacher, H. W.; Füser, H.; Bieler, M.; Bauer, A.; Pfleiderer, C. Influence of the magnetovolume effect on the transient reflectivity of MnSi Journal Article Phys. Rev. B 110, 014415 (2024). @article{kalin_influence_2024,
title = {Influence of the magnetovolume effect on the transient reflectivity of MnSi},
author = {J. Kalin and S. Sievers and H. W. Schumacher and H. Füser and M. Bieler and A. Bauer and C. Pfleiderer},
doi = {10.1103/PhysRevB.110.014415},
year = {2024},
date = {2024-07-11},
urldate = {2024-07-11},
journal = {Phys. Rev. B},
volume = {110},
number = {1},
pages = {014415},
abstract = {The magnetovolume effect is a well established yet frequently overlooked phenomenon in magnetic materials that may affect a wide range of physical properties. Our study explores the influence of the magnetovolume effect on the transient reflectivity of MnSi, a well-known chiral magnet with strong magnetoelastic coupling. We observe a unipolar reflectivity transient in the paramagnetic phase, contrasting with a bipolar response in phases with magnetic long-range order. Comparing our findings with thermal expansion from literature, we establish that the bipolar response originates in the magnetovolume effect which dominates the thermal expansion and influences the optical reflectivity. Our results highlight not only that the magnetovolume effect must be considered when discussing transient reflectivity measurements of magnetic materials but also that such measurements permit to study the characteristic time scales of the magnetovolume effect itself, contributing to a deeper understanding of this often-neglected phenomenon.},
keywords = {C1, C3},
pubstate = {published},
tppubtype = {article}
}
The magnetovolume effect is a well established yet frequently overlooked phenomenon in magnetic materials that may affect a wide range of physical properties. Our study explores the influence of the magnetovolume effect on the transient reflectivity of MnSi, a well-known chiral magnet with strong magnetoelastic coupling. We observe a unipolar reflectivity transient in the paramagnetic phase, contrasting with a bipolar response in phases with magnetic long-range order. Comparing our findings with thermal expansion from literature, we establish that the bipolar response originates in the magnetovolume effect which dominates the thermal expansion and influences the optical reflectivity. Our results highlight not only that the magnetovolume effect must be considered when discussing transient reflectivity measurements of magnetic materials but also that such measurements permit to study the characteristic time scales of the magnetovolume effect itself, contributing to a deeper understanding of this often-neglected phenomenon. |  |
Pichler, F.; Kadow, W.; Kuhlenkamp, C.; Knap, M. Probing magnetism in moiré heterostructures with quantum twisting microscopes Journal Article Phys. Rev. B 110, 045116 (2024), datadoi: 10.5281/zenodo.10611915. @article{pichlerProbingMagnetismMoire2024,
title = {Probing magnetism in moiré heterostructures with quantum twisting microscopes},
author = {F. Pichler and W. Kadow and C. Kuhlenkamp and M. Knap},
url = {https://doi.org/10.1103/PhysRevB.110.045116},
doi = {10.1103/PhysRevB.110.045116},
year = {2024},
date = {2024-07-09},
urldate = {2024-07-09},
journal = {Phys. Rev. B},
volume = {110},
number = {4},
pages = {045116},
abstract = {Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum resolved spectrum of single-particle and collective excitations, can be used as a novel tool to distinguish between different types of magnetic order. To this end, we calculate the single-particle spectral function and the dynamical spin-structure factor for both a ferromagnetic and antiferromagnetic generalized Wigner crystal formed in fractionally filled moiré superlattices of transition metal dichalcogenide heterostructures. We demonstrate that magnetic order can be clearly identified in these response functions. Furthermore, we explore signatures of quantum phase transitions in the quantum twisting microscope response. We focus on the specific case of triangular moiré lattices at half filling that have been proposed to host a topological phase transition between a chiral spin liquid and a 120° ordered state. Our work demonstrates the potential for quantum twisting microscopes to characterize quantum magnetism in moiré heterostructures.},
note = {datadoi: 10.5281/zenodo.10611915},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum resolved spectrum of single-particle and collective excitations, can be used as a novel tool to distinguish between different types of magnetic order. To this end, we calculate the single-particle spectral function and the dynamical spin-structure factor for both a ferromagnetic and antiferromagnetic generalized Wigner crystal formed in fractionally filled moiré superlattices of transition metal dichalcogenide heterostructures. We demonstrate that magnetic order can be clearly identified in these response functions. Furthermore, we explore signatures of quantum phase transitions in the quantum twisting microscope response. We focus on the specific case of triangular moiré lattices at half filling that have been proposed to host a topological phase transition between a chiral spin liquid and a 120° ordered state. Our work demonstrates the potential for quantum twisting microscopes to characterize quantum magnetism in moiré heterostructures. |  |
Chen, A.; Heyl, M. Empowering deep neural quantum states through efficient optimization Journal Article Nat. Phys. 20, 1476 (2024), datadoi: (10.5281/zenodo.7657551). @article{chenEmpoweringDeepNeural2024,
title = {Empowering deep neural quantum states through efficient optimization},
author = {A. Chen and M. Heyl},
url = {https://doi.org/10.1038/s41567-024-02566-1},
doi = {10.1038/s41567-024-02566-1},
year = {2024},
date = {2024-07-01},
urldate = {2024-07-01},
journal = {Nat. Phys.},
volume = {20},
number = {9},
pages = {1476},
abstract = {Computing the ground state of interacting quantum matter is a long-standing challenge, especially for complex two-dimensional systems. Recent developments have highlighted the potential of neural quantum states to solve the quantum many-body problem by encoding the many-body wavefunction into artificial neural networks. However, this method has faced the critical limitation that existing optimization algorithms are not suitable for training modern large-scale deep network architectures. Here, we introduce a minimum-step stochastic-reconfiguration optimization algorithm, which allows us to train deep neural quantum states with up to 106 parameters. We demonstrate our method for paradigmatic frustrated spin-1/2 models on square and triangular lattices, for which our trained deep networks approach machine precision and yield improved variational energies compared to existing results. Equipped with our optimization algorithm, we find numerical evidence for gapless quantum-spin-liquid phases in the considered models, an open question to date. We present a method that captures the emergent complexity in quantum many-body problems through the expressive power of large-scale artificial neural networks.},
note = {datadoi: (10.5281/zenodo.7657551)},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Computing the ground state of interacting quantum matter is a long-standing challenge, especially for complex two-dimensional systems. Recent developments have highlighted the potential of neural quantum states to solve the quantum many-body problem by encoding the many-body wavefunction into artificial neural networks. However, this method has faced the critical limitation that existing optimization algorithms are not suitable for training modern large-scale deep network architectures. Here, we introduce a minimum-step stochastic-reconfiguration optimization algorithm, which allows us to train deep neural quantum states with up to 106 parameters. We demonstrate our method for paradigmatic frustrated spin-1/2 models on square and triangular lattices, for which our trained deep networks approach machine precision and yield improved variational energies compared to existing results. Equipped with our optimization algorithm, we find numerical evidence for gapless quantum-spin-liquid phases in the considered models, an open question to date. We present a method that captures the emergent complexity in quantum many-body problems through the expressive power of large-scale artificial neural networks. |  |
Das, P.; Leeb, V.; Knolle, J.; Knap, M. Realizing altermagnetism in fermi-hubbard models with ultracold atoms Journal Article Phys. Rev. Lett. 132, 263402 (2024), datadoi: 10.5281/zenodo.10391823. @article{dasRealizingAltermagnetismFermihubbard2024,
title = {Realizing altermagnetism in fermi-hubbard models with ultracold atoms},
author = {P. Das and V. Leeb and J. Knolle and M. Knap},
url = {https://doi.org/10.1103/PhysRevLett.132.263402},
doi = {10.1103/PhysRevLett.132.263402},
year = {2024},
date = {2024-06-26},
urldate = {2024-06-01},
journal = {Phys. Rev. Lett.},
volume = {132},
number = {26},
pages = {263402},
abstract = {Altermagnetism represents a type of collinear magnetism, that is in some aspects distinct from ferromagnetism and from conventional antiferromagnetism. In contrast to the latter, sublattices of opposite spin are related by spatial rotations and not only by translations and inversions. As a result, altermagnets have spin-split bands leading to unique experimental signatures. Here, we show theoretically how a 𝑑-wave altermagnetic phase can be realized with ultracold fermionic atoms in optical lattices. We propose an altermagnetic Hubbard model with anisotropic next-nearest neighbor hopping and obtain the Hartree-Fock phase diagram. The altermagnetic phase separates in a metallic and an insulating phase and is robust over a large parameter regime. We show that one of the defining characteristics of altermagnetism, the anisotropic spin transport, can be probed with trap-expansion experiments.},
note = {datadoi: 10.5281/zenodo.10391823},
keywords = {C6},
pubstate = {published},
tppubtype = {article}
}
Altermagnetism represents a type of collinear magnetism, that is in some aspects distinct from ferromagnetism and from conventional antiferromagnetism. In contrast to the latter, sublattices of opposite spin are related by spatial rotations and not only by translations and inversions. As a result, altermagnets have spin-split bands leading to unique experimental signatures. Here, we show theoretically how a 𝑑-wave altermagnetic phase can be realized with ultracold fermionic atoms in optical lattices. We propose an altermagnetic Hubbard model with anisotropic next-nearest neighbor hopping and obtain the Hartree-Fock phase diagram. The altermagnetic phase separates in a metallic and an insulating phase and is robust over a large parameter regime. We show that one of the defining characteristics of altermagnetism, the anisotropic spin transport, can be probed with trap-expansion experiments. |  |
Shen, B.; Ginga, V. A.; Arévalo-López, A. M.; Garbarino, G.; Uykur, E.; Goncalves-Faria, M.; Mukharjee, P. K.; Gegenwart, P.; Tsirlin, A. A. Magnetic vs. nonmagnetic polymorphs of RuBr3 under pressure Journal Article Phys. Rev. B 109, 224402 (2024), datadoi: 10.5281/zenodo.10863362. @article{shenMagneticVsNonmagnetic2024,
title = {Magnetic vs. nonmagnetic polymorphs of RuBr_{3} under pressure},
author = {B. Shen and V. A. Ginga and A. M. Arévalo-López and G. Garbarino and E. Uykur and M. Goncalves-Faria and P. K. Mukharjee and P. Gegenwart and A. A. Tsirlin},
url = {https://doi.org/10.1103/PhysRevB.109.224402},
doi = {10.1103/PhysRevB.109.224402},
year = {2024},
date = {2024-06-03},
urldate = {2024-03-01},
journal = {Phys. Rev. B},
volume = {109},
number = {22},
pages = {224402},
abstract = {Pressure evolution of the crystal structure and magnetism of the honeycomb 𝛼-RuBr_3 is studied using high-pressure x-ray diffraction, magnetometry, and density-functional band-structure calculations. Hydrostatic compression transforms antiferromagnetic 𝛼-RuBr_3 (R-3) into paramagnetic 𝛼'-RuBr_3 (P-1) where short Ru-Ru bonds cause magnetism collapse above 1.3 GPa at 0 K and 2.5 GPa at 295 K. Below this critical pressure, the Ntextbackslash'eel temperature of 𝛼-RuBr_3 increases with the slope of 1.8 K/GPa. Pressure tunes 𝛼-RuBr_3 away from the Kitaev limit, whereas increased third-neighbor in-plane coupling and interlayer coupling lead to a further stabilization of the collinear zigzag state. Both 𝛼- and 𝛼'-RuBr_3 are metastable at ambient pressure, but their transformation into the thermodynamically stable 𝛽-polymorph is kinetically hindered at room temperature.},
note = {datadoi: 10.5281/zenodo.10863362},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Pressure evolution of the crystal structure and magnetism of the honeycomb 𝛼-RuBr_3 is studied using high-pressure x-ray diffraction, magnetometry, and density-functional band-structure calculations. Hydrostatic compression transforms antiferromagnetic 𝛼-RuBr_3 (R-3) into paramagnetic 𝛼'-RuBr_3 (P-1) where short Ru-Ru bonds cause magnetism collapse above 1.3 GPa at 0 K and 2.5 GPa at 295 K. Below this critical pressure, the Ntextbackslash'eel temperature of 𝛼-RuBr_3 increases with the slope of 1.8 K/GPa. Pressure tunes 𝛼-RuBr_3 away from the Kitaev limit, whereas increased third-neighbor in-plane coupling and interlayer coupling lead to a further stabilization of the collinear zigzag state. Both 𝛼- and 𝛼'-RuBr_3 are metastable at ambient pressure, but their transformation into the thermodynamically stable 𝛽-polymorph is kinetically hindered at room temperature. |  |
Leeb, V.; Mook, A.; Šmejkal, L.; Knolle, J. Spontaneous Formation of Altermagnetism from Orbital Ordering Journal Article Phys. Rev. Lett. 132, 236701 (2024), datadoi: 10.5281/zenodo.10222641. @article{leebSpontaneousFormationAltermagnetism2024,
title = {Spontaneous Formation of Altermagnetism from Orbital Ordering},
author = {V. Leeb and A. Mook and L. Šmejkal and J. Knolle},
url = {https://link.aps.org/doi/10.1103/PhysRevLett.132.236701},
doi = {10.1103/PhysRevLett.132.236701},
year = {2024},
date = {2024-06-03},
urldate = {2024-06-01},
journal = {Phys. Rev. Lett.},
volume = {132},
number = {23},
pages = {236701},
abstract = {Altermagnetism has emerged as a third type of collinear magnetism. In contrast to standard ferromagnets and antiferromagnets, altermagnets exhibit extra even-parity wave spin order parameters resulting in a spin splitting of electronic bands in momentum space. In real space, sublattices of opposite spin polarization are anisotropic and related by rotational symmetry. In the hitherto identified altermagnetic candidate materials, the anisotropies arise from the local crystallographic symmetry. Here, we show that altermagnetism can also form as an interaction-induced electronic instability in a lattice without the crystallographic sublattice anisotropy. We provide a microscopic example of a two-orbital model showing that the coexistence of staggered antiferromagnetic and orbital order can realize robust altermagnetism. We quantify the spin-splitter conductivity as a key experimental observable and discuss material candidates for the interaction-induced realization of altermagnetism.},
note = {datadoi: 10.5281/zenodo.10222641},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Altermagnetism has emerged as a third type of collinear magnetism. In contrast to standard ferromagnets and antiferromagnets, altermagnets exhibit extra even-parity wave spin order parameters resulting in a spin splitting of electronic bands in momentum space. In real space, sublattices of opposite spin polarization are anisotropic and related by rotational symmetry. In the hitherto identified altermagnetic candidate materials, the anisotropies arise from the local crystallographic symmetry. Here, we show that altermagnetism can also form as an interaction-induced electronic instability in a lattice without the crystallographic sublattice anisotropy. We provide a microscopic example of a two-orbital model showing that the coexistence of staggered antiferromagnetic and orbital order can realize robust altermagnetism. We quantify the spin-splitter conductivity as a key experimental observable and discuss material candidates for the interaction-induced realization of altermagnetism. | |
Hirschberger, M.; Szigeti, B. G.; Hemmida, M.; Hirschmann, M. M.; Esser, S.; Ohsumi, H.; Tanaka, Y.; Spitz, L.; Gao, S.; Kolincio, K. K.; Sagayama, H.; Nakao, H.; Yamasaki, Y.; Forró, L.; von Nidda, H. -A. Krug; Kézsmárki, I.; Arima, T.; Tokura, Y. Lattice-commensurate skyrmion texture in a centrosymmetric breathing kagome magnet Journal Article npj Quantum Mater. 9, 45 (2024). @article{hirschberger_lattice-commensurate_2024,
title = {Lattice-commensurate skyrmion texture in a centrosymmetric breathing kagome magnet},
author = {M. Hirschberger and B. G. Szigeti and M. Hemmida and M. M. Hirschmann and S. Esser and H. Ohsumi and Y. Tanaka and L. Spitz and S. Gao and K. K. Kolincio and H. Sagayama and H. Nakao and Y. Yamasaki and L. Forró and H. -A. Krug von Nidda and I. Kézsmárki and T. Arima and Y. Tokura},
doi = {10.1038/s41535-024-00654-2},
year = {2024},
date = {2024-05-23},
urldate = {2024-05-01},
journal = {npj Quantum Mater.},
volume = {9},
pages = {45},
abstract = {Skyrmion lattices (SkL) in centrosymmetric materials typically have a magnetic period on the nanometer-scale, so that the coupling between magnetic superstructures and the underlying crystal lattice cannot be neglected. We reveal the commensurate locking of a SkL to the atomic lattice in Gd3Ru4Al12 via high-resolution resonant elastic x-ray scattering (REXS). Weak easy-plane magnetic anisotropy, demonstrated here by a combination of ferromagnetic resonance and REXS, penalizes placing a skyrmion core on a site of the atomic lattice. Under these conditions, a commensurate SkL, locked to the crystal lattice, is stable at finite temperatures – but gives way to a competing incommensurate ground state upon cooling. We discuss the role of Umklapp-terms in the Hamiltonian for the formation of this lattice-locked state, its magnetic space group, and the role of slight discommensurations, or (line) defects in the magnetic texture. We also contrast our findings with the case of SkLs in noncentrosymmetric material platforms.},
keywords = {B4, B5},
pubstate = {published},
tppubtype = {article}
}
Skyrmion lattices (SkL) in centrosymmetric materials typically have a magnetic period on the nanometer-scale, so that the coupling between magnetic superstructures and the underlying crystal lattice cannot be neglected. We reveal the commensurate locking of a SkL to the atomic lattice in Gd3Ru4Al12 via high-resolution resonant elastic x-ray scattering (REXS). Weak easy-plane magnetic anisotropy, demonstrated here by a combination of ferromagnetic resonance and REXS, penalizes placing a skyrmion core on a site of the atomic lattice. Under these conditions, a commensurate SkL, locked to the crystal lattice, is stable at finite temperatures – but gives way to a competing incommensurate ground state upon cooling. We discuss the role of Umklapp-terms in the Hamiltonian for the formation of this lattice-locked state, its magnetic space group, and the role of slight discommensurations, or (line) defects in the magnetic texture. We also contrast our findings with the case of SkLs in noncentrosymmetric material platforms. |  |
Matsumoto, Y.; Schnierer, S.; Bruin, J. A. N.; Nuss, J.; Reiss, P.; Jackeli, G.; Kitagawa, K.; Takagi, H. A quantum critical Bose gas of magnons in the quasi-two-dimensional antiferromagnet YbCl3 under magnetic fields Journal Article Nat. Phys. 20, 1131–1138 (2024), datadoi: 10.1038/s41567-024-02498-w. @article{matsumotoQuantumCriticalBose2024,
title = {A quantum critical Bose gas of magnons in the quasi-two-dimensional antiferromagnet YbCl_{3} under magnetic fields},
author = {Y. Matsumoto and S. Schnierer and J. A. N. Bruin and J. Nuss and P. Reiss and G. Jackeli and K. Kitagawa and H. Takagi},
url = {https://doi.org/10.1038/s41567-024-02498-w},
doi = {10.1038/s41567-024-02498-w},
year = {2024},
date = {2024-05-09},
urldate = {2024-05-01},
journal = {Nat. Phys.},
volume = {20},
number = {7},
pages = {1131–1138},
abstract = {Bose–Einstein condensation (BEC) is a quantum phenomenon in which a macroscopic number of bosons occupy the lowest energy state and acquire coherence at low temperatures. In three-dimensional antiferromagnets, a magnetic-field-induced transition has been successfully described as a magnon BEC. For a strictly two-dimensional (2D) system, it is known that BEC cannot take place due to the presence of a finite density of states at zero energy. However, in a realistic quasi-2D magnet consisting of stacked magnetic layers, a small but finite interlayer coupling stabilizes marginal BEC but such that 2D physics is still expected to dominate. This 2D-limit BEC behaviour has been reported in a few materials but only at very high magnetic fields that are difficult to access. The honeycomb S = 1/2 Heisenberg antiferromagnet YbCl3 exhibits a transition to a fully polarized state at a relatively low in-plane magnetic field. Here, we demonstrate the formation of a quantum critical 2D Bose gas at the transition field, which, with lowering the field, experiences a BEC marginally stabilized by an extremely small interlayer coupling. Our observations establish YbCl3, previously a Kitaev quantum spin liquid material, as a realization of a quantum critical BEC in the 2D limit.},
note = {datadoi: 10.1038/s41567-024-02498-w},
keywords = {A3},
pubstate = {published},
tppubtype = {article}
}
Bose–Einstein condensation (BEC) is a quantum phenomenon in which a macroscopic number of bosons occupy the lowest energy state and acquire coherence at low temperatures. In three-dimensional antiferromagnets, a magnetic-field-induced transition has been successfully described as a magnon BEC. For a strictly two-dimensional (2D) system, it is known that BEC cannot take place due to the presence of a finite density of states at zero energy. However, in a realistic quasi-2D magnet consisting of stacked magnetic layers, a small but finite interlayer coupling stabilizes marginal BEC but such that 2D physics is still expected to dominate. This 2D-limit BEC behaviour has been reported in a few materials but only at very high magnetic fields that are difficult to access. The honeycomb S = 1/2 Heisenberg antiferromagnet YbCl3 exhibits a transition to a fully polarized state at a relatively low in-plane magnetic field. Here, we demonstrate the formation of a quantum critical 2D Bose gas at the transition field, which, with lowering the field, experiences a BEC marginally stabilized by an extremely small interlayer coupling. Our observations establish YbCl3, previously a Kitaev quantum spin liquid material, as a realization of a quantum critical BEC in the 2D limit. |  |
Kunze, J.; Köpf, M.; Cao, W.; Qi, Y.; Kuntscher, C. A. Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R = La, Ce, Pr, Nd, Sm) Journal Article Phys. Rev. B 109, 195130 (2024). @article{kunze_optical_2024,
title = {Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R = La, Ce, Pr, Nd, Sm)},
author = {J. Kunze and M. Köpf and W. Cao and Y. Qi and C. A. Kuntscher},
url = {https://link.aps.org/doi/10.1103/PhysRevB.109.195130},
doi = {10.1103/PhysRevB.109.195130},
year = {2024},
date = {2024-05-09},
urldate = {2024-05-09},
journal = {Phys. Rev. B},
volume = {109},
number = {19},
pages = {195130},
abstract = {Weyl semimetals with magnetic ordering provide a promising platform for the investigation of rare topological effects such as the anomalous Hall effect, resulting from the interplay of nontrivial bands with various spin configurations. The materials RAlSi, where R represents a rare-earth element, are prominent representatives of Weyl semimetals, where the Weyl states are induced by space inversion symmetry breaking, and in addition, for several rare-earth elements R, enhanced by time-reversal symmetry breaking through the formation of a magnetic order at low temperature. We report optical signatures of Weyl fermions in the magnetic compounds CeAlSi, PrAlSi, NdAlSi, and SmAlSi as well as the nonmagnetic family member LaAlSi by broad-frequency infrared spectroscopy at room temperature, i.e., in the paramagnetic phase. A similar profile of the optical conductivity spectrum and a metallic character are observed for all compounds, with LaAlSi showing the strongest free charge-carrier contribution. Furthermore, the linear-in-frequency behavior of the optical conductivity of all investigated compounds indicates the presence of Weyl nodes in close proximity to the Fermi energy, resulting from inversion symmetry breaking in noncentrosymmetric structures. According to the characteristics of these linear slopes, the RAlSi compounds are expected to host mainly type-II Weyl states with overtilted Weyl cones. The results are compared to the optical response of the closely related RAlGe materials, which are considered as potential hybridization-driven Weyl-Kondo systems.},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
Weyl semimetals with magnetic ordering provide a promising platform for the investigation of rare topological effects such as the anomalous Hall effect, resulting from the interplay of nontrivial bands with various spin configurations. The materials RAlSi, where R represents a rare-earth element, are prominent representatives of Weyl semimetals, where the Weyl states are induced by space inversion symmetry breaking, and in addition, for several rare-earth elements R, enhanced by time-reversal symmetry breaking through the formation of a magnetic order at low temperature. We report optical signatures of Weyl fermions in the magnetic compounds CeAlSi, PrAlSi, NdAlSi, and SmAlSi as well as the nonmagnetic family member LaAlSi by broad-frequency infrared spectroscopy at room temperature, i.e., in the paramagnetic phase. A similar profile of the optical conductivity spectrum and a metallic character are observed for all compounds, with LaAlSi showing the strongest free charge-carrier contribution. Furthermore, the linear-in-frequency behavior of the optical conductivity of all investigated compounds indicates the presence of Weyl nodes in close proximity to the Fermi energy, resulting from inversion symmetry breaking in noncentrosymmetric structures. According to the characteristics of these linear slopes, the RAlSi compounds are expected to host mainly type-II Weyl states with overtilted Weyl cones. The results are compared to the optical response of the closely related RAlGe materials, which are considered as potential hybridization-driven Weyl-Kondo systems. |  |
Reinhoffer, C.; Esser, S.; Esser, S.; Mashkovich, E.; Germanskiy, S.; Gegenwart, P.; Anders, F.; Loosdrecht, P. H. M.; Wang, Z. Strong Terahertz Third-Harmonic Generation by Kinetic Heavy Quasiparticles in CaRuO3 Journal Article Phys. Rev. Lett. 132, 196501 (2024). @article{reinhoffer_strong_2024,
title = {Strong Terahertz Third-Harmonic Generation by Kinetic Heavy Quasiparticles in CaRuO_{3}},
author = {C. Reinhoffer and S. Esser and S. Esser and E. Mashkovich and S. Germanskiy and P. Gegenwart and F. Anders and P. H. M. Loosdrecht and Z. Wang},
url = {https://link.aps.org/doi/10.1103/PhysRevLett.132.196501},
doi = {10.1103/PhysRevLett.132.196501},
year = {2024},
date = {2024-05-08},
urldate = {2024-05-08},
journal = {Phys. Rev. Lett.},
volume = {132},
number = {19},
pages = {196501},
abstract = {We report on time-resolved nonlinear terahertz spectroscopy of a strongly correlated ruthenate, CaRuO_{3}, as a function of temperature, frequency, and terahertz field strength. Third-harmonic radiation for frequencies up to 2.1 THz is observed evidently at low temperatures below 80 K, where the low-frequency linear dynamical response deviates from the Drude model and a coherent heavy quasiparticle band emerges by strong correlations associated with the Hund’s coupling. Phenomenologically, by taking an experimentally observed frequency-dependent scattering rate, the deviation of the field driven kinetics from the Drude behavior is reconciled in a time-dependent Boltzmann description, which allows an attribution of the observed third-harmonic generation to the terahertz field driven nonlinear kinetics of the heavy quasiparticles.},
keywords = {B1, B5},
pubstate = {published},
tppubtype = {article}
}
We report on time-resolved nonlinear terahertz spectroscopy of a strongly correlated ruthenate, CaRuO3, as a function of temperature, frequency, and terahertz field strength. Third-harmonic radiation for frequencies up to 2.1 THz is observed evidently at low temperatures below 80 K, where the low-frequency linear dynamical response deviates from the Drude model and a coherent heavy quasiparticle band emerges by strong correlations associated with the Hund’s coupling. Phenomenologically, by taking an experimentally observed frequency-dependent scattering rate, the deviation of the field driven kinetics from the Drude behavior is reconciled in a time-dependent Boltzmann description, which allows an attribution of the observed third-harmonic generation to the terahertz field driven nonlinear kinetics of the heavy quasiparticles. |  |
Ebad-Allah, J.; Jiang, M. -C.; Borkenhagen, R.; Meggle, F.; Prodan, L.; Tsurkan, V.; Schilberth, F.; Guo, G. -Y.; Arita, R.; Kézsmárki, I.; Kuntscher, C. A. Optical anisotropy of the kagome magnet FeSn: Dominant role of excitations between kagome and Sn layers Journal Article Phys. Rev. B 109, L201106 (2024). @article{ebad-allah_optical_2024,
title = {Optical anisotropy of the kagome magnet FeSn: Dominant role of excitations between kagome and Sn layers},
author = {J. Ebad-Allah and M. -C. Jiang and R. Borkenhagen and F. Meggle and L. Prodan and V. Tsurkan and F. Schilberth and G. -Y. Guo and R. Arita and I. Kézsmárki and C. A. Kuntscher},
doi = {10.1103/PhysRevB.109.L201106},
year = {2024},
date = {2024-05-07},
urldate = {2024-05-01},
journal = {Phys. Rev. B},
volume = {109},
number = {20},
pages = {L201106},
abstract = {Antiferromagnetic FeSn is considered to be a close realization of the ideal two-dimensional (2D) kagome lattice, hosting Dirac cones, van Hove singularities, and flat bands, as it comprises Fe3Sn kagome layers well separated by Sn buffer layers. We observe a pronounced optical anisotropy, with the low-energy optical conductivity being surprisingly higher perpendicular to the kagome planes than along the layers. This finding contradicts the prevalent picture of dominantly 2D electronic structure for FeSn. Our material-specific theory reproduces the measured conductivity spectra remarkably well. A site-specific decomposition of the optical response to individual excitation channels shows that the optical conductivity for polarizations both parallel and perpendicular to the kagome plane is dominated by interlayer transitions between kagome layers and adjacent Sn-based layers. Moreover, the matrix elements corresponding to these transitions are highly anisotropic, leading to larger out-of-plane conductivity. Our results evidence the crucial role of interstitial layers in charge dynamics even in seemingly 2D systems.},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
Antiferromagnetic FeSn is considered to be a close realization of the ideal two-dimensional (2D) kagome lattice, hosting Dirac cones, van Hove singularities, and flat bands, as it comprises Fe3Sn kagome layers well separated by Sn buffer layers. We observe a pronounced optical anisotropy, with the low-energy optical conductivity being surprisingly higher perpendicular to the kagome planes than along the layers. This finding contradicts the prevalent picture of dominantly 2D electronic structure for FeSn. Our material-specific theory reproduces the measured conductivity spectra remarkably well. A site-specific decomposition of the optical response to individual excitation channels shows that the optical conductivity for polarizations both parallel and perpendicular to the kagome plane is dominated by interlayer transitions between kagome layers and adjacent Sn-based layers. Moreover, the matrix elements corresponding to these transitions are highly anisotropic, leading to larger out-of-plane conductivity. Our results evidence the crucial role of interstitial layers in charge dynamics even in seemingly 2D systems. |  |
Huber, N.; Mishra, S.; Sheikin, I.; Alpin, K.; Schnyder, A. P.; Benka, G.; Bauer, A.; Pfleiderer, C.; Wilde, M. A. Fermi surface of the chiral topological semimetal CoSi Journal Article Phys. Rev. B 109, 205115 (2024). @article{huber_fermi_2024,
title = {Fermi surface of the chiral topological semimetal CoSi},
author = {N. Huber and S. Mishra and I. Sheikin and K. Alpin and A. P. Schnyder and G. Benka and A. Bauer and C. Pfleiderer and M. A. Wilde},
doi = {10.1103/PhysRevB.109.205115},
year = {2024},
date = {2024-05-06},
urldate = {2024-05-06},
journal = {Phys. Rev. B},
volume = {109},
number = {20},
pages = {205115},
abstract = {We report a study of the Fermi surface of the chiral semimetal CoSi and its relationship to a network of multifold topological crossing points, Weyl points, and topological nodal planes in the electronic band structure. Combining quantum oscillations in the Hall resistivity, magnetization, and torque magnetization with ab initio electronic structure calculations, we identify two groups of Fermi-surface sheets, one centered at the 𝑅 point and the other centered at the Γ point. The presence of topological nodal planes at the Brillouin zone boundary enforces topological protectorates on the Fermi-surface sheets centered at the 𝑅 point. In addition, Weyl points exist close to the Fermi-surface sheets centered at the 𝑅 and the Γ points. In contrast, topological crossing points at the 𝑅 point and the Γ point, which have been advertised to feature exceptionally large Chern numbers, are located at a larger distance to the Fermi level. Representing a unique example in which the multitude of topological band crossings has been shown to form a complex network, our observations in CoSi highlight the need for detailed numerical calculations of the Berry curvature at the Fermi level, regardless of the putative existence and the possible character of topological band crossings in the band structure.},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
We report a study of the Fermi surface of the chiral semimetal CoSi and its relationship to a network of multifold topological crossing points, Weyl points, and topological nodal planes in the electronic band structure. Combining quantum oscillations in the Hall resistivity, magnetization, and torque magnetization with ab initio electronic structure calculations, we identify two groups of Fermi-surface sheets, one centered at the 𝑅 point and the other centered at the Γ point. The presence of topological nodal planes at the Brillouin zone boundary enforces topological protectorates on the Fermi-surface sheets centered at the 𝑅 point. In addition, Weyl points exist close to the Fermi-surface sheets centered at the 𝑅 and the Γ points. In contrast, topological crossing points at the 𝑅 point and the Γ point, which have been advertised to feature exceptionally large Chern numbers, are located at a larger distance to the Fermi level. Representing a unique example in which the multitude of topological band crossings has been shown to form a complex network, our observations in CoSi highlight the need for detailed numerical calculations of the Berry curvature at the Fermi level, regardless of the putative existence and the possible character of topological band crossings in the band structure. |  |
Kosior, A.; Heyl, M. Vortex loop dynamics and dynamical quantum phase transitions in three-dimensional fermion matter Journal Article Phys. Rev. B 109, L140303 (2024), datadoi: (10.5281/zenodo.10837585). @article{kosiorVortexLoopDynamics2024,
title = {Vortex loop dynamics and dynamical quantum phase transitions in three-dimensional fermion matter},
author = {A. Kosior and M. Heyl},
url = {https://doi.org/10.1103/PhysRevB.109.L140303},
doi = {10.1103/physrevb.109.l140303},
year = {2024},
date = {2024-04-15},
urldate = {2024-04-01},
journal = {Phys. Rev. B},
volume = {109},
number = {14},
pages = {L140303},
abstract = {Over the past decade, dynamical quantum phase transitions (DQPTs) have emerged as a paradigm shift in understanding nonequilibrium quantum many-body systems. However, the challenge lies in identifying order parameters that effectively characterize the associated dynamic phases. In this study we investigate the behavior of vortex singularities in the phase of the Green's function for a broad class of fermion lattice models in three dimensions after an instantaneous quench in both interacting and noninteracting systems. We find that the full set of vortices form one-dimensional dynamical objects, which we call vortex loops. We propose that the number of such vortex loops can be interpreted as a quantized order parameter that distinguishes between different nonequilibrium phases. Our results establish an explicit link between variations in the order parameter and DQPTs in the noninteracting scenario. Moreover, we show that the vortex loops are robust in the weakly interacting case, even though there is no direct relation between the Loschmidt amplitude and the Green's function. Finally, we observe that vortex loops can form complex dynamical patterns in momentum space. Our findings provide valuable insights for developing definitions of dynamical order parameters in nonequilibrium systems.},
note = {datadoi: (10.5281/zenodo.10837585)},
keywords = {B6},
pubstate = {published},
tppubtype = {article}
}
Over the past decade, dynamical quantum phase transitions (DQPTs) have emerged as a paradigm shift in understanding nonequilibrium quantum many-body systems. However, the challenge lies in identifying order parameters that effectively characterize the associated dynamic phases. In this study we investigate the behavior of vortex singularities in the phase of the Green's function for a broad class of fermion lattice models in three dimensions after an instantaneous quench in both interacting and noninteracting systems. We find that the full set of vortices form one-dimensional dynamical objects, which we call vortex loops. We propose that the number of such vortex loops can be interpreted as a quantized order parameter that distinguishes between different nonequilibrium phases. Our results establish an explicit link between variations in the order parameter and DQPTs in the noninteracting scenario. Moreover, we show that the vortex loops are robust in the weakly interacting case, even though there is no direct relation between the Loschmidt amplitude and the Green's function. Finally, we observe that vortex loops can form complex dynamical patterns in momentum space. Our findings provide valuable insights for developing definitions of dynamical order parameters in nonequilibrium systems. |  |
Luo, M.; Trivedi, R.; Bañuls, M. C.; Cirac, J. I. Probing off-diagonal eigenstate thermalization with tensor networks Journal Article Phys. Rev. B 109, 134304 (2024). @article{luo_probing_2024,
title = {Probing off-diagonal eigenstate thermalization with tensor networks},
author = {M. Luo and R. Trivedi and M. C. Bañuls and J. I. Cirac},
doi = {10.1103/PhysRevB.109.134304},
year = {2024},
date = {2024-04-08},
urldate = {2024-04-01},
journal = {Phys. Rev. B},
volume = {109},
number = {13},
pages = {134304},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
|  |
Boesl, J.; Zechmann, P.; Feldmeier, J.; Knap, M. Deconfinement Dynamics of Fractons in Tilted Bose-Hubbard Chains Journal Article Phys. Rev. Lett. 132, 143401 (2024), datadoi: (10.5281/zenodo.10035551). @article{boeslDeconfinementDynamicsFractons2024,
title = {Deconfinement Dynamics of Fractons in Tilted Bose-Hubbard Chains},
author = {J. Boesl and P. Zechmann and J. Feldmeier and M. Knap},
url = {https://doi.org/10.1103/PhysRevLett.132.143401},
doi = {10.1103/PhysRevLett.132.143401},
year = {2024},
date = {2024-04-02},
urldate = {2024-04-02},
journal = {Phys. Rev. Lett.},
volume = {132},
number = {14},
pages = {143401},
abstract = {Fractonic constraints can lead to exotic properties of quantum many-body systems. Here, we investigate the dynamics of fracton excitations on top of the ground states of a one-dimensional, dipole-conserving Bose-Hubbard model. We show that nearby fractons undergo a collective motion mediated by exchanging virtual dipole excitations, which provides a powerful dynamical tool to characterize the underlying ground-state phases. We find that, in the gapped Mott insulating phase, fractons are confined to each other as motion requires the exchange of massive dipoles. When crossing the phase transition into a gapless Luttinger liquid of dipoles, fractons deconfine. Their transient deconfinement dynamics scales diffusively and exhibits strong but subleading contributions described by a quantum Lifshitz model. We examine prospects for the experimental realization in tilted Bose-Hubbard chains by numerically simulating the adiabatic state preparation and subsequent time evolution and find clear signatures of the low-energy fracton dynamics.},
note = {datadoi: (10.5281/zenodo.10035551)},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Fractonic constraints can lead to exotic properties of quantum many-body systems. Here, we investigate the dynamics of fracton excitations on top of the ground states of a one-dimensional, dipole-conserving Bose-Hubbard model. We show that nearby fractons undergo a collective motion mediated by exchanging virtual dipole excitations, which provides a powerful dynamical tool to characterize the underlying ground-state phases. We find that, in the gapped Mott insulating phase, fractons are confined to each other as motion requires the exchange of massive dipoles. When crossing the phase transition into a gapless Luttinger liquid of dipoles, fractons deconfine. Their transient deconfinement dynamics scales diffusively and exhibits strong but subleading contributions described by a quantum Lifshitz model. We examine prospects for the experimental realization in tilted Bose-Hubbard chains by numerically simulating the adiabatic state preparation and subsequent time evolution and find clear signatures of the low-energy fracton dynamics. |  |
Jones, D.; Östlin, A.; Weh, A.; Beiuşeanu, F.; Eckern, U.; Vitos, L.; Chioncel, L. Superconducting transition temperatures of pure vanadium and vanadium-titanium alloys in the presence of dynamical electronic correlations Journal Article Phys. Rev. B 109, 165107 (2024). @article{jones_superconducting_2024,
title = {Superconducting transition temperatures of pure vanadium and vanadium-titanium alloys in the presence of dynamical electronic correlations},
author = {D. Jones and A. Östlin and A. Weh and F. Beiuşeanu and U. Eckern and L. Vitos and L. Chioncel},
doi = {10.1103/PhysRevB.109.165107},
year = {2024},
date = {2024-04-01},
urldate = {2024-04-12},
journal = {Phys. Rev. B},
volume = {109},
number = {16},
pages = {165107},
abstract = {Ordinary superconductors are widely assumed insensitive to small concentrations of random nonmagnetic impurities, whereas strong disorder suppresses superconductivity, ultimately leading to a superconductor-insulator transition. In between these limiting cases, a most fascinating regime may emerge where disorder enhances superconductivity. This effect is discussed here for the β phase of vanadium-titanium alloys. Disorder is modeled using the coherent potential approximation while local electronic interactions are treated using dynamical mean-field theory. The McMillan formula is employed to estimate the superconducting transition temperature, showing a maximum at a Ti concentration of around 0.33 for a local Coulomb interaction U in the range of 2 eV to 3 eV. Our calculations quantitatively agree with the experimentally observed concentration-dependent increase of Tc, and its maximal value of about 20%.},
keywords = {A5},
pubstate = {published},
tppubtype = {article}
}
Ordinary superconductors are widely assumed insensitive to small concentrations of random nonmagnetic impurities, whereas strong disorder suppresses superconductivity, ultimately leading to a superconductor-insulator transition. In between these limiting cases, a most fascinating regime may emerge where disorder enhances superconductivity. This effect is discussed here for the β phase of vanadium-titanium alloys. Disorder is modeled using the coherent potential approximation while local electronic interactions are treated using dynamical mean-field theory. The McMillan formula is employed to estimate the superconducting transition temperature, showing a maximum at a Ti concentration of around 0.33 for a local Coulomb interaction U in the range of 2 eV to 3 eV. Our calculations quantitatively agree with the experimentally observed concentration-dependent increase of Tc, and its maximal value of about 20%. |  |
Zechmann, P.; Boesl, J.; Feldmeier, J.; Knap, M. Dynamical Spectral Response of Fractonic Quantum Matter Journal Article Phys. Rev. B 109, 125137 (2024), datadoi: (10.5281/zenodo.10014288). @article{zechmannDynamicalSpectralResponse2024,
title = {Dynamical Spectral Response of Fractonic Quantum Matter},
author = {P. Zechmann and J. Boesl and J. Feldmeier and M. Knap},
doi = {10.1103/physrevb.109.125137},
year = {2024},
date = {2024-03-21},
urldate = {2024-03-21},
journal = {Phys. Rev. B},
volume = {109},
number = {12},
pages = {125137},
abstract = {Quantum many-body systems with fractonic excitations can realize fascinating phases of matter. Here, we study the low-energy excitations of a constrained Bose-Hubbard model in one dimension, which conserves the center of mass or, equivalently, the dipole moment in addition to the particle number. This model is known to realize fractonic phases, including a dipole Mott insulator, a dipole Luttinger liquid, and a metastable dipole supersolid. We use tensor network methods to compute spectral functions from the dynamical response of the system and verify predictions from low-energy field theories of the corresponding ground-state phases. We demonstrate the existence of gapped excitations compatible with strong coupling results in a dipole Mott insulator, linear sound modes characteristic of a Luttinger liquid of dipoles, and soft quadratic modes at both zero and finite momenta in a supersolid state with charge density wave order and phase coherence at noninteger filling.},
note = {datadoi: (10.5281/zenodo.10014288)},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Quantum many-body systems with fractonic excitations can realize fascinating phases of matter. Here, we study the low-energy excitations of a constrained Bose-Hubbard model in one dimension, which conserves the center of mass or, equivalently, the dipole moment in addition to the particle number. This model is known to realize fractonic phases, including a dipole Mott insulator, a dipole Luttinger liquid, and a metastable dipole supersolid. We use tensor network methods to compute spectral functions from the dynamical response of the system and verify predictions from low-energy field theories of the corresponding ground-state phases. We demonstrate the existence of gapped excitations compatible with strong coupling results in a dipole Mott insulator, linear sound modes characteristic of a Luttinger liquid of dipoles, and soft quadratic modes at both zero and finite momenta in a supersolid state with charge density wave order and phase coherence at noninteger filling. |  |
Kadow, W.; Jin, H. -K.; Knolle, J.; Knap, M. Single-hole spectra of Kitaev spin liquids: From dynamical Nagaoka ferromagnetism to spin-hole fractionalization Journal Article npj Quantum Mater. 9, 32 (2024), datadoi: 10.5281/zenodo.8363616. @article{kadowSingleholeSpectraKitaev2024,
title = {Single-hole spectra of Kitaev spin liquids: From dynamical Nagaoka ferromagnetism to spin-hole fractionalization},
author = {W. Kadow and H. -K. Jin and J. Knolle and M. Knap},
url = {https://doi.org/10.1038/s41535-024-00641-7},
doi = {10.1038/s41535-024-00641-7},
year = {2024},
date = {2024-03-21},
urldate = {2024-03-21},
journal = {npj Quantum Mater.},
volume = {9},
number = {1},
pages = {32},
note = {datadoi: 10.5281/zenodo.8363616},
keywords = {B6, C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Choi, W.; Knap, M.; Pollmann, F. Finite Temperature Entanglement Negativity of Fermionic Symmetry Protected Topological Phases and Quantum Critical Points in One Dimension Journal Article Phys. Rev. B 109, 115132 (2024), datadoi: (10.5281/zenodo.10058475). @article{choiFiniteTemperatureEntanglement2024,
title = {Finite Temperature Entanglement Negativity of Fermionic Symmetry Protected Topological Phases and Quantum Critical Points in One Dimension},
author = {W. Choi and M. Knap and F. Pollmann},
url = {https://doi.org/10.1103/PhysRevB.109.115132},
doi = {10.1103/PhysRevB.109.115132},
year = {2024},
date = {2024-03-18},
urldate = {2024-03-01},
journal = {Phys. Rev. B},
volume = {109},
number = {11},
pages = {115132},
abstract = {We study the logarithmic entanglement negativity of symmetry-protected topological (SPT) phases and quantum critical points (QCPs) of one-dimensional noninteracting fermions at finite temperatures. In particular, we consider a free fermion model that realizes not only quantum phase transitions between gapped phases but also an exotic topological phase transition between quantum critical states in the form of the fermionic Lifshitz transition. The bipartite entanglement negativity between adjacent fermion blocks reveals the crossover boundary of the quantum critical fan near the QCP between two gapped phases. Along the critical phase boundary between the gapped phases, the sudden decrease in the entanglement negativity signals the fermionic Lifshitz transition responsible for the change in the topological nature of the QCPs. In addition, the tripartite entanglement negativity between spatially separated fermion blocks counts the number of topologically protected boundary modes for both SPT phases and topologically nontrivial QCPs at zero temperature. However, the long-distance entanglement between the boundary modes vanishes at finite temperatures due to the instability of SPTs, the phases themselves.},
note = {datadoi: (10.5281/zenodo.10058475)},
keywords = {C5},
pubstate = {published},
tppubtype = {article}
}
We study the logarithmic entanglement negativity of symmetry-protected topological (SPT) phases and quantum critical points (QCPs) of one-dimensional noninteracting fermions at finite temperatures. In particular, we consider a free fermion model that realizes not only quantum phase transitions between gapped phases but also an exotic topological phase transition between quantum critical states in the form of the fermionic Lifshitz transition. The bipartite entanglement negativity between adjacent fermion blocks reveals the crossover boundary of the quantum critical fan near the QCP between two gapped phases. Along the critical phase boundary between the gapped phases, the sudden decrease in the entanglement negativity signals the fermionic Lifshitz transition responsible for the change in the topological nature of the QCPs. In addition, the tripartite entanglement negativity between spatially separated fermion blocks counts the number of topologically protected boundary modes for both SPT phases and topologically nontrivial QCPs at zero temperature. However, the long-distance entanglement between the boundary modes vanishes at finite temperatures due to the instability of SPTs, the phases themselves. |  |
Kawano, M.; Pollmann, F.; Knap, M. Unconventional spin transport in strongly correlated kagome systems Journal Article Phys. Rev. B 109, L121111 (2024), datadoi: 10.5281/zenodo.8183105. @article{kawanoUnconventionalSpinTransport2024,
title = {Unconventional spin transport in strongly correlated kagome systems},
author = {M. Kawano and F. Pollmann and M. Knap},
url = {https://doi.org/10.1103/PhysRevB.109.L121111},
doi = {10.1103/physrevb.109.l121111},
issn = {2469-9969},
year = {2024},
date = {2024-03-18},
urldate = {2024-03-01},
journal = {Phys. Rev. B},
volume = {109},
number = {12},
pages = {L121111},
publisher = {American Physical Society (APS)},
note = {datadoi: 10.5281/zenodo.8183105},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
|  |
Solana-Madruga, E.; Mentre, O.; Tsirlin, A. A.; Huve, M.; Khalyavin, D.; Ritter, C.; Arevalo-Lopez, A. M. CoVO3 High-Pressure Polymorphs: To Order or Not to Order? Journal Article Adv. Sci. 11, 2307766 (2024). @article{solana-madruga_covo_3_2023,
title = {CoVO_{3} High-Pressure Polymorphs: To Order or Not to Order?},
author = {E. Solana-Madruga and O. Mentre and A. A. Tsirlin and M. Huve and D. Khalyavin and C. Ritter and A. M. Arevalo-Lopez},
doi = {10.1002/advs.202307766},
year = {2024},
date = {2024-03-06},
urldate = {2023-12-01},
journal = {Adv. Sci.},
volume = {11},
number = {9},
pages = {2307766},
abstract = {Materials properties are determined by their compositions and structures. In ABO(3) oxides different cation orderings lead to mainly perovskite- or corundum like derivatives with exciting physical properties. Sometimes, a material can be stabilized in more than one structural modification, providing a unique opportunity to explore structure-properties relationship. Here, CoVO3 obtained in both ilmenite-(CoVO3-I) and LiNbO3-type (CoVO3-II) polymorphs at moderate (8-12 GPa) and high pressures (22 GPa), respectively are presented. Their distinctive cation distributions affect drastically the magnetic properties as CoVO3-II shows a cluster-glass behavior while CoVO3-I hosts a honeycomb zigzag magnetic structure in the cobalt network. First principles calculations show that the influence of vanadium is crucial for CoVO3-I, although it is previously considered as non-magnetic in a dimerized spin-singlet state. Contrarily, CoVO3-II shows two independent interpenetrating antiferromagnetic Co- and ferromagnetic V-hcp sublattices, which intrinsically frustrate any possible magnetic order. CoVO3-II is also remarkable as the first oxide crystallizing with the LiNbO3-type structure where both metals contain free d electrons. CoVO3 polymorphs pinpoint therefore as well to a much broader phase field of high-pressure A-site Cobaltites.},
keywords = {B1, B3},
pubstate = {published},
tppubtype = {article}
}
Materials properties are determined by their compositions and structures. In ABO(3) oxides different cation orderings lead to mainly perovskite- or corundum like derivatives with exciting physical properties. Sometimes, a material can be stabilized in more than one structural modification, providing a unique opportunity to explore structure-properties relationship. Here, CoVO3 obtained in both ilmenite-(CoVO3-I) and LiNbO3-type (CoVO3-II) polymorphs at moderate (8-12 GPa) and high pressures (22 GPa), respectively are presented. Their distinctive cation distributions affect drastically the magnetic properties as CoVO3-II shows a cluster-glass behavior while CoVO3-I hosts a honeycomb zigzag magnetic structure in the cobalt network. First principles calculations show that the influence of vanadium is crucial for CoVO3-I, although it is previously considered as non-magnetic in a dimerized spin-singlet state. Contrarily, CoVO3-II shows two independent interpenetrating antiferromagnetic Co- and ferromagnetic V-hcp sublattices, which intrinsically frustrate any possible magnetic order. CoVO3-II is also remarkable as the first oxide crystallizing with the LiNbO3-type structure where both metals contain free d electrons. CoVO3 polymorphs pinpoint therefore as well to a much broader phase field of high-pressure A-site Cobaltites. |  |
Daul, W. G.; Hirrle, M.; Eisfeld, B.; Kraft, M.; von Nidda, H. -A. Krug; Volkmer, D. Heteropentanuclear Ru(II)Cu(II)4 Kuratowski Complexes Assembled from a Ruthenium(II) Precursor Complex to Study Competing Exchange Interactions in M(II)(ta)2 Networks [ta(−) = 1,2,3-Triazolate] Journal Article Inorg. Chem. 63, 5027–5039 (2024), datadoi: 10.1021/acs.inorgchem.3c04478. @article{daulHeteropentanuclearRuIICuII4Kuratowski2024,
title = {Heteropentanuclear Ru(II)Cu(II)4 Kuratowski Complexes Assembled from a Ruthenium(II) Precursor Complex to Study Competing Exchange Interactions in M(II)(ta)2 Networks [ta(−) = 1,2,3-Triazolate]},
author = {W. G. Daul and M. Hirrle and B. Eisfeld and M. Kraft and H. -A. Krug von Nidda and D. Volkmer},
url = {https://doi.org/10.1021/acs.inorgchem.3c04478},
doi = {10.1021/acs.inorgchem.3c04478},
year = {2024},
date = {2024-03-05},
urldate = {2024-03-01},
journal = {Inorg. Chem.},
volume = {63},
number = {11},
pages = {5027–5039},
abstract = {We report a directed two-step synthesis toward pentanuclear Kuratowski complexes. First, six 5,6-dimethylbenzo[1,2,3]triazole ligands (Me2btaH) are coordinated to a single Ru(II) ion, providing a topologically ideal template for the addition of further metal ions. The synthesis and crystal structures of [RuCu4X4(Me2bta)6] [X = acetylacetonate (acac) and tris(3,5-dimethyl-1-pyrazolyl)borate (Tp*)] are described. Both represent new members of the family of so-called Kuratowski (K3,3) complexes. The coordination units feature triazolato-bridged metal-centered MM4 tetrahedra, which are known for frustrated magnetic interactions in both complexes and metal–organic frameworks. The novel Ru(II)-centered complexes were synthesized in order to investigate the influence of the presence or absence of a paramagnetic central metal ion in the Kuratowski complex. Superconducting quantum interference device and electron spin resonance measurements demonstrate that small deviations in bond lengths and valence angles can lead to the formation of pairs of magnetic exchange-coupled Cu(II) ions. Which Cu(II) ions pair up can be predicted in Jahn–Teller active compounds by the overlap of the respective orbitals. These data are compared with those gleaned for M(II)(ta)2 (ta = 1,2,3-triazolate) lattices, in which structurally similar MM4 tetrahedra constitute the secondary building units.},
note = {datadoi: 10.1021/acs.inorgchem.3c04478},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
We report a directed two-step synthesis toward pentanuclear Kuratowski complexes. First, six 5,6-dimethylbenzo[1,2,3]triazole ligands (Me2btaH) are coordinated to a single Ru(II) ion, providing a topologically ideal template for the addition of further metal ions. The synthesis and crystal structures of [RuCu4X4(Me2bta)6] [X = acetylacetonate (acac) and tris(3,5-dimethyl-1-pyrazolyl)borate (Tp*)] are described. Both represent new members of the family of so-called Kuratowski (K3,3) complexes. The coordination units feature triazolato-bridged metal-centered MM4 tetrahedra, which are known for frustrated magnetic interactions in both complexes and metal–organic frameworks. The novel Ru(II)-centered complexes were synthesized in order to investigate the influence of the presence or absence of a paramagnetic central metal ion in the Kuratowski complex. Superconducting quantum interference device and electron spin resonance measurements demonstrate that small deviations in bond lengths and valence angles can lead to the formation of pairs of magnetic exchange-coupled Cu(II) ions. Which Cu(II) ions pair up can be predicted in Jahn–Teller active compounds by the overlap of the respective orbitals. These data are compared with those gleaned for M(II)(ta)2 (ta = 1,2,3-triazolate) lattices, in which structurally similar MM4 tetrahedra constitute the secondary building units. | ![Heteropentanuclear Ru(II)Cu(II)4 Kuratowski Complexes Assembled from a Ruthenium(II) Precursor Complex to Study Competing Exchange Interactions in M(II)(ta)2 Networks [ta(−) = 1,2,3-Triazolate]](https://www.trr360.de/wp-content/uploads/2024/03/CQM_Logo_BB.png) |
d'Ornellas, P.; Knolle, J. Kitaev-Heisenberg model on the star lattice: From chiral Majorana fermions to chiral triplons Journal Article Phys. Rev. B 109, 094421 (2024). @article{dornellas_kitaev-heisenberg_2024,
title = {Kitaev-Heisenberg model on the star lattice: From chiral Majorana fermions to chiral triplons},
author = {P. d'Ornellas and J. Knolle},
doi = {10.1103/PhysRevB.109.094421},
year = {2024},
date = {2024-03-01},
urldate = {2024-04-12},
journal = {Phys. Rev. B},
volume = {109},
number = {9},
pages = {094421},
abstract = {The interplay of frustrated interactions and lattice geometry can lead to a variety of exotic quantum phases. Here we unearth a particularly rich phase diagram of the Kitaev-Heisenberg model on the star lattice, a triangle decorated honeycomb lattice breaking sublattice symmetry. In the antiferromagnetic regime, the interplay of Heisenberg coupling and geometric frustration leads to the formation of valence bond solid (VBS) phases—a singlet VBS and a bond selective triplet VBS stabilized by the Kitaev exchange. We show that the ratio of the Kitaev versus Heisenberg exchange tunes between these VBS phases and chiral quantum spin-liquid regimes. Remarkably, the VBS phases host a whole variety of chiral triplon excitations with high Chern numbers in the presence of a weak magnetic field. We discuss our results in light of a recently synthesized star lattice material and other decorated lattice systems.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
The interplay of frustrated interactions and lattice geometry can lead to a variety of exotic quantum phases. Here we unearth a particularly rich phase diagram of the Kitaev-Heisenberg model on the star lattice, a triangle decorated honeycomb lattice breaking sublattice symmetry. In the antiferromagnetic regime, the interplay of Heisenberg coupling and geometric frustration leads to the formation of valence bond solid (VBS) phases—a singlet VBS and a bond selective triplet VBS stabilized by the Kitaev exchange. We show that the ratio of the Kitaev versus Heisenberg exchange tunes between these VBS phases and chiral quantum spin-liquid regimes. Remarkably, the VBS phases host a whole variety of chiral triplon excitations with high Chern numbers in the presence of a weak magnetic field. We discuss our results in light of a recently synthesized star lattice material and other decorated lattice systems. | |
Wang, L.; Liu, H.; Zimmermann, V.; Yogi, A. K.; Isobe, M.; Minola, M.; Hepting, M.; Khaliullin, G.; Keimer, B. Spin-Orbit Excitons in a Correlated Metal: Raman Scattering Study of Sr2RhO4 Journal Article Phys. Rev. Lett. 132, 116502 (2024). @article{wang_spin-orbit_2024,
title = {Spin-Orbit Excitons in a Correlated Metal: Raman Scattering Study of Sr_{2}RhO_{4}},
author = {L. Wang and H. Liu and V. Zimmermann and A. K. Yogi and M. Isobe and M. Minola and M. Hepting and G. Khaliullin and B. Keimer},
doi = {10.1103/PhysRevLett.132.116502},
year = {2024},
date = {2024-03-01},
urldate = {2024-03-01},
journal = {Phys. Rev. Lett.},
volume = {132},
number = {11},
pages = {116502},
abstract = {Using Raman spectroscopy to study the correlated 4d-electron metal Sr2RhO4, we observe pronounced excitations at 220 meV and 240 meV with A1g and B1g symmetries, respectively. We identify them as transitions between the spin-orbit multiplets of the Rh ions, in close analogy to the spin-orbit excitons in the Mott insulators Sr2IrO4 and α−RuCl3. This observation provides direct evidence for the unquenched spin-orbit coupling in Sr2RhO4. A quantitative analysis of the data reveals that the tetragonal crystal field Δ in Sr2RhO4 has a sign opposite to that in insulating Sr2IrO4, which enhances the planar xy orbital character of the effective J=1/2 wave function. This supports a metallic ground state, and suggests that c-axis compression of Sr2RhO4 may transform it into a quasi-two-dimensional antiferromagnetic insulator.},
keywords = {B2},
pubstate = {published},
tppubtype = {article}
}
Using Raman spectroscopy to study the correlated 4d-electron metal Sr2RhO4, we observe pronounced excitations at 220 meV and 240 meV with A1g and B1g symmetries, respectively. We identify them as transitions between the spin-orbit multiplets of the Rh ions, in close analogy to the spin-orbit excitons in the Mott insulators Sr2IrO4 and α−RuCl3. This observation provides direct evidence for the unquenched spin-orbit coupling in Sr2RhO4. A quantitative analysis of the data reveals that the tetragonal crystal field Δ in Sr2RhO4 has a sign opposite to that in insulating Sr2IrO4, which enhances the planar xy orbital character of the effective J=1/2 wave function. This supports a metallic ground state, and suggests that c-axis compression of Sr2RhO4 may transform it into a quasi-two-dimensional antiferromagnetic insulator. |  |
Simeth, W.; Rahn, M. C.; Bauer, A.; Meven, M.; Pfleiderer, C. Topological aspects of multi-k antiferromagnetism in cubic rare-earth compounds Journal Article J. Phys.: Condens. Matter 36, 215602 (2024), datadoi: (10.5281/zenodo.10047782). @article{simethTopologicalAspectsMultik2024,
title = {Topological aspects of multi-k antiferromagnetism in cubic rare-earth compounds},
author = {W. Simeth and M. C. Rahn and A. Bauer and M. Meven and C. Pfleiderer},
doi = {10.1088/1361-648x/ad24bb},
year = {2024},
date = {2024-02-29},
urldate = {2024-02-29},
journal = {J. Phys.: Condens. Matter},
volume = {36},
number = {21},
pages = {215602},
abstract = {We advertise rare-earth intermetallics with high-symmetry crystal structures and competing interactions as a possible materials platform hosting spin structures with non-trivial topological properties. Focusing on the series of cubic RCu compounds, where R = Ho, Er, Tm, the bulk properties of these systems display exceptionally rich magnetic phase diagrams hosting an abundance of different phase pockets characteristic of antiferromagnetic order in the presence of delicately balanced interactions. The electrical transport properties exhibit large anomalous contributions suggestive of topologically non-trivial winding in the electronic and magnetic structures. Neutron diffraction identifies spontaneous long-range magnetic order in terms of commensurate and incommensurate variations of
antiferromagnetism with the possibility for various multi-k configurations. Motivated by general trends in these materials, we discuss the possible existence of topologically non-trivial winding in real and reciprocal space in the class of RCu compounds including antiferromagnetic skyrmion lattices. Putatively bringing together different limits of non-trivial topological winding in the same material, the combination of properties in RCu systems promises access to advanced functionalities.},
note = {datadoi: (10.5281/zenodo.10047782)},
keywords = {C1},
pubstate = {published},
tppubtype = {article}
}
We advertise rare-earth intermetallics with high-symmetry crystal structures and competing interactions as a possible materials platform hosting spin structures with non-trivial topological properties. Focusing on the series of cubic RCu compounds, where R = Ho, Er, Tm, the bulk properties of these systems display exceptionally rich magnetic phase diagrams hosting an abundance of different phase pockets characteristic of antiferromagnetic order in the presence of delicately balanced interactions. The electrical transport properties exhibit large anomalous contributions suggestive of topologically non-trivial winding in the electronic and magnetic structures. Neutron diffraction identifies spontaneous long-range magnetic order in terms of commensurate and incommensurate variations of
antiferromagnetism with the possibility for various multi-k configurations. Motivated by general trends in these materials, we discuss the possible existence of topologically non-trivial winding in real and reciprocal space in the class of RCu compounds including antiferromagnetic skyrmion lattices. Putatively bringing together different limits of non-trivial topological winding in the same material, the combination of properties in RCu systems promises access to advanced functionalities. |  |
Leeb, V.; Knolle, J. Interband scattering-and nematicity-induced quantum oscillation frequency in FeSe Journal Article Phys. Rev. B 109, L081109 (2024), datadoi: 10.5281/zenodo.8225406. @article{leebInterbandScatteringandNematicityinduced2024,
title = {Interband scattering-and nematicity-induced quantum oscillation frequency in FeSe},
author = {V. Leeb and J. Knolle},
url = {https://doi.org/10.1103/PhysRevB.109.L081109},
doi = {10.1103/physrevb.109.l081109},
year = {2024},
date = {2024-02-24},
urldate = {2024-02-01},
journal = {Phys. Rev. B},
volume = {109},
number = {8},
pages = {L081109},
abstract = {Understanding the nematic phase observed in the iron-chalcogenide materials is crucial for describing their superconducting pairing. Experiments on FeSe1−𝑥S𝑥 showed that one of the slow Shubnikov-de Haas quantum oscillation frequencies disappears when tuning the material out of the nematic phase via chemical substitution or pressure, which has been interpreted as a Lifshitz transition [Coldea et al., npj Quantum Mater. 4, 2 (2019); Reiss et al., Nat. Phys. 16, 89 (2020)]. Here, we present a generic, alternative scenario for a nematicity-induced sharp quantum oscillation frequency, which disappears in the tetragonal phase and is not connected to an underlying Fermi surface pocket. We show that different microscopic interband scattering mechanisms—for example, orbital-selective scattering—in conjunction with nematic order can give rise to this quantum oscillation frequency beyond the standard Onsager relation. We discuss implications for iron-chalcogenides and the interpretation of quantum oscillations in other correlated materials.},
note = {datadoi: 10.5281/zenodo.8225406},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Understanding the nematic phase observed in the iron-chalcogenide materials is crucial for describing their superconducting pairing. Experiments on FeSe1−𝑥S𝑥 showed that one of the slow Shubnikov-de Haas quantum oscillation frequencies disappears when tuning the material out of the nematic phase via chemical substitution or pressure, which has been interpreted as a Lifshitz transition [Coldea et al., npj Quantum Mater. 4, 2 (2019); Reiss et al., Nat. Phys. 16, 89 (2020)]. Here, we present a generic, alternative scenario for a nematicity-induced sharp quantum oscillation frequency, which disappears in the tetragonal phase and is not connected to an underlying Fermi surface pocket. We show that different microscopic interband scattering mechanisms—for example, orbital-selective scattering—in conjunction with nematic order can give rise to this quantum oscillation frequency beyond the standard Onsager relation. We discuss implications for iron-chalcogenides and the interpretation of quantum oscillations in other correlated materials. | |
Hu, Y.; Ma, J.; Li, Y.; Jiang, Y.; Gawryluk, D. J.; Hu, T.; Teyssier, J.; Multian, V.; Yin, Z.; Xu, S.; others, Phonon promoted charge density wave in topological kagome metal ScV6Sn6 Journal Article Nat. Commun. 15, 1658 (2024), datadoi: 10.24435/materialscloud:mz-ng. @article{huPhononPromotedCharge2024,
title = {Phonon promoted charge density wave in topological kagome metal ScV_{6}Sn_{6}},
author = {Y. Hu and J. Ma and Y. Li and Y. Jiang and D. J. Gawryluk and T. Hu and J. Teyssier and V. Multian and Z. Yin and S. Xu and others},
url = {https://doi.org/10.1038/s41467-024-45859-y},
doi = {10.1038/s41467-024-45859-y},
year = {2024},
date = {2024-02-23},
urldate = {2024-02-01},
journal = {Nat. Commun.},
volume = {15},
number = {1},
pages = {1658},
abstract = {Charge density wave (CDW) orders in vanadium-based kagome metals have recently received tremendous attention, yet their origin remains a topic of debate. The discovery of ScV6Sn6, a bilayer kagome metal featuring an intriguing sqrt(3)xsqrt(3)x3 CDW order, offers a novel platform to explore the underlying mechanism behind the unconventional CDW. Here, we combine high-resolution angle-resolved photoemission spectroscopy, Raman scattering and density functional theory to investigate the electronic structure and phonon modes of ScV6Sn6. We identify topologically nontrivial surface states and multiple van Hove singularities (VHSs) in the vicinity of the Fermi level, with one VHS aligning with the in-plane component of the CDW vector near the K point. Additionally, Raman measurements indicate a strong electron-phonon coupling, as evidenced by a two-phonon mode and new emergent modes. Our findings highlight the fundamental role of lattice degrees of freedom in promoting the CDW in ScV6Sn6.},
note = {datadoi: 10.24435/materialscloud:mz-ng},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
Charge density wave (CDW) orders in vanadium-based kagome metals have recently received tremendous attention, yet their origin remains a topic of debate. The discovery of ScV6Sn6, a bilayer kagome metal featuring an intriguing sqrt(3)xsqrt(3)x3 CDW order, offers a novel platform to explore the underlying mechanism behind the unconventional CDW. Here, we combine high-resolution angle-resolved photoemission spectroscopy, Raman scattering and density functional theory to investigate the electronic structure and phonon modes of ScV6Sn6. We identify topologically nontrivial surface states and multiple van Hove singularities (VHSs) in the vicinity of the Fermi level, with one VHS aligning with the in-plane component of the CDW vector near the K point. Additionally, Raman measurements indicate a strong electron-phonon coupling, as evidenced by a two-phonon mode and new emergent modes. Our findings highlight the fundamental role of lattice degrees of freedom in promoting the CDW in ScV6Sn6. |  |
Romen, A.; Birnkammer, S.; Knap, M. Deconfined quantum criticality in the long-range, anisotropic Heisenberg chain Journal Article SciPost Phys. Core 7, 008 (2024), datadoi: 10.5281/zenodo.10102981. @article{romenDeconfinedQuantumCriticality2024,
title = {Deconfined quantum criticality in the long-range, anisotropic Heisenberg chain},
author = {A. Romen and S. Birnkammer and M. Knap},
url = {https://scipost.org/10.21468/SciPostPhysCore.7.1.008},
doi = {10.21468/scipostphyscore.7.1.008},
year = {2024},
date = {2024-02-22},
urldate = {2024-02-22},
journal = {SciPost Phys. Core},
volume = {7},
number = {1},
pages = {008},
abstract = {Deconfined quantum criticality describes continuous phase transitions that are not captured by the Landau-Ginzburg paradigm. Here, we investigate deconfined quantum critical points in the long-range, anisotropic Heisenberg chain. With matrix product state simulations, we show that the model undergoes a continuous phase transition from a valence bond solid to an antiferromagnet. We extract the critical exponents of the transition and connect them to an effective field theory obtained from bosonization techniques. We show that beyond stabilizing the valance bond order, the long-range interactions are irrelevant and the transition is well described by a double frequency sine-Gordon model. We propose how to realize and probe deconfined quantum criticality in our model with trapped-ion quantum simulators.},
note = {datadoi: 10.5281/zenodo.10102981},
keywords = {C5, C6},
pubstate = {published},
tppubtype = {article}
}
Deconfined quantum criticality describes continuous phase transitions that are not captured by the Landau-Ginzburg paradigm. Here, we investigate deconfined quantum critical points in the long-range, anisotropic Heisenberg chain. With matrix product state simulations, we show that the model undergoes a continuous phase transition from a valence bond solid to an antiferromagnet. We extract the critical exponents of the transition and connect them to an effective field theory obtained from bosonization techniques. We show that beyond stabilizing the valance bond order, the long-range interactions are irrelevant and the transition is well described by a double frequency sine-Gordon model. We propose how to realize and probe deconfined quantum criticality in our model with trapped-ion quantum simulators. |  |
Müller, M.; Weber, J.; Engelhardt, F.; Bittencourt, V. A. S. V.; Luschmann, T.; Cherkasskii, M.; Opel, M.; Goennenwein, S. T. B.; Kusminskiy, S. V.; Geprägs, S.; Gross, R.; Althammer, M.; Huebl, H. Chiral phonons and phononic birefringence in ferromagnetic metal–bulk acoustic resonator hybrids Journal Article Phys. Rev. B 109, 024430 (2024). @article{muller_chiral_2024,
title = {Chiral phonons and phononic birefringence in ferromagnetic metal–bulk acoustic resonator hybrids},
author = {M. Müller and J. Weber and F. Engelhardt and V. A. S. V. Bittencourt and T. Luschmann and M. Cherkasskii and M. Opel and S. T. B. Goennenwein and S. V. Kusminskiy and S. Geprägs and R. Gross and M. Althammer and H. Huebl},
doi = {10.1103/PhysRevB.109.024430},
year = {2024},
date = {2024-01-23},
urldate = {2024-01-01},
journal = {Phys. Rev. B},
volume = {109},
number = {2},
pages = {024430},
abstract = {Magnomechanical devices, in which magnetic excitations couple to mechanical vibrations, have been discussed as efficient and broadband microwave signal transducers in the classical and quantum limit. We experimentally investigate the resonant magnetoelastic coupling between the ferromagnetic resonance modes in metallic Co25Fe75 thin films, featuring ultralow magnetic damping as well as sizable magnetostriction, and standing transverse elastic phonon modes in sapphire, silicon, and gadolinium gallium garnet at cryogenic temperatures. For all substrates, we observe a coherent interaction between the acoustic and magnetic modes. We identify the phonon modes as transverse shear waves propagating with slightly different velocities (Δv/v≃10−5); i.e., all investigated substrates show potential for phononic birefringence as well as phonon-mediated angular momentum transport. Our magnon-phonon hybrid systems operate in a coupling regime analogous to the Purcell enhanced damping in cavity magnonics.},
keywords = {C3},
pubstate = {published},
tppubtype = {article}
}
Magnomechanical devices, in which magnetic excitations couple to mechanical vibrations, have been discussed as efficient and broadband microwave signal transducers in the classical and quantum limit. We experimentally investigate the resonant magnetoelastic coupling between the ferromagnetic resonance modes in metallic Co25Fe75 thin films, featuring ultralow magnetic damping as well as sizable magnetostriction, and standing transverse elastic phonon modes in sapphire, silicon, and gadolinium gallium garnet at cryogenic temperatures. For all substrates, we observe a coherent interaction between the acoustic and magnetic modes. We identify the phonon modes as transverse shear waves propagating with slightly different velocities (Δv/v≃10−5); i.e., all investigated substrates show potential for phononic birefringence as well as phonon-mediated angular momentum transport. Our magnon-phonon hybrid systems operate in a coupling regime analogous to the Purcell enhanced damping in cavity magnonics. |  |
Zhao, K.; Tokiwa, Y.; Chen, H.; Gegenwart, P. Discrete degeneracies distinguished by the anomalous Hall effect in a metallic kagome ice compound Journal Article Nat. Phys. 20, 442 (2024), datadoi: 10.1038/s41567-023-02307-w. @article{zhaoDiscreteDegeneraciesDistinguished2024,
title = {Discrete degeneracies distinguished by the anomalous Hall effect in a metallic kagome ice compound},
author = {K. Zhao and Y. Tokiwa and H. Chen and P. Gegenwart},
url = {https://doi.org/10.1038/s41567-023-02307-w},
doi = {10.1038/s41567-023-02307-w},
year = {2024},
date = {2024-01-10},
urldate = {2024-01-01},
journal = {Nat. Phys.},
volume = {20},
pages = {442},
abstract = {In magnetic crystals, despite the explicit breaking of time-reversal symmetry, two equilibrium states related by time reversal are always energetically degenerate. In ferromagnets, this time-reversal degeneracy is reflected in the hysteresis of the magnetic field dependence of the magnetization and, if metallic, in that of the anomalous Hall effect (AHE). Under time-reversal, both these quantities change signs but not their magnitude. Here we show that a time-reversal-like degeneracy appears in the metallic kagome spin ice HoAgGe when magnetic fields are applied parallel to the kagome plane. We find vanishing hysteresis in the field dependence of the magnetization at low temperature, but finite hysteresis in the field-dependent AHE. This suggests the emergence of states with nearly the same energy and net magnetization but different sizes of the AHE and of the longitudinal magnetoresistance. By analysing the experimental data and a minimal tight-binding model, we identify a time-reversal-like operation connecting these near-degenerate states, which is related to the non-trivial distortion of the kagome lattice in HoAgGe. Our work demonstrates the diagnostic power of transport phenomena for identifying hidden symmetries in frustrated spin systems. Transport measurements of the metallic kagome spin ice HoAgGe show that it has an emergent discrete symmetry that is not apparent from measurements of its magnetization.},
note = {datadoi: 10.1038/s41567-023-02307-w},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
In magnetic crystals, despite the explicit breaking of time-reversal symmetry, two equilibrium states related by time reversal are always energetically degenerate. In ferromagnets, this time-reversal degeneracy is reflected in the hysteresis of the magnetic field dependence of the magnetization and, if metallic, in that of the anomalous Hall effect (AHE). Under time-reversal, both these quantities change signs but not their magnitude. Here we show that a time-reversal-like degeneracy appears in the metallic kagome spin ice HoAgGe when magnetic fields are applied parallel to the kagome plane. We find vanishing hysteresis in the field dependence of the magnetization at low temperature, but finite hysteresis in the field-dependent AHE. This suggests the emergence of states with nearly the same energy and net magnetization but different sizes of the AHE and of the longitudinal magnetoresistance. By analysing the experimental data and a minimal tight-binding model, we identify a time-reversal-like operation connecting these near-degenerate states, which is related to the non-trivial distortion of the kagome lattice in HoAgGe. Our work demonstrates the diagnostic power of transport phenomena for identifying hidden symmetries in frustrated spin systems. Transport measurements of the metallic kagome spin ice HoAgGe show that it has an emergent discrete symmetry that is not apparent from measurements of its magnetization. |  |
Wu, X.; Chakraborty, D.; Schnyder, A. P.; Greco, A. Crossover between electron-electron and electron-phonon mediated pairing on the Kagome lattice Journal Article Phys. Rev. B 109, 014517 (2024). @article{wu_crossover_2024,
title = {Crossover between electron-electron and electron-phonon mediated pairing on the Kagome lattice},
author = {X. Wu and D. Chakraborty and A. P. Schnyder and A. Greco},
doi = {10.1103/physrevb.109.014517},
year = {2024},
date = {2024-01-01},
urldate = {2024-01-01},
journal = {Phys. Rev. B},
volume = {109},
number = {1},
pages = {014517},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
|  |
Kutko, K.; Bernáth, B.; Khrustalyov, V.; Young, O.; Engelkamp, H.; Christianen, P. C. M.; Prodan, L.; Skourski, Y.; Pourovskii, L. V.; Khmelevskyi, S.; Kamenskyi, D. High-field magnetization of KEr(MoO4)2 Journal Article Phys. Rev. B 109, 024438 (2024). @article{kutko_high-field_2024,
title = {High-field magnetization of KEr(MoO_{4})_{2}},
author = {K. Kutko and B. Bernáth and V. Khrustalyov and O. Young and H. Engelkamp and P. C. M. Christianen and L. Prodan and Y. Skourski and L. V. Pourovskii and S. Khmelevskyi and D. Kamenskyi},
doi = {10.1103/PhysRevB.109.024438},
year = {2024},
date = {2024-01-01},
urldate = {2024-01-01},
journal = {Phys. Rev. B},
volume = {109},
number = {2},
pages = {024438},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
| |
Alpin, K. Perturbative description of high-T_c superconductivity in the Hubbard model via unitary transformation and classical spins Unpublished (2024), arXiv.2403.09765. @unpublished{alpin_perturbative_2024,
title = {Perturbative description of high-T_c superconductivity in the Hubbard model via unitary transformation and classical spins},
author = {K. Alpin},
doi = {10.48550/arXiv.2403.09765},
year = {2024},
date = {2024-03-01},
urldate = {2024-04-12},
abstract = {A unitary transformation is applied to the Hubbard model, which maps the Hubbard interaction to a single particle term. The resulting Hamiltonian consists of unconstrained fermions, which is then mapped to a Hamiltonian of spinless fermions coupled to pseudospins. The fermions are integrated out using second order perturbation theory in $1/U$, resulting in an effective spin Hamiltonian. An order parameter is identified, stabilizing d-wave superconductivity. The groundstate energy of classical spin configurations is minimized at a finite value of this order parameter after a critical chemical potential, resulting in d-wave superconductivity at non-zero doping. This suggests, that the onset of high-$T_c$ superconductivity is governed by the groundstate of a classical spin system.},
note = {arXiv.2403.09765},
keywords = {},
pubstate = {published},
tppubtype = {unpublished}
}
A unitary transformation is applied to the Hubbard model, which maps the Hubbard interaction to a single particle term. The resulting Hamiltonian consists of unconstrained fermions, which is then mapped to a Hamiltonian of spinless fermions coupled to pseudospins. The fermions are integrated out using second order perturbation theory in $1/U$, resulting in an effective spin Hamiltonian. An order parameter is identified, stabilizing d-wave superconductivity. The groundstate energy of classical spin configurations is minimized at a finite value of this order parameter after a critical chemical potential, resulting in d-wave superconductivity at non-zero doping. This suggests, that the onset of high-$T_c$ superconductivity is governed by the groundstate of a classical spin system. |  |
2023
|
Panther, A.; Tsirlin, A. A.; Rousochatzakis, I. Frustration relief and reorientation transition in the kagomelike dolerophanite Cu2OSO4 Journal Article Phys. Rev. B 108, 224410 (2023), datadoi: 10.5281/zenodo.8219316. @article{pantherFrustrationReliefReorientation2023,
title = {Frustration relief and reorientation transition in the kagomelike dolerophanite Cu_{2}OSO_{4}},
author = {A. Panther and A. A. Tsirlin and I. Rousochatzakis},
url = {https://doi.org/10.1103/PhysRevB.108.224410},
doi = {10.1103/PhysRevB.108.224410},
year = {2023},
date = {2023-12-06},
urldate = {2023-12-01},
journal = {Phys. Rev. B},
volume = {108},
number = {22},
pages = {224410},
abstract = {We present a theoretical study of dolerophanite Cu2OSO4, a layered kagomelike spin-21 magnetic insulator that can be described either as a system of chains coupled through dimers or as a kagome lattice where every third spin is replaced by a ferromagnetic spin dimer. Building on insights from ab initio calculations, classical numerical minimizations, and semiclassical expansions, we arrive at a minimal microscopic description that accounts for the experimental data reported so far, including the nature of the magnetic order, the reported spin length, and the observed anisotropy. The latter arises by a peculiar competition between the antisymmetric (DzyaloshinskiiMoriya) and the symmetric part of the exchange anisotropy, which gives rise to a two-step reorientation process involving two successive continuous phase transitions. In this paper, we uncover mechanisms stabilizing canted ferrimagnetic order in kagome systems and highlight strong magnetic anisotropy in the presence of dissimilar magnetic orbitals on crystallographically nonequivalent Cu sites. We also show how these anisotropy terms affect the spin-wave spectrum and how they can be tracked experimentally.},
note = {datadoi: 10.5281/zenodo.8219316},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
We present a theoretical study of dolerophanite Cu2OSO4, a layered kagomelike spin-21 magnetic insulator that can be described either as a system of chains coupled through dimers or as a kagome lattice where every third spin is replaced by a ferromagnetic spin dimer. Building on insights from ab initio calculations, classical numerical minimizations, and semiclassical expansions, we arrive at a minimal microscopic description that accounts for the experimental data reported so far, including the nature of the magnetic order, the reported spin length, and the observed anisotropy. The latter arises by a peculiar competition between the antisymmetric (DzyaloshinskiiMoriya) and the symmetric part of the exchange anisotropy, which gives rise to a two-step reorientation process involving two successive continuous phase transitions. In this paper, we uncover mechanisms stabilizing canted ferrimagnetic order in kagome systems and highlight strong magnetic anisotropy in the presence of dissimilar magnetic orbitals on crystallographically nonequivalent Cu sites. We also show how these anisotropy terms affect the spin-wave spectrum and how they can be tracked experimentally. |  |
Breitner, F. A.; Kaiser, J.; Jesche, A.; Gegenwart, P. Metallic conductivity in Na-deficient structural domain walls in the spin-orbit Mott insulator Na2IrO3 Journal Article Phys. Rev. B 108, 235130 (2023). @article{breitner_metallic_2023,
title = {Metallic conductivity in Na-deficient structural domain walls in the spin-orbit Mott insulator Na_{2}IrO_{3}},
author = {F. A. Breitner and J. Kaiser and A. Jesche and P. Gegenwart},
doi = {10.1103/PhysRevB.108.235130},
year = {2023},
date = {2023-12-01},
urldate = {2023-12-01},
journal = {Phys. Rev. B},
volume = {108},
number = {23},
pages = {235130},
abstract = {Honeycomb Na2IrO3 is a prototype spin-orbit Mott insulator and Kitaev magnet. We report a combined structural and electrical resistivity study of Na2IrO3 single crystals. Laue back-scattering diffraction indicates twinning with +/- 120 degrees rotation around the c* axis while scanning electron microscopy displays nanothin lines parallel to all three b-axis orientations of twin domains. Energy dispersive x-ray analysis line scans across such domain walls indicate no change of the Ir signal intensity, i.e., intact honeycomb layers, while the Na intensity is reduced down to similar to 2/3 of its original value at the domain walls, implying significant hole doping. Utilizing focused-ion-beam microsectioning, the temperature dependence of the electrical resistance of individual domain walls is studied. It demonstrates the tuning through the metal-insulator transition into a correlated-metal ground state by increasing hole doping.},
keywords = {B1},
pubstate = {published},
tppubtype = {article}
}
Honeycomb Na2IrO3 is a prototype spin-orbit Mott insulator and Kitaev magnet. We report a combined structural and electrical resistivity study of Na2IrO3 single crystals. Laue back-scattering diffraction indicates twinning with +/- 120 degrees rotation around the c* axis while scanning electron microscopy displays nanothin lines parallel to all three b-axis orientations of twin domains. Energy dispersive x-ray analysis line scans across such domain walls indicate no change of the Ir signal intensity, i.e., intact honeycomb layers, while the Na intensity is reduced down to similar to 2/3 of its original value at the domain walls, implying significant hole doping. Utilizing focused-ion-beam microsectioning, the temperature dependence of the electrical resistance of individual domain walls is studied. It demonstrates the tuning through the metal-insulator transition into a correlated-metal ground state by increasing hole doping. |  |
Alpin, K.; Hirschmann, M. M.; Heinsdorf, N.; Leonhardt, A.; Yau, W. Y.; Wu, X.; Schnyder, A. P. Fundamental laws of chiral band crossings: Local constraints, global constraints, and topological phase diagrams Journal Article Phys. Rev. Research 5, 043165 (2023). @article{alpin_fundamental_2023,
title = {Fundamental laws of chiral band crossings: Local constraints, global constraints, and topological phase diagrams},
author = {K. Alpin and M. M. Hirschmann and N. Heinsdorf and A. Leonhardt and W. Y. Yau and X. Wu and A. P. Schnyder},
doi = {10.1103/PhysRevResearch.5.043165},
year = {2023},
date = {2023-11-01},
urldate = {2023-11-01},
journal = {Phys. Rev. Research},
volume = {5},
number = {4},
pages = {043165},
abstract = {We derive two fundamental laws of chiral band crossings: (i) a local constraint relating the Chern number to phase jumps of rotation eigenvalues and (ii) a global constraint determining the number of chiral crossings on rotation axes. Together with the fermion doubling theorem, these laws describe all conditions that a network of chiral band crossing must satisfy. We apply the fundamental laws to prove the existence of enforced double Weyl points, nodal planes, and generic Weyl points, among others. In addition, we show that chiral space group symmetries can not stabilize nodal lines with finite Chern numbers. Combining the local constraint with explicit low-energy models, we determine the generic topological phase diagrams of all multifold crossings. Remarkably, we find a fourfold crossing with Chern number 5, which exceeds the previously conceived maximum Chern number of 4. We identify materials crystallizing in space group 198, such as B20 materials and BaAsPt, as suitable compounds with this Chern number 5 crossing.},
keywords = {A6},
pubstate = {published},
tppubtype = {article}
}
We derive two fundamental laws of chiral band crossings: (i) a local constraint relating the Chern number to phase jumps of rotation eigenvalues and (ii) a global constraint determining the number of chiral crossings on rotation axes. Together with the fermion doubling theorem, these laws describe all conditions that a network of chiral band crossing must satisfy. We apply the fundamental laws to prove the existence of enforced double Weyl points, nodal planes, and generic Weyl points, among others. In addition, we show that chiral space group symmetries can not stabilize nodal lines with finite Chern numbers. Combining the local constraint with explicit low-energy models, we determine the generic topological phase diagrams of all multifold crossings. Remarkably, we find a fourfold crossing with Chern number 5, which exceeds the previously conceived maximum Chern number of 4. We identify materials crystallizing in space group 198, such as B20 materials and BaAsPt, as suitable compounds with this Chern number 5 crossing. |  |
Bader, V. P.; Ritter, C.; Papke, E.; Gegenwart, P.; Tsirlin, A. A. Geometrical frustration and incommensurate magnetic order in Na3RuO4 with two triangular motifs Journal Article Phys. Rev. B 108, 144424 (2023), datadoi: 10.5281/zenodo.8226429. @article{baderGeometricalFrustrationIncommensurate2023,
title = {Geometrical frustration and incommensurate magnetic order in Na_{3}RuO_{4} with two triangular motifs},
author = {V. P. Bader and C. Ritter and E. Papke and P. Gegenwart and A. A. Tsirlin},
url = {https://doi.org/10.1103/PhysRevB.108.144424},
doi = {10.1103/PhysRevB.108.144424},
year = {2023},
date = {2023-10-19},
urldate = {2023-01-01},
journal = {Phys. Rev. B},
volume = {108},
number = {14},
pages = {144424},
abstract = {Incommensurate magnetic order in the spin-3/2 antiferromagnet Na3RuO4 is uncovered by neutron diffraction combined with ab initio calculations. The crystal structure of Na3RuO4 contains two triangular motifs on different length scales. The magnetic Ru5+ ions form a lozenge (diamond) configuration, with tetramers composed of two isosceles triangles. These tetramers are further arranged in layers, such that an effective triangular lattice is formed. The tetramers are nearly antiferromagnetic but frustration between them leads to an incommensurately modulated magnetic structure described by the propagation vector 𝑘=(0.242(1),0,0.313(1)). We show that the long-range Ru-O-O-Ru couplings between the tetramers play a major role in Na3RuO4 and suggest an effective description in terms of the spatially anisotropic triangular lattice if the tetramers are treated as single sites.},
note = {datadoi: 10.5281/zenodo.8226429},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
Incommensurate magnetic order in the spin-3/2 antiferromagnet Na3RuO4 is uncovered by neutron diffraction combined with ab initio calculations. The crystal structure of Na3RuO4 contains two triangular motifs on different length scales. The magnetic Ru5+ ions form a lozenge (diamond) configuration, with tetramers composed of two isosceles triangles. These tetramers are further arranged in layers, such that an effective triangular lattice is formed. The tetramers are nearly antiferromagnetic but frustration between them leads to an incommensurately modulated magnetic structure described by the propagation vector 𝑘=(0.242(1),0,0.313(1)). We show that the long-range Ru-O-O-Ru couplings between the tetramers play a major role in Na3RuO4 and suggest an effective description in terms of the spatially anisotropic triangular lattice if the tetramers are treated as single sites. |  |
Mohanty, S.; Islam, S. S.; Winterhalter-Stocker, N.; Jesche, A.; Simutis, G.; Wang, Ch; Guguchia, Z.; Sichelschmidt, J.; Baenitz, M.; Tsirlin, A. A.; others, Disordered ground state in the spin-orbit coupled Jeff = 1/2 distorted honeycomb magnet BiYbGeO5 Journal Article Phys. Rev. B 108, 134408 (2023), datadoi: 10.5281/zenodo.8406218. @article{mohantyDisorderedGroundState2023,
title = {Disordered ground state in the spin-orbit coupled J_{eff} = 1/2 distorted honeycomb magnet BiYbGeO_{5}},
author = {S. Mohanty and S. S. Islam and N. Winterhalter-Stocker and A. Jesche and G. Simutis and Ch Wang and Z. Guguchia and J. Sichelschmidt and M. Baenitz and A. A. Tsirlin and others},
url = {https://doi.org/10.1103/PhysRevB.108.134408},
doi = {10.1103/PhysRevB.108.134408},
year = {2023},
date = {2023-10-09},
urldate = {2023-01-01},
journal = {Phys. Rev. B},
volume = {108},
number = {13},
pages = {134408},
abstract = {We delineate quantum magnetism in the strongly spin-orbit coupled distorted honeycomb lattice antiferromagnet BiYbGeO5. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective J(eff) = 1/2 Kramers doublet of Yb3+. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity can be modeled well assuming isolated spin dimers with anisotropic exchange interactions J(Z) similar or equal to 2.6 K and J(XY) similar or equal to 1.3 K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80 mK both in zero field and in applied fields. This sets BiYbGeO5 apart from Yb2Si2O7, with its unusual regime of magnon Bose-Einstein condensation, and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice.},
note = {datadoi: 10.5281/zenodo.8406218},
keywords = {B3},
pubstate = {published},
tppubtype = {article}
}
We delineate quantum magnetism in the strongly spin-orbit coupled distorted honeycomb lattice antiferromagnet BiYbGeO5. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective J(eff) = 1/2 Kramers doublet of Yb3+. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity can be modeled well assuming isolated spin dimers with anisotropic exchange interactions J(Z) similar or equal to 2.6 K and J(XY) similar or equal to 1.3 K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80 mK both in zero field and in applied fields. This sets BiYbGeO5 apart from Yb2Si2O7, with its unusual regime of magnon Bose-Einstein condensation, and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice. |  |
Huber, N.; Leeb, V.; Bauer, A.; Benka, G.; Knolle, J.; Pfleiderer, C.; Wilde, M. A. Quantum oscillations of the quasiparticle lifetime in a metal Journal Article Nature 621, 276 (2023), datadoi: 10.5281/zenodo.7957066. @article{huberQuantumOscillationsQuasiparticle2023,
title = {Quantum oscillations of the quasiparticle lifetime in a metal},
author = {N. Huber and V. Leeb and A. Bauer and G. Benka and J. Knolle and C. Pfleiderer and M. A. Wilde},
url = {https://doi.org/10.1038/s41586-023-06330-y},
doi = {10.1038/s41586-023-06330-y},
issn = {0028-0836},
year = {2023},
date = {2023-08-02},
urldate = {2023-08-02},
journal = {Nature},
volume = {621},
pages = {276},
abstract = {Following nearly a century of research, it remains a puzzle that the low-lying excitations of metals are remarkably well explained by effective single-particle theories of non-interacting bands(1-4). The abundance of interactions in real materials raises the question of direct spectroscopic signatures of phenomena beyond effective single-particle, single-band behaviour. Here we report the identification of quantum oscillations (QOs) in the three-dimensional topological semimetal CoSi, which defy the standard description in two fundamental aspects. First, the oscillation frequency corresponds to the difference of semiclassical quasiparticle (QP) orbits of two bands, which are forbidden as half of the trajectory would oppose the Lorentz force. Second, the oscillations exist up to above 50 K, in strong contrast to all other oscillatory components, which vanish below a few kelvin. Our findings are in excellent agreement with generic model calculations of QOs of the QP lifetime (QPL). Because the only precondition for their existence is a nonlinear coupling of at least two electronic orbits, for example, owing to QP scattering on defects or collective excitations, such QOs of the QPL are generic for any metal featuring Landau quantization with several orbits. They are consistent with certain frequencies in topological semimetals(5-9), unconventional superconductors(10,11), rare-earth compounds(12-14) and Rashba systems(15), and permit to identify and gauge correlation phenomena, for example, in two-dimensional materials(16,17) and multiband metals(18).},
note = {datadoi: 10.5281/zenodo.7957066},
keywords = {A6, B6, C1},
pubstate = {published},
tppubtype = {article}
}
Following nearly a century of research, it remains a puzzle that the low-lying excitations of metals are remarkably well explained by effective single-particle theories of non-interacting bands(1-4). The abundance of interactions in real materials raises the question of direct spectroscopic signatures of phenomena beyond effective single-particle, single-band behaviour. Here we report the identification of quantum oscillations (QOs) in the three-dimensional topological semimetal CoSi, which defy the standard description in two fundamental aspects. First, the oscillation frequency corresponds to the difference of semiclassical quasiparticle (QP) orbits of two bands, which are forbidden as half of the trajectory would oppose the Lorentz force. Second, the oscillations exist up to above 50 K, in strong contrast to all other oscillatory components, which vanish below a few kelvin. Our findings are in excellent agreement with generic model calculations of QOs of the QP lifetime (QPL). Because the only precondition for their existence is a nonlinear coupling of at least two electronic orbits, for example, owing to QP scattering on defects or collective excitations, such QOs of the QPL are generic for any metal featuring Landau quantization with several orbits. They are consistent with certain frequencies in topological semimetals(5-9), unconventional superconductors(10,11), rare-earth compounds(12-14) and Rashba systems(15), and permit to identify and gauge correlation phenomena, for example, in two-dimensional materials(16,17) and multiband metals(18). |  |
Ghara, S.; Barts, E.; Vasin, K. V.; Kamenskyi, D.; Prodan, L.; Tsurkan, V.; Kézsmárki, I.; Mostovoy, M.; Deisenhofer, J. Magnetization reversal through an antiferromagnetic state Journal Article Nat. Commun. 14, 5174 (2023). @article{ghara_magnetization_2023,
title = {Magnetization reversal through an antiferromagnetic state},
author = {S. Ghara and E. Barts and K. V. Vasin and D. Kamenskyi and L. Prodan and V. Tsurkan and I. Kézsmárki and M. Mostovoy and J. Deisenhofer},
doi = {10.1038/s41467-023-40722-y},
year = {2023},
date = {2023-08-01},
urldate = {2023-08-01},
journal = {Nat. Commun.},
volume = {14},
number = {1},
pages = {5174},
abstract = {Magnetization reversal in ferro- and ferrimagnets is a well-known archetype of non-equilibrium processes, where the volume fractions of the oppositely magnetized domains vary and perfectly compensate each other at the coercive magnetic field. Here, we report on a fundamentally new pathway for magnetization reversal that is mediated by an antiferromagnetic state. Consequently, an atomic-scale compensation of the magnetization is realized at the coercive field, instead of the mesoscopic or macroscopic domain cancellation in canonical reversal processes. We demonstrate this unusual magnetization reversal on the Zn-doped polar magnet Fe2Mo3O8. Hidden behind the conventional ferrimagnetic hysteresis loop, the surprising emergence of the antiferromagnetic phase at the coercive fields is disclosed by a sharp peak in the field-dependence of the electric polarization. In addition, at the magnetization reversal our THz spectroscopy studies reveal the reappearance of the magnon mode that is only present in the pristine antiferromagnetic state. According to our microscopic calculations, this unusual process is governed by the dominant intralayer coupling, strong easy-axis anisotropy and spin fluctuations, which result in a complex interplay between the ferrimagnetic and antiferromagnetic phases. Such antiferro-state-mediated reversal processes offer novel concepts for magnetization control, and may also emerge for other ferroic orders.},
keywords = {A1, C4},
pubstate = {published},
tppubtype = {article}
}
Magnetization reversal in ferro- and ferrimagnets is a well-known archetype of non-equilibrium processes, where the volume fractions of the oppositely magnetized domains vary and perfectly compensate each other at the coercive magnetic field. Here, we report on a fundamentally new pathway for magnetization reversal that is mediated by an antiferromagnetic state. Consequently, an atomic-scale compensation of the magnetization is realized at the coercive field, instead of the mesoscopic or macroscopic domain cancellation in canonical reversal processes. We demonstrate this unusual magnetization reversal on the Zn-doped polar magnet Fe2Mo3O8. Hidden behind the conventional ferrimagnetic hysteresis loop, the surprising emergence of the antiferromagnetic phase at the coercive fields is disclosed by a sharp peak in the field-dependence of the electric polarization. In addition, at the magnetization reversal our THz spectroscopy studies reveal the reappearance of the magnon mode that is only present in the pristine antiferromagnetic state. According to our microscopic calculations, this unusual process is governed by the dominant intralayer coupling, strong easy-axis anisotropy and spin fluctuations, which result in a complex interplay between the ferrimagnetic and antiferromagnetic phases. Such antiferro-state-mediated reversal processes offer novel concepts for magnetization control, and may also emerge for other ferroic orders. |  |
Prodan, L.; Evans, D. M.; Griffin, S. M.; Oestlin, A.; Altthaler, M.; Lysne, E.; Filippova, I. G.; Shova, S.; Chioncel, L.; Tsurkan, V.; Kézsmárki, I. Large ordered moment with strong easy-plane anisotropy and vortex-domain pattern in the kagome ferromagnet Fe3Sn Journal Article Appl. Phys. Lett. 123, 021901 (2023). @article{prodan_large_2023,
title = {Large ordered moment with strong easy-plane anisotropy and vortex-domain pattern in the kagome ferromagnet Fe_{3}Sn},
author = {L. Prodan and D. M. Evans and S. M. Griffin and A. Oestlin and M. Altthaler and E. Lysne and I. G. Filippova and S. Shova and L. Chioncel and V. Tsurkan and I. Kézsmárki},
doi = {10.1063/5.0155295},
issn = {0003-6951},
year = {2023},
date = {2023-07-01},
urldate = {2023-07-01},
journal = {Appl. Phys. Lett.},
volume = {123},
number = {2},
pages = {021901},
abstract = {We report the magnetic anisotropy of kagome bilayer ferromagnet Fe3Sn probed by the bulk magnetometry and magnetic force microscopy (MFM) on high-quality single crystals. The dependence of magnetization on the orientation of the external magnetic field reveals strong easyplane magnetocrystalline anisotropy and anisotropy of the saturation magnetization. The leading magnetocrystalline anisotropy constant shows a monotonous increase from K-1 approximate to -1.0 x 10(6) J/m(3) at 300K to -1.3 x 10(6) J/m(3) at 2K. Our ab initio electronic structure calculations yield the value of total magnetic moment of 7.1 mu(B)=f.u. and a magnetocrystalline anisotropy energy density of -0.57meV=f.u. (-1.62 x 10(6)J/m(3)) both being in reasonable agreement with the experimental values. The MFM imaging reveals micrometer-scale magnetic vortices with weakly pinned cores that vanish at the saturation field of similar to 3T applied perpendicular to the kagome plane. The observed vortex-domain structure is well reproduced by the micromagnetic simulations, using the experimentally determined value of the anisotropy and exchange stiffness. (c) 2023 Author(s).},
keywords = {A4, A5},
pubstate = {published},
tppubtype = {article}
}
We report the magnetic anisotropy of kagome bilayer ferromagnet Fe3Sn probed by the bulk magnetometry and magnetic force microscopy (MFM) on high-quality single crystals. The dependence of magnetization on the orientation of the external magnetic field reveals strong easyplane magnetocrystalline anisotropy and anisotropy of the saturation magnetization. The leading magnetocrystalline anisotropy constant shows a monotonous increase from K-1 approximate to -1.0 x 10(6) J/m(3) at 300K to -1.3 x 10(6) J/m(3) at 2K. Our ab initio electronic structure calculations yield the value of total magnetic moment of 7.1 mu(B)=f.u. and a magnetocrystalline anisotropy energy density of -0.57meV=f.u. (-1.62 x 10(6)J/m(3)) both being in reasonable agreement with the experimental values. The MFM imaging reveals micrometer-scale magnetic vortices with weakly pinned cores that vanish at the saturation field of similar to 3T applied perpendicular to the kagome plane. The observed vortex-domain structure is well reproduced by the micromagnetic simulations, using the experimentally determined value of the anisotropy and exchange stiffness. (c) 2023 Author(s). |  |
Deyerling, A.; Wilde, M. A.; Pfleiderer, C. Electronic structure of CeAuAl3 using density functional theory Journal Article SciPost Phys. Proc. 11, 008 (2023). @article{deyerling_electronic_2023,
title = {Electronic structure of CeAuAl_{3} using density functional theory},
author = {A. Deyerling and M. A. Wilde and C. Pfleiderer},
doi = {10.21468/SciPostPhysProc.11.008},
year = {2023},
date = {2023-06-05},
urldate = {2023-06-05},
journal = {SciPost Phys. Proc.},
volume = {11},
pages = {008},
abstract = {We studied the magnetic properties and electronic structure of CeAuAl3 using density functional theory. This compound shows a large Sommerfeld coefficient, a Kondo temperature, TK=4K and antiferromagnetic order below TN=1.1K. We calculated the magnetic groundstate of CeAuAl3 and the magnetic anisotropy energies. Treating the 4f-electrons as localized with DFT+U we obtain a good match with the magnetic properties observed experimentally. We also report salient features of the electronic structure of CeAuAl3, including features of the Fermi surface and associated quantum oscillatory spectra, when the 4f-electrons are treated either as localized or itinerant.},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
We studied the magnetic properties and electronic structure of CeAuAl3 using density functional theory. This compound shows a large Sommerfeld coefficient, a Kondo temperature, TK=4K and antiferromagnetic order below TN=1.1K. We calculated the magnetic groundstate of CeAuAl3 and the magnetic anisotropy energies. Treating the 4f-electrons as localized with DFT+U we obtain a good match with the magnetic properties observed experimentally. We also report salient features of the electronic structure of CeAuAl3, including features of the Fermi surface and associated quantum oscillatory spectra, when the 4f-electrons are treated either as localized or itinerant. |  |
Kumar, V.; Bauer, A.; Franz, C.; Spallek, J.; Schönmann, R.; Stekiel, M.; Schneidewind, A.; Wilde, M. A.; Pfleiderer, C. Low-temperature antiferromagnetic order in orthorhombic CePdAl3 Journal Article Phys. Rev. Research 5, 023157 (2023). @article{kumar_low-temperature_2023,
title = {Low-temperature antiferromagnetic order in orthorhombic CePdAl_{3}},
author = {V. Kumar and A. Bauer and C. Franz and J. Spallek and R. Schönmann and M. Stekiel and A. Schneidewind and M. A. Wilde and C. Pfleiderer},
doi = {10.1103/PhysRevResearch.5.023157},
year = {2023},
date = {2023-06-01},
urldate = {2023-06-01},
journal = {Phys. Rev. Research},
volume = {5},
number = {2},
pages = {023157},
abstract = {We report the magnetization, ac susceptibility, and specific heat of optically float-zoned single crystals of CePdAl3. In comparison to the properties of polycrystalline CePdAl3 reported in the literature, which displays a tetragonal crystal structure and no long-range magnetic order, our single crystals exhibit an orthorhombic structure (𝐶𝑚𝑐𝑚) and antiferromagnetic order below a Néel temperature 𝑇1=5.6 K. The specific heat at zero field shows two anomalies, namely, a broad transition at 𝑇1=5.6 K followed by a 𝜆-anomaly at 𝑇2=5.4 K. A conservative estimate of the Sommerfeld coefficient of the electronic specific heat, 𝛾=121mJK−2mol−1, indicates a moderately enhanced heavy-fermion ground state. A twin microstructure evolves in the family of planes spanned by the basal plane lattice vectors 𝐚o and 𝐜o , with the magnetic hard axis 𝐛o common to all twins. The antiferromagnetic state is characterized by a strong ao, co easy-plane magnetic anisotropy where the ao direction is the easy axis in the easy plane. A spin-flop transition induced under magnetic field along the easy directions, results in complex magnetic phase diagrams. Taken together, our results reveal a high sensitivity of the magnetic and electronic properties of CePdAl3 to its structural modifications.},
keywords = {A6, C1},
pubstate = {published},
tppubtype = {article}
}
We report the magnetization, ac susceptibility, and specific heat of optically float-zoned single crystals of CePdAl3. In comparison to the properties of polycrystalline CePdAl3 reported in the literature, which displays a tetragonal crystal structure and no long-range magnetic order, our single crystals exhibit an orthorhombic structure (𝐶𝑚𝑐𝑚) and antiferromagnetic order below a Néel temperature 𝑇1=5.6 K. The specific heat at zero field shows two anomalies, namely, a broad transition at 𝑇1=5.6 K followed by a 𝜆-anomaly at 𝑇2=5.4 K. A conservative estimate of the Sommerfeld coefficient of the electronic specific heat, 𝛾=121mJK−2mol−1, indicates a moderately enhanced heavy-fermion ground state. A twin microstructure evolves in the family of planes spanned by the basal plane lattice vectors 𝐚o and 𝐜o , with the magnetic hard axis 𝐛o common to all twins. The antiferromagnetic state is characterized by a strong ao, co easy-plane magnetic anisotropy where the ao direction is the easy axis in the easy plane. A spin-flop transition induced under magnetic field along the easy directions, results in complex magnetic phase diagrams. Taken together, our results reveal a high sensitivity of the magnetic and electronic properties of CePdAl3 to its structural modifications. |  |
Schilberth, F.; Jiang, M. -C.; Minami, S.; Kassem, M. A.; Mayr, F.; Koretsune, T.; Tabata, Y.; Waki, T.; Nakamura, H.; Guo, G. -Y.; Arita, R.; Kézsmárki, I.; Bordacs, S. Nodal-line resonance generating the giant anomalous Hall effect of Co3Sn2S2 Journal Article Phys. Rev. B 107, 214441 (2023). @article{schilberth_nodal-line_2023,
title = {Nodal-line resonance generating the giant anomalous Hall effect of Co_{3}Sn_{2}S_{2}},
author = {F. Schilberth and M. -C. Jiang and S. Minami and M. A. Kassem and F. Mayr and T. Koretsune and Y. Tabata and T. Waki and H. Nakamura and G. -Y. Guo and R. Arita and I. Kézsmárki and S. Bordacs},
doi = {10.1103/PhysRevB.107.214441},
issn = {2469-9950},
year = {2023},
date = {2023-06-01},
urldate = {2023-06-01},
journal = {Phys. Rev. B},
volume = {107},
number = {21},
pages = {214441},
abstract = {Giant anomalous Hall effect (AHE) and magneto-optical activity can emerge in magnets with topologically nontrivial degeneracies. However, identifying the specific band-structure features such as Weyl points, nodal lines, or planes which generate the anomalous response is a challenging issue. Since the low-energy interband transitions can govern the static AHE, we addressed this question in the prototypical magnetic Weyl semimetal Co3Sn2S2 also hosting nodal lines by broadband polarized reflectivity and magneto-optical Kerr effect spectroscopy with a focus on the far-infrared range. In the linear dichroism spectrum we observe a strong resonance at 40 meV, which also appears in the optical Hall conductivity and primarily determines the static AHE, and thus confirms its intrinsic origin. Our material-specific theory reproduces the experimental data remarkably well and shows that strongly tilted nodal-line segments around the Fermi energy generate the resonance. While the Weyl points only give vanishing contributions, these segments of the nodal lines gapped by the spin-orbit coupling dominate the low-energy optical response and generate the giant AHE.},
keywords = {A1},
pubstate = {published},
tppubtype = {article}
}
Giant anomalous Hall effect (AHE) and magneto-optical activity can emerge in magnets with topologically nontrivial degeneracies. However, identifying the specific band-structure features such as Weyl points, nodal lines, or planes which generate the anomalous response is a challenging issue. Since the low-energy interband transitions can govern the static AHE, we addressed this question in the prototypical magnetic Weyl semimetal Co3Sn2S2 also hosting nodal lines by broadband polarized reflectivity and magneto-optical Kerr effect spectroscopy with a focus on the far-infrared range. In the linear dichroism spectrum we observe a strong resonance at 40 meV, which also appears in the optical Hall conductivity and primarily determines the static AHE, and thus confirms its intrinsic origin. Our material-specific theory reproduces the experimental data remarkably well and shows that strongly tilted nodal-line segments around the Fermi energy generate the resonance. While the Weyl points only give vanishing contributions, these segments of the nodal lines gapped by the spin-orbit coupling dominate the low-energy optical response and generate the giant AHE. |  |
Tóth, B.; Amelin, K.; Rõõm, T.; Nagel, U.; Bauernfeind, A.; Tsurkan, V.; Prodan, L.; von Nidda, H. -A. Krug; Scheffler, M.; Kézsmárki, I.; others, Broadband magnetic resonance spectroscopy in MnSc2S4 Journal Article Sci. Rep. 13, 11069 (2023). @article{toth_broadband_2023,
title = {Broadband magnetic resonance spectroscopy in MnSc_{2}S_{4}},
author = {B. Tóth and K. Amelin and T. Rõõm and U. Nagel and A. Bauernfeind and V. Tsurkan and L. Prodan and H. -A. Krug von Nidda and M. Scheffler and I. Kézsmárki and others},
doi = {10.1038/s41598-023-37911-6},
year = {2023},
date = {2023-01-01},
urldate = {2023-01-01},
journal = {Sci. Rep.},
volume = {13},
number = {1},
pages = {11069},
abstract = {Recent neutron scattering experiments suggested that frustrated magnetic interactions give rise to antiferromagnetic spiral and fractional skyrmion lattice phases in MnSc2S4. Here, to trace the signatures of these modulated phases, we studied the spin excitations of MnSc2S4 by THz spectroscopy at 300 mK and in magnetic fields up to 12 T and by broadband microwave spectroscopy at various temperatures up to 50 GHz. We found a single magnetic resonance with frequency linearly increasing in field. The small deviation of the Mn2+ ion g-factor from 2},
keywords = {B4},
pubstate = {published},
tppubtype = {article}
}
Recent neutron scattering experiments suggested that frustrated magnetic interactions give rise to antiferromagnetic spiral and fractional skyrmion lattice phases in MnSc2S4. Here, to trace the signatures of these modulated phases, we studied the spin excitations of MnSc2S4 by THz spectroscopy at 300 mK and in magnetic fields up to 12 T and by broadband microwave spectroscopy at various temperatures up to 50 GHz. We found a single magnetic resonance with frequency linearly increasing in field. The small deviation of the Mn2+ ion g-factor from 2 |  |
Müller, M.; Weber, J.; Goennenwein, S. T. B.; Kusminskiy, S. V.; Gross, R.; Althammer, M.; Huebl, H. Temperature dependence of the magnon-phonon interaction in high overtone bulk acoustic resonator-ferromagnetic thin film hybrids Journal Article Phy. Rev. Applied 21, 034032 (2023). @article{muller_temperature_2023,
title = {Temperature dependence of the magnon-phonon interaction in high overtone bulk acoustic resonator-ferromagnetic thin film hybrids},
author = {M. Müller and J. Weber and S. T. B. Goennenwein and S. V. Kusminskiy and R. Gross and M. Althammer and H. Huebl},
doi = {10.1103/PhysRevApplied.21.034032},
year = {2023},
date = {2023-01-01},
urldate = {2023-01-01},
journal = {Phy. Rev. Applied},
volume = {21},
number = {3},
pages = {034032},
keywords = {C3},
pubstate = {published},
tppubtype = {article}
}
|  |
Evans, D. M.; Conroy, M.; Puntigam, L.; Croitori, D.; Prodan, L.; Douglas, J. O.; Gault, B.; Tsurkan, V. Direct imaging of spatial heterogeneities in type II superconductors Unpublished (2023), arXiv:2310.20017. @unpublished{evans_direct_2023,
title = {Direct imaging of spatial heterogeneities in type II superconductors},
author = {D. M. Evans and M. Conroy and L. Puntigam and D. Croitori and L. Prodan and J. O. Douglas and B. Gault and V. Tsurkan},
doi = {10.48550/arXiv.2310.20017},
year = {2023},
date = {2023-01-01},
urldate = {2023-01-01},
note = {arXiv:2310.20017},
keywords = {},
pubstate = {published},
tppubtype = {unpublished}
}
| |